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21.发明授权公开(公告)号：US08444951B2
公开(公告)日：2013-05-21
申请号：US12924876
申请日：2010-10-06
IPC分类号： C01B3/26
CPC分类号： B01F3/04049 , B01D2253/112 , B01D2257/304 , B01F5/045 , B01J8/0214 , B01J8/0221 , B01J8/0278 , B01J8/0285 , B01J8/043 , B01J2208/00203 , B01J2208/0053 , B01J2208/00646 , B01J2208/00716 , C01B3/382 , C01B2203/0244 , C01B2203/0455 , C01B2203/0485 , C01B2203/0894 , C01B2203/1276 , F01N2240/30 , F02M25/12 , F02M27/02 , F02M31/125 , Y02T10/121 , Y02T10/126
摘要： The present invention provides a process and apparatus for the gasification of a liquid fuel and includes providing a supply of a liquid fuel, a supply of oxidant, and a supply of liquid water; atomizing the liquid fuel and mixing it with the oxidant and steam; catalytically reacting the fuel-oxidant-steam mixture in a catalyst bed; initiating the catalytic reaction with an ignition source; positioning a heat exchanger in proximity with the catalyst bed so as to convert the liquid water to steam; and feeding the steam into the catalytic reaction, thereby eliminating the need for a liquid fuel vaporizer. A preferred catalyst bed includes an ultra-short-channel-length metal substrate.
摘要翻译： 本发明提供一种用于液化燃料气化的方法和装置，包括提供液体燃料，氧化剂供应和液态水的供应; 雾化液体燃料并将其与氧化剂和蒸汽混合; 在催化剂床中催化反应燃料 - 氧化剂 - 蒸汽混合物; 引发与点火源的催化反应; 将热交换器定位在催化剂床附近，以便将液态水转化成蒸汽; 并将蒸汽进料到催化反应中，从而不再需要液体燃料蒸发器。 优选的催化剂床包括超短通道长度的金属基材。
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公开(公告)号：US08337757B2
公开(公告)日：2012-12-25
申请号：US12322970
申请日：2009-02-09
申请人： Subir Roychoudhury , Joel M. Desjardins , David Spence , Richard Mastanduno , Dennis E. Walsh , William C. Pfefferle
发明人： Subir Roychoudhury , Joel M. Desjardins , David Spence , Richard Mastanduno , Dennis E. Walsh , William C. Pfefferle
IPC分类号： G05B13/00
CPC分类号： C01B3/26 , C10J3/723 , C10J2200/06 , G05D23/1931 , Y10T436/207497 , Y10T436/218
摘要： A method is provided for controlling the operating temperature of a catalytic reactor using a closed-loop system that provides for varying the reactor input and other operating parameters in order to maintain the operating temperature of the reactor at or near the initial setpoint temperature for operation of the reactor. In one example, maximum and minimum operating temperatures with a catalytic partial oxidation reactor are controlled, as well as maintaining control over the corresponding minimum required ratio of oxygen atoms to carbon atoms, such that the operating temperature within the reactor is maintained below the material limits but above threshold temperatures for coking.
摘要翻译： 提供了一种用于使用闭环系统来控制催化反应器的操作温度的方法，所述闭环系统提供改变反应器输入和其它操作参数，以便将反应器的操作温度保持在或接近初始设定点温度，以操作 反应堆。 在一个实例中，控制具有催化部分氧化反应器的最大和最小操作温度，以及保持对氧原子与碳原子的相应最小所需比例的控制，使得反应器内的操作温度保持在材料极限以下 但高于焦化阈值温度。
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23.发明授权Process for oxidative conversion of methane to higher hydrocarbons using metal sulfide oxidizing agent 失效使用金属硫化物氧化剂将甲烷氧化转化成高级烃的方法
公开(公告)号：US5191138A
公开(公告)日：1993-03-02
申请号：US794560
申请日：1991-11-19
IPC分类号： C07C2/82
CPC分类号： C07C2/82 , Y10S585/943
摘要： There is provided a process for converting methane to hydrocarbons having at least two carbon atoms (i.e. higher hydrocarbons). The process involves oxidizing methane with a metal sulfide oxidizing agent. After this conversion of methane, the reduced metal sulfide may be regenerated by oxidation of the reduced metal sulfide.
摘要翻译： 提供了将甲烷转化为具有至少两个碳原子的烃（即高级烃）的方法。 该方法涉及用金属硫化物氧化剂氧化甲烷。 在甲烷转化后，还原的金属硫化物可以通过还原的金属硫化物的氧化再生。
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公开(公告)号：US5105044A
公开(公告)日：1992-04-14
申请号：US597220
申请日：1990-10-15
IPC分类号： C07C2/84
CPC分类号： C07C2/84 , C07C2523/06 , C07C2523/34 , Y10S585/943
摘要： There is provided a catalyst and a process for the direct partial oxidation of methane with oxygen, whereby hydrocarbons having at least two carbon atoms are produced. The catalyst used in this reaction is a spinel oxide, such as MgMn.sub.2 O.sub.4 or CaMn.sub.2 O.sub.4, modified with an alkali metal, such as Li or Na.
摘要翻译： 提供了用氧气直接部分氧化甲烷的催化剂和方法，由此产生具有至少两个碳原子的烃。 在该反应中使用的催化剂是用碱金属如Li或Na改性的尖晶石氧化物，例如MgMn 2 O 4或CaMn 2 O 4。
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25.发明授权
公开(公告)号：US5068486A
公开(公告)日：1991-11-26
申请号：US597221
申请日：1990-10-15
IPC分类号： C07C2/82
CPC分类号： C07C2/82 , Y10S585/943
摘要： There is provided a process for converting methane to hydrocarbons having at least two carbon atoms. The process involves contacting methane with an oxidizing agent, such as oxygen, at a relatively moderate temperature of less than about 700.degree. C. and a relatively high pressure of greater than about 20 atmospheres.
摘要翻译： 提供了将甲烷转化为具有至少两个碳原子的烃的方法。 该方法包括在低于约700℃的相对中等温度和大于约20个大气压的较高压力下使甲烷与氧化剂（例如氧）接触。
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公开(公告)号：US5023393A
公开(公告)日：1991-06-11
申请号：US454534
申请日：1989-12-21
CPC分类号： C07C2/84 , C07C29/50 , C07C2529/46 , Y10S585/943
摘要： There is provided a process for the direct partial oxidation of methane with oxygen, whereby organic compounds comprising higher hydrocarbons are produced. The catalyst used in this reaction is an NiZSM-5 catalyst. This catalyst may be prepared by ion exchanging or impregnating a ZSM-5 catalyst with a suitable nickel salt such as nickel nitrate.
摘要翻译： 提供了用氧直接部分氧化甲烷的方法，由此产生包含高级烃的有机化合物。 在该反应中使用的催化剂是NiZSM-5催化剂。 该催化剂可以通过用合适的镍盐如硝酸镍离子交换或浸渍ZSM-5催化剂来制备。
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公开(公告)号：US5004856A
公开(公告)日：1991-04-02
申请号：US459218
申请日：1989-12-29
CPC分类号： C07C2/84 , B01J23/34 , C07C2523/06 , C07C2523/34 , Y10S585/943
摘要： There is provided a process for the direct partial oxidation of methane with oxygen, whereby hydrocarbons having at least two carbon atoms are produced. The catalyst used in this reaction is a cadmium-manganese oxide catalyst.
摘要翻译： 提供了用氧直接部分氧化甲烷的方法，由此产生具有至少两个碳原子的烃。 该反应中使用的催化剂是镉 - 锰氧化物催化剂。
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公开(公告)号：US4877581A
公开(公告)日：1989-10-31
申请号：US239257
申请日：1988-09-01
申请人： Nai Y. Chen , Dennis E. Walsh
发明人： Nai Y. Chen , Dennis E. Walsh
摘要： A paraffin conversion process for hydroisomerizing a nitrogen and wax-containing hydrocarbon feedstock comprising contacting the feedstock with a catalyst including a ZSM-11 zeolite characterized by an alpha value from about 10 to 50, in combination with a Group VIII metal hydrogenation-dehydrogenation component of platinum or palladium at a temperature of about 400.degree. F. to about 850.degree. F. and at a pressure of from about 200 to about 2000 psig.
摘要翻译： 一种用于使含氮和含蜡的烃原料加氢异构化的链烷烃转化方法，包括使原料与包含Z值为约10至50的α值的ZSM-11沸石的催化剂结合，与第VIII族金属加氢脱氢组分 铂或钯，温度为约400°F至约850°F，压力为约200至约2000psig。
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29.发明授权
公开(公告)号：US4515092A
公开(公告)日：1985-05-07
申请号：US569816
申请日：1984-01-11
申请人： Dennis E. Walsh , Gary J. Green
发明人： Dennis E. Walsh , Gary J. Green
CPC分类号： F23C13/00 , F23C10/002
摘要： A combustion enhancing catalyst is deposited on a particulate refractory substrate such as sand. The solid fuel is contacted with the impregnated substrate and burned, for example, in a fluidized bed combustor. The substrate and catalyst remains in the combustor thereby obviating problems of catalyst loss and adverse effects of emitted metal particles.
摘要翻译： 燃烧增强催化剂沉积在颗粒耐火基材如砂上。 固体燃料与浸渍的基材接触并在例如流化床燃烧器中燃烧。 衬底和催化剂保留在燃烧器中，从而消除了催化剂损失和发射的金属颗粒的不利影响的问题。
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公开(公告)号：US09102531B2
公开(公告)日：2015-08-11
申请号：US13613153
申请日：2012-09-13
申请人： Subir Roychoudhury , Joel M DesJardins , David Spence , Richard Mastanduno , Dennis E. Walsh , Lisa Burns
发明人： Subir Roychoudhury , Joel M DesJardins , David Spence , Richard Mastanduno , Dennis E. Walsh , William C. Pfefferle
CPC分类号： C01B3/26 , C10J3/723 , C10J2200/06 , G05D23/1931 , Y10T436/207497 , Y10T436/218
摘要： A method is provided for controlling the operating temperature of a catalytic reactor using a closed-loop system that provides for varying the reactor input and other operating parameters in order to maintain the operating temperature of the reactor at or near the initial setpoint temperature for operation of the reactor. In one example, maximum and minimum operating temperatures with a catalytic partial oxidation reactor are controlled, as well as maintaining control over the corresponding minimum required ratio of oxygen atoms to carbon atoms, such that the operating temperature within the reactor is maintained below the material limits but above threshold temperatures for coking.
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