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公开(公告)号：US20140336422A1
公开(公告)日：2014-11-13
申请号：US13885611
申请日：2011-11-04
申请人： Jihad M. Dakka , Teng Xu , Edward A. Lemon , James R. Lattner , Jane C. Cheng
发明人： Jihad M. Dakka , Teng Xu , Edward A. Lemon , James R. Lattner , Jane C. Cheng
CPC分类号： C07C2/66 , C07C37/07 , C07C37/08 , C07C45/53 , C07C2529/08 , C07C2529/18 , C07C2529/70 , Y02P20/127 , C07C13/28
摘要： In a process for producing mono-cycloalkyl-substituted aromatic compound, benzene and cyclic monoolefin are contacted with a catalyst under alkylation conditions to produce an effluent containing mono-cycloalkyl-substituted aromatic compound. The catalyst comprises a molecular sieve.
摘要翻译： 在制备单环烷基取代的芳族化合物的方法中，苯和环状单烯烃在烷基化条件下与催化剂接触以产生含有单环烷基取代的芳族化合物的流出物。 催化剂包括分子筛。
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公开(公告)号：US08633343B2
公开(公告)日：2014-01-21
申请号：US13264464
申请日：2010-04-14
申请人： Kun Wang , Jane C. Cheng , Terry E. Helton
发明人： Kun Wang , Jane C. Cheng , Terry E. Helton
CPC分类号： C07C409/14 , C07C2/74 , C07C6/126 , C07C37/08 , C07C45/53 , C07C407/00 , C07C2521/04 , C07C2521/06 , C07C2529/08 , C07C2529/18 , C07C2529/70 , C07C2601/14 , Y02P20/52 , C07C13/28 , C07C39/04 , C07C49/403
摘要： In a process for the transalkylation of polycyclohexylbenzenes, a feed containing at least one polycyclohexylbenzene is contacted with benzene under transalkylation conditions with a catalyst comprising a zeolite USY having a silica to alumina molar ratio in excess of 10 to convert at least part of said polycyclohexylbenzene to cyclohexylbenzene.
摘要翻译： 在聚环己基苯的烷基转移的方法中，将含有至少一种聚环己基苯的进料在烷基转移条件下与苯接触，其中催化剂包含二氧化硅与氧化铝摩尔比超过10的沸石USY，以将至少部分所述多环己基苯转化为 环己基苯。
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公开(公告)号：US08440864B2
公开(公告)日：2013-05-14
申请号：US13060773
申请日：2009-08-04
CPC分类号： C07C7/163 , C07C2/66 , C07C7/14891 , C07C37/08 , C07C37/20 , C07C45/53 , C07C407/00 , C07C409/08 , C07C2529/70 , Y02P20/127 , C07C15/02 , C07C11/08 , C07C49/10 , C07C39/04 , C07C39/16
摘要： In a process for producing sec-butylbenzene, a C4 olefinic hydrocarbon feedstock comprising isobutene and at least one n-butene is contacted with methanol and/or water in the presence of an acid catalyst to selectively oxygenate isobutene to produce an effluent stream rich in n-butene and containing less isobutene than the feedstock. The effluent stream is then contacted with benzene under alkylation conditions and in the presence of an alkylation catalyst to produce alkylation stream comprising sec-butylbenzene.
摘要翻译： 在制备仲丁基苯的方法中，包含异丁烯和至少一个正丁烯的C 4烯烃原料在酸催化剂的存在下与甲醇和/或水接触以选择性地使异丁烯氧化以产生富含n 并且含有比原料少的异丁烯。 然后在烷基化条件下和在烷基化催化剂的存在下将流出物流与苯接触以产生包含仲丁基苯的烷基化流。
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公开(公告)号：US08436213B2
公开(公告)日：2013-05-07
申请号：US13060335
申请日：2009-08-04
申请人： Jihad M. Dakka , Jane C. Cheng , John S. Buchanan
发明人： Jihad M. Dakka , Jane C. Cheng , John S. Buchanan
CPC分类号： C07C37/08 , C07C2/08 , C07C2/66 , C07C5/03 , C07C6/126 , C07C7/14858 , C07C45/53 , C07C2529/08 , C07C2529/18 , C07C2529/70 , C07C9/12 , C07C15/02 , C07C49/10 , C07C39/04
摘要： In a process for reducing the level of tert-butylbenzene in a mixed butylbenzene feed comprising tert-butylbenzene and sec-butylbenzene, the feed is contacted under dealkylation conditions with a catalyst system comprising a dealkylation catalyst whereby the tert-butylbenzene is selectively dealkylated to produce an effluent stream which comprises benzene and which has a lower concentration of tert-butylbenzene than said feed.
摘要翻译： 在降低包含叔丁基苯和仲丁基苯的混合丁苯进料中的叔丁基苯含量的方法中，进料在脱烷基化条件下与包含脱烷基化催化剂的催化剂体系接触，由此使叔丁基苯选择性脱烷基化以产生 包含苯并且具有比所述进料更低浓度的叔丁基苯的流出物流。
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公开(公告)号：US08247627B2
公开(公告)日：2012-08-21
申请号：US12933935
申请日：2009-03-16
申请人： Jihad M. Dakka , J. Scott Buchanan , Jane C. Cheng , Tan-Jen Chen , Lorenzo C. DeCaul , Terry E. Helton , Jon E. Stanat , Francisco M. Benitez
发明人： Jihad M. Dakka , J. Scott Buchanan , Jane C. Cheng , Tan-Jen Chen , Lorenzo C. DeCaul , Terry E. Helton , Jon E. Stanat , Francisco M. Benitez
CPC分类号： C07C37/08 , B01J29/064 , B01J29/7215 , B01J29/7276 , C07C2/74 , C07C37/07 , C07C45/53 , C07C407/00 , C07C409/14 , C07C2601/14 , Y02P20/52 , C07C13/28 , C07C49/403 , C07C39/04
摘要： In a process for producing phenol and/or cyclohexanone, benzene and hydrogen are contacted with a first catalyst in a hydroalkylation step to produce a first effluent stream comprising cyclohexylbenzene, cyclohexane, and unreacted benzene. At least part of the first effluent stream is supplied to a first separation system to divide the first effluent stream part into a cyclohexylbenzene-rich stream and a C6 product stream comprising unreacted benzene and cyclohexane.
摘要翻译： 在制备苯酚和/或环己酮的方法中，苯和氢在加氢烷基化步骤中与第一催化剂接触以产生包含环己基苯，环己烷和未反应苯的第一流出料流。 将第一流出物流的至少一部分供应到第一分离系统，以将第一流出物流部分分解成富含环己基苯的物流和包含未反应的苯和环己烷的C6产物流。
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公开(公告)号：US08178728B2
公开(公告)日：2012-05-15
申请号：US12920383
申请日：2009-02-24
申请人： Jane C. Cheng , Tan-Jen Chen , Prasenjeet Ghosh
发明人： Jane C. Cheng , Tan-Jen Chen , Prasenjeet Ghosh
CPC分类号： B01J29/7088 , B01J21/04 , B01J23/44 , B01J29/7476 , B01J29/7676 , B01J35/0006 , B01J37/0009 , B01J2229/42 , C07C2/74 , C07C6/126 , C07C37/07 , C07C37/08 , C07C45/53 , C07C407/00 , C07C409/14 , C07C2521/04 , C07C2521/06 , C07C2523/44 , C07C2529/74 , C07C2529/76 , C07C2601/14 , Y02P20/52 , C07C13/28 , C07C49/403 , C07C39/04
摘要： In a process for producing cyclohexylbenzene, benzene and hydrogen are contacted under hydroalkylation conditions with a catalyst system comprising a MCM-22 family molecular sieve and at least one hydrogenation metal. The conditions comprise a temperature of about 140° C. to about 175° C., a pressure of about 135 psig to about 175 psig (931 kPag to 1207 kPag), a hydrogen to benzene molar ratio of about 0.30 to about 0.65 and a weight hourly space velocity of benzene of about 0.26 to about 1.05 hr−1.
摘要翻译： 在制备环己基苯的方法中，苯和氢在加氢烷基化条件下与包含MCM-22族分子筛和至少一种氢化金属的催化剂体系接触。 条件包括约140℃至约175℃的温度，约135psig至约175psig（931kPag至1207kPag）的压力，约0.30至约0.65的氢至苯摩尔比和 苯的重时空速为约0.26至约1.05小时-1。
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公开(公告)号：US20120046499A1
公开(公告)日：2012-02-23
申请号：US13264464
申请日：2010-04-14
申请人： Kun Wang , Jane C. Cheng , Terry E. Helton
发明人： Kun Wang , Jane C. Cheng , Terry E. Helton
CPC分类号： C07C409/14 , C07C2/74 , C07C6/126 , C07C37/08 , C07C45/53 , C07C407/00 , C07C2521/04 , C07C2521/06 , C07C2529/08 , C07C2529/18 , C07C2529/70 , C07C2601/14 , Y02P20/52 , C07C13/28 , C07C39/04 , C07C49/403
摘要： In a process for the transalkylation of polycyclohexylbenzenes, a feed containing at least one polycyclohexylbenzene is contacted with benzene under transalkylation conditions with a catalyst comprising a zeolite USY having a silica to alumina molar ratio in excess of 10 to convert at least part of said polycyclohexylbenzene to cyclohexylbenzene.
摘要翻译： 在聚环己基苯的烷基转移的方法中，将含有至少一种聚环己基苯的进料在烷基转移条件下与苯接触，其中催化剂包含二氧化硅与氧化铝摩尔比超过10的沸石USY，以将至少部分所述多环己基苯转化为 环己基苯。
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公开(公告)号：US20110160489A1
公开(公告)日：2011-06-30
申请号：US13060335
申请日：2009-08-04
申请人： Jihad M. Dakka , Jane C. Cheng , John Buchanan
发明人： Jihad M. Dakka , Jane C. Cheng , John Buchanan
CPC分类号： C07C37/08 , C07C2/08 , C07C2/66 , C07C5/03 , C07C6/126 , C07C7/14858 , C07C45/53 , C07C2529/08 , C07C2529/18 , C07C2529/70 , C07C9/12 , C07C15/02 , C07C49/10 , C07C39/04
摘要： In a process for reducing the level of tert-butylbenzene in a mixed butylbenzene feed comprising tert-butylbenzene and sec-butylbenzene, the feed is contacted under dealkylation conditions with a catalyst system comprising a dealkylation catalyst whereby the tert-butylbenzene is selectively dealkylated to produce an effluent stream which comprises benzene and which has a lower concentration of tert-butylbenzene than said feed.
摘要翻译： 在降低包含叔丁基苯和仲丁基苯的混合丁苯进料中的叔丁基苯含量的方法中，进料在脱烷基化条件下与包含脱烷基化催化剂的催化剂体系接触，由此叔丁基苯选择性脱烷基化以产生 包含苯并且具有比所述进料更低浓度的叔丁基苯的流出物流。
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公开(公告)号：US07939693B2
公开(公告)日：2011-05-10
申请号：US12666333
申请日：2008-07-11
申请人： Jane C. Cheng , Jihad M. Dakka , Travis A. Reine , Jon E. Stanat
发明人： Jane C. Cheng , Jihad M. Dakka , Travis A. Reine , Jon E. Stanat
IPC分类号： C07C45/00 , C07C37/08 , C07C15/067
CPC分类号： C07C409/08 , C07C2/66 , C07C37/08 , C07C45/53 , C07C407/00 , Y02P20/127 , C07C15/02 , C07C49/10 , C07C39/04
摘要： A process for producing sec-butylbenzene comprises feeding reactants comprising benzene and a C4 olefin to a distillation column reactor having a first reaction zone containing an alkylation catalyst and a second distillation zone, which is located below said first reaction zone and which is substantially free of alkylation catalyst, wherein the ratio of the number of distillation stages in said first reaction zone to the number of distillation stages in said second distillation zone is less than 1:1. Concurrently in the distillation reactor, the reactants are contacted with the alkylation catalyst in the first reaction zone under conditions such that the C4 olefin reacts with the benzene to produce sec-butylbenzene and the sec-butylbenzene is fractioned from the unreacted C4 olefin. The sec-butylbenzene thereby passes as a liquid phase stream from the first reaction zone to the second distillation zone and the liquid phase steam is withdrawn from the distillation column reactor as bottoms.
摘要翻译： 一种生产仲丁基苯的方法包括将含有苯和C 4烯烃的反应物进料到具有含有烷基化催化剂和第二蒸馏区的第一反应区的蒸馏塔反应器中，所述第一反应区位于所述第一反应区之下且基本上不含 烷基化催化剂，其中所述第一反应区中的蒸馏级数与所述第二蒸馏区中的蒸馏级数之比小于1:1。 同时在蒸馏反应器中，使反应物与第一反应区中的烷基化催化剂接触，使得C 4烯烃与苯反应产生仲丁基苯，仲丁基苯从未反应的C 4烯烃中分馏。 因此，仲丁基苯作为液相物流从第一反应区流向第二蒸馏区，液相蒸汽作为底部从蒸馏塔反应器中排出。
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公开(公告)号：US07910779B2
公开(公告)日：2011-03-22
申请号：US12904215
申请日：2010-10-14
IPC分类号： C07C45/27 , C07C27/08 , C07C2/68 , C07C15/067
CPC分类号： C07C2/74 , C07C37/08 , C07C45/53 , C07C2521/04 , C07C2521/06 , C07C2523/06 , C07C2523/14 , C07C2523/44 , C07C2523/46 , C07C2523/75 , C07C2523/755 , C07C2529/70 , C07C2529/74 , C07C2601/14 , Y02P20/52 , C07C13/28 , C07C39/04 , C07C49/403
摘要： In a process for producing cyclohexylbenzene, benzene and hydrogen are fed to at least one reaction zone. The benzene and hydrogen are then contacted in the at least one reaction zone under hydroalkylation conditions with a catalyst system comprising a molecular sieve having an X-ray diffraction pattern including d-spacing maxima at 12.4±0.25, 6.9±0.15, 3.57±0.07 and 3.42±0.07 Angstrom, and at least one hydrogenation metal to produce an effluent containing cyclohexylbenzene. The catalyst system has an acid-to-metal molar ratio of from about 75 to about 750.
摘要翻译： 在生产环己基苯的方法中，将苯和氢气进料至至少一个反应区。 然后使苯和氢在加氢烷基化条件下在至少一个反应区中与包含分子筛的催化剂体系接触，所述催化剂体系包含具有12.4±0.25,6.9±0.15,3.57±0.07的d间距最大值的X射线衍射图， 3.42±0.07埃，和至少一种氢化金属，以生产含有环己基苯的流出物。 催化剂体系具有约75-约750的酸 - 金属摩尔比。
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