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    Organic materials able to detect analytes
    26.
    发明授权
    Organic materials able to detect analytes 失效
    有机材料能够检测分析物

    公开(公告)号：US08298830B2

    公开(公告)日：2012-10-30

    申请号：US12795279

    申请日：2010-06-07

    Applicant: Aimee Rose ,  Timothy M. Swager ,  Zhengguo Zhu ,  Vladimir Bulovic ,  Conor Francis Madigan

    Inventor： Aimee Rose ,  Timothy M. Swager ,  Zhengguo Zhu ,  Vladimir Bulovic ,  Conor Francis Madigan

    IPC: G01N33/00

    CPC classification number: G01N21/7703 ,  G01N33/0057 ,  H01S3/067 ,  H01S3/178 ,  H01S5/12 ,  H01S5/36 ,  H01S2301/02

    Abstract: The present invention generally relates to polymers with lasing characteristics that allow the polymers to be useful in detecting analytes. In one aspect, the polymer, upon an interaction with an analyte, may exhibit a change in a lasing characteristic that can be determined in some fashion. For example, interaction of an analyte with the polymer may affect the ability of the polymer to reach an excited state that allows stimulated emission of photons to occur, which may be determined, thereby determining the analyte. In another aspect, the polymer, upon interaction with an analyte, may exhibit a change in stimulated emission that is at least 10 times greater with respect to a change in the spontaneous emission of the polymer upon interaction with the analyte. The polymer may be a conjugated polymer in some cases. In one set of embodiments, the polymer includes one or more hydrocarbon side chains, which may be parallel to the polymer backbone in some instances. In another set of embodiments, the polymer may include one or more pendant aromatic rings. In yet another set of embodiments, the polymer may be substantially encapsulated in a hydrocarbon. In still another set of embodiments, the polymer may be substantially resistant to photobleaching. In certain aspects, the polymer may be useful in the detection of explosive agents, such as 2,4,6-trinitrotoluene (TNT) and 2,4-dinitrotoluene (DNT).

    Abstract translation: 本发明一般涉及具有允许聚合物用于检测分析物的激光特性的聚合物。 在一个方面，聚合物在与分析物相互作用时可以表现出可以以某种方式确定的激光特性的变化。 例如，分析物与聚合物的相互作用可能影响聚合物达到允许发生光子的受激发射的激发态的能力，这可以被确定，从而确定分析物。 在另一方面，聚合物在与分析物相互作用时可能表现出相对于与分析物相互作用时聚合物自发发射变化的至少10倍的受激发射的变化。 在某些情况下，聚合物可以是共轭聚合物。 在一组实施方案中，聚合物包括一个或多个烃侧链，其在一些情况下可以平行于聚合物主链。 在另一组实施方案中，聚合物可以包括一个或多个芳族环。 在又一组实施方案中，聚合物可以基本上包封在烃中。 在又一组实施方案中，聚合物可以基本上抵抗光漂白。 在某些方面，聚合物可用于检测爆炸剂，例如2,4,6-三硝基甲苯（TNT）和2,4-二硝基甲苯（DNT）。

    Polymers with high internal free volume
    30.
    发明申请
    Polymers with high internal free volume 审中-公开
    高内部自由体积的聚合物

    公开(公告)号：US20080188634A1

    公开(公告)日：2008-08-07

    申请号：US11880868

    申请日：2007-07-23

    Applicant: Timothy M. Swager ,  Timothy M. Long ,  Zhengguo Zhu

    Inventor： Timothy M. Swager ,  Timothy M. Long ,  Zhengguo Zhu

    IPC: C08F32/00

    CPC classification number: H01L21/02118 ,  C08G61/02 ,  C08G61/10 ,  C08G61/12 ,  C08L101/12 ,  C09K11/06 ,  C09K19/38 ,  H01B1/12 ,  H01L21/312 ,  H01L51/0044 ,  H01L51/0058 ,  H01L51/0065 ,  Y10T428/10 ,  Y10T428/1036

    Abstract: Shape-persistent organic materials, including polymers, with large degrees of interior free volume are described, along with behaviors and phenomena enabled by their unique properties. One class of such a material is built up from triptycene base moieties wherein three benzene rings are bridged together about a [2.2.2] tricyclic ring system. These units can be assembled into discreet molecules and polymers. These materials and/or formulations thereof with liquid crystals or polymers are useful for the complexation of chemicals and/or polymers; they have very low dielectric constants for use as coatings in dielectric circuits, they provide additional ordering mechanisms in liquid crystals, and they display unusual mechanical responses when subjected to electrochemical, chemical, or mechanical stimuli.

    Abstract translation: 描述了具有大度内部自由体积的形状持久的有机材料，包括聚合物，以及由它们独特的性质实现的行为和现象。 一类这样的材料由三环己基部分构成，其中三个苯环围绕[2.2.2]三环系统桥联在一起。 这些单元可以组装成离散的分子和聚合物。 这些具有液晶或聚合物的材料和/或配方可用于化合物和/或聚合物的络合; 它们具有非常低的介电常数用作介电电路中的涂层，它们在液晶中提供附加的排序机制，并且当经受电化学，化学或机械刺激时它们显示出不寻常的机械响应。

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