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公开(公告)号：US07238303B2
公开(公告)日：2007-07-03
申请号：US10928516
申请日：2004-08-27
申请人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
发明人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
CPC分类号： C09K11/595 , C09K11/7734 , C09K11/778 , H01J1/63 , H01J2211/42
摘要： Phosphor and a plasma display device are provided whose deterioration in brightness of phosphors and a degree of change in chromaticity are alleviated and whose discharge characteristics are improved and that has excellent initial characteristics. Phosphor of the present invention is an alkaline-earth metal aluminate phosphor containing an element M (where M denotes at least one type of element selected from the group consisting of Nb, Ta, W and B). In this phosphor, a concentration of M in the vicinity of a surface of the phosphor particles is higher than the average concentration of M in the phosphor particles as a whole. A plasma display device according to the present invention includes a plasma display panel in which a plurality of discharge cells in one color or in a plurality of colors are arranged and phosphor layers are arranged so as to correspond to the discharge cells in colors and in which light is emitted by exciting the phosphor layers with ultraviolet rays. The phosphor layers include blue phosphor, where the afore-mentioned phosphor is used as the blue phosphor.
摘要翻译： 提供了荧光体和等离子体显示装置，其荧光体的亮度劣化和色度变化程度得到缓解，其放电特性得到改善并具有优异的初始特性。 本发明的荧光体是含有元素M的碱土金属铝酸盐荧光体（其中M表示选自Nb，Ta，W和B中的至少一种元素）。 在该荧光体中，荧光体粒子表面附近的M浓度高于荧光体粒子的M的平均浓度。 根据本发明的等离子体显示装置包括等离子体显示面板，其中排列有一种颜色或多种颜色的多个放电单元，并且荧光体层被布置为与颜色的放电单元相对应，并且其中 通过用紫外线激发荧光体层来发射光。 荧光体层包括蓝色荧光体，其中上述荧光体用作蓝色荧光体。
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公开(公告)号：US20050062417A1
公开(公告)日：2005-03-24
申请号：US10928516
申请日：2004-08-27
申请人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
发明人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
IPC分类号： C09K11/08 , C09K11/55 , C09K11/59 , C09K11/64 , C09K11/67 , C09K11/68 , C09K11/77 , C09K11/80 , H01J1/62 , H01J1/63 , H01J11/00 , H01J11/22 , H01J11/24 , H01J11/34 , H01J11/42 , H01J63/04 , H01J17/49
CPC分类号： C09K11/595 , C09K11/7734 , C09K11/778 , H01J1/63 , H01J2211/42
摘要： Phosphor and a plasma display device are provided whose deterioration in brightness of phosphors and a degree of change in chromaticity are alleviated and whose discharge characteristics are improved and that has excellent initial characteristics. Phosphor of the present invention is an alkaline-earth metal aluminate phosphor containing an element M (where M denotes at least one type of element selected from the group consisting of Nb, Ta, W and B). In this phosphor, a concentration of M in the vicinity of a surface of the phosphor particles is higher than the average concentration of M in the phosphor particles as a whole. A plasma display device according to the present invention includes a plasma display panel in which a plurality of discharge cells in one color or in a plurality of colors are arranged and phosphor layers are arranged so as to correspond to the discharge cells in colors and in which light is emitted by exciting the phosphor layers with ultraviolet rays. The phosphor layers include blue phosphor, where the afore-mentioned phosphor is used as the blue phosphor.
摘要翻译： 提供了荧光体和等离子体显示装置，其荧光体的亮度劣化和色度变化程度得到缓解，其放电特性得到改善并具有优异的初始特性。 本发明的荧光体是含有元素M的碱土金属铝酸盐荧光体（其中M表示选自Nb，Ta，W和B中的至少一种元素）。 在该荧光体中，荧光体粒子表面附近的M浓度高于荧光体粒子的M的平均浓度。 根据本发明的等离子体显示装置包括等离子体显示面板，其中排列有一种颜色或多种颜色的多个放电单元，并且荧光体层被布置为与颜色的放电单元相对应，并且其中 通过用紫外线激发荧光体层来发射光。 荧光体层包括蓝色荧光体，其中上述荧光体用作蓝色荧光体。
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3.发明授权Plasma display device having blue phosphor layers with alkaline earth metal aluminate containing molybdenum or tungsten 有权具有含有钼或钨的碱土金属铝酸盐的蓝色荧光体层的等离子体显示装置公开(公告)号：US07285913B2
公开(公告)日：2007-10-23
申请号：US10927265
申请日：2004-08-26
申请人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
发明人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
IPC分类号： H01J17/49
CPC分类号： C09K11/595 , C09K11/7734 , C09K11/778 , H01J1/63 , H01J2211/42
摘要： A plasma display device is provided in which deterioration in brightness of phosphor layers can be avoided. The plasma display device includes a plasma display panel in which a plurality of discharge cells in one color or in a plurality of colors are arranged and phosphor layers are arranged so as to correspond to the discharge cells in colors and in which light is emitted by exciting the phosphor layers with ultraviolet rays. The phosphor layers include blue phosphor, the blue phosphor being composed of an alkaline-earth metal aluminate phosphor containing at least one element selected from the group consisting of Mo and W. The addition of hexavalent ions (Mo, W) in the blue phosphor allows the elimination of oxygen defects in the vicinity of a layer containing Ba atoms (Ba—O layer), the suppression of adsorption of water to the surface of the blue phosphor and the improvement of deterioration in brightness and a change in chromaticity for the respective phosphors and discharge characteristics.
摘要翻译： 提供了一种能够避免荧光体层的亮度劣化的等离子体显示装置。 等离子体显示装置包括等离子体显示面板，其中排列有一种颜色或多种颜色的多个放电单元，并且荧光体层被布置成与颜色对应于放电单元并且通过激发发光 具有紫外线的荧光体层。 荧光体层包括蓝色荧光体，蓝色荧光体由含有选自Mo和W中的至少一种元素的碱土金属铝酸盐荧光体构成。在蓝色荧光体中添加六价离子（Mo，W）允许 消除含有Ba原子（Ba-O层）的层附近的氧缺陷，抑制水对蓝色荧光体表面的吸附以及改善亮度劣化和各种荧光体的色度变化 和放电特性。
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公开(公告)号：US20050046330A1
公开(公告)日：2005-03-03
申请号：US10927265
申请日：2004-08-26
申请人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
发明人： Kojiro Okuyama , Takehiro Zukawa , Masahiro Sakai , Seigo Shiraishi , Kazuhiko Sugimoto , Masaki Aoki , Junichi Hibino
IPC分类号： C09K11/08 , C09K11/55 , C09K11/59 , C09K11/64 , C09K11/67 , C09K11/68 , C09K11/77 , C09K11/80 , H01J1/62 , H01J1/63 , H01J11/00 , H01J11/22 , H01J11/24 , H01J11/34 , H01J11/42 , H01J63/04
CPC分类号： C09K11/595 , C09K11/7734 , C09K11/778 , H01J1/63 , H01J2211/42
摘要： A plasma display device is provided in which deterioration in brightness of phosphor layers can be avoided. The plasma display device includes a plasma display panel in which a plurality of discharge cells in one color or in a plurality of colors are arranged and phosphor layers are arranged so as to correspond to the discharge cells in colors and in which light is emitted by exciting the phosphor layers with ultraviolet rays. The phosphor layers include blue phosphor, the blue phosphor being composed of an alkaline-earth metal aluminate phosphor containing at least one element selected from the group consisting of Mo and W. The addition of hexavalent ions (Mo, W) in the blue phosphor allows the elimination of oxygen defects in the vicinity of a layer containing Ba atoms (Ba—O layer), the suppression of adsorption of water to the surface of the blue phosphor and the improvement of deterioration in brightness and a change in chromaticity for the respective phosphors and discharge characteristics.
摘要翻译： 提供了一种能够避免荧光体层的亮度劣化的等离子体显示装置。 等离子体显示装置包括等离子体显示面板，其中排列有一种颜色或多种颜色的多个放电单元，并且荧光体层被布置成与颜色相对应的放电单元并且通过激发发光 具有紫外线的荧光体层。 荧光体层包括蓝色荧光体，蓝色荧光体由含有选自Mo和W中的至少一种元素的碱土金属铝酸盐荧光体构成。在蓝色荧光体中添加六价离子（Mo，W）允许 消除含有Ba原子（Ba-O层）的层附近的氧缺陷，抑制水对蓝色荧光体表面的吸附以及改善亮度劣化和各种荧光体的色度变化 和放电特性。
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公开(公告)号：US20080203893A1
公开(公告)日：2008-08-28
申请号：US11910832
申请日：2006-04-06
申请人： Masahiro Sakai , Seigo Shiraishi , Takehiro Zukawa , Kojiro Okuyama , Junichi Hibino , Kazuhiko Sugimoto
发明人： Masahiro Sakai , Seigo Shiraishi , Takehiro Zukawa , Kojiro Okuyama , Junichi Hibino , Kazuhiko Sugimoto
CPC分类号： C09K11/7734 , H01J1/63 , H01J11/12 , H01J11/42 , H01J61/44
摘要： The present invention is a light-emitting device which is provided with a phosphor layer containing a blue phosphor, wherein the phosphor layer includes an aluminate phosphor, as the blue phosphor, that contains Ba, Sr, Eu, Mg, Al and O as constituting elements at an atom-number ratio Ba:Sr:Eu:Mg:Al:O=p:q:r:1:w:17 wherein 0.70≦p≦0.95, 0≦q≦0.15, 0.05≦r≦0.20, p+q+r≧1, and 9.8≦w≦10.5 are satisfied, and a value of a linear coupling function s represented by a formula: s=−11622+2043.07La+199.24L1−116.91L2 is 1 or less, when a lattice constant is La(Å), an interatomic distance between Al(2) and O(5) is L1(Å), and an interatomic distance between Al(1) and O(4) is L2(Å), which are obtained by an X-ray crystal structure analysis assuming that the aluminate phosphor belongs to a space group P63/mmc.
摘要翻译： 本发明是一种发光装置，其具有含有蓝色荧光体的荧光体层，其中，荧光体层含有作为蓝色荧光体的铝酸盐荧光体，其含有Ba，Sr，Eu，Mg，Al，O作为构成 元素原子数比Ba：Sr：Eu：Mg：Al：O = p：q：r：1：w：17其中0.70 <= p <= 0.95,0 <= q <= 0.15,0.05 < 满足r <= 0.20，p + q + r> = 1和9.8 <= w <= 10.5，并且由公式表示的线性耦合函数s的值：<？in-line-formula description =“In -line公式“end =”lead“？> s = -11622 + 2043.07L 199.24L -116.91L <2> 在线公式描述=“在线公式”end =“tail”？>为1以下，当晶格常数为L（a）时，Al（2）之间的原子间距离 ）和O（5）是L 1（A），Al（1）和O（4）之间的原子间距离是L 2（），它们是 通过假设铝酸盐荧光体属于空间群P6
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公开(公告)号：US08366965B2
公开(公告)日：2013-02-05
申请号：US13180171
申请日：2011-07-11
IPC分类号： C09K11/68
CPC分类号： C09K11/7736 , H01J11/12 , H01J11/42 , H01J61/44
摘要： The present invention provides a blue phosphor that exhibits high luminance and shows less luminance degradation during driving of a light-emitting device. The present invention is a blue phosphor represented by the general formula aBaO.bSrO.(1−a−b)EuO.cMgO.dAlO3/2.eWO3, where 0.70≦a≦0.95, 0≦b≦0.15, 0.95≦c≦1.15, 9.00≦d≦11.00, 0.001≦e≦0.100, and a+b≦0.97 are satisfied. In this blue phosphor, two peaks whose tops are located in a range of diffraction angle 2θ=13.0 to 13.6 degrees are present in an X-ray diffraction pattern obtained by measurement on the blue phosphor using an X-ray with a wavelength of 0.774 Å.
摘要翻译： 本发明提供了一种在发光装置的驱动期间显示出高亮度并且显示出较少亮度劣化的蓝色荧光体。 本发明是由通式aBaO.bSrO（1-a-b）EuO.cMgO.dAlO3 / 2eWO3表示的蓝色荧光体，其中0.70和nlE; a＆nlE; 0.95,0和nlE; b＆nlE; 0.15,0.95＆ c＆nlE; 1.15,9.00和nlE; d＆nlE; 11.00,0.001和nlE; e＆nlE; 0.100和a + b＆nlE; 0.97。 在这种蓝色荧光体中，其顶部位于衍射角2的范围内的两个峰位于13.0至13.6度的X射线衍射图中，其通过使用波长为0.774的X射线在蓝色荧光体上测量而获得 一个。
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公开(公告)号：US08410677B2
公开(公告)日：2013-04-02
申请号：US12595159
申请日：2008-03-25
CPC分类号： C09K11/7736 , H01J61/44 , H01J2211/42
摘要： The present invention provides a blue phosphor having high luminance and showing less luminance degradation during driving of a light-emitting device. The present invention is a blue phosphor that includes: an alkaline earth metal aluminate represented by a general formula aBaO.bSrO.(1−a−b)EuO.cMgO.dAlO3/2, where 0.70≦a≦0.95, 0≦b≦0.15, 0.95≦c≦1.15, 9.00≦d≦11.00, and a+b≦0.97 are satisfied; and 0.008 mol to 0.800 mol of MWO4 with respect to 1 mol of the aluminate, where M is at least one element selected from a group consisting of Ba, Sr, and Ca.
摘要翻译： 本发明提供一种具有高亮度的蓝色荧光体，并且在发光装置的驱动期间显示出较少的亮度劣化。 本发明是一种蓝色荧光体，其包括：由通式aBaO.bSrO（1-a-b）EuO·c·MgO·AlO 3/2表示的碱土金属铝酸盐，其中0.70和nlE; a＆nlE; 0.95,0和nlE; b＆ ; 0.15,0.95＆nlE; c＆nlE; 1.15,9.00＆amp; nlE; d＆nlE; 11.00和a + b＆nlE; 0.97; 和相对于1mol铝酸盐为0.008mol至0.800mol的MWO4，其中M为选自Ba，Sr和Ca中的至少一种元素。
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公开(公告)号：US08040063B2
公开(公告)日：2011-10-18
申请号：US12595174
申请日：2008-03-25
CPC分类号： C09K11/7736 , H01J11/12 , H01J11/42 , H01J61/44
摘要： The present invention provides a blue phosphor that exhibits high luminance and shows less luminance degradation during driving of a light-emitting device. The present invention is a blue phosphor represented by the general formula aBaO.bSrO.(1−a−b)EuO.cMgO.dAlO3/2.eWO3, where 0.70≦a≦0.95, 0≦b≦0.15, 0.95≦c≦1.15, 9.00≦d≦11.00, 0.001≦e≦0.100, and a+b≦0.97 are satisfied. In this blue phosphor, two peaks whose tops are located in a range of diffraction angle 2θ=13.0 to 13.6 degrees are present in an X-ray diffraction pattern obtained by measurement on the blue phosphor using an X-ray with a wavelength of 0.774 Å.
摘要翻译： 本发明提供了一种在发光装置的驱动期间显示出高亮度并且显示出较少亮度劣化的蓝色荧光体。 本发明是由通式aBaO.bSrO（1-a-b）EuO.cMgO.dAlO3 / 2eWO3表示的蓝色荧光体，其中0.70和nlE; a＆nlE; 0.95,0和nlE; b＆nlE; 0.15,0.95＆ c＆nlE; 1.15,9.00和nlE; d＆nlE; 11.00,0.001和nlE; e＆nlE; 0.100和a + b＆nlE; 0.97。 在这种蓝色荧光体中，其顶部位于衍射角2的范围内的两个峰位于13.0至13.6度的X射线衍射图中，其通过使用波长为0.774的X射线在蓝色荧光体上测量而获得 一个。
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公开(公告)号：US20100052506A1
公开(公告)日：2010-03-04
申请号：US12595159
申请日：2008-03-25
CPC分类号： C09K11/7736 , H01J61/44 , H01J2211/42
摘要： The present invention provides a blue phosphor having high luminance and showing less luminance degradation during driving of a light-emitting device. The present invention is a blue phosphor that includes: an alkaline earth metal aluminate represented by a general formula aBaO.bSrO.(1−a−b)EuO.cMgO.dAlO3/2, where 0.70≦a≦0.95, 0≦b≦0.15, 0.95≦c≦1.15, 9.00≦d≦11.00, and a+b≦0.97 are satisfied; and 0.008 mol to 0.800 mol of MWO4 with respect to 1 mol of the aluminate, where M is at least one element selected from a group consisting of Ba, Sr, and Ca.
摘要翻译： 本发明提供一种具有高亮度的蓝色荧光体，并且在发光装置的驱动期间显示出较少的亮度劣化。 本发明是一种蓝色荧光体，其包括：由通式aBaO.bSrO（1-a-b）EuO·c·MgO·AlO 3/2表示的碱土金属铝酸盐，其中0.70和nlE; a＆nlE; 0.95,0和nlE; b＆ ; 0.15,0.95＆nlE; c＆nlE; 1.15,9.00＆amp; nlE; d＆nlE; 11.00和a + b＆nlE; 0.97; 和相对于1mol铝酸盐为0.008mol至0.800mol的MWO4，其中M为选自Ba，Sr和Ca中的至少一种元素。
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公开(公告)号：US20100141113A1
公开(公告)日：2010-06-10
申请号：US12595174
申请日：2008-03-25
CPC分类号： C09K11/7736 , H01J11/12 , H01J11/42 , H01J61/44
摘要： The present invention provides a blue phosphor that exhibits high luminance and shows less luminance degradation during driving of a light-emitting device. The present invention is a blue phosphor represented by the general formula aBaO.bSrO.(1−a−b)EuO.cMgO.dAlO3/2.eWO3, where 0.70≦a≦0.95, 0≦b≦0.15, 0.95≦c≦1.15, 9.00≦d≦11.00, 0.001≦e≦0.100, and a+b≦0.97 are satisfied. In this blue phosphor, two peaks whose tops are located in a range of diffraction angle 2θ=13.0 to 13.6 degrees are present in an X-ray diffraction pattern obtained by measurement on the blue phosphor using an X-ray with a wavelength of 0.774 Å.
摘要翻译： 本发明提供了一种在发光装置的驱动期间显示出高亮度并且显示出较少亮度劣化的蓝色荧光体。 本发明是由通式aBaO.bSrO（1-a-b）EuO.cMgO.dAlO3 / 2eWO3表示的蓝色荧光体，其中0.70和nlE; a＆nlE; 0.95,0和nlE; b＆nlE; 0.15,0.95＆ c＆nlE; 1.15,9.00和nlE; d＆nlE; 11.00,0.001和nlE; e＆nlE; 0.100和a + b＆nlE; 0.97。 在这种蓝色荧光体中，其顶部位于衍射角2的范围内的两个峰位于13.0至13.6度的X射线衍射图中，其通过使用波长为0.774的X射线在蓝色荧光体上测量而获得 一个。
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