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公开(公告)号：US09255227B2
公开(公告)日：2016-02-09
申请号：US12518616
申请日：2007-11-20
申请人： Finn Joensen , Poul Erik Højlund Nielsen , Niels Christian Schiødt , Ton V. W. Janssens , Bodil Voss
发明人： Finn Joensen , Poul Erik Højlund Nielsen , Niels Christian Schiødt , Ton V. W. Janssens , Bodil Voss
CPC分类号： C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2300/805 , C10G2400/02 , C10G2400/20 , Y02P30/20
摘要： Process for the synthesis of hydrocarbon constituents of gasoline comprising catalytic conversion in a gasoline synthesis step of an oxygenate-containing feed comprising methanol and/or dimethyl ether and a mixture of at least on a total oxygenate basis 0.05 wt % C3+ higher alcohols and/or their oxygenate equivalents to hydrocarbon constituents of gasoline.
摘要翻译： 在包含甲醇和/或二甲醚的含氧化合物进料的汽油合成步骤和至少在总含氧化合物基础上的混合物，基于0.05重量％的C3 +高级醇和/或 它们的含氧化合物等同于汽油的烃成分。
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公开(公告)号：US08677762B2
公开(公告)日：2014-03-25
申请号：US12674272
申请日：2008-08-13
IPC分类号： F02C6/18
CPC分类号： C07C29/1518 , C07C41/01 , C10G3/42 , C10G2300/1022 , C10G2400/02 , Y02E20/14 , Y02P30/20 , C07C31/04 , C07C43/043
摘要： A process for the preparation of hydrocarbon products and for the generation of power that includes the steps of (a) providing a synthesis gas having a hydrogen to carbon monoxide ratio of between 0.1 and 1; (b) contacting the synthesis gas with one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates comprising methanol and dimethyl ether with a dimethyl ether to methanol ratio of higher than 2 and a carbon dioxide content of above 20 mole %; (c) contacting the carbon dioxide containing oxygenate mixture at an inlet temperature of between 240° and 4000° C. with a catalyst being active in the conversion of oxygenate to higher hydrocarbons and a tail gas being rich in carbon dioxide; (d) combusting the carbon dioxide rich tail gas in a gas turbine combustion chamber to flue gas; and (e) expanding the flue gas stream through a gas turbine for the generation of power.
摘要翻译： 一种用于制备烃产物和产生动力的方法，包括以下步骤：（a）提供氢与一氧化碳比为0.1至1的合成气; （b）使合成气与一种或多种催化剂接触，这些催化剂一起催化氢和一氧化碳与包含甲醇和二甲醚的含氧化合物的反应，甲醚与甲醇的比例高于2，二氧化碳含量高于20摩尔％ ; （c）在240℃和4000℃之间的入口温度下与含氧化合物混合物的接触与在含氧化合物转化为高级烃和富含二氧化碳的尾气中具有活性的催化剂接触; （d）将燃气轮机燃烧室中的富含二氧化碳的尾气燃烧成烟道气; 和（e）通过用于发电的燃气轮机扩大烟气流。
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公开(公告)号：US20110314834A1
公开(公告)日：2011-12-29
申请号：US12674272
申请日：2008-08-13
IPC分类号： F02C6/18
CPC分类号： C07C29/1518 , C07C41/01 , C10G3/42 , C10G2300/1022 , C10G2400/02 , Y02E20/14 , Y02P30/20 , C07C31/04 , C07C43/043
摘要： A process for the preparation of hydrocarbon products and for the generation of power comprising the steps of (a) providing a synthesis gas having a hydrogen to carbon monoxide ratio of between 0.1 and 1; (b) contacting the synthesis gas with one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates comprising methanol and dimethyl ether with a dimethyl ether to methanol ratio of higher than 2 and a carbon dioxide content of above 20 mole %; (c) contacting the carbon dioxide containing oxygenate mixture at an inlet temperature of between 240 and 4000 C with a catalyst being active in the conversion of oxygenate to higher hydrocarbons and a tail gas being rich in carbon dioxide; (d) combusting the carbon dioxide rich tail gas, optionally admixed with fresh carbon monoxide rich synthesis gas in a gas turbine combustion chamber to flue gas; and (e) expanding the flue gas stream through a gas turbine for the generation of power.
摘要翻译： 一种用于制备烃产物和产生动力的方法，包括以下步骤：（a）提供氢与一氧化碳比为0.1至1的合成气; （b）使合成气与一种或多种催化剂接触，这些催化剂一起催化氢和一氧化碳与包含甲醇和二甲醚的含氧化合物的反应，甲醚与甲醇的比例高于2，二氧化碳含量高于20摩尔％ ; （c）在240至4000℃的入口温度下使含二氧化碳混合物与含氧化合物转化为高级烃和富含二氧化碳的尾气有活性的催化剂接触; （d）燃烧富含二氧化碳的尾气，任选地与燃气轮机燃烧室中的新鲜的富含一氧化碳的合成气混合成烟道气; 和（e）通过用于发电的燃气轮机扩大烟气流。
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公开(公告)号：US08202413B2
公开(公告)日：2012-06-19
申请号：US12209499
申请日：2008-09-12
CPC分类号： C10G3/49 , C10G2300/4081 , C10G2400/02 , Y02P30/20
摘要： A process for the preparation of hydrocarbon products including the steps of (a) providing a stream containing oxygenates; (b) mixing the stream with a recycle stream to form a gasoline feed stream; (c) contacting the gasoline feed stream with one or more gasoline synthesis catalysts to obtain an effluent stream with higher hydrocarbons boiling in the gasoline range; (d) withdrawing from step (c) the effluent stream; and (e) splitting a part of the effluent stream to form the recycle stream which is optionally further reduced in content of water or enriched in hydrogen, then pressurized and recycled to step (b).
摘要翻译： 一种制备烃产物的方法，包括以下步骤：（a）提供含有氧化物的料流; （b）将料流与再循环料流混合以形成汽油进料流; （c）使汽油进料流与一种或多种汽油合成催化剂接触以获得在汽油范围内沸腾的高级烃的流出物流; （d）从步骤（c）退出流出物流; 和（e）分离一部分流出物流以形成循环物流，其任选地进一步减少水的含量或富含氢气，然后加压并再循环至步骤（b）。
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公开(公告)号：US08038906B2
公开(公告)日：2011-10-18
申请号：US12431240
申请日：2009-04-28
CPC分类号： C01B3/36 , C01B3/32 , C01B3/50 , C01B3/52 , C01B2203/0415 , C01B2203/047 , C01B2203/0475 , C07C41/01 , D21C11/125 , C07C43/043
摘要： A process for the adjustment of the composition of a synthesis gas produced in a high temperature black liquor gasifier. The process includes the steps of (a) generating a gasifier effluent stream from black liquor in the gasifier by a blast and optionally an atomising stream; (b) optionally quenching the gasifier effluent stream with a gas stream to form a gas quenched effluent stream; (c) quenching the gasifier effluent of step (a) or the gas quenched effluent gas stream of step (b) with a water stream to form a raw synthesis gas; (d) further cooling and cleaning and separating the raw synthesis gas to form a purified unprocessed synthesis gas with an appropriate H2/CO ratio; (e) partly converting the purified synthesis gas to dimethyl ether in a synthesis section, producing at least a product stream of DME and a hydrogen rich purge stream of processed; (f) splitting and recycling individual or combinations of split streams of the processed or the unprocessed synthesis gas to step a and/or step (b); and recycling a by-product stream of CO2 being further generated in step (e) in part or completely to step (a) and/or step (b).
摘要翻译： 用于调节在高温黑液气化器中生产的合成气的组成的方法。 该方法包括以下步骤：（a）通过鼓风和任选的雾化流从气化器中的黑液生成气化器流出物流; （b）任选地用气流骤冷气化器流出物流以形成气体骤冷流出物流; （c）用水流淬火步骤（a）的气化器流出物或步骤（b）的气体骤冷流出物气流，以形成原始合成气; （d）进一步冷却和清洗并分离原始合成气以形成具有合适H 2 / CO比的纯化未加工合成气; （e）在合成部分中部分地将纯化的合成气转化为二甲醚，至少产生DME的产物流和加氢的富氢吹扫流; （f）将经处理或未经处理的合成气的分流或分离流分离和回收到步骤a和/或步骤（b）; 并且在步骤（e）中再次产生副产物二氧化碳流，部分或完全是步骤（a）和/或步骤（b）。
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6.发明授权公开(公告)号：US08471060B2
公开(公告)日：2013-06-25
申请号：US12624019
申请日：2009-11-23
IPC分类号： C07C51/00
CPC分类号： C07C45/38 , B01J8/04 , C07C51/235 , C07C47/06 , C07C53/08
摘要： A process and reactor for the production of acetic acid comprising the steps of: passing a feed stream containing ethanol and water together with a predetermined feed rate of an oxygen containing atmosphere in presence of one or more catalysts being active in simultaneous non-oxidative and oxidative conversion of ethanol to a product stream with acetic acid; recovering from the product stream a stream of acetic acid; optionally recovering reactive derivatives of acetic acid and recycling these to step (a).
摘要翻译： 一种用于生产乙酸的方法和反应器，包括以下步骤：在一种或多种催化剂的存在下，使含有乙醇和水的进料流与预定的含氧气氛的进料速率一起通过同时进行的非氧化和氧化 用乙酸将乙醇转化成产物流; 从产物流中回收乙酸流; 任选地回收乙酸的活性衍生物并将其再循环到步骤（a）。
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7.发明申请公开(公告)号：US20100130776A1
公开(公告)日：2010-05-27
申请号：US12624019
申请日：2009-11-23
IPC分类号： C07C51/235 , B01J8/04
CPC分类号： C07C45/38 , B01J8/04 , C07C51/235 , C07C47/06 , C07C53/08
摘要： A process and reactor for the production of acetic acid comprising the steps of: passing a feed stream containing ethanol and water together with a predetermined feed rate of an oxygen containing atmosphere in presence of one or more catalysts being active in simultaneous non-oxidative and oxidative conversion of ethanol to a product stream with acetic acid; recovering from the product stream a stream of acetic acid; optionally recovering reactive derivatives of acetic acid and recycling these to step (a).
摘要翻译： 一种用于生产乙酸的方法和反应器，包括以下步骤：在一种或多种催化剂的存在下，使含有乙醇和水的进料流与预定的含氧气氛的进料速率一起通过同时进行的非氧化和氧化 用乙酸将乙醇转化成产物流; 从产物流中回收乙酸流; 任选地回收乙酸的活性衍生物并将其再循环到步骤（a）。
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公开(公告)号：US20100130775A1
公开(公告)日：2010-05-27
申请号：US12622820
申请日：2009-11-20
IPC分类号： C07C53/08
摘要： Process for the preparation of acetic acid comprising the steps of: providing a feed stream of water and ethanol; adding the feed stream to a recycle stream comprising unconverted ethanol and water; heating the admixture to a predetermined reaction temperature and passing the thus heated admixture over a catalyst being active in non-oxidative conversion of ethanol to acetic acid to obtain an effluent being rich in acetic acid; optionally cooling the effluent; separating the effluent into a stream rich in acetic acid being essentially free of water, a hydrogen containing stream, and a stream with unconverted amounts of ethanol, water and reactive derivates of acetic acid and optionally ethyl acetate; recycling the stream with unconverted amounts of ethanol and water to step (a); determining the amount of water in the recycle stream and adjusting the composition of the ethanol and water feed stream in step (a) to a water/ethanol mole ratio of between 0.3/0.7 to 0.6/0.4.
摘要翻译： 制备乙酸的方法，包括以下步骤：提供水和乙醇的进料流; 将进料流加入到包含未转化的乙醇和水的再循环流中; 将混合物加热到预定的反应温度，并将如此加热的混合物通过催化剂，在乙醇非氧化转化成乙酸中有活性的催化剂，得到富含乙酸的流出液; 任选地冷却流出物; 将流出物分离成富含乙酸的物流，其基本上不含水，含氢气流，以及具有未转化量的乙醇，水和乙酸和任选的乙酸乙酯的反应性衍生物的物流; 将未转化量的乙醇和水回收到步骤（a）; 确定再循环流中的水量，并将步骤（a）中的乙醇和水进料流的组成调节至0.3 / 0.7-0.6 / 0.4之间的水/乙醇摩尔比。
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公开(公告)号：US20100036186A1
公开(公告)日：2010-02-11
申请号：US12518616
申请日：2007-11-20
申请人： Finn Joensen , Poul Erik Hojlund Nielsen , Niels Christian Schiodt , Ton V.W. Janssens , Bodil Voss
发明人： Finn Joensen , Poul Erik Hojlund Nielsen , Niels Christian Schiodt , Ton V.W. Janssens , Bodil Voss
IPC分类号： C07C1/20
CPC分类号： C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2300/805 , C10G2400/02 , C10G2400/20 , Y02P30/20
摘要： Process for the synthesis of hydrocarbon constituents of gasoline comprising catalytic conversion in a gasoline synthesis step of an oxygenate-containing feed comprising methanol and/or dimethyl ether and a mixture of at least on a total oxygenate basis 0.05 wt % C3+ higher alcohols and/or their oxygenate equivalents to hydrocarbon constituents of gasoline.
摘要翻译： 在包含甲醇和/或二甲醚的含氧化合物进料的汽油合成步骤和至少在总含氧化合物基础上的混合物，基于0.05重量％的C3 +高级醇和/或 它们的含氧化合物等同于汽油的烃成分。
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公开(公告)号：US5908963A
公开(公告)日：1999-06-01
申请号：US894066
申请日：1997-12-12
申请人： Bodil Voss , Finn Joensen , John Bogild Hansen
发明人： Bodil Voss , Finn Joensen , John Bogild Hansen
CPC分类号： C07C41/01
摘要： A process for the preparation of dimethyl ether. The process prepares fuel grade dimethyl ether from a hydrogen and carbon oxides synthesis gas.
摘要翻译： PCT No.PCT / DK96 / 00047 Sec。 371日期1997年12月12日 102（e）日期1997年12月12日PCT 1996年1月29日PCT PCT。 公开号WO96 / 23755 日期1996年8月8日制备二甲醚的方法。 该方法由氢和碳氧化物合成气制备燃料级二甲醚。
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