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    PROCESS FOR CONVERTING METHANE INTO A HIGHER ALKANE MIXTURE.
    7.
    发明申请
    PROCESS FOR CONVERTING METHANE INTO A HIGHER ALKANE MIXTURE. 审中-公开
    将甲烷转化为较高的烷烃混合物的方法。

    公开(公告)号：WO2008075031A1

    公开(公告)日：2008-06-26

    申请号：PCT/GB2007/004866

    申请日：2007-12-18

    Applicant: BP OIL INTERNATIONAL LIMITED ,  BASSET, Jean-Marie ,  CHAKKA, Sudhakar ,  SOULIVONG, Daravong ,  TAOUFIK, Mostafa ,  THIVOLLE-CAZAT, Jean

    Inventor： BASSET, Jean-Marie ,  CHAKKA, Sudhakar ,  SOULIVONG, Daravong ,  TAOUFIK, Mostafa ,  THIVOLLE-CAZAT, Jean

    IPC: C07C6/10 ,  C07C9/08 ,  C07C9/10 ,  C07C9/14

    CPC classification number: C07C6/10 ,  C07C2521/08 ,  C07C2531/12 ,  C07C9/10 ,  C07C9/14 ,  C07C9/08

    Abstract: The present invention relates to a process for converting methane into a higher alkane mixture, preferably a liquid alkane mixture, comprising (C 3+ ) alkanes having 3 carbon atoms and more, preferably (C 4+ ) alkanes having 4 carbon atoms, especially (C 5+ ) alkanes having 5 carbon atoms and more. The process comprises: - a stage (1) comprising contacting methane with a metal catalyst (C1) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C-C and/or C-H and/or C-metal bonds, so as to form by a non-oxidative methane coupling reaction a mixture (M1) comprising ethane and hydrogen, - preferably a stage (2) comprising fractionating the mixture (M1) so as to separate and to isolate the ethane, and - a stage (3) comprising, preferably simultaneously, (i) contacting the mixture (M1) or preferably the ethane isolated in stage (2) with a metal catalyst (C2) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C-C and/or C-H and/or C-metal bonds, said catalyst being identical to or different from catalyst (C1), so as to form by simultaneous ethane self- and cross-metathesis reactions a mixture (M2) comprising methane and the higher alkane mixture, and (ii) fractionating the mixture (M2) so as to separate and to isolate said higher alkane mixture, preferably in liquid form, and particularly the methane which is preferably recycled into stage (1). The hydrogen produced in stage (1) is preferably separated and isolated in stage (2) and then used for various applications and stages, e.g. for producing thermal and/or electrical energies preferably employed to run the process.

    Abstract translation: 本发明涉及一种将甲烷转化为高级烷烃混合物，优选液体烷烃混合物的方法，其包含具有3个碳原子的（C 3+ +）烷烃和更多（优选（C 4） 具有4个碳原子的烷烃，特别是具有5个碳原子的（C 5+ +）烷烃等。 该方法包括： - 阶段（1），其包括使甲烷与能够与烷烃接触的金属催化剂（C1）接触涉及CC和/或CH和/或C - 金属键的分解和重组的反应，因此 通过非氧化甲烷偶联反应形成包含乙烷和氢气的混合物（M1），优选包括分级分离混合物（M1）的阶段（2），以分离和分离乙烷，和 - 阶段 3）优选同时包含（i）将阶段（2）中分离的混合物（M1）或优选乙烷与能够与烷烃接触的金属催化剂（C2）接触涉及CC的分解和重组的反应 和/或CH和/或C - 金属键，所述催化剂与催化剂（C1）相同或不同，以便通过同时进行乙烷自身和交叉复分解反应形成包含甲烷和高级烷烃的混合物（M2） 混合物，和（ii）将混合物（M2）分馏 分离并分离所述高级烷烃混合物，优选液体形式，特别是优选循环至级（1）的甲烷。 在阶段（1）中产生的氢优选在阶段（2）中分离和分离，然后用于各种应用和阶段，例如， 用于产生优选用于运行该过程的热能和/或电能。

    GAS TO LIQUID CONVERSION PROCESS
    9.
    发明申请
    GAS TO LIQUID CONVERSION PROCESS 审中-公开
    气体转化过程

    公开(公告)号：WO2003080546A1

    公开(公告)日：2003-10-02

    申请号：PCT/US2003/008078

    申请日：2003-03-17

    Applicant: ENERGY TECHNOLOGIES GROUP, INC.

    Inventor： SHERWOOD, Steven, P.

    IPC: C07C2/00

    CPC classification number: C07C2/76 ,  C07C9/08

    Abstract: A process is disclosed for the conversion of lower molecular weight hydrocarbons, such as methane, into higher molecular weight hydrocarbon products, such as hydrocarbons having between 4 and 29 carbons. The process includes forming hydrated electrons, such as by mixing the lower molecular weight hydrocarbons with water and contacting the mixture with an energy source to form hydrated electrons. The hydrated electrons react with the methane to form hydrogen and higher molecular weight hydrocarbon products. Also disclosed is a related process for converting higher molecular weight hydrocarbons to lower molecular weight hydrocarbons by forming a mixture of higher molecular weight hydrocarbons and water and contacting the mixture with an energy source to form hydrated electrons that react with the higher molecular weight hydrocarbons to form hydrogen and lower molecular weight hydrocarbon products.

    Abstract translation: 公开了一种将较低分子量烃如甲烷转化为较高分子量烃产物如具有4至29个碳原子的烃的方法。 该方法包括形成水合电子，例如通过将低分子量烃与水混合并使该混合物与能量源接触以形成水合电子。 水合电子与甲烷反应形成氢气和较高分子量的烃产物。 还公开了通过形成较高分子量烃和水的混合物将较高分子量烃转化为较低分子量烃并使该混合物与能量源接触以形成与较高分子量烃反应形成的水合电子的相关方法 氢和低分子量烃产物。

    PROPANE RECOVERY PROCESS
    10.
    发明申请
    PROPANE RECOVERY PROCESS 审中-公开
    丙烷回收方法

    公开(公告)号：WO1997016505A1

    公开(公告)日：1997-05-09

    申请号：PCT/IB1996001249

    申请日：1996-11-01

    Applicant: McDERMOTT ENGINEERS & CONSTRUCTORS (CANADA) LTD.

    Inventor： McDERMOTT ENGINEERS & CONSTRUCTORS (CANADA) LTD. ,  SORENSEN, James, N.

    IPC: C10G05/04

    CPC classification number: B01D53/1418 ,  C07C7/005 ,  C10G5/04 ,  F25J3/0209 ,  F25J3/0233 ,  F25J3/0242 ,  F25J2200/04 ,  F25J2200/08 ,  F25J2200/70 ,  F25J2200/74 ,  F25J2200/78 ,  F25J2205/02 ,  F25J2235/60 ,  F25J2245/02 ,  F25J2270/04 ,  C07C9/08

    Abstract: Increased recovery of propane, butane and other heavier components found in a natural gas stream is achieved by installing an absorber upstream from an expander and a separator. The separator is downstream from the expander and returns the liquid stream generated by the separator back to the absorber. Additionally, the recovery of propane, butane and other heavier components is enhanced by combining the upper gas stream from a distillation column with the upper gas stream from the absorber prior to injecting this combination into the separator. The upper gas stream removed from the separator is then subsequently processed for the recovery of a predominantely methane and ethane gas stream while the bottom liquid stream from the absorber is subsequently distilled for the generation of a stream consisting predominantely of propane, butane and other heavy hydrocarbon components. Alternate embodiments include an additional reflux separator in the system, or substitution of an additional absorber for the separator.

    Abstract translation: 在天然气流中发现的丙烷，丁烷和其它较重组分的回收率增加是通过在膨胀机和分离器的上游安装吸收器来实现的。 分离器在膨胀器的下游，并将由分离器产生的液体流返回吸收器。 此外，通过将来自蒸馏塔的上部气体流与来自吸收器的上部气体流组合，然后将该组合注入分离器，可以提高丙烷，丁烷和其他较重组分的回收率。 然后从分离器中除去的上部气体流随后被处理以回收主要的甲烷和乙烷气体流，同时来自吸收器的底部液体物流随后被蒸馏以产生主要由丙烷，丁烷和其它重质烃组成的物流 组件。 替代实施方案包括系统中的另外的回流分离器或用于分离器的另外的吸收剂的取代。

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