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    Isobutane alkylation
    31.
    发明申请
    Isobutane alkylation 有权
    异丁烷烷基化

    公开(公告)号：US20050250972A1

    公开(公告)日：2005-11-10

    申请号：US11126859

    申请日：2005-05-10

    申请人： William Pfefferle

    发明人： William Pfefferle

    IPC分类号： B01J4/00 ,  B01J19/24 ,  B01J37/02 ,  C07C2/58 ,  C07C2/66 ,  C07C2/68

    CPC分类号： C07C2/66 ,  B01J4/00 ,  B01J19/2485 ,  B01J37/0246 ,  C07C2/58

    摘要： A method for isobutane alkylation is provided using a fixed-bed catalytic alkylation reactor comprises at least one catalytic flow channel. A feed stream comprising a compound to be alkylated is passed into a flow channel having an alkylation catalyst positioned on at least a portion of the flow channel inner surface in the flow channel downstream region. Olefin is injected into the feed stream at a point beyond a flow channel entrance region whereby the olefin contacts the alkylation catalyst by diffusion to the flow channel inner surface thereby reacting the compound with the olefin and produces an alkylate product.

    摘要翻译： 使用包含至少一个催化流动通道的固定床催化烷基化反应器提供异丁烷烷基化的方法。 将包含待烷基化化合物的进料流送入具有位于流动通道下游区域中的流路内表面的至少一部分上的烷基化催化剂的流动通道。 烯烃在超过流动通道入口区域的点处注入进料流中，由此烯烃通过扩散到流动通道内表面与烷基化催化剂接触，由此使化合物与烯烃反应并产生烷基化产物。

    Selective zeolite catalyst modification
    35.
    发明授权
    Selective zeolite catalyst modification 有权
    选择性沸石催化剂改性

    公开(公告)号：US06943131B1

    公开(公告)日：2005-09-13

    申请号：US10790948

    申请日：2004-03-02

    申请人： Ashim Kumar Ghosh ,  Pamela Harvey

    发明人： Ashim Kumar Ghosh ,  Pamela Harvey

    IPC分类号： B01J29/00 ,  B01J29/04 ,  B01J29/40 ,  B01J29/87 ,  B01J35/00 ,  B01J37/00 ,  B01J37/02 ,  C07C2/68 ,  C07C5/27

    CPC分类号： B01J29/40 ,  B01J35/002 ,  B01J37/009 ,  B01J37/0236 ,  B01J37/28 ,  B01J2229/12 ,  B01J2229/37 ,  C07C2/864 ,  C07C2529/40 ,  Y02P20/52 ,  C07C15/08

    摘要： A method of modifying a zeolite catalyst to increase selectivity of the catalyst is achieved by dissolving alumina in a phosphorus-containing acid solution, and treating the zeolite catalyst with the dissolved alumina solution. A method of preparing an aromatic product, such as a xylene product, is also achieved by contacting the modified zeolite catalyst with an aromatic hydrocarbon, such as toluene, and an alkylating agent, such as methanol, under reaction conditions suitable for aromatic alkylation. For xylene products the aromatic hydrocarbon may be toluene and the reaction conditions may be suitable for at least one of toluene methylation and transalkylation.

    摘要翻译： 通过将氧化铝溶解在含磷酸溶液中并用溶解氧化铝溶液处理沸石催化剂，可以实现改性沸石催化剂以提高催化剂选择性的方法。 通过在适于芳族烷基化的反应条件下使改性沸石催化剂与芳族烃如甲苯和烷基化剂如甲醇接触来制备芳族产物如二甲苯产物的方法。 对于二甲苯产物，芳族烃可以是甲苯，反应条件可适用于甲苯甲基化和烷基转移中的至少一种。

    SELECTIVE ZEOLITE CATALYST MODIFICATION
    36.
    发明申请
    SELECTIVE ZEOLITE CATALYST MODIFICATION 有权
    选择性沸石催化剂改性

    公开(公告)号：US20050197245A1

    公开(公告)日：2005-09-08

    申请号：US10790948

    申请日：2004-03-02

    申请人： Ashim Ghosh ,  Pamela Harvey

    发明人： Ashim Ghosh ,  Pamela Harvey

    IPC分类号： B01J29/00 ,  B01J29/04 ,  B01J29/40 ,  B01J29/87 ,  B01J35/00 ,  B01J37/00 ,  B01J37/02 ,  C07C2/68 ,  C07C5/27

    CPC分类号： B01J29/40 ,  B01J35/002 ,  B01J37/009 ,  B01J37/0236 ,  B01J37/28 ,  B01J2229/12 ,  B01J2229/37 ,  C07C2/864 ,  C07C2529/40 ,  Y02P20/52 ,  C07C15/08

    摘要： A method of modifying a zeolite catalyst to increase selectivity of the catalyst is achieved by dissolving alumina in a phosphorus-containing acid solution, and treating the zeolite catalyst with the dissolved alumina solution. A method of preparing an aromatic product, such as a xylene product, is also achieved by contacting the modified zeolite catalyst with an aromatic hydrocarbon, such as toluene, and an alkylating agent, such as methanol, under reaction conditions suitable for aromatic alkylation. For xylene products the aromatic hydrocarbon may be toluene and the reaction conditions may be suitable for at least one of toluene methylation and transalkylation.

    摘要翻译： 通过将氧化铝溶解在含磷酸溶液中并用溶解氧化铝溶液处理沸石催化剂，可以实现改性沸石催化剂以提高催化剂选择性的方法。 通过在适于芳族烷基化的反应条件下使改性沸石催化剂与芳族烃如甲苯和烷基化剂如甲醇接触来制备芳族产物如二甲苯产物的方法。 对于二甲苯产物，芳族烃可以是甲苯，反应条件可适用于甲苯甲基化和烷基转移中的至少一种。

    Process for the production of phenylalkanes using a hydrocarbon fraction that is obtained from the Fischer-Tropsch process
    37.
    发明申请
    Process for the production of phenylalkanes using a hydrocarbon fraction that is obtained from the Fischer-Tropsch process 审中-公开
    使用从费 - 托方法获得的烃馏分生产苯基烷烃的方法

    公开(公告)号：US20050187417A1

    公开(公告)日：2005-08-25

    申请号：US11061573

    申请日：2005-02-22

    申请人： Patrick Briot ,  Emmanuelle Guillon ,  Francois Hugues ,  Marie-Claire Marion

    发明人： Patrick Briot ,  Emmanuelle Guillon ,  Francois Hugues ,  Marie-Claire Marion

    IPC分类号： C07C2/66 ,  C10G29/20 ,  C07C1/20 ,  C07C2/68

    CPC分类号： C10G29/205 ,  C07C2/66 ,  C07C15/107

    摘要： A process for the production of phenylalkanes comprising a reaction for alkylation of at least one aromatic compound by at least one hydrocarbon fraction that is directly obtained from the Fischer-Tropsch process comprising linear olefins that have 9 to 16 carbon atoms per molecule and oxygenated compounds is described. Said alkylation reaction is carried out in a catalytic reactor that contains at least one reaction zone that comprises at least one acidic solid catalyst, and said hydrocarbon fraction does not undergo any purification treatment prior to its introduction into said reaction zone.

    摘要翻译： 一种制备苯基烷烃的方法，其包括通过至少一种直接从费 - 托法得到的烃馏分烷基化至少一种芳族化合物的反应，该方法包括每分子具有9-16个碳原子的直链烯烃和含氧化合物 描述。 所述烷基化反应在包含至少一个包含至少一种酸性固体催化剂的反应区的催化反应器中进行，所述烃馏分在其引入所述反应区之前不进行任何纯化处理。

    Process for producing alkylbenzene
    38.
    发明申请
    Process for producing alkylbenzene 失效
    生产烷基苯的方法

    公开(公告)号：US20050054890A1

    公开(公告)日：2005-03-10

    申请号：US10880072

    申请日：2004-11-12

    申请人： Brendan Murray ,  Garo Vaporciyan

    发明人： Brendan Murray ,  Garo Vaporciyan

    IPC分类号： C07C1/22 ,  C07C15/085 ,  C07C1/20 ,  C07C2/68

    CPC分类号： C07C15/085 ,  C07C1/22 ,  C07C2523/40 ,  C07C2523/44 ,  C07C2523/72 ,  C07C2523/74 ,  C07C2529/22 ,  Y02P20/127 ,  Y10S203/06

    摘要： A process for producing an alkylbenzene from an alkylphenyl alcohol involving the steps of: (a) feeding a feed stream containing alkylphenyl a reactor having a catalytic distillation zone; and, (b) concurrently in the reactor (i) contacting the feed stream containing alkylphenyl alcohol with hydrogen in the catalytic distillation zone to convert alkylphenyl alcohol to alkylbenzene over a catalyst containing Group VIII or a Group IB metal; and, (ii) separating alkylbenzene from the reaction mixture by fractional distillation to produce an overhead stream containing alkylbenzene having a reduced concentration of alkylphenyl alcohol than the feed stream from the distillation column reactor. Examples of the alkylphenyl alcohol include cumyl alcohol, phenyl ethyl alcohol, or di(2-hydroxyl 2-propyl)benzene, and that for the alkylbenzene include cumene and di-ethyl benzene, or di(2-hydroxyl-2-propyl)benzene.

    摘要翻译： 包括以下步骤生产烷基苯的方法：（a）将含有烷基苯基的进料流输送到具有催化蒸馏区的反应器; 和（b）在反应器中同时（i）在催化蒸馏区中使含有烷基苯基醇的进料流与氢气接触，以使烷基苯醇在含有VIII族或IB族金属的催化剂上转化为烷基苯; 和（ii）通过分馏从反应混合物中分离出烷基苯，以产生含有烷基苯醇浓度低于来自蒸馏塔反应器的进料流的烷基苯的塔顶液流。 烷基苯醇的实例包括枯基醇，苯基乙醇或二（2-羟基-2-丙基）苯，对于烷基苯包括枯烯和二乙基苯，或二（2-羟基-2-丙基）苯 。

    Toluene methylation process
    40.
    发明申请
    Toluene methylation process 有权
    甲苯甲基化过程

    公开(公告)号：US20050027151A1

    公开(公告)日：2005-02-03

    申请号：US10632254

    申请日：2003-08-01

    申请人： Ashim Ghosh ,  Pamela Harvey

    发明人： Ashim Ghosh ,  Pamela Harvey

    IPC分类号： C07C2/66 ,  C07C2/86 ,  C07C2/68

    CPC分类号： C07C2/864 ,  C07C2529/40 ,  Y02P20/52 ,  C07C15/08

    摘要： A method of preparing a xylene product is carried out in a reactor containing a phosphorus-treated ZSM-5-type zeolite catalyst. The method includes initiating a unique start-up of a toluene methylation reaction by contacting the catalyst with a toluene/methanol feed and a cofeed of hydrogen introduced into the reactor at certain start-up conditions. By utilizing the start-up conditions high selectivity for p-xylene can be achieved while providing stable catalytic activity over extended periods.

    摘要翻译： 制备二甲苯产物的方法在含有磷处理的ZSM-5型沸石催化剂的反应器中进行。 该方法包括通过在某些启动条件下使催化剂与甲苯/甲醇进料和引入反应器的氢的共进料接触来引发甲苯甲基化反应的独特启动。 通过利用启动条件，可以在长时间提供稳定的催化活性的同时实现对二甲苯的高选择性。