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    Multi component catalyst and its use in catalytic cracking
    1.
    发明授权
    Multi component catalyst and its use in catalytic cracking 有权
    多组分催化剂及其在催化裂化中的应用

    公开(公告)号：US07326332B2

    公开(公告)日：2008-02-05

    申请号：US10671080

    申请日：2003-09-25

    申请人： Tan-Jen Chen ,  John Scott Buchanan ,  Brian Erik Henry ,  Paul F. Keusenkothen ,  Philip A. Ruziska ,  David L. Stern

    发明人： Tan-Jen Chen ,  John Scott Buchanan ,  Brian Erik Henry ,  Paul F. Keusenkothen ,  Philip A. Ruziska ,  David L. Stern

    IPC分类号： C10G11/00 ,  C10G11/05

    CPC分类号： C10G11/05 ,  B01J29/005 ,  B01J29/40 ,  B01J29/85

    摘要： A multi component catalyst and catalytic cracking process for selectively producing C3 olefins. The catalyst comprises a first molecular sieve having an intermediate pore size, a second molecular sieve and, optionally a third molecular sieve having a large pore size. At least one of the channels of the second molecular sieve has a pore size index that is less than the pore size index of at least one channel of the first molecular sieve. The process is carried out by contacting a feedstock containing hydrocarbons having at least 5 carbon atoms is contacted, under catalytic cracking conditions, with the multi component catalyst. The catalyst finds application in the cracking of naphtha and heavy hydrocarbon feedstocks.

    摘要翻译： 用于选择性制备C 3 O 3烯烃的多组分催化剂和催化裂解方法。 催化剂包括具有中等孔径的第一分子筛，第二分子筛和任选的具有大孔径的第三分子筛。 第二分子筛的至少一个通道的孔径指数小于第一分子筛的至少一个通道的孔径指数。 该方法通过使含有至少5个碳原子的烃的原料在催化裂化条件下与多组分催化剂接触来进行。 该催化剂可用于石脑油和重质烃原料的裂解。

    Hydrothermally stable catalyst and its use in catalytic cracking
    2.
    发明授权
    Hydrothermally stable catalyst and its use in catalytic cracking 失效
    水热稳定催化剂及其在催化裂化中的应用

    公开(公告)号：US07615143B2

    公开(公告)日：2009-11-10

    申请号：US10903152

    申请日：2004-07-30

    申请人： Tan-Jen Chen ,  Paul F. Keusenkothen ,  J. Jason Wu ,  John Scott Buchanan ,  Guang Cao ,  Larry L. Iaccino ,  David L. Stern ,  Matthew J. Vincent

    发明人： Tan-Jen Chen ,  Paul F. Keusenkothen ,  J. Jason Wu ,  John Scott Buchanan ,  Guang Cao ,  Larry L. Iaccino ,  David L. Stern ,  Matthew J. Vincent

    IPC分类号： C10G11/05

    CPC分类号： C10G11/05 ,  C10G2400/20

    摘要： There is provided a catalyst composition having improved hydrothermal stability for the catalytic cracking of a hydrocarbon feedstock to selectively produce propylene. The catalyst composition comprises a first crystalline molecular sieve selected from the group consisting of IM-5, MWW, ITH, FER, MFS, AEL, and AFO and an effective amount of a stabilization metal (copper, zirconium, or mixtures thereof) exchanged into the molecular sieve. The catalyst finds application in the cracking of naphtha and heavy hydrocarbon feedstocks. When used in the catalytic cracking of heavier hydrocarbon feedstocks, the catalyst composition preferably comprises a second molecular sieve having a pore size that is greater than the pore size of the first molecular sieve. The process is carried out by contacting a feedstock containing hydrocarbons having at least 4 carbon atoms is contacted, under catalytic cracking conditions, with the catalyst composition.

    摘要翻译： 提供了一种具有改进的水热稳定性用于烃原料的催化裂化以选择性地生产丙烯的催化剂组合物。 催化剂组合物包含选自由IM-5，MWW，ITH，FER，MFS，AEL和AFO组成的组的第一结晶分子筛和有效量的稳定金属（铜，锆或其混合物）交换成 分子筛。 该催化剂可用于石脑油和重质烃原料的裂解。 当用于较重烃原料的催化裂化时，催化剂组合物优选包含具有大于第一分子筛孔径的孔径的第二分子筛。 该方法通过使含有至少4个碳原子的烃的原料在催化裂化条件下与催化剂组合物接触来进行。

    Method for selectively producing propylene by catalytically cracking an olefinic hydrocarbon feedstock
    3.
    发明授权
    Method for selectively producing propylene by catalytically cracking an olefinic hydrocarbon feedstock 失效
    通过催化裂化烯烃原料选择性生产丙烯的方法

    公开(公告)号：US06429348B1

    公开(公告)日：2002-08-06

    申请号：US09073148

    申请日：1998-05-05

    申请人： Tan-Jen Chen ,  S. Mark Davis ,  Luc R. M. Martens ,  Marcel J. G. Janssen ,  Philip A. Ruziska

    发明人： Tan-Jen Chen ,  S. Mark Davis ,  Luc R. M. Martens ,  Marcel J. G. Janssen ,  Philip A. Ruziska

    IPC分类号： C07C406

    CPC分类号： C07C4/06 ,  B01J29/85 ,  C07C2529/84 ,  C07C2529/85 ,  C10G2400/20 ,  Y02P20/52

    摘要： The invention provides a method for converting an olefinic hydrocarbon feedstock to propylene comprising: contacting a hydrocarbon feedstock under catalytic cracking conditions with a catalyst comprising a catalyst selected from the group consisting of SAPO catalysts, MeAPO catalysts, MeASPO catalysts, ElAPO catalysts, ElASPO catalysts, rare earth exchanged catalysts from any of the preceding groups, and mixtures thereof, under cracking conditions to selectively produce propylene. The invention further provides a method for stabilizing a catalyst to steam from the foregoing group by ion exchange with a rare earth metal. A catalyst has enhanced stability as used herein when treated with a rare earth metal or metals in a concentration effective to provide a catalyst which exhibits a higher conversion of a hydrocarbon feedstock to propylene than does an equal quantity of an untreated sample of the same catalyst under the same conditions following exposure of each catalyst to steam for a period of at least 10 hours.

    摘要翻译： 本发明提供了一种将烯烃原料转化成丙烯的方法，包括：在催化裂化条件下使烃原料与包含选自SAPO催化剂，MeAPO催化剂，MeASPO催化剂，ElAPO催化剂，ElASPO催化剂， 在裂化条件下稀土交换任何前述基团的催化剂及其混合物，以选择性地生产丙烯。 本发明还提供了一种通过与稀土金属离子交换将催化剂稳定化成来自上述组的蒸汽的方法。 当用稀土金属或金属处理时，催化剂具有增强的稳定性，该稀土金属或金属的浓度有效地提供催化剂，其表现出比同样催化剂下的相同催化剂的等量的未处理样品的烃原料比丙烯更高的转化率 在每种催化剂暴露于蒸汽至少10小时的时间后，相同的条件。

    Process for producing cyclohexylbenzene
    6.
    发明授权
    Process for producing cyclohexylbenzene 有权
    生产环己基苯的方法

    公开(公告)号：US07906685B2

    公开(公告)日：2011-03-15

    申请号：US12601572

    申请日：2008-08-12

    申请人： Tan-Jen Chen ,  Francisco M. Benitez ,  Jane C. Cheng ,  Jon E. Stanat ,  John Scott Buchanan

    发明人： Tan-Jen Chen ,  Francisco M. Benitez ,  Jane C. Cheng ,  Jon E. Stanat ,  John Scott Buchanan

    IPC分类号： C07C45/27 ,  C07C27/08 ,  C07C2/68 ,  C07C15/067

    CPC分类号： C07C2/74 ,  Y02P20/52 ,  C07C13/28

    摘要： In a process for producing cyclohexylbenzene, benzene and hydrogen are fed to at least one reaction zone. The benzene and hydrogen are then contacted in the at least one reaction zone under hydroalkylation conditions with a catalyst system comprising a molecular sieve having an X-ray diffraction pattern including d-spacing maxima at 12.4±0.25, 6.9±0.15, 3.57±0.07 and 3.42±0.07 Angstrom, and at least one hydrogenation metal to produce an effluent containing cyclohexylbenzene. The ratio of the total number of moles of hydrogen fed to said at least one reaction zone to the number of moles of benzene fed to said at least one reaction zone is between 0.4 and 0.9:1.

    摘要翻译： 在生产环己基苯的方法中，将苯和氢气进料至至少一个反应区。 然后使苯和氢在加氢烷基化条件下在至少一个反应区中与包含分子筛的催化剂体系接触，所述催化剂体系包含具有12.4±0.25,6.9±0.15,3.57±0.07的d间距最大值的X射线衍射图， 3.42±0.07埃，和至少一种氢化金属，以生产含有环己基苯的流出物。 供给到所述至少一个反应区的氢的总摩尔数与进料到所述至少一个反应区的苯的摩尔数之比为0.4-0.9:1。

    Process For Producing Cyclohexylbenzene
    8.
    发明申请
    Process For Producing Cyclohexylbenzene 有权
    生产环己基苯的方法

    公开(公告)号：US20100197971A1

    公开(公告)日：2010-08-05

    申请号：US12601572

    申请日：2008-08-12

    申请人： Tan-Jen Chen ,  Francisco M. Benitez ,  Jane C. Cheng ,  Jon E. Stanat ,  John Scott Buchanan

    发明人： Tan-Jen Chen ,  Francisco M. Benitez ,  Jane C. Cheng ,  Jon E. Stanat ,  John Scott Buchanan

    IPC分类号： C07C5/10 ,  C07C45/27 ,  C07C37/08

    CPC分类号： C07C2/74 ,  Y02P20/52 ,  C07C13/28

    摘要： In a process for producing cyclohexylbenzene, benzene and hydrogen are fed to at least one reaction zone. The benzene and hydrogen are then contacted in the at least one reaction zone under hydroalkylation conditions with a catalyst system comprising a molecular sieve having an X-ray diffraction pattern including d-spacing maxima at 12.4±0.25, 6.9±0.15, 3.57±0.07 and 3.42±0.07 Angstrom, and at least one hydrogenation metal to produce an effluent containing cyclohexylbenzene. The ratio of the total number of moles of hydrogen fed to said at least one reaction zone to the number of moles of benzene fed to said at least one reaction zone is between 0.4 and 0.9:1.

    摘要翻译： 在生产环己基苯的方法中，将苯和氢气进料至至少一个反应区。 然后使苯和氢在加氢烷基化条件下在至少一个反应区中与包含分子筛的催化剂体系接触，所述催化剂体系包含具有12.4±0.25,6.9±0.15,3.57±0.07的d间距最大值的X射线衍射图， 3.42±0.07埃，和至少一种氢化金属，以生产含有环己基苯的流出物。 供给到所述至少一个反应区的氢的总摩尔数与进料到所述至少一个反应区的苯的摩尔数之比为0.4-0.9:1。