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1.发明授权
公开(公告)号：US5310833A
公开(公告)日：1994-05-10
申请号：US20758
申请日：1993-02-22
申请人： Kunimichi Kubo , Motokazu Watanabe , Mamoru Yoshikawa , Masatoshi Morikawa , Yoshihisa Yamaguchi
发明人： Kunimichi Kubo , Motokazu Watanabe , Mamoru Yoshikawa , Masatoshi Morikawa , Yoshihisa Yamaguchi
CPC分类号： B01J19/26 , B01J3/02 , B01J8/0005 , B01J8/0015 , B01J8/0035 , B01J8/004 , B01J8/24 , C08F10/00 , B01J2208/00265 , B01J2208/00548 , B01J2208/00752 , Y10S526/901
摘要： A process for feeding a powder catalyst with a gas intermittently to a high-pressure fluidized bed reactor for the vapor phase polymerization of olefin, wherein the cross section of a catalyst feed pipe is reduced midway through the pipe to thereby make continual catalyst feeding possible and prevent the formation of a lump polymer.
摘要翻译： 一种将气体间歇地供给到高压流化床反应器的粉末催化剂进行烯烃气相聚合的方法，其中催化剂进料管的横截面通过管中途减少，从而使连续的催化剂进料成为可能， 防止形成块状聚合物。
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2.发明授权Process for feeding catalyst to fluidized bed for vapor phase polymerization 失效将催化剂输送到流化床用于蒸气相聚合的方法
公开(公告)号：US5202396A
公开(公告)日：1993-04-13
申请号：US842094
申请日：1992-03-19
申请人： Kunimichi Kubo , Motokazu Watanabe , Mamoru Yoshikawa , Masatoshi Morikawa , Yoshihisa Yamaguchi
发明人： Kunimichi Kubo , Motokazu Watanabe , Mamoru Yoshikawa , Masatoshi Morikawa , Yoshihisa Yamaguchi
CPC分类号： B01J19/26 , B01J3/02 , B01J8/0005 , B01J8/0015 , B01J8/0035 , B01J8/004 , B01J8/24 , C08F10/00 , B01J2208/00265 , B01J2208/00548 , B01J2208/00752 , Y10S526/901
摘要： A process for feeding a powder catalyst with a gas intermittently to a high-pressure fluidized bed reactor for the vapor phase polymerization of olefin, wherein the cross section of a catalyst feed pipe is reduced midway through the pipe to thereby make continual catalyst feeding possible and prevent the formation of a lump polymer.
摘要翻译： PCT No.PCT / JP91 / 00968 Sec。 371日期：1992年3月19日 102（e）1992年3月19日PCT PCT 1991年7月19日PCT公布。 出版物WO92 / 01722 日期：1992年2月6日。一种将气体间歇地送入用于烯烃气相聚合的高压流化床反应器的粉末催化剂的方法，其中催化剂进料管的横截面通过管中途减少至 从而使连续的催化剂进料成为可能，并防止形成块状聚合物。
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公开(公告)号：US5525687A
公开(公告)日：1996-06-11
申请号：US328083
申请日：1994-10-24
申请人： Yoshihisa Yamaguchi , Shinjiro Suga , Masatoshi Morikawa , Kunimichi Kubo , Motokazu Watanabe , Yasuhiko Sano
发明人： Yoshihisa Yamaguchi , Shinjiro Suga , Masatoshi Morikawa , Kunimichi Kubo , Motokazu Watanabe , Yasuhiko Sano
CPC分类号： C08F10/00 , Y10S526/901
摘要： A process for producing polyolefin with a vapor-phase fluidized-bed reactor, wherein the reaction is started after filling the reactor with particles which contain moisture and/or molecular oxygen and can form a fluidized bed in order to prevent the formation of molten resin which is liable to occur at the start of the reaction and to attain a smooth operation of the reactor.
摘要翻译： 一种用气相流化床反应器生产聚烯烃的方法，其中反应开始于含有水分和/或分子氧的颗粒填充反应器之后，可形成流化床，以防止形成熔融树脂， 在反应开始时容易发生，从而使反应器顺利运行。
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公开(公告)号：US5385991A
公开(公告)日：1995-01-31
申请号：US844590
申请日：1992-03-27
申请人： Yoshihisa Yamaguchi , Shinjiro Suga , Masatoshi Morikawa , Kunimichi Kubo , Motokazu Watanabe , Yasuhiko Sano
发明人： Yoshihisa Yamaguchi , Shinjiro Suga , Masatoshi Morikawa , Kunimichi Kubo , Motokazu Watanabe , Yasuhiko Sano
CPC分类号： C08F10/00 , Y10S526/901
摘要： A process for producing polyolefin with a vapor-phase fluidized-bed reactor, wherein the reaction is started after filling the reactor with particles which contain moisture and/or molecular oxygen and can form a fluidized bed in order to prevent the formation of molten resin which is liable to occur at the start of the reaction and to attain a smooth operation of the reactor.
摘要翻译： PCT No.PCT / JP91 / 01010 Sec。 371日期：1992年3月27日 102（e）1992年3月27日PCT PCT 1991年7月26日PCT公布。 出版物WO92 / 02563 日本1992年2月20日。一种用气相流化床反应器生产聚烯烃的方法，其中反应开始于含有水分和/或分子氧的颗粒填充反应器之后，可形成流化床，以便 防止在反应开始时易于发生的熔融树脂的形成，并使反应器顺利地进行操作。
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公开(公告)号：US4525548A
公开(公告)日：1985-06-25
申请号：US406435
申请日：1982-08-09
CPC分类号： B01J8/38 , B01F7/04 , B01J8/10 , C08F10/00 , B01J2219/182 , Y10S526/901
摘要： Provided is a method for vapor phase polymerization of olefins. An olefin gas is fed into a horizontal cylindrical vessel having a lower curved surface corresponding to 30 to 180 degrees of the circumference of the vessel and extending substantially the length of the vessel formed by a perforated plate having a multiplicity of holes spaced at intervals in the range of from 0.5 to 50 mm, through said plate from an olefin feed chamber mounted below and covering the plate. A polymer catalyst is fed into the horizontal cylindrical vessel through a polymerization catalyst inlet port located in a portion of the vessel other than the lower curved surface formed by the perforated plate. The olefin is reacted in the presence of a catalyst with agitation to form polymer. Unreacted olefin is removed through a discharge port located in a portion of the vessel other than the lower curved surface formed by the perforated plate. Polymer is removed through an outlet port located in a portion of the vessel other than the lower curved surface formed by the perforated plate.
摘要翻译： 提供了一种烯烃气相聚合方法。 将烯烃气体进料到具有对应于容器圆周的30至180度的较低弯曲表面的水平圆柱形容器中，并且基本上延伸由多孔板形成的容器的长度，所述多孔板具有多个孔， 范围为0.5至50mm，通过所述板从安装在下方并覆盖板的烯烃进料室。 聚合物催化剂通过聚合催化剂入口进入水平圆筒形容器中，所述聚合催化剂入口位于容器的除多孔板形成的下弯曲表面之外的部分中。 烯烃在催化剂存在下与搅拌反应形成聚合物。 未反应的烯烃通过位于容器的除多孔板形成的下弯曲表面以外的排出口除去。 聚合物通过位于容器的除多孔板形成的下弯曲表面以外的一部分的出口除去。
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公开(公告)号：US4372919A
公开(公告)日：1983-02-08
申请号：US242308
申请日：1981-03-10
CPC分类号： B01J8/382 , B01J8/10 , C08F10/00 , B01J2219/182 , Y10S526/901
摘要： A horizontal agitation bed type vapor phase polymerization apparatus for olefins, having a lower curved surface constructed by a perforated plate so as to allow a olefin gas to be fed uniformly throughout the reaction system through the said perforated plate.
摘要翻译： 一种用于烯烃的卧式搅拌床型气相聚合装置，具有由多孔板构成的下弯曲表面，以使烯烃气体通过所述多孔板均匀地供给到整个反应系统中。
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公开(公告)号：US5571879A
公开(公告)日：1996-11-05
申请号：US595520
申请日：1996-02-01
申请人： Makoto Jimbo , Mamoru Yoshikawa , Shinjiro Suga , Yoshihisa Yamaguchi , Masahiro Niwa , Eiko Kobayashi , Kunimichi Kubo
发明人： Makoto Jimbo , Mamoru Yoshikawa , Shinjiro Suga , Yoshihisa Yamaguchi , Masahiro Niwa , Eiko Kobayashi , Kunimichi Kubo
CPC分类号： C08F10/00 , Y10S526/901
摘要： In the polymerization of olefins with a vapor phase fluidized bed reactor, the improvement comprises the steps of feeding seed polymer particles and the reaction is then started after feeding an organoaluminum compound on a prescribed basis, thereby avoiding the formation of sheet-like polymer in the initial period of the reaction and the lowering of the bulk density of the product polymer.
摘要翻译： 在用气相流化床反应器进行烯烃聚合反应时，改进之处包括进料种子聚合物颗粒的步骤，然后在规定的基础上加入有机铝化合物之后开始反应，从而避免了在 反应的初始阶段和产物聚合物的堆积密度的降低。
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公开(公告)号：US4438073A
公开(公告)日：1984-03-20
申请号：US315616
申请日：1981-10-28
CPC分类号： B01J8/382 , B01J8/10 , C08F10/00 , B01J2219/182
摘要： A horizontal agitation bed type vapor phase polymerization apparatus for olefins provided on its lower curved surface with plural cells each having an opening facing on the polymerization reaction system and further having small holes formed in its side wall portion for feeding a starting olefin gas.
摘要翻译： 一种用于烯烃的卧式搅拌床型气相聚合装置，在其下曲面上设置有多个单元，每个单元均具有面向聚合反应系统的开口，并且在其侧壁部分中形成有用于进料起始烯烃气体的小孔。
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公开(公告)号：US5648581A
公开(公告)日：1997-07-15
申请号：US598334
申请日：1996-02-08
CPC分类号： B01J8/1809 , B01J19/002 , C08F10/00 , B01J2208/00044 , B01J2208/00734
摘要： A method for polymerizing or copolymerizing .alpha.-olefin in a vapor phase condition by supplying to a reactor a catalyst composed of a solid catalyst component containing at least titanium and/or vanadium as well as magnesium and an organic aluminum compound wherein the current due to the electric charge transferred from polymer particles electrified to an electrode disposed at a position where sheet-like polymers will be produced in a reactor, as a result of contact of the polymer particles in the reactor with the electrode is determined, and the polymerization or copolymerization is carried out under such condition where the mean value of current is zero or a positive value. As a result, it becomes possible to prevent production of sheet-like polymers and to stably continue the reaction for polymerization.
摘要翻译： 一种通过向反应器中提供由至少含有钛和/或钒的固体催化剂组分以及镁和有机铝化合物组成的催化剂，从而在气相条件下聚合或共聚α-烯烃的方法，其中由于 测定从聚合物粒子的电荷转移到布置在反应器中将产生片状聚合物的位置处的电极，由于反应器中的聚合物颗粒与电极的接触，聚合或共聚是 在电流的平均值为零或正值的条件下进行。 结果，可以防止片状聚合物的生产并稳定地继续聚合反应。
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公开(公告)号：US5543478A
公开(公告)日：1996-08-06
申请号：US174269
申请日：1993-12-28
申请人： Masahiro Niwa , Yuji Sugano , Ken-ichi Uenishi , Hideto Kitada , Yoshihisa Yamaguchi , Eiko Kobayashi , Kunimichi Kubo , Akira Sano
发明人： Masahiro Niwa , Yuji Sugano , Ken-ichi Uenishi , Hideto Kitada , Yoshihisa Yamaguchi , Eiko Kobayashi , Kunimichi Kubo , Akira Sano
CPC分类号： C08F10/00
摘要： In the preparation of polyolefin in a vapor phase polymerization using catalysts comprising a solid catalyst component containing titanium and/or vanadium; and magnesium and an organoaluminum compound, when the reaction is stopped for a certain period of time, the restarting of reaction is possible by feeding in the first place an organoaluminum compound into the reaction system with retaining of polymer particles in the reactor.
摘要翻译： 在使用包含含有钛和/或钒的固体催化剂组分的催化剂进行气相聚合的聚烯烃的制备中; 和镁和有机铝化合物，当反应停止一定时间时，通过在反应器中保持聚合物颗粒首先将有机铝化合物进料到反应体系中，可以重新开始反应。
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