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    Homopolymers with high photoinduceable double refraction
    91.
    发明授权
    Homopolymers with high photoinduceable double refraction 有权
    具有高光诱导双折射的均聚物

    公开(公告)号：US06441113B1

    公开(公告)日：2002-08-27

    申请号：US09423499

    申请日：1999-11-08

    Applicant: Horst Berneth ,  Uwe Claussen ,  Serguei Kostromine ,  Ralf Neigl ,  Hans-Joachim Vedder

    Inventor： Horst Berneth ,  Uwe Claussen ,  Serguei Kostromine ,  Ralf Neigl ,  Hans-Joachim Vedder

    IPC: C08F12058

    CPC classification number: G11C13/0014 ,  B82Y10/00 ,  C08F120/36 ,  G11B7/244 ,  G11B7/245 ,  G11B7/2467 ,  G11B7/25 ,  G11B7/253 ,  G11C13/0016 ,  G11C13/04 ,  G11C13/042

    Abstract: A homopolymer formed from monomers which contain groupings which are at least trinuclear, which are capable of absorbing the electromagnetic radiation of visible light, and which are structured so that in their thermodynamically stable state they are distended and strongly anisometric, is disclosed. The trinuclear groups of the homopolymer include at least one electron-attracting substituent which gives rise to a dipole moment which forms an angle of at least 20° with the longitudinal axis of the trinuclear groups. The homopolymer contains covalently bonded side groups branching from the backbone represented by the following formula, —§—T—Q—E. In the formula: § represents one of oxygen, sulphur and NR1; T represents a (CH2)n radical, optionally interrupted by, for example, —O—; Q represents a divalent linking group; and E represents the trinuclear group, e.g., represented by the following formula (VII),

    Abstract translation: 公开了由包含至少三核的能够吸收可见光的电磁辐射的组的单体形成的均聚物，并且其结构使得在其热力学稳定状态下它们膨胀并且具有强烈的不规则性。 均聚物的三核基团包括至少一个吸电子取代基，其产生与三核基团的纵轴形成至少20°的角度的偶极矩。 均聚物含有由下式表示的骨架分支的共价键合的侧基。在下式中：§代表氧，硫和NR1中的一个; T表示（CH 2）n基团，任选地被例如-O-间隔; Q表示二价连接基团; E表示例如由下式（VII）表示的三核基团，

    Electrochromic system
    92.
    发明授权
    Electrochromic system 失效
    电致变色系

    公开(公告)号：US06183878B2

    公开(公告)日：2001-02-06

    申请号：US09147615

    申请日：1999-05-25

    Applicant: Horst Berneth ,  Uwe Claussen ,  Dietrich Haarer ,  Jochen Schaller ,  Jürgen Simmerer

    Inventor： Horst Berneth ,  Uwe Claussen ,  Dietrich Haarer ,  Jochen Schaller ,  Jürgen Simmerer

    IPC: C09K902

    CPC classification number: G02F1/1521 ,  C09K9/02 ,  G02F2001/1502 ,  G02F2001/1512 ,  Y10T428/12271

    Abstract: The invention concerns an electrochrome system comprising a mixture of reducible and oxidizable substances RED1 and OX2, at lest one RED1′-OX2′ pair being covalently interlinked via a bridge and, for at least one RED1″ or OX2″ substance, the reciprocal conversion of the oxidized form and the reduced form being brought about by the fracture or formation of a &sgr;-bond. The electrochrome system is characterized by simplified electron transfer and reduced secondary reactions.

    Abstract translation: 本发明涉及一种包含可还原和可氧化物质RED1和OX2的混合物的电化学系统，至少一个RED1'-OX2对通过桥联共价连接，并且对于至少一种RED1“或OX2”物质， 通过σ-键的断裂或形成引起的氧化形式和还原形式的转化。 电子照相系统的特征在于简化的电子转移和二次反应的减少。

    Cationic 1,3,4-thiadiazole dyestuffs
    97.
    发明授权
    Cationic 1,3,4-thiadiazole dyestuffs 失效

    公开(公告)号：US5208325A

    公开(公告)日：1993-05-04

    申请号：US805147

    申请日：1991-12-11

    Applicant: Horst Berneth ,  Klaus Leverenz

    Inventor： Horst Berneth ,  Klaus Leverenz

    IPC: C09B44/20 ,  C07D285/12 ,  C07D285/135 ,  C09B44/10 ,  C09D11/00 ,  C09D11/02 ,  D06P1/08 ,  D06P3/76 ,  D21H21/28

    CPC classification number: C07D285/135 ,  C09B44/107

    Abstract: Cationic 1,3,4-thiadiazole dyestuff of the formula ##STR1##in whichR.sup.1 and R.sup.2, independently of one another, denote hydrogen, alkyl, alkenyl, cycloalkyl, aralkyl, aryl, a heterocycle, said heterocycle having a direct bond to the nitrogen atom, or being bound through a methylene or ethylene group, or R.sup.1 and R.sup.2, together with the nitrogen atom to which they are attached form a heterocycle,R.sup.3 denotes alkyl, alkenyl or aralkyl,R.sup.4 denotes hydrogen or alkyl,R.sup.5 denotes acyl,R.sup.6 and R.sup.7, independently of one another, denote hydrogen, alkyl, alkoxy, aryloxy or halogen andR.sup.8 and R.sup.9, independently of one another, denote hydrogen, alkyl, alkenyl, cycloalkyl, aralkyl, aryl, a heterocycle, said heterocycle having a direct bond to the nitrogen atom, or being bound through a methylene or ethylene group, or R.sup.8 and R.sup.9, together with the nitrogen atom to which they are attached form a heterocycle, orR.sup.6 and R.sup.8 together with the nitrogen to which R.sup.8 is attached completes a heterocyclic, said R.sup.6 and R.sup.8 having a total of from 2 to 4 atoms, one of which can be oxygen or nitrogen, said heterocyclic being either unsubstituted or substituted with from 1 to 3 alkyl groups orR.sup.7 and R.sup.9, together with the nitrogen to which R.sup.9 is bound completes a heterocyclic, said R.sup.7 and R.sup.9 having a total of from 2 to 4 atoms, one of which may be oxygen or nitrogen, said heterocyclic being either unsubstituted or substituted with from 1 to 3 alkyl groups, andX.sup.e denotes an anion andin which all alkyl, alkenyl, cycloalkyl, aralkyl, aryl, alkoxy and heterocyclic radicals present may be substituted by nonionic substitutents, carboxyl groups, ammonium groups and/or pyridinium groups wherein the nonionic substituents are substituents selected from the group consisting of cyano, hydroxyl, fluorine, chlorine, bromine, nitro, alkyl, monoalkylamino, dialkylamino, alkoxy, phenyl, acyloxy, acylamino, alkoxycarbonyl and alkoxycarbonyloxy.

    Bis(indolyl)ethylene compounds
    98.
    发明授权
    Bis(indolyl)ethylene compounds 失效
    双（吲哚基）乙烯化合物

    公开(公告)号：US4931567A

    公开(公告)日：1990-06-05

    申请号：US409186

    申请日：1989-09-19

    Applicant: Hubertus Psaar ,  Horst Berneth

    Inventor： Hubertus Psaar ,  Horst Berneth

    IPC: C07D209/14 ,  C07D209/08 ,  C07D209/24

    CPC classification number: C07D209/08 ,  C07D209/24

    Abstract: Bis(indolyl)ethylenes of the formula ##STR1## wherein R.sub.1 denotes hydrogen, alkyl, aralkyl or aryl,R.sub.2 denotes hydrogen, alkyl or aryl,R.sub.3 denotes hydrogen, alkyl, alkenyl, COOH or aryl andR.sub.4 denotes hydrogen, alkyl, alkoxy, cycloalkoxy or halogen, andthese substituents, in turn, can carry non-ionic radicals or a carboxyl group, are obtained by reaction of indoles of the formula ##STR2## with carboxylic acids of the formulaR.sub.3 --CH.sub.2 --COOH (III)their chlorides, esters, for example alkyl esters, or anhydrides in the presence of phosphorus oxychloride.

    Chromogenic 3,1-benzoxazines
    99.
    发明授权
    Chromogenic 3,1-benzoxazines 失效
    显色3,1-苯并恶嗪

    公开(公告)号：US4835270A

    公开(公告)日：1989-05-30

    申请号：US810797

    申请日：1988-12-18

    Applicant: Horst Berneth

    Inventor： Horst Berneth

    IPC: B41M5/136 ,  B41M5/323 ,  C07D265/16 ,  C07D413/04 ,  C07D413/10 ,  C07D413/12 ,  C09B11/02 ,  C09B11/04 ,  C09B19/00 ,  G02F1/17

    CPC classification number: C09B11/04 ,  B41M5/136 ,  B41M5/323 ,  C07D265/16 ,  C07D413/04 ,  C09B11/02

    Abstract: Compounds of the formula ##STR1## wherein Z.sup.1 denotes hydrogen, alkyl, cycloalkyl or ##STR2## R.sup.1 denotes hydrogen, alkyl, cycloalkyl, aralkyl, aryl, heteroalkyl or heteryl,X.sup.1, X.sup.2 and X.sup.3 denote hydrogen, halogen, alkyl, cycloalkyl, aryl, alkanoylamino, aroylamino or heteryl, and at least one of these radicals denotes NH.sup.1 Y.sup.2, OY.sup.3 or SY.sup.3,Y.sup.1, Y.sup.2 and Y.sup.3 denote hydrogen, alkyl, cycloalkyl, aralkyl, aryl or heteryl andY.sup.1 +Y.sup.2 denote the remaining members of a 5-membered or 6-membered ring which optionally contains further hetero-atoms,are outstandingly suitable as colour-forming agents for pressure-sensitive, heat-sensitive and electrosensitive recording materials with an acid developer. Deep copies which are fast to light are obtained.

    Abstract translation: 式（I）的化合物其中Z1表示氢，烷基，环烷基或R1表示氢，烷基，环烷基，芳烷基，芳基，杂烷基或杂芳基，X1，X2和X3表示氢，卤素，烷基， 环烷基，芳基，烷酰基氨基，芳酰基氨基或杂芳基，并且这些基团中的至少一个表示NH1Y2，OY3或SY3，Y1，Y2和Y3表示氢，烷基，环烷基，芳烷基，芳基或杂芳基，Y1 + Y2表示 任选地含有其它杂原子的5元或6元环非常适合用作用于具有酸显影剂的压敏，热敏和电敏记录材料的着色剂。 获得快速光照的深色复印件。

    Chromogenic 3,1-benzoxazines
    100.
    发明授权
    Chromogenic 3,1-benzoxazines 失效
    显色3,1-苯并恶嗪

    公开(公告)号：US4831141A

    公开(公告)日：1989-05-16

    申请号：US56569

    申请日：1987-06-01

    Applicant: Horst Berneth ,  Gert Jabs

    Inventor： Horst Berneth ,  Gert Jabs

    IPC: B41M5/136 ,  B41M5/145 ,  B41M5/323 ,  C07D265/16 ,  C07D413/04 ,  C09B19/00 ,  C09B67/22

    CPC classification number: B41M5/20 ,  B41M5/136 ,  B41M5/323 ,  C09B19/00

    Abstract: The invention relates to chromogenic 3,1-benzoxazines of the formula ##STR1## wherein X.sup.1 denotes hydrogen, C.sub.1 -C.sub.4 -alkyl, chlorine or OY.sup.1,X.sup.2 denotes NY.sup.2 Y.sup.3,X.sup.3 denotes OY.sup.4 or NY.sup.5 Y.sup.6,R.sup.1 -R.sup.3 independently of one another denote hydrogen, C.sub.1 -C.sub.4 -alkyl, chlorine, C.sub.1 -C.sub.4 -alkoxy or C.sub.1 -C.sub.4 -mono- or -dialkylamino, orR.sup.1 together with Y.sup.2,R.sup.2 or R.sup.3 together with Y.sup.4 or Y.sup.5, orR.sup.2 and R.sup.3 simultaneously with Y.sup.5 and Y.sup.6 denote a 2 to 4-membered bridge which can contain one oxygen atom or one nitrogen atom and can carry up to 4 methyl groups, and whereinR.sup.1 and R.sup.3 simultaneously represent hydrogen only if R.sup.2 with Y.sup.4 or Y.sup.5 forms one of the abovementioned bridges,R.sup.4 denotes hydrogen, methyl or chlorine,Y.sup.1 and Y.sup.4 independently of one another denote C.sub.1 -C.sub.4 -alkyl, cyclohexyl or benzyl and Y.sup.2, Y.sup.3, Y.sup.5 and Y.sup.6 independently of one another denote hydrogen, C.sub.1 -C.sub.4 -alkyl, cyclohexyl or benzyl,are used for pressure-copying, thermoreactive or electrochromic recording materials.

    Abstract translation: 本发明涉及式IMAMA的显色3,1-苯并恶嗪，其中X1表示氢，C1-C4-烷基，氯或OY1，X2表示NY2Y3，X3表示OY4或NY5Y6，R1-R3彼此独立地表示氢 ，C1-C4-烷基，氯，C1-C4-烷氧基或C1-C4-单 - 或二烷基氨基，或R1与Y2，R2或R3一起与Y4或Y5或R2和R3同时与Y5和Y6表示 可以含有一个氧原子或一个氮原子并且可以携带多达4个甲基的2至4元桥，其中只有当具有Y 4或Y 5的R 2形成上述桥之一时，R 1和R 3同时表示氢，R 4表示 氢，甲基或氯，Y1和Y4彼此独立地表示C1-C4-烷基，环己基或苄基，Y2，Y3，Y5和Y6彼此独立地表示氢，C1-C4-烷基，环己基或苄基 用于压力复制，热反应或电致变色记录材料。

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