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公开(公告)号：US20130213107A1
公开(公告)日：2013-08-22
申请号：US13882572
申请日：2011-12-15
申请人： Koichi Sakairi , Kunihiro Tanaka , Muneki Nakamura , Fumie Seki
发明人： Koichi Sakairi , Kunihiro Tanaka , Muneki Nakamura , Fumie Seki
摘要： The present invention is a metallic wire rod comprising iridium or an iridium-containing alloy and, the wire rod has in the cross section thereof biaxial crystal orientation of 50% or more of abundance proportion of textures in which crystallographic orientation has preferred orientation to direction. In the present invention, crystal orientation in the outer periphery from semicircle of the cross section which is the periphery of the wire rod is important, and in this zone, abundance proportion of textures in which crystallographic orientation has preferred orientation to direction is preferably not less than 50%.
摘要翻译： 本发明是一种包含铱或含铱合金的金属线材，该线材的横截面为双轴晶体取向为50％以上，其结晶取向优选取向为<100 >方向。 在本发明中，作为线材周边的横截面的半圆的外周的晶体取向是重要的，在该区域中，结晶取向优选朝向<100>方向的织构的丰度比例为 优选不小于50％。
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2.发明授权Electrode for polymer electrolyte electrochemical cell and process of preparing same 失效电极用于聚合物电解质电化学电池及其制备方法
公开(公告)号：US5728485A
公开(公告)日：1998-03-17
申请号：US873760
申请日：1997-06-12
申请人： Masahiro Watanabe , Koichi Sakairi
发明人： Masahiro Watanabe , Koichi Sakairi
CPC分类号： H01M4/926 , H01M4/8605 , H01M8/1004 , H01M2300/0082
摘要： Disclosed an electrode for a polymer electrolyte electrochemical cell which comprises catalyst supports carrying catalyst particles, a first solid polymer electrolyte layer insoluble in water and an organic solvent formed on the particles and a second solid polymer electrolyte layer insoluble or soluble in the organic solvent formed on part of the surface of the first solid polymer electrolyte layer and a process of preparing same.
摘要翻译： 公开了一种用于聚合物电解质电化学电池的电极，其包括载有催化剂颗粒的催化剂载体，不溶于水的第一固体聚合物电解质层和形成在颗粒上的有机溶剂，以及第二固体聚合物电解质层，其不溶于或可溶于形成于 第一固体聚合物电解质层的表面的一部分及其制备方法。
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3.发明授权Conductive fine particle and metal paste for electrode formation, and electrode 有权用于电极形成的导电细颗粒和金属膏，以及电极公开(公告)号：US08771553B2
公开(公告)日：2014-07-08
申请号：US13387976
申请日：2011-07-08
申请人： Takuya Hosoi , Nobuhisa Okamoto , Koichi Sakairi
发明人： Takuya Hosoi , Nobuhisa Okamoto , Koichi Sakairi
CPC分类号： C09D5/24 , G01N27/4075 , H01B1/02 , H01B1/22 , Y10T428/2991
摘要： An object of the present invention is to provide a conductive fine particle for producing a metal paste that can produce an electrode film having a low resistance, and a metal paste utilizing the conductive fine particle. The present invention is a conductive particle for electrode formation having a core/shell structure, and the conductive particle comprises a core particle made of Pt or a Pt alloy and having a particle diameter of 10 to 200 nm, and a shell made of a ceramic containing Al2O3 or ZrO2 and covers at least a part of the core particle, wherein the ceramic constituting the shell is added in an amount of 0.5 to 15% by weight based on the core particle to cover the core. The core particle is preferably Pt or a Pt alloy alloyed with Pd, Au, Ag, or Rh.
摘要翻译： 本发明的目的在于提供一种用于制造能够制造具有低电阻的电极膜的金属膏的导电性微粒和利用该导电性微粒的金属糊。 本发明是具有核/壳结构的电极形成用导电性粒子，导电性粒子由Pt或Pt合金制成的粒径为10〜200nm的核心粒子和由陶瓷制成的壳体 含有Al 2 O 3或ZrO 2并且覆盖核心颗粒的至少一部分，其中构成壳的陶瓷的添加量为0.5〜15重量％，基于芯颗粒覆盖芯。 核心颗粒优选为与Pd，Au，Ag或Rh合金化的Pt或Pt合金。
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4.发明申请NOBEL METAL ALLOY FOR SPARK PLUG AND METHOD FOR PRODUCING AND PROCESSING THE SAME 有权用于火花塞的NOBEL金属合金及其生产和加工方法公开(公告)号：US20090293995A1
公开(公告)日：2009-12-03
申请号：US12064665
申请日：2007-07-24
CPC分类号： C22C5/00 , B22F2998/10 , C22C1/0466 , C22F1/14 , C23C6/00 , C23C26/02 , H01T13/39 , H01T21/02 , B22F1/0003 , B22F2202/07 , B22F2203/11 , B22F7/062 , B22F3/17 , B22F3/18 , B22F3/20 , B22F3/24
摘要： An object of the present invention is to provide a material for a precious metal tip of a spark plug, which has more excellent durability, particularly oxidation wear resistance than a conventional one. The precious metal alloy for the spark plug according to the present invention contains 0.2 to 6.0 wt. % Cr as an essential component, further at least any one of Fe or Ni, and the balance being Ir. Here, the amount of Fe and Ni to be added is preferably 2.0 to 12.0 wt. % in total. According to the present invention, the surface may be oxidized to form an oxide layer made from a Cr—Fe oxide, a Cr—Ni oxide or a Cr—Fe—Ni oxide. The oxide layer is formed by a diffusion treatment by heating the precious metal alloy at 300 to 900° C. in an oxidative atmosphere, and preferably has a thickness of 5 to 100 μm.
摘要翻译： 本发明的目的是提供一种用于火花塞的贵金属端头的材料，其耐久性更优异，特别是比常规的耐氧化耐磨性更好。 本发明的火花塞用贵金属合金含有0.2〜6.0重量％ ％Cr作为必要成分，还含有Fe或Ni中的至少任一种，余量为Ir。 这里，Fe和Ni的添加量优选为2.0〜12.0重量％。 ％ 总共。 根据本发明，可以将表面氧化形成由Cr-Fe氧化物，Cr-Ni氧化物或Cr-Fe-Ni氧化物制成的氧化物层。 通过在氧化气氛中在300〜900℃下加热贵金属合金进行扩散处理而形成氧化物层，优选为5〜100μm的厚度。
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公开(公告)号：US5294232A
公开(公告)日：1994-03-15
申请号：US999303
申请日：1992-12-31
申请人： Koichi Sakairi , Yumi Yamamoto
发明人： Koichi Sakairi , Yumi Yamamoto
CPC分类号： H01M8/1004 , H01M2300/0082 , Y02P70/56 , Y10T29/49115
摘要： Disclosed herein is a process of preparing a solid polymer electrolyte type fuel cell formed by combining a cathode current collector, a cathode containing cathode particles, an ion exchange membrane, an anode containing anode particles and an anode current collector characterized by comprising reducing a catalyst metal salt in an organic solution with the solid polymer electrolyte, depositing the reduced catalyst metal in the solid polymer electrolyte to form the cathode and/or the anode, interposing the cathode and/or the anode between the respective current collectors and the ion exchange membrane and pressing for assembling the fuel cell.Also disclosed is the same process as above except that the support is present in the solid polymer electrolyte.In the fuel cells prepared in accordance with the present invention, the catalyst metal always exists in the solid polymer electrolyte, and even if a cavity is formed in the solid polymer electrolyte, the catalyst metal is not exposed to the cavity. Accordingly, almost all the catalyst metals can be utilized to generate energy at the high efficiency.
摘要翻译： 本发明公开了一种制备固体聚合物电解质型燃料电池的方法，该固体聚合物电解质型燃料电池通过组合阴极集电器，含阴极颗粒的阴极，离子交换膜，含阳极颗粒的阳极和阳极集电器而形成，其特征在于包括还原催化剂金属 在固体聚合物电解质的有机溶液中加入盐，将还原的催化剂金属沉积在固体聚合物电解质中以形成阴极和/或阳极，将阴极和/或阳极插入相应的集电体和离子交换膜之间，以及 按压组装燃料电池。 还公开了与上述相同的方法，只是载体存在于固体聚合物电解质中。 在根据本发明制备的燃料电池中，催化剂金属总是存在于固体聚合物电解质中，并且即使在固体聚合物电解质中形成空腔，催化剂金属也不暴露于空腔。 因此，几乎所有的催化剂金属都可以用于以高效率产生能量。
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公开(公告)号：US10047415B2
公开(公告)日：2018-08-14
申请号：US13882572
申请日：2011-12-15
申请人： Koichi Sakairi , Kunihiro Tanaka , Muneki Nakamura , Fumie Seki
发明人： Koichi Sakairi , Kunihiro Tanaka , Muneki Nakamura , Fumie Seki
摘要： The present invention is a metallic wire rod comprising iridium or an iridium-containing alloy and, the wire rod has in the cross section thereof biaxial crystal orientation of 50% or more of abundance proportion of textures in which crystallographic orientation has preferred orientation to direction. In the present invention, crystal orientation in the outer periphery from semicircle of the cross section which is the periphery of the wire rod is important, and in this zone, abundance proportion of textures in which crystallographic orientation has preferred orientation to direction is preferably not less than 50%.
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7.发明申请CONDUCTIVE FINE PARTICLE AND METAL PASTE FOR ELECTRODE FORMATION, AND ELECTRODE 有权导电精细颗粒和金属电极用于电极形成和电极公开(公告)号：US20120126183A1
公开(公告)日：2012-05-24
申请号：US13387976
申请日：2011-07-08
申请人： Takuya Hosoi , Nobuhisa Okamoto , Koichi Sakairi
发明人： Takuya Hosoi , Nobuhisa Okamoto , Koichi Sakairi
IPC分类号： H01B1/02
CPC分类号： C09D5/24 , G01N27/4075 , H01B1/02 , H01B1/22 , Y10T428/2991
摘要： An object of the present invention is to provide a conductive fine particle for producing a metal paste that can produce an electrode film having a low resistance, and a metal paste utilizing the conductive fine particle. The present invention is a conductive particle for electrode formation having a core/shell structure, and the conductive particle comprises a core particle made of Pt or a Pt alloy and having a particle diameter of 10 to 200 nm, and a shell made of a ceramic containing Al2O3 or ZrO2 and covers at least a part of the core particle, wherein the ceramic constituting the shell is added in an amount of 0.5 to 15% by weight based on the core particle to cover the core. The core particle is preferably Pt or a Pt alloy alloyed with Pd, Au, Ag, or Rh.
摘要翻译： 本发明的目的在于提供一种用于制造能够制造具有低电阻的电极膜的金属膏的导电性微粒和利用该导电性微粒的金属糊。 本发明是具有核/壳结构的电极形成用导电性粒子，导电性粒子由Pt或Pt合金制成的粒径为10〜200nm的核心粒子和由陶瓷制成的壳体 含有Al 2 O 3或ZrO 2并且覆盖核心颗粒的至少一部分，其中构成壳的陶瓷的添加量为0.5〜15重量％，基于芯颗粒覆盖芯。 核心颗粒优选为与Pd，Au，Ag或Rh合金化的Pt或Pt合金。
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8.发明授权Noble metal alloy for spark plug and method for producing and processing the same 有权用于火花塞的贵金属合金及其制造和加工方法公开(公告)号：US08029628B2
公开(公告)日：2011-10-04
申请号：US12064665
申请日：2007-07-24
IPC分类号： C22C5/04
CPC分类号： C22C5/00 , B22F2998/10 , C22C1/0466 , C22F1/14 , C23C6/00 , C23C26/02 , H01T13/39 , H01T21/02 , B22F1/0003 , B22F2202/07 , B22F2203/11 , B22F7/062 , B22F3/17 , B22F3/18 , B22F3/20 , B22F3/24
摘要： An object of the present invention is to provide a material for a precious metal tip of a spark plug, which has more excellent durability, particularly oxidation wear resistance than a conventional one. The precious metal alloy for the spark plug according to the present invention contains 0.2 to 6.0 wt. % Cr as an essential component, further at least any one of Fe or Ni, and the balance being Ir. Here, the amount of Fe and Ni to be added is preferably 2.0 to 12.0 wt. % in total. According to the present invention, the surface may be oxidized to form an oxide layer made from a Cr—Fe oxide, a Cr—Ni oxide or a Cr—Fe—Ni oxide. The oxide layer is formed by a diffusion treatment by heating the precious metal alloy at 300 to 900° C. in an oxidative atmosphere, and preferably has a thickness of 5 to 100 μm.
摘要翻译： 本发明的目的是提供一种用于火花塞的贵金属端头的材料，其耐久性更优异，特别是比常规的耐氧化耐磨性更好。 本发明的火花塞用贵金属合金含有0.2〜6.0重量％ ％Cr作为必要成分，还含有Fe或Ni中的至少任一种，余量为Ir。 这里，Fe和Ni的添加量优选为2.0〜12.0重量％。 ％ 总共。 根据本发明，可以将表面氧化形成由Cr-Fe氧化物，Cr-Ni氧化物或Cr-Fe-Ni氧化物制成的氧化物层。 通过在氧化气氛下在300〜900℃下加热贵金属合金进行扩散处理而形成氧化物层，优选为5〜100μm的厚度。
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公开(公告)号：US5453332A
公开(公告)日：1995-09-26
申请号：US125636
申请日：1993-09-22
申请人： Koichi Sakairi , Masahiro Watanabe
发明人： Koichi Sakairi , Masahiro Watanabe
CPC分类号： H01M4/926 , H01M4/96 , H01M8/1004 , H01M2300/0082
摘要： Disclosed is an electrode structure for fuel cell having a carbon support of which an apparent density is between 0.05 g/cm.sup.3 and 1.2 g/cm.sup.3.In this electrode structure, the sufficient diffusion of gases can be secured because the sufficient cavities are securely formed in the catalyst electrode layer by the carbon support having a smaller apparent density or a larger porosity even if the thickness of the catalyst electrode layer increases.
摘要翻译： 公开了一种具有碳载体的燃料电池的电极结构，其表观密度为0.05g / cm 3至1.2g / cm 3。 在该电极结构中，即使催化剂电极层的厚度增加，由于通过具有较小表观密度或更大孔隙率的碳载体的催化剂电极层中牢固地形成足够的空腔，因此可以确保气体的充分扩散。
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