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公开(公告)号：US4668594A
公开(公告)日：1987-05-26
申请号：US812889
申请日：1985-12-05
IPC分类号： H01M10/052 , H01M4/485 , H01M10/0566 , H01M4/48 , H01M10/40
CPC分类号： H01M10/052 , H01M4/485
摘要： A rechargeable electrochemical device composed of a negative electrode (4) which comprises an alkali metal as an active material, a non-aqueous electrolyte (6), and a positive electrode (1). The positive electrode (1) is composed of an oxide of chromium and vanadium represented by the general formula:Cr.sub.x V.sub.2(1-x) O.sub.5-(2+y)x(wherein 0.2.ltoreq.x.ltoreq.0.9, 0.1.ltoreq.y.ltoreq.1.0). The rechargeable electrochemical device offers a high discharge voltage, a large discharge capacity, linear discharge voltage, and the capacity to withstand over-charging.
摘要翻译： PCT No.PCT / JP85 / 00162 Sec。 371日期1985年12月5日第 102（e）1985年12月5日日期PCT提交1985年4月3日PCT公布。 公开号WO85 / 04763 日期：1985年10月24日。一种由负极（4）构成的可充电电化学装置，其包含作为活性物质的碱金属，非水电解质（6）和正极（1）。 正极（1）由以下通式表示的铬和钒的氧化物构成：CrxV2（1-x）O5-（2 + y）x（其中0.2
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公开(公告)号：US4658498A
公开(公告)日：1987-04-21
申请号：US681848
申请日：1984-12-04
CPC分类号： H01M10/05 , H01M4/40 , H01M4/66 , Y10T29/49108
摘要： An alloy capable of reversibly absorbing and desorbing lithium ions in a non-aqueous electrolyte containing lithium ions on charging and discharging has excellent applicability to anode for rechargeable electrochemical devices. However, such alloy, when absorbed with lithium, loses its flexibility, so that when it is incorporated in a device in a charged state, it is subject to trouble such as cracking and can not display its properties. This invention adopts a method in which anode alloy is combined with lithium by connecting them so as to be electronically conductive to each other and this combination is fitted into the device, and then the electrolyte is supplied into the device to have lithium absorbed in anode alloy in the device. According to this method, cracking of cathode can be prevented.
摘要翻译： PCT No.PCT / JP84 / 00171 Sec。 371日期1984年12月4日第 102（e）日期1984年12月4日PCT提交1984年4月5日PCT公布。 WO94 / 04001 PCT出版物 日期：1984年10月11日。在充电和放电的含有锂离子的非水电解质中能够可逆吸收和解吸锂离子的合金对于可再充电电化学装置的阳极具有极好的适用性。 然而，当用锂吸收时，这种合金失去其柔性，使得当其以带电状态并入设备时，其遭受诸如破裂的故障，并且不能显示其性能。 本发明采用一种方法，其中将阳极合金与锂组合以使其彼此电子导电，并将该组合装配到装置中，然后将电解质供应到装置中以将锂吸收在阳极合金中 在设备中。 根据该方法，可以防止阴极开裂。
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公开(公告)号：US4851309A
公开(公告)日：1989-07-25
申请号：US935169
申请日：1986-11-24
摘要： A rechargeable negative electrode for an electrochemical apparatus using nonaqueous electrolytes, said electrode comprising an alloy comprising (1) at least one metal selected from the group consisting of Sn, Pn, In and Bi and (2) Zn or Zn and Cd, as well as a rechargeable electrochemical apparatus comprising a combination of said negative electrode with a positive electrode having reversibility in charging and discharging. The above-mentioned negative electrode reversibly absorbs and desorbs alkali metal ions, as the result of charge and discharge, in nonaqueous electrolyte containing alkali metal ions. It undergoes no pulverization even after repeated charge and discharge, and maintains its shape stably, so that it has a long charge-and-discharge cycle life. Further, since it can absorb a large quantity of alkali metal per unit volume, it is of high energy density.
摘要翻译： PCT No.PCT / JP84 / 00088 Sec。 371日期1984年11月5日 102（e）日期1984年11月5日PCT提交1984年3月6日PCT公布。 出版物WO84 / 03591 日本9月13日，1984年。一种用于使用非水电解质的电化学装置的可再充电负极，所述电极包括合金，其包含（1）选自Sn，Pn，In和Bi中的至少一种金属和（2）Zn 或Zn和Cd，以及可充电电化学装置，其包括所述负极与正电极的组合，其具有充电和放电的可逆性。 在含有碱金属离子的非水电解质中，上述负极作为充放电的结果可逆地吸收和解吸碱金属离子。 即使重复进行充放电，也不会发生粉碎，并且保持其形状稳定，因此其充放电循环寿命长。 此外，由于每单位体积吸收大量碱金属，所以能量密度高。
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公开(公告)号：US4683182A
公开(公告)日：1987-07-28
申请号：US873093
申请日：1986-06-04
摘要： The present invention relates to a rechargeable negative electrode for an electrochemical apparatus using nonaqueous electrolyte, said electrode comprising an alloy comprising Cd and at least one metal selected from the group consisting of Sn, Pb, In and Bi, as well as to a rechargeable electrochemical apparatus comprising a combination of said negative electrode with a positive electrode having reversibility in charge and discharge.The above-mentioned negative electrode reversibly absorbs and desorbs alkali metal ions, as the result of charge and discharge, in nonaqueous electrolyte containing alkali metal ions. It undergoes no pulverization even after repeated charge and discharge and maintains its shape stably, so that it has a long chargeand-discharge life. Further, since it can absorb a large quantity of alkali metal per unit volume, it is of high energy density.
摘要翻译： PCT No.PCT / JP84 / 00086 Sec。 371日期1984年11月5日 102（e）日期1984年11月5日PCT提交1984年3月6日PCT公布。 公开号WO84 / 03590 日期：1984年9月13日。本发明涉及一种使用非水电解质的电化学装置的可再充电负极，所述电极包括含有Cd和选自Sn，Pb，In和Bi中的至少一种金属的合金， 以及包括所述负极与正电极的组合的可再充电电化学装置，其具有充电和放电的可逆性。 在含有碱金属离子的非水电解质中，上述负极作为充放电的结果可逆地吸收和解吸碱金属离子。 即使在重复充放电之后也不会发生粉碎，并且其形状稳定，从而具有长的充放电寿命。 此外，由于每单位体积吸收大量碱金属，所以能量密度高。
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5.发明授权Nonaqueous electrolyte for secondary battery and secondary battery including the same 失效用于二次电池和二次电池的非水电解质包括其公开(公告)号：US07851093B2
公开(公告)日：2010-12-14
申请号：US11792246
申请日：2005-12-06
申请人： Masaki Deguchi , Tooru Matsui , Hiroshi Yoshizawa
发明人： Masaki Deguchi , Tooru Matsui , Hiroshi Yoshizawa
CPC分类号： H01M10/0567 , H01M4/131 , H01M4/133 , H01M10/0525 , H01M10/0568 , H01M10/0587 , H01M10/4235 , Y02T10/7011
摘要： A non-aqueous electrolyte for a secondary battery, including a non-aqueous solvent in which a solute is dissolved, a first additive and a second additive, wherein the first additive is a vinyl monomer having an electron donating group, the second additive is a carbonic acid ester having at least one carbon-carbon unsaturated bond, and an e value, which is a polarization factor of the vinyl monomer having an electron donating group, is a negative value.
摘要翻译： 一种二次电池用非水电解质，包括其中溶解有溶质的非水溶剂，第一添加剂和第二添加剂，其中所述第一添加剂是具有给电子基团的乙烯基单体，所述第二添加剂为 具有至少一个碳 - 碳不饱和键的碳酸酯和作为具有给电子基团的乙烯基单体的极化因子的e值为负值。
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公开(公告)号：US20090325076A1
公开(公告)日：2009-12-31
申请号：US12489940
申请日：2009-06-23
申请人： Tooru Matsui , Tetsuo Nanno , Hiroshi Yoshizawa
发明人： Tooru Matsui , Tetsuo Nanno , Hiroshi Yoshizawa
IPC分类号： H01M6/16
CPC分类号： H01M10/0569 , H01M10/052 , H01M10/0565 , H01M2300/0037 , H01M2300/004
摘要： A non-aqueous electrolyte secondary battery is produced using a non-aqueous electrolyte including: a non-aqueous solvent that primarily contains a solvent mixture of ethylene carbonate and propylene carbonate and includes a fluorine-substituted ether having a divalent group represented by a formula: —CFX—CH(CH3)—O—, where X is a hydrogen atom or fluorine atom, in a molecule thereof; and a lithium salt that is dissolved in the non-aqueous solvent. The non-aqueous electrolyte has favorable wettability towards a polyolefin separator, and improves the cycle characteristics and the load characteristics of the non-aqueous electrolyte secondary battery.
摘要翻译： 使用非水电解质制造非水电解质二次电池，所述非水电解质包括：主要含有碳酸亚乙酯和碳酸亚丙酯的溶剂混合物的非水溶剂，并且包括具有由下式表示的二价基团的氟取代的醚： -CFX-CH（CH 3）-O-，其中X为氢原子或氟原子; 和溶解在非水溶剂中的锂盐。 非水电解质对聚烯烃隔膜具有良好的润湿性，并且提高了非水电解质二次电池的循环特性和负载特性。
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公开(公告)号：US07468225B2
公开(公告)日：2008-12-23
申请号：US11547172
申请日：2005-03-31
IPC分类号： H01M6/18
CPC分类号： H01M4/505 , H01M4/131 , H01M4/133 , H01M4/525 , H01M6/168 , H01M10/0525 , H01M10/0567 , H01M10/0569 , H01M10/0587 , H01M10/4235 , H01M2004/8689 , H01M2300/0025 , Y02T10/7011
摘要： A non-aqueous electrolyte secondary battery including a positive electrode and a negative electrode each capable of absorbing and desorbing lithium, a separator interposed therebetween, and a non-aqueous electrolyte, wherein the positive electrode includes a positive electrode active material represented by: LiM1-xLxO2 where 0.005≦x≦0.1 is satisfied, M is at least one selected from the group consisting of Mn, Co and Ni, and L is at least one selected from the group consisting of Mg, Al, Ti, Sr, Zn, B, Ca, Cr, Si, Ga, Sn, P, V, Sb, Nb, Ta, Mo, W, Zr, Y and Fe, and the non-aqueous electrolyte includes a phosphinate compound represented by: where R1, R2 and R3 are each independently an aryl group, or an alkyl group, an alkenyl group or an alkynyl group each having 1 to 5 carbon atoms.
摘要翻译： 一种非水电解质二次电池，包括能够吸收和解吸锂的正极和负极，隔着隔板的非水电解质二次电池和非水电解质，其中所述正极包括由LiM1- xLxO2，其中满足0.005 <= x <= 0.1，M是选自Mn，Co和Ni中的至少一种，L是选自Mg，Al，Ti，Sr，Zn ，B，Ca，Cr，Si，Ga，Sn，P，V，Sb，Nb，Ta，Mo，W，Zr，Y和Fe，非水电解质包括由下式表示的次膦酸盐化合物：其中R1，R2 和R 3各自独立地为具有1〜5个碳原子的芳基或烷基，烯基或炔基。
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公开(公告)号：US6043975A
公开(公告)日：2000-03-28
申请号：US294553
申请日：1999-04-20
申请人： Teruhisa Kanbara , Tooru Matsui , Kenichi Takeyama
发明人： Teruhisa Kanbara , Tooru Matsui , Kenichi Takeyama
摘要： An ion-conductive polymer electrolyte having a high ionic conductivity and a high stability in both of physical and chemical properties is disclosed. It has a polymer containing at least one monomer selected from the group containing of a hydroxyalkyl acrylate, a hydroxyalkyl methacrylate and vinylene carbonate as its polymerizable ingredient, and at least one electrolyte salt. An aluminum electrolytic capacitor and an electric double-layer capacitor configured with the electrolyte are also disclosed.
摘要翻译： 公开了一种离子导电聚合物电解质，其具有高的离子导电性和物理和化学性质的高稳定性。 它具有含有至少一种选自丙烯酸羟烷基酯，甲基丙烯酸羟烷基酯和碳酸亚乙烯酯作为其可聚合成分的单体和至少一种电解质盐的聚合物。 还公开了一种铝电解电容器和配置有电解质的双电层电容器。
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9.发明授权
公开(公告)号：US5558953A
公开(公告)日：1996-09-24
申请号：US319761
申请日：1994-10-07
申请人： Tooru Matsui , Kenichi Takeyama
发明人： Tooru Matsui , Kenichi Takeyama
CPC分类号： H01M4/13 , C25D3/42 , H01M4/0438 , H01M4/0452 , C25D17/10 , H01M2300/0025 , H01M6/164
摘要： A non-aqueous electrolyte secondary battery having a long cycle life and a high reliability with substantially no internal short-circuit is provided by incorporating crystalline metal lithium as its negative electrode. The crystalline metal lithium is electrochemically deposited on a metal substrate in an electrolyte including a tetrahydrofran derivative or a 1,3-dioxolan derivative as a solvent.
摘要翻译： 通过结晶金属锂作为其负极，提供了具有长的循环寿命和高可靠性，基本上没有内部短路的非水电解质二次电池。 结晶金属锂电化学沉积在包含四氢呋喃衍生物或1,3-二氧戊环衍生物作为溶剂的电解质的金属基底上。
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公开(公告)号：US08470475B2
公开(公告)日：2013-06-25
申请号：US11287446
申请日：2005-11-28
申请人： Masaki Deguchi , Tooru Matsui , Hiroshi Yoshizawa
发明人： Masaki Deguchi , Tooru Matsui , Hiroshi Yoshizawa
IPC分类号： H01M4/13
CPC分类号： C01G51/42 , C01G45/1228 , C01G51/50 , C01G53/42 , C01G53/50 , C01P2002/52 , C01P2002/54 , C01P2006/40 , H01M4/131 , H01M4/485 , H01M4/505 , H01M4/525 , H01M10/0525 , H01M10/0569
摘要： A non-aqueous electrolyte secondary battery includes: a positive electrode capable of absorbing and desorbing lithium; a negative electrode capable of absorbing and desorbing lithium; a separator interposed between the positive electrode and the negative electrode; and a non-aqueous electrolyte. The positive electrode includes a composite oxide represented by formula (1): LiNixM1-x-yLyO2 as an active material. The formula (1) satisfies 0.3≦x≦0.9 and 0≦y≦0.1. The element M is at least one selected from the group consisting of Co and Mn, and the element L is at least one selected from the group consisting of Mg, Al, Ti, Sr, Zn, B, Ca, Cr, Si, Ga, Sn, P, V, Sb, Nb, Ta, Mo, W, Zr, Y and Fe. The non-aqueous electrolyte includes a main solvent, a solute and vinyl ethylene carbonate.
摘要翻译： 非水电解质二次电池包括：能够吸收和解吸锂的正极; 能够吸收和解吸锂的负极; 夹在正极和负极之间的隔膜; 和非水电解质。 正极包括由式（1）表示的复合氧化物：LiNixM1-x-yLyO2作为活性材料。 式（1）满足0.3 @ x @ 0.9和0 @ y @ 0.1。 元素M是选自Co和Mn中的至少一种元素，元素L是选自Mg，Al，Ti，Sr，Zn，B，Ca，Cr，Si，Ga中的至少一种 ，Sn，P，V，Sb，Nb，Ta，Mo，W，Zr，Y和Fe。 非水电解质包括主溶剂，溶质和乙烯基碳酸亚乙酯。
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