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公开(公告)号：US5747182A
公开(公告)日：1998-05-05
申请号：US379503
申请日：1995-04-03
申请人： Richard Henry Friend , Andrew Bruce Holmes , Donal Donat Conor Bradley , Paul Leslie Burn , Arno Kraft , Adam Richard Brown , Jeremy Henley Burroughes , Neil Clement Greenham
发明人： Richard Henry Friend , Andrew Bruce Holmes , Donal Donat Conor Bradley , Paul Leslie Burn , Arno Kraft , Adam Richard Brown , Jeremy Henley Burroughes , Neil Clement Greenham
CPC分类号： H01L51/5012 , C08G61/00 , C09K11/06 , H05B33/10 , H05B33/14 , Y10S428/917
摘要： In an electroluminescent device which comprises a layer of a semiconductive conjugated polymer between positive and negative charge carrier injecting electrodes, a barrier layer is arranged between the layer of semiconductive conjugated polymer and the charge carrier injecting layer for negative charge carriers. The barrier layer protects the layer of semiconductive conjugated polymer from for example mobile ions released by the reactive charge carrier injecting layer. The barrier layer can in some circumstances also itself be light-emissive.
摘要翻译： PCT No.PCT / GB93 / 01573 Sec。 371日期：1995年4月3日 102（e）日期1995年4月3日PCT提交1993年7月26日PCT公布。 公开号WO94 / 03030 日期：1994年2月3日在含有负电荷载流子注入电极的半导体共轭聚合物层的电致发光器件中，在半导体共轭聚合物层和负电荷载体的电荷载流子注入层之间配置阻挡层。 阻挡层保护半导体共轭聚合物层免受例如由反应性电荷载体注入层释放的移动离子的影响。 在某些情况下，阻挡层本身也可以是发光的。
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公开(公告)号：US5807627A
公开(公告)日：1998-09-15
申请号：US848952
申请日：1997-04-30
申请人： Richard Henry Friend , Andrew Bruce Holmes , Donal Donat Conor Bradley , Paul Leslie Burn , Arno Kraft , Adam Richard Brown , Jeremy Henley Burroughes , Neil Clement Greenham
发明人： Richard Henry Friend , Andrew Bruce Holmes , Donal Donat Conor Bradley , Paul Leslie Burn , Arno Kraft , Adam Richard Brown , Jeremy Henley Burroughes , Neil Clement Greenham
IPC分类号： C08G61/00 , C08G61/02 , C09K11/06 , H01L51/00 , H01L51/30 , H01L51/50 , H05B33/10 , H05B33/14 , B05D1/38
CPC分类号： H05B33/14 , C08G61/00 , C08G61/02 , C09K11/06 , H01L51/0043 , H01L51/5036 , H05B33/10 , H01L51/0038 , Y10S428/917 , Y10T428/24942 , Y10T428/31504 , Y10T428/31678
摘要： An electroluminescent device has at least two active semiconductive conjugated polymer light emitting layers arranged between a cathode and an anode. The layers are arranged so that at least part of at least two layers lie in an emission zone of the device.
摘要翻译： PCT No.PCT / GB93 / 01574 Sec。 371日期1995年3月31日 102（e）1995年3月31日PCT PCT 1993年7月26日PCT公布。 公开号WO94 / 03031 日期1994年2月3日电致发光器件具有布置在阴极和阳极之间的至少两个有源半导体共轭高分子发光层。 这些层被布置成使得至少两层的至少一部分位于装置的发射区域中。
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3.发明授权
公开(公告)号：US5653914A
公开(公告)日：1997-08-05
申请号：US481379
申请日：1995-10-02
申请人： Andrew Bruce Holmes , Arno Kraft , Paul Leslie Burn , Stephen Carl Moratti , Richard Henry Friend , Donal Donat Conor Bradley , Neil Clement Greenham , Adam Richard Brown , Josef Herbert Ferdinand Martens , Franco Cacialli , Johannes Gruener
发明人： Andrew Bruce Holmes , Arno Kraft , Paul Leslie Burn , Stephen Carl Moratti , Richard Henry Friend , Donal Donat Conor Bradley , Neil Clement Greenham , Adam Richard Brown , Josef Herbert Ferdinand Martens , Franco Cacialli , Johannes Gruener
摘要： An electroluminescent device is provided incorporating an emissive layer comprising a processible polymer matrix such as poly(methylmethacrylate) and a chromophoric component such as an asymmetric stilbene or distyrylbenzene. The chromophoric component is blended with the polymer matrix or covalently attached thereto as a side chain and is selected to emit radiation in the region 400 nm to 500 nm when excited to luminesce.
摘要翻译： PCT No.PCT / GB93 / 02586 Sec。 371 1995年10月2日日期 102（e）日期1995年10月2日PCT 1993年12月17日PCT PCT。 公开号WO94 / 15441 日期1994年7月7日提供一种电致发光器件，其结合有包含可加工聚合物基质如聚（甲基丙烯酸甲酯）和发色组分如不对称二苯乙烯或二苯乙烯基苯的发射层。 将发色组分与聚合物基质共混或共价连接到其上作为侧链，并且当激发发光时，其选择为在400nm至500nm的区域中发射辐射。
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公开(公告)号：US5672678A
公开(公告)日：1997-09-30
申请号：US506201
申请日：1995-09-18
申请人： Andrew Holmes , Donal Donat Bradley , Richard Henry Friend , Arno Kraft , Paul Burn , Adam Brown
发明人： Andrew Holmes , Donal Donat Bradley , Richard Henry Friend , Arno Kraft , Paul Burn , Adam Brown
IPC分类号： C08G61/02 , C07C43/205 , C07C43/225 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01B1/12 , H01L33/00 , H01L51/00 , H01L51/30 , H01L51/50 , H01L51/56 , H05B33/10 , H05B33/12 , H05B33/14 , C08G75/00
CPC分类号： H05B33/14 , C07C43/2055 , C07C43/225 , C08G61/00 , C09K11/06 , H01B1/127 , H01B1/128 , H01L51/0036 , H01L51/0038 , H01L51/0043 , H01L51/5012 , H01L51/5036 , H01L51/56 , Y10T428/3158 , Y10T428/31587 , Y10T428/31645
摘要： A semiconductive conjugated copolymer comprises at least two chemically different monomer units which, when existing in their individual homopolymer forms, have different semiconductor bandgaps. The proportion of said at least two chemically different monomer units in the copolymer is selected to control the semiconductor bandgap of the copolymer so as to control the optical properties of the copolymer. The copolymer is formed in a manner enabling it to be laid down as a film without substantially affecting the luminescent characteristics of the copolymer and is stable at operational temperature. The semiconductor bandgap may be spatially modulated so as to increase the quantum efficiency of the copolymer when excited to luminesce, to select the wavelength of radiation omitted during luminescence or to select the refractive index of the copolymer.
摘要翻译： 半导体共轭共聚物包含至少两种化学上不同的单体单元，当其各自的均聚物形式存在时，其具有不同的半导体带隙。 选择共聚物中所述至少两种化学上不同的单体单元的比例以控制共聚物的半导体带隙，从而控制共聚物的光学性能。 共聚物的形成方式使得其能够以膜形式放置而基本上不影响共聚物的发光特性，并且在操作温度下是稳定的。 半导体带隙可以被空间调制，以便当激发发光时提高共聚物的量子效率，以选择在发光期间省略的辐射波长或选择共聚物的折射率。
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公开(公告)号：US06403809B1
公开(公告)日：2002-06-11
申请号：US09508035
申请日：2000-05-30
申请人： Andrew Bruce Holmes , Stephen Carl Moratti , Xiao-Chang Li , Henning Sirringhaus , Arno Kraft , Michael Mark Murray
发明人： Andrew Bruce Holmes , Stephen Carl Moratti , Xiao-Chang Li , Henning Sirringhaus , Arno Kraft , Michael Mark Murray
IPC分类号： C07D33350
CPC分类号： H01L51/0036 , C07D495/04 , C07D495/14 , C08G61/126 , H01L51/0068 , H01L51/0074 , H01L51/0508 , Y10S362/80
摘要： The present invention provides a compound or complex comprising at least two moieties, each moiety being comprised of two or more thiophenes fused directly to each other. Also provided is a method for the production of the compounds of the present invention, which method comprises the coupling of one fused thiophene derivative to another fused thiophene derivative.
摘要翻译： 本发明提供了包含至少两个部分的化合物或复合物，每个部分由两个或更多个彼此直接融合的噻吩组成。 还提供了制备本发明化合物的方法，该方法包括将一种稠合噻吩衍生物与另一稠合噻吩衍生物的偶合。
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公开(公告)号：US06626566B2
公开(公告)日：2003-09-30
申请号：US10155823
申请日：2002-05-24
申请人： Andrew Bruce Holmes , Stephen Carl Moratti , Xiao-Chang Li , Henning Sirringhaus , Arno Kraft , Michael Mark Murray
发明人： Andrew Bruce Holmes , Stephen Carl Moratti , Xiao-Chang Li , Henning Sirringhaus , Arno Kraft , Michael Mark Murray
IPC分类号： G02F1136
CPC分类号： H01L51/0036 , C07D495/04 , C07D495/14 , C08G61/126 , H01L51/0068 , H01L51/0074 , H01L51/0508 , Y10S362/80
摘要： The present invention provides a compound or complex comprising at least two moieties, each moiety being comprised of two or more thiophenes fused directly to each other. Also provided is a method for the production of the compounds of the present invention, which method comprises the coupling of one fused thiophene derivative to another fused thiophene derivative.
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公开(公告)号：US5512654A
公开(公告)日：1996-04-30
申请号：US246269
申请日：1994-05-19
申请人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
发明人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
IPC分类号： C08G61/02 , C07C43/205 , C07C43/225 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01B1/12 , H01L33/00 , H01L51/00 , H01L51/30 , H01L51/50 , H01L51/56 , H05B33/10 , H05B33/12 , H05B33/14 , C08G75/00
CPC分类号： H05B33/14 , C07C43/2055 , C07C43/225 , C08G61/00 , C09K11/06 , H01B1/127 , H01B1/128 , H01L51/0036 , H01L51/0038 , H01L51/0043 , H01L51/5012 , H01L51/5036 , H01L51/56 , Y10T428/3158 , Y10T428/31587 , Y10T428/31645
摘要： A semiconductive conjugated copolymer comprises at least two chemically different monomer units which, when existing in their individual homopolymer forms, have different semiconductor bandgaps. The proportion of said at least two chemically different monomer units in the copolymer is selected to control the semiconductor bandgap of the copolymer so as to control the optical properties of the copolymer. The copolymer is formed in a manner enabling it to be laid down as a film without substantially affecting the luminescent characteristics of the copolymer and is stable at operational temperature.The semiconductor bandgap may be spatially modulated so as to increase the quantum efficiency of the copolymer when excited to luminesce, to select the wavelength of radiation emitted during luminescence or to select the refractive index of the copolymer.
摘要翻译： 半导体共轭共聚物包含至少两种化学上不同的单体单元，当其各自的均聚物形式存在时，其具有不同的半导体带隙。 选择共聚物中所述至少两种化学上不同的单体单元的比例以控制共聚物的半导体带隙，从而控制共聚物的光学性能。 共聚物的形成方式使得其能够以膜形式放置而基本上不影响共聚物的发光特性，并且在操作温度下是稳定的。 可以对半导体带隙进行空间调制，以便在激发发光时提高共聚物的量子效率，以选择在发光期间发射的辐射的波长或选择共聚物的折射率。
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公开(公告)号：US5425125A
公开(公告)日：1995-06-13
申请号：US199036
申请日：1994-02-18
申请人： Andrew B. Holmes , Donal D. Bradley , Richard H. Friend , Paul L. Burn , Arno Kraft , Adam R. Brown
发明人： Andrew B. Holmes , Donal D. Bradley , Richard H. Friend , Paul L. Burn , Arno Kraft , Adam R. Brown
IPC分类号： C08G61/02 , C07C43/205 , C07C43/225 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01B1/12 , H01L33/00 , H01L51/00 , H01L51/30 , H01L51/50 , H01L51/56 , H05B33/10 , H05B33/12 , H05B33/14 , G02B6/10
CPC分类号： H05B33/14 , C07C43/2055 , C07C43/225 , C08G61/00 , C09K11/06 , H01B1/127 , H01B1/128 , H01L51/0036 , H01L51/0038 , H01L51/0043 , H01L51/5012 , H01L51/5036 , H01L51/56 , Y10T428/3158 , Y10T428/31587 , Y10T428/31645
摘要： A method is provided for forming in a semiconductive conjugated polymer at least first and second legions having different optical properties. The method comprises: forming a layer of a precursor polymer and permitting the first region to come into contact with a reactant, such as an acid, and heat while permitting the second region to come into contact with a lower concentration of the reactant. The reactant affects the conversion conditions of the precursor polymer in such a way as to control the optical properties of at least the first region so that the optical properties of the first region are different from those of the second region. The precursor polymer may comprise a poly(arylene-1, 2-ethanediyl) polymer, at least some of the ethane groups of which include a modifier group whose susceptibility to elimination is increased in the presence of the reactant.
摘要翻译： 提供一种在半导体共轭聚合物中形成具有不同光学特性的至少第一和第二团粒的方法。 该方法包括：形成前体聚合物层，并允许第一区域与反应物（例如酸）接触并加热，同时允许第二区域与较低浓度的反应物接触。 反应物以这样的方式影响前体聚合物的转化条件，以便控制至少第一区域的光学性质，使得第一区域的光学性质与第二区域的光学性质不同。 前体聚合物可以包含聚（亚芳基-1,2-乙二基）聚合物，其中至少一些乙烷基团包括在反应物存在下易于消除的易感性的改性剂基团。
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公开(公告)号：US5401827A
公开(公告)日：1995-03-28
申请号：US748777
申请日：1991-08-22
申请人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
发明人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
IPC分类号： C08G61/02 , C07C43/205 , C07C43/225 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01B1/12 , H01L33/00 , H01L51/00 , H01L51/30 , H01L51/50 , H01L51/56 , H05B33/10 , H05B33/12 , H05B33/14 , C08G75/04
CPC分类号： H05B33/14 , C07C43/2055 , C07C43/225 , C08G61/00 , C09K11/06 , H01B1/127 , H01B1/128 , H01L51/0036 , H01L51/0038 , H01L51/0043 , H01L51/5012 , H01L51/5036 , H01L51/56 , Y10T428/3158 , Y10T428/31587 , Y10T428/31645
摘要： A semiconductive conjugated copolymer comprises at least two chemically different monomer units which, when existing in their individual homopolymer forms, have different semiconductor bandgaps. The proportion of said at least two chemically different monomer units in the copolymer is selected to control the semiconductor bandgap of the copolymer so as to control the optical properties of the copolymer. The copolymer is formed in a manner enabling it to be laid down as a film without substantially affecting the luminescent characteristics of the copolymer and is stable at operational temperature.The semiconductor bandgap may be spatially modulated so as to increase the quantum efficiency of the copolymer when excited to luminesce, to select the wavelength of radiation omitted during luminescence or to select the refractive index of the copolymer.
摘要翻译： 半导体共轭共聚物包含至少两种化学上不同的单体单元，当其各自的均聚物形式存在时，其具有不同的半导体带隙。 选择共聚物中所述至少两种化学上不同的单体单元的比例以控制共聚物的半导体带隙，从而控制共聚物的光学性能。 共聚物的形成方式使得其能够以膜形式放置而基本上不影响共聚物的发光特性，并且在操作温度下是稳定的。 半导体带隙可以被空间调制，以便当激发发光时提高共聚物的量子效率，以选择在发光期间省略的辐射波长或选择共聚物的折射率。
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公开(公告)号：US5328809A
公开(公告)日：1994-07-12
申请号：US748795
申请日：1991-08-22
申请人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
发明人： Andrew Holmes , Donal D. Bradley , Richard H. Friend , Arno Kraft , Paul Burn , Adam Brown
IPC分类号： C08G61/02 , C07C43/205 , C07C43/225 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01B1/12 , H01L33/00 , H01L51/00 , H01L51/30 , H01L51/50 , H01L51/56 , H05B33/10 , H05B33/12 , H05B33/14 , B05D1/32 , G03C5/00
CPC分类号： H05B33/14 , C07C43/2055 , C07C43/225 , C08G61/00 , C09K11/06 , H01B1/127 , H01B1/128 , H01L51/0036 , H01L51/0038 , H01L51/0043 , H01L51/5012 , H01L51/5036 , H01L51/56 , Y10T428/3158 , Y10T428/31587 , Y10T428/31645
摘要： A method is provided for forming in a semiconductive conjugated polymer at least first and second regions having different optical properties. The method comprises: forming a layer of a precursor polymer and permitting the first region to come into contact with a reactant, such as an acid, and heat while permitting the second region to come into contact with a lower concentration of the reactant. The reactant affects the conversion conditions of the precursor polymer in such a way as to control the optical properties of at least the first region so that the optical properties of the first region are different from those of the second region.The precursor polymer may comprise a poly(arylene-1,2-ethanediyl) polymer, at least some of the ethane groups of which include a modifier group whose susceptibility to elimination is increased in the presence of the reactant.
摘要翻译： 提供一种在半导体共轭聚合物中形成具有不同光学特性的至少第一和第二区域的方法。 该方法包括：形成前体聚合物层，并允许第一区域与反应物（例如酸）接触并加热，同时允许第二区域与较低浓度的反应物接触。 反应物以这样的方式影响前体聚合物的转化条件，以便控制至少第一区域的光学性质，使得第一区域的光学性质与第二区域的光学性质不同。 前体聚合物可以包含聚（亚芳基-1,2-乙二基）聚合物，其中至少一些乙烷基团包括其在反应物存在下易于消除的易感性的改性剂基团。
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