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公开(公告)号：WO2013015989A2
公开(公告)日：2013-01-31
申请号：PCT/US2012046202
申请日：2012-07-11
Applicant: UOP LLC , KALNES TOM N , CHEN JOHN Q , KOCAL JOSEPH A
Inventor： KALNES TOM N , CHEN JOHN Q , KOCAL JOSEPH A
CPC classification number: C07C29/132 , C07C31/20
Abstract: A catalytic process for generating at least one polyol from a feedstock comprising cellulose is performed in a continuous manner. The process involves, contacting, continuously, hydrogen, water, and a feedstock comprising cellulose, with a catalyst to generate an effluent stream comprising at least one polyol, water, hydrogen, and at least one co-product. The water, hydrogen, and at least one co-product are separated from the effluent stream and recycled to the reaction zone. The polyol is recovered from the effluent stream.
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公开(公告)号：WO2012012047A2
公开(公告)日：2012-01-26
申请号：PCT/US2011/040601
申请日：2011-06-16
Applicant: UOP LLC , BORESKOV INSTITUTE OF CATALYSIS , BHATTACHARYYA, Alakananda , KOCAL, Joseph, A. , WALENGA, Joel, T. , ADONIN, Nikolay, Y. , KUZNETSOVA, Nina, I. , BAL'ZHINIMAEV, Bair, S.
Inventor： BHATTACHARYYA, Alakananda , KOCAL, Joseph, A. , WALENGA, Joel, T. , ADONIN, Nikolay, Y. , KUZNETSOVA, Nina, I. , BAL'ZHINIMAEV, Bair, S.
CPC classification number: C07C51/265 , C07C51/42 , Y02P20/52 , Y02P20/542 , C07C63/26
Abstract: A solid terephthalic acid composition and a process for producing terephthalic acid from para-xylene. The process comprises forming a mixture comprising the para-xylene, a solvent, a bromine source, and a catalyst; and oxidizing the para-xylene by contacting the mixture with an oxidizing agent at oxidizing conditions to produce a solid oxidation product comprising terephthalic acid, para-toluic acid, 4-carboxybenzaldehyde. The solvent comprises a carboxylic acid having from 1 to 7 carbon atoms and an dialkyl imidazolium ionic liquid; and the catalyst comprises at least one of cobalt, titanium, manganese, chromium, copper, nickel, vanadium, iron, molybdenum, tin, cerium, and zirconium. The solid terephthalic acid composition comprises, less than about 4,000 ppm-
Abstract translation: 固体对苯二甲酸组合物和由对二甲苯制备对苯二甲酸的方法。 该方法包括形成包含对二甲苯，溶剂，溴源和催化剂的混合物; 并在氧化条件下使该混合物与氧化剂接触以氧化对二甲苯以产生包含对苯二甲酸，对甲苯甲酸，4-羧基苯甲醛的固体氧化产物。 溶剂包括具有1至7个碳原子的羧酸和二烷基咪唑离子液体; 催化剂包括钴，钛，锰，铬，铜，镍，钒，铁，钼，锡，铈和锆中的至少一种。 固体对苯二甲酸组合物包含小于约4,000ppm-
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公开(公告)号：WO2012012045A2
公开(公告)日：2012-01-26
申请号：PCT/US2011/040502
申请日：2011-06-15
Applicant: UOP LLC , BORESKOV INSTITUTE OF CATALYSIS , BHATTACHARYYA, Alakananda , KOCAL, Joseph, A. , WALENGA, Joel, T. , ADONIN, Nikolay, Y. , KUZNETSOVA, Nina, I. , BAL'ZHINIMAEV, Bair, S.
Inventor： BHATTACHARYYA, Alakananda , KOCAL, Joseph, A. , WALENGA, Joel, T. , ADONIN, Nikolay, Y. , KUZNETSOVA, Nina, I. , BAL'ZHINIMAEV, Bair, S.
CPC classification number: C07C51/265 , C07C63/16 , C07C63/24 , C07C63/26 , C07C63/06
Abstract: A process and a mixture for oxidizing an alkyl-aromatic compound comprises forming a mixture comprising the alkyl-aromatic compound, a solvent, a bromine source, and a catalyst; and contacting the mixture with an oxidizing agent at oxidizing conditions to produce an oxidation product comprising at least one of an aromatic aldehyde, an aromatic alcohol, an aromatic ketone, and an aromatic carboxylic acid. The solvent comprises a carboxylic acid having from 1 to 7 carbon atoms and an ionic liquid selected from the group consisting of an imidazolium ionic liquid, a pyridinium ionic liquid, a phosphonium ionic liquid, a tetra alkyl ammonium ionic liquid, and combinations thereof. The catalyst comprises at least one of cobalt, titanium, manganese, chromium, copper, nickel, vanadium, iron, molybdenum, tin, cerium, and zirconium.
Abstract translation: 用于氧化烷基 - 芳族化合物的方法和混合物包括形成包含烷基 - 芳族化合物，溶剂，溴源和催化剂的混合物; 以及在氧化条件下使所述混合物与氧化剂接触以产生包含芳族醛，芳族醇，芳族酮和芳族羧酸中的至少一种的氧化产物。 溶剂包括具有1至7个碳原子的羧酸和选自咪唑鎓离子液体，吡啶鎓离子液体，鏻离子液体，四烷基铵离子液体及其组合的离子液体。 催化剂包括钴，钛，锰，铬，铜，镍，钒，铁，钼，锡，铈和锆中的至少一种。
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24.发明申请LOW OXYGEN BIOMASS-DERIVED PYROLYSIS OILS AND METHODS FOR PRODUCING THE SAME 审中-公开低氧生物质衍生的热解油及其生产方法
公开(公告)号：WO2011103047A3
公开(公告)日：2011-12-08
申请号：PCT/US2011024688
申请日：2011-02-14
Applicant: UOP LLC , KOCAL JOSEPH A , MARINANGELI RICHARD , LUPTON FRANCIS STEPHEN , KING LISA
Inventor： KOCAL JOSEPH A , MARINANGELI RICHARD , LUPTON FRANCIS STEPHEN , KING LISA
CPC classification number: C10G3/45 , C01B3/12 , C01B3/323 , C01B3/38 , C01B2203/0233 , C01B2203/0283 , C01B2203/1211 , C01B2203/1241 , C10B49/22 , C10B53/02 , C10B57/06 , C10C5/00 , C10G3/50 , C10G2300/1011 , Y02E50/14 , Y02P20/145 , Y02P30/20
Abstract: Methods are provided for producing low oxygen biomass-derived pyrolysis oil from carbonaceous biomass feedstock. The carbonaceous biomass feedstock is pyrolyzed in the presence of a steam reforming catalyst to produce char and pyrolysis gases. During pyrolysis, a portion of the oxygenated hydrocarbons in the pyrolysis gases is converted into hydrocarbons by steam reforming also yielding carbon oxides and hydrogen gas. The hydrogen gas at least partially deoxygenates a residual portion of the oxygenated hydrocarbons. Additional hydrogen gas may also be produced by water-gas shift reactions to deoxygenate the residual portion of the oxygenated hydrocarbons in the pyrolysis gases. Deoxygenation may occur in the presence of a hydroprocessing catalyst. A condensable portion of the pyrolysis gases is condensed to form low oxygen biomass-derived pyrolysis oil.
Abstract translation: 提供用于从含碳生物质原料生产低氧生物质衍生的热解油的方法。 碳水生物质原料在蒸汽重整催化剂存在下热解生成焦炭和裂解气。 在热解过程中，热分解气体中的一部分氧化烃通过也可产生碳氧化物和氢气的蒸汽重整转化为烃。 氢气至少部分地使氧化烃的残留部分脱氧。 还可以通过水煤气变换反应产生另外的氢气，以使热解气体中的氧化烃的残余部分脱氧。 脱氧可能在加氢处理催化剂存在下进行。 热解气体的可冷凝部分被冷凝以形成低氧生物质衍生的热解油。
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公开(公告)号：WO2011090616A2
公开(公告)日：2011-07-28
申请号：PCT/US2010060718
申请日：2010-12-16
Applicant: UOP LLC , BHATTACHARYYA ALAKANANDA , SERBAN MANUELA , MEZZA BECKAY J , VANDEN BUSSCHE KURT M , NICHOLAS CHRISTOPHER P , KOCAL JOSEPH A , BENNION WARREN K
Inventor： BHATTACHARYYA ALAKANANDA , SERBAN MANUELA , MEZZA BECKAY J , VANDEN BUSSCHE KURT M , NICHOLAS CHRISTOPHER P , KOCAL JOSEPH A , BENNION WARREN K
CPC classification number: C10G21/08 , B01D11/043 , B01D11/0492 , C10G21/28 , C10G2300/1074 , C10G2300/206 , C10G2300/4081 , C10G2300/805 , C10G2400/06
Abstract: A process for removing a metal from a vacuum gas oil feed includes contacting the vacuum gas oil feed comprising the metal with a VGO-immiscible ionic liquid to produce a vacuum gas oil and VGO-immiscible ionic liquid mixture, and separating the mixture to produce a vacuum gas oil effluent having a reduced metal content relative to the vacuum gas oil feed.
Abstract translation: 从真空瓦斯油原料中除去金属的方法包括使包含金属的减压瓦斯油原料与VGO不溶混离子液体接触以产生真空瓦斯油和VGO不溶混性离子液体混合物，并分离该混合物以产生 相对于真空瓦斯油原料具有降低的金属含量的真空瓦斯油流出物。
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Patent Agency Ranking26.发明申请SELECTIVE OXIDATION AGENT OF HYDROCARBONS TO SYNTHESIS GAS BASED ON SEPARATE PARTICLES OF O-CARRIER AND HYDROCARBON ACTIVATOR 审中-公开选择性氧化剂基于O载体和碳氢化合物的分离颗粒合成气体
公开(公告)号：WO2009064591A3
公开(公告)日：2009-08-13
申请号：PCT/US2008080710
申请日：2008-10-22
Applicant: UOP LLC , JAN DENG-YANG , WALENGA JOEL T , VANDEN BUSSCHE KURT M , KOCAL JOSEPH A , KING LISA M
Inventor： JAN DENG-YANG , WALENGA JOEL T , VANDEN BUSSCHE KURT M , KOCAL JOSEPH A , KING LISA M
IPC: B01J23/00
CPC classification number: C01B13/0203 , C01B3/386 , C01B2203/0261 , C01B2203/0805 , C01B2203/0866 , C01B2203/1047 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1094 , C01B2203/1241 , Y02P20/52
Abstract: A solid material is presented for the partial oxidation of natural gas. The solid material includes a solid oxygen carrying agent and a hydrocarbon activation agent. The material precludes the need for gaseous oxygen for the partial oxidation and provides better control over the reaction.
Abstract translation: 提供固体材料用于天然气的部分氧化。 固体材料包括固体氧气载体和烃活化剂。 该材料排除了对氧气进行部分氧化的需要，并提供对反应的更好控制。
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公开(公告)号：WO2013015997A3
公开(公告)日：2013-01-31
申请号：PCT/US2012/046348
申请日：2012-07-12
Applicant: UOP LLC , DALIAN INSTITUTE OF CHEMICAL PHYSICS , ZHANG, Tao , WANG, Aiqin , ZHENG, Mingyuan , LI, Changzhi , PANG, Jifeng , KALNES, Tom N. , CHEN, John Q. , KOCAL, Joseph A.
Inventor： ZHANG, Tao , WANG, Aiqin , ZHENG, Mingyuan , LI, Changzhi , PANG, Jifeng , KALNES, Tom N. , CHEN, John Q. , KOCAL, Joseph A.
Abstract: A catalytic process for generating at least one polyol from a feedstock comprising cellulose is performed in a continuous manner using a catalyst comprising nickel tungsten carbide. The process involves, contacting, continuously, hydrogen, water, and a feedstock comprising cellulose, with the catalyst to generate an effluent stream comprising at least one polyol and recovering the polyol from the effluent stream.
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公开(公告)号：WO2012091899A1
公开(公告)日：2012-07-05
申请号：PCT/US2011/064347
申请日：2011-12-12
Applicant: UOP LLC , KOCAL, Joseph A.
Inventor： KOCAL, Joseph A.
Abstract: Methods are disclosed for producing, from renewable carbon sources, acetic acid in an economical manner. In particular, these methods are directed to the separation and recovery of acetic acid as a substantial product (e.g., as much as 5% by weight or more) of biomass pyrolysis. For a given commercial biomass pyrolysis unit, the acetic acid yield can represent a significant quantity of that used in a major industrial applications such as purified terephthalic acid (PTA) production. According to some embodiments, pyrolysis conditions and/or flow schemes advantageously improve the recovery of acetic acid for a given purity level.
Abstract translation: 公开了从可再生碳源以经济的方式生产乙酸的方法。 特别地，这些方法涉及作为生物质热解的实质产物（例如多达5重量％以上）的乙酸的分离和回收。 对于给定的商业生物质热解单元，乙酸产率可以代表在主要工业应用中使用的显着量，例如纯化的对苯二甲酸（PTA）生产。 根据一些实施方案，热解条件和/或流程方案有利地改善了给定纯度水平下乙酸的回收率。
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公开(公告)号：WO2012012048A3
公开(公告)日：2012-04-19
申请号：PCT/US2011040602
申请日：2011-06-16
Applicant: UOP LLC , BORESKOVA INST KATALIZA SIBIR , BHATTACHARYYA ALAKANANDA , KOCAL JOSEPH A , WALENGA JOEL T , ADONIN NIKOLAY Y , KUZNETSOVA NINA I , BAL ZHINIMAEV BAIR S
Inventor： BHATTACHARYYA ALAKANANDA , KOCAL JOSEPH A , WALENGA JOEL T , ADONIN NIKOLAY Y , KUZNETSOVA NINA I , BAL ZHINIMAEV BAIR S
CPC classification number: C07C51/265 , C07C51/43 , C07C63/26
Abstract: A solid terephthalic acid composition and a process for producing terephthalic acid from para-xylene. The process comprises forming a mixture comprising the para-xylene, a solvent, a bromine source, and a catalyst; and oxidizing the para-xylene by contacting the mixture with an oxidizing agent at oxidizing conditions to produce a solid oxidation product comprising terephthalic acid, para-toluic acid, 4-carboxybenzaldehyde. The solvent comprises a carboxylic acid having from 1 to 7 carbon atoms and an dialkyl imidazolium ionic liquid; and the catalyst comprises at least one of cobalt, titanium, manganese, chromium, copper, nickel, vanadium, iron, molybdenum, tin, cerium, and zirconium. The solid terephthalic acid composition comprises, less than about 4,000 ppm-wt 4-carboxybenzaldehyde content, and more than about 2,000 ppm-wt a para-toluic acid.
Abstract translation: 固体对苯二甲酸组合物和由对二甲苯生产对苯二甲酸的方法。 该方法包括形成包含对二甲苯，溶剂，溴源和催化剂的混合物; 并通过在氧化条件下将氧化剂与氧化剂接触来氧化对二甲苯以产生包含对苯二甲酸，对甲苯甲酸，4-羧基苯甲醛的固体氧化产物。 溶剂包括具有1至7个碳原子的羧酸和二烷基咪唑鎓离子液体; 催化剂包括钴，钛，锰，铬，铜，镍，钒，铁，钼，锡，铈和锆中的至少一种。 固体对苯二甲酸组合物包含小于约4,000ppm重量的4-羧基苯甲醛含量和大于约2,000ppm重量的对甲苯甲酸。
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公开(公告)号：WO2012012046A3
公开(公告)日：2012-04-12
申请号：PCT/US2011040515
申请日：2011-06-15
Applicant: UOP LLC , BORESKOVA INST KATALIZA SIBIR , BHATTACHARYYA ALAKANANDA , KOCAL JOSEPH A , WALENGA JOEL T , ADONIN NIKOLAY Y , KUZNETSOVA NINA I , BAL ZHINIMAEV BAIR S
Inventor： BHATTACHARYYA ALAKANANDA , KOCAL JOSEPH A , WALENGA JOEL T , ADONIN NIKOLAY Y , KUZNETSOVA NINA I , BAL ZHINIMAEV BAIR S
CPC classification number: C07C51/265 , C07C63/06 , C07C63/16 , C07C63/26
Abstract: A process and a mixture for oxidizing an alkyl-aromatic compound comprises forming a mixture comprising the alkyl-aromatic compound, a solvent, a bromine source, and a catalyst; and contacting the mixture with an oxidizing agent at oxidizing conditions to produce an oxidation product comprising at least one of an aromatic aldehyde, an aromatic alcohol, an aromatic ketone, and an aromatic carboxylic acid. The solvent comprises a carboxylic acid having from 1 to 7 carbon atoms and an ionic liquid selected from the group consisting of an imidazolium ionic liquid, a pyridinium ionic liquid, a phosphonium ionic liquid, a tetra alkyl ammonium ionic liquid, and combinations thereof. The catalyst comprises at least one of cobalt, titanium, manganese, chromium, copper, nickel, vanadium, iron, molybdenum, tin, cerium, and zirconium.
Abstract translation: 用于氧化烷基芳族化合物的方法和混合物包括形成包含烷基芳族化合物，溶剂，溴源和催化剂的混合物; 以及在氧化条件下使混合物与氧化剂接触以产生包含芳族醛，芳族醇，芳族酮和芳族羧酸中的至少一种的氧化产物。 溶剂包含具有1至7个碳原子的羧酸和选自由咪唑鎓离子液体，吡啶鎓离子液体，鏻离子液体，四烷基铵离子液体及其组合组成的组的离子液体。 催化剂包含钴，钛，锰，铬，铜，镍，钒，铁，钼，锡，铈和锆中的至少一种。
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