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公开(公告)号：US4895638A
公开(公告)日：1990-01-23
申请号：US339284
申请日：1989-04-17
摘要： A process for the catalytic cracking of heavy petroleum fractions into lower hydrocarbons, such as fuel products. The process comprises contacting the petroleum fractions at an elevated temperature with a cracking catalyst comprising (a) a layered metal oxide of the titanometallate type intercalated with an interspathic polymeric chalcogenide, e.g., polymeric silica and, optionally (b) a porous crystalline silicate component such as a large pore zeolite material.
摘要翻译： 将重质石油馏分催化裂化成低级烃，如燃料产品的方法。 该方法包括在升高的温度下使石油馏分与裂解催化剂接触，所述裂化催化剂包含（a）层状金属氧化物，金属螯合物层状金属氧化物，其插入有间位聚合硫属化物，例如聚合二氧化硅，和任选地（b）多孔结晶硅酸盐组分， 作为大孔沸石材料。
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52.发明授权Catalysts comprising silica supported on alumina, their preparation and use 失效包含负载在氧化铝上的二氧化硅的催化剂，其制备和用途
公开(公告)号：US4778779A
公开(公告)日：1988-10-18
申请号：US37506
申请日：1987-04-13
摘要： Useful cracking catalysts and catalyst supports comprising silica supported on alumina are prepared by compositing particles of silica or silica precursor with particles of porous alumina and subjecting the resulting composite to high temperature steaming in a non-reducing environment at a temperature of at least about 500.degree. C. for a time sufficient to disperse at least a portion of the silica over the alumina surface. The silica wets, spreads out and reactions with the surface hydroxyul groups of the alumina. The supported silica on alumina composites that can be made from this process may exhibit properties of both bulk silica and bulk alumina at the same time, bulk silica and alumina whose exterior surface only has been modified with silica as wells as composites exhibiting surface properties different from both bulk silica and bulk alumina.
摘要翻译： 通过将二氧化硅或二氧化硅前体的颗粒与多孔氧化铝的颗粒合成，并将所得的复合材料在至少约500℃的非还原性环境中进行高温蒸汽来制备包含负载在氧化铝上的二氧化硅的有用的裂解催化剂和催化剂载体 在足以在氧化铝表面上分散二氧化硅的至少一部分的时间。 二氧化硅湿润，扩散和与氧化铝的表面羟基的反应。 可以由该方法制备的负载二氧化硅的氧化铝复合材料可以同时显示本体二氧化硅和本体氧化铝的本体二氧化硅和氧化铝的性质，其外表面仅仅用二氧化硅作为表面改性的复合材料，表现出与 本体二氧化硅和体积氧化铝。
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公开(公告)号：US4728635A
公开(公告)日：1988-03-01
申请号：US848955
申请日：1986-04-07
IPC分类号： B01D53/50 , B01D53/81 , B01D53/86 , B01J23/00 , B01J23/10 , B01J23/22 , C01F7/16 , C10G11/04 , B01J21/04 , B01J23/02
CPC分类号： C01F7/162 , B01J23/005 , B01J23/10 , B01J23/22 , C10G11/04 , C01P2006/12 , C01P2006/21 , Y10S502/524
摘要： A process for the production of an alkaline earth metal, aluminum-containing spinel composition comprises: (a) combining (1) an acidic, aluminum-containing composition in which the aluminum is present in a positively charged species, and (2) a basic, alkaline earth metal-containing composition to form a mixture; and (b) calcining the mixture to form the alkaline earth metal, aluminum-containing spinel composition. Alkaline earth metal, aluminum-containing spinels having both high surface areas and high attrition resistance, and processes for using spinel compositions, e.g., as sulfur oxide and nitrogen oxide removal agent, are also disclosed.
摘要翻译： 一种制备碱土金属的含铝尖晶石组合物的方法包括：（a）将（1）其中铝以带正电的物质存在的酸性含铝组合物和（2）碱性 ，含碱土金属的组合物以形成混合物; 和（b）煅烧该混合物以形成碱土金属的含铝尖晶石组合物。 还公开了具有高表面积和高耐磨性的碱土金属，含铝尖晶石，以及使用尖晶石组合物如硫氧化物和氮氧化物去除剂的方法。
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公开(公告)号：US4698321A
公开(公告)日：1987-10-06
申请号：US763514
申请日：1985-08-08
申请人： Allan S. Myerson , William R. Ernst
发明人： Allan S. Myerson , William R. Ernst
摘要： Regeneration of HDS catalysts by sulfiding under controlled conditions and leaching the sulfided catalyst with an acidic aqueous ferric ion containing solution to remove contaminating nickel and vanadium compounds and recovering catalyst of increased BET surface area and pore diameter.
摘要翻译： 在控制条件下通过硫化再生HDS催化剂，并用含酸性含铁离子的溶液浸提硫化催化剂以除去污染的镍和钒化合物并回收增加的BET表面积和孔径的催化剂。
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公开(公告)号：US4668655A
公开(公告)日：1987-05-26
申请号：US840240
申请日：1986-03-17
申请人： Paul H. Lewis , Eugene P. Dai , Edward H. Holst
发明人： Paul H. Lewis , Eugene P. Dai , Edward H. Holst
CPC分类号： B01D53/8609 , B01J23/02 , B01J23/10 , C10G11/04
摘要： A catalyst composition for catalytic cracking contains a catalytic cracking catalyst and 1-10 weight %, of the total, of additive containing a porous refractory support bearing 0.5-10 weight % of at least one of bismuth, chromium or a rare earth metal and 0.4-10 weight % of an alkali metal.
摘要翻译： 用于催化裂化的催化剂组合物含有催化裂化催化剂，总共含有1-10重量％的添加剂，该添加剂含有0.5-10重量％的铋，铬或稀土金属中的至少一种的多孔耐火材料支撑体和0.4 -10重量％的碱金属。
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公开(公告)号：US4664779A
公开(公告)日：1987-05-12
申请号：US840228
申请日：1986-03-17
申请人： Brent J. Bertus , Dwight L. McKay , H. Wayne Mark
发明人： Brent J. Bertus , Dwight L. McKay , H. Wayne Mark
CPC分类号： C10G11/04 , B01J29/06 , B01J29/90 , B01J2229/34 , B01J2229/40 , Y10S502/521
摘要： A method to restore the activity of a cracking catalyst which has been deactivated at least partially by metals contamination which involves contacting the cracking catalyst with an aluminum containing treating agent.
摘要翻译： 一种恢复至少部分被金属污染物去除的裂化催化剂的活性的方法，所述金属污染包括使裂化催化剂与含铝处理剂接触。
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公开(公告)号：US4595772A
公开(公告)日：1986-06-17
申请号：US672558
申请日：1984-11-19
CPC分类号： C10G11/04 , C07F9/902 , Y10S502/521
摘要： Novel organic water-soluble antimony compounds are prepared by reacting an alkanolamine with a hydroxycarboxylic acid to form an intermediate product and then reacting the intermediate product with an antimony oxide. These compounds are useful for use as catalyst metal poison passivators.
摘要翻译： 通过使烷醇胺与羟基羧酸反应形成中间产物，然后使中间产物与氧化锑反应制备新的有机水溶性锑化合物。 这些化合物可用作催化剂金属毒物钝化剂。
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公开(公告)号：US4535066A
公开(公告)日：1985-08-13
申请号：US585667
申请日：1984-03-02
CPC分类号： C10G11/04 , B01J21/20 , B01J23/18 , B01J29/076 , Y10S502/521
摘要： A cracking catalyst used to crack oil to produce gasoline or higher-boiling hydrocarbon fuel is contacted with both (A) antimony or a compound thereof such as antimony tris(0,0-dipropyl phosphorodithioate) and (B) a modifying composition consisting essentially of carbon, hydrogen, nitrogen, and sulfur produced by the treatment of a metal salt of a dialkyl dithiocarbamate with a hydrolyzable germanium (IV) compound such as germanium tetrachloride, the contacting of the catalyst with (A) and (B) prior to, during, or after use of the catalyst in a cracking process being effective in precluding or reducing adverse effects of metals such as nickel, vanadium, and iron.
摘要翻译： 用于裂解油以生产汽油或高沸点烃燃料的裂化催化剂与（A）锑或其化合物（例如三（0-二丙基二硫代磷酸锑））和（B）基本上由 通过用可水解的锗（IV）化合物如四氯化锗处理二烷基二硫代氨基甲酸金属盐产生的碳，氢，氮和硫，催化剂与（A）和（B）之间的催化剂在 或者在裂化过程中使用催化剂有效地排除或减少金属如镍，钒和铁的不利影响。
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公开(公告)号：US4504379A
公开(公告)日：1985-03-12
申请号：US525787
申请日：1983-08-23
CPC分类号： C10G11/04 , Y10S502/521
摘要： A method for passivating metal contaminants present in a hydrocarbon feedstock which become deposited on cracking catalyst is described. The method is directed at passing the cracking catalyst through a passivation zone having a reducing atmosphere maintained at an elevated temperature. The reducing atmosphere comprises a process reducing gas stream which has been passed through a guard bed adapted to selectively remove an unsaturated hydrocarbon prior to the process reducing gas being added to the passivation zone.
摘要翻译： 描述了一种钝化沉积在裂化催化剂上的烃原料中存在的金属污染物的方法。 该方法涉及使裂化催化剂通过具有保持在高温下的还原气氛的钝化区。 还原气氛包括一种工艺还原气流，其已经通过适合于选择性除去不饱和烃的保护床，在还原气体被加入钝化区之前。
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公开(公告)号：US4495304A
公开(公告)日：1985-01-22
申请号：US494604
申请日：1983-05-16
申请人： Jin S. Yoo , John A. Jaecker
发明人： Jin S. Yoo , John A. Jaecker
CPC分类号： C10G11/04 , B01J21/005 , B01J23/005 , B01J37/04
摘要： An improved process for converting hydrocarbons using a catalyst which is periodically regenerated to remove carbonaceous deposits, the catalyst being comprised of a mixture containing, as a major component, solid particles capable of promoting hydrocarbon conversion at hydrocarbon conversion conditions, and, as a minor component, discrete entities comprising at least one spinel, preferably alkaline earth metal-containing spinel; thereby reducing the amount of sulfur oxides exiting the catalyst regeneration zone.Improved hydrocarbon conversion catalysts are also disclosed.
摘要翻译： 一种使用周期性再生以除去含碳沉积物的催化剂转化烃的改进方法，该催化剂由含有作为主要组分的能够在烃转化条件下促进烃转化的固体颗粒和作为次要组分的混合物 包括至少一种尖晶石，优选含碱土金属的尖晶石的离散实体; 从而减少离开催化剂再生区的硫氧化物的量。 还公开了改进的烃转化催化剂。
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