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公开(公告)号：US20100087693A1
公开(公告)日：2010-04-08
申请号：US12633253
申请日：2009-12-08
IPC分类号： C07C1/00
CPC分类号： C10G11/16 , C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/14 , C10G2300/4081 , C10G2400/20 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.
摘要翻译： 改进含氧化合物原料的加工，以提高轻质烯烃的生产或产率。 这种处理涉及含氧化合物转化为烯烃并随后开裂较重的烯烃，其中使用普通的压缩机将来自每个反应器的产物的至少一部分在压力下升高，然后被送至共同的产物分馏和回收段。 在一个具体实施方案中，可以处理裂化产物气体以从其中除去酸性气体。 在另一个实施方案中，烯烃裂解反应器是移动床反应器。
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公开(公告)号：US20100048965A1
公开(公告)日：2010-02-25
申请号：US12610108
申请日：2009-10-30
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.
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53.发明申请公开(公告)号：US20100004497A1
公开(公告)日：2010-01-07
申请号：US12511617
申请日：2009-07-29
申请人： Bryan K. Glover , Stephen W. Sohn , Mark G. Riley , Dean E. Rende
发明人： Bryan K. Glover , Stephen W. Sohn , Mark G. Riley , Dean E. Rende
IPC分类号： C07C2/00
CPC分类号： C07C15/107 , C07C2/66 , C07C5/333 , C07C2521/12 , Y02P20/125
摘要： Integrated processes for making detergent range alkylbenzenes from C5-C6-containing feeds involve feed pretreatment and/or selective hydrogenation to enable acceptable quality alkylbenzene production at attractive capital and operating costs.
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54.发明授权Selective conversion of oxygenate to propylene using moving bed technology and a hydrothermally stabilized dual-function catalyst 有权使用移动床技术和水热稳定的双功能催化剂选择性地将含氧化合物转化为丙烯公开(公告)号：US07408092B2
公开(公告)日：2008-08-05
申请号：US10988136
申请日：2004-11-12
申请人： Bryan K. Glover , John Q. Chen , Peter R. Pujado , Bipin V. Vora
发明人： Bryan K. Glover , John Q. Chen , Peter R. Pujado , Bipin V. Vora
IPC分类号： C07C1/00
CPC分类号： C07C11/06 , B01J8/082 , B01J8/085 , B01J8/12 , B01J2208/00274 , B01J2208/00283 , B01J2208/00292 , C07C1/20 , C07C2521/04 , C07C2529/40 , C07C2529/84 , C07C2529/85 , Y02P20/52
摘要： The average propylene cycle selectivity of an oxygenate to propylene (OTP) process using a dual-function oxygenate conversion catalyst is substantially enhanced by the use of a combination of: 1) moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of the fixed bed technology of the prior art; 2) a hydrothermally stabilized and dual-functional catalyst system comprising a molecular sieve having dual-function capability dispersed in a phosphorus-modified alumina matrix containing labile phosphorus and/or aluminum anions; and 3) a catalyst on-stream cycle time of 400 hours or less. These provisions stabilize the catalyst against hydrothermal deactivation and hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of average propylene cycle yield near or at essentially start-of-cycle levels.
摘要翻译： 使用双功能含氧化合物转化催化剂的含氧化合物对丙烯（OTP）方法的平均丙烯循环选择性通过使用以下组合来显着增强：1）OTP流程图的烃合成部分中的移动床反应器技术 现有技术的固定床技术的代替; 2）水热稳定和双功能催化剂体系，其包含具有分散在含有不稳定磷和/或铝阴离子的磷改性氧化铝基质中的双功能能力的分子筛; 和3）催化剂在流循环时间为400小时以下。 这些规定稳定催化剂以防止水热失活，并将催化剂上焦炭沉积物的积聚保持在基本上不降低双功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而使维持平均丙烯循环产率接近或 基本上是循环周期的水平。
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55.发明申请Fluidized Bed Reactor with Back-Mixing for Dehydrogenation of Light Paraffins 有权流化床反应器，用于轻质石蜡脱氢反向混合公开(公告)号：US20080161624A1
公开(公告)日：2008-07-03
申请号：US11954153
申请日：2007-12-11
IPC分类号： C07C5/333
CPC分类号： C07C5/324 , C07C5/325 , C07C2521/04 , C07C2521/08 , C07C2521/16 , C07C2523/26 , C07C2523/28 , C07C2523/30 , C07C2523/36 , C07C2523/42 , C07C2523/44 , C07C2523/745 , C07C2523/75 , C07C2523/755 , Y02P20/584 , C07C11/02
摘要： An improved process and system for the endothermic dehydrogenation of an alkane stream is described. The process and system of the present invention comprise a back-mixed fluidized bed reactor. The alkane stream is dehydrogenated in a single reactor stage by contacting the alkane stream with a back-mixed fluidized bed of catalyst. Deactivated catalyst is withdrawn from the back-mixed fluidized reactor and heated to produce hot regenerated catalyst. The hot regenerated catalyst is returned to the back-mixed fluidized bed reactor at a rate sufficient to maintain the back-mixed fluidized bed reactor at substantially isothermal conditions.
摘要翻译： 描述了用于烷烃流的吸热脱氢的改进方法和系统。 本发明的方法和系统包括反混流化床反应器。 通过使烷烃流与催化剂的反混合流化床接触，在单个反应器阶段使烷烃流脱氢。 将脱活催化剂从反混合流化反应器中取出并加热以产生热再生催化剂。 热再生催化剂以足以将反混流化床反应器保持在基本等温条件的速率返回到反混流化床反应器。
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公开(公告)号：US20080154078A1
公开(公告)日：2008-06-26
申请号：US11643604
申请日：2006-12-21
申请人： Andrea G. Bozzano , Bryan K. Glover
发明人： Andrea G. Bozzano , Bryan K. Glover
摘要： A processing scheme and system for enhanced light olefin production, particularly for increased relative yield of propylene, involves oxygenate conversion to olefins and subsequent oxygenate conversion effluent stream treatment including dimerization of ethylene to butene and metathesis of butenes and/or hexenes with ethylene. The processing scheme and system may further involve isomerization of at least a portion of 1-butene to 2-butene to produce additional propylene.
摘要翻译： 用于增强轻烯烃生产的加工方案和系统，特别是用于提高丙烯的相对产率，涉及含氧化合物转化为烯烃和随后的含氧化合物转化流出物流处理，包括将乙烯二聚成丁烯和使乙烯和/或己烯与乙烯的复分解。 加工方案和系统可进一步包括将至少一部分1-丁烯异构化成2-丁烯以产生另外的丙烯。
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57.发明授权
公开(公告)号：US5849979A
公开(公告)日：1998-12-15
申请号：US812800
申请日：1997-03-06
IPC分类号： C07C7/11
CPC分类号： C07C7/11
摘要： A process for the removal of trace quantities of polynuclear aromatic compounds from the vapor effluent of a hydrocarbon dehydrogenation zone containing normally gaseous olefinic hydrocarbons, trace mononuclear aromatic compounds and trace polynuclear aromatic compounds by contacting the hot vapor effluent of a hydrocarbon dehydrogenation zone with a cold lean liquid absorption stream to absorb at least a portion of the trace polynuclear aromatic compounds to produce a rich liquid absorption stream and a gaseous olefin-containing hydrocarbon stream having a reduced concentration of polynuclear aromatic compounds.
摘要翻译： 通过使碳氢化合物脱氢区的热蒸气流出物与冷却物接触，从含有通常气态的烯烃，痕量单核芳族化合物和痕量多核芳族化合物的烃脱氢区的蒸气流出物中除去痕量的多核芳族化合物的方法 贫吸液体吸收流以吸收至少一部分痕量多核芳族化合物以产生富液体吸收流和具有降低的多核芳族化合物浓度的含气态烯烃的烃流。
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公开(公告)号：US09192916B2
公开(公告)日：2015-11-24
申请号：US12563591
申请日：2009-09-21
申请人： Mark G. Riley , Bryan K. Glover
发明人： Mark G. Riley , Bryan K. Glover
IPC分类号： C07C5/05 , B01J23/58 , B01J21/04 , B01J23/44 , B01J35/00 , B01J35/10 , C07C5/09 , C07C15/107
CPC分类号： B01J23/58 , B01J21/04 , B01J23/44 , B01J35/0026 , B01J35/1014 , B01J35/1019 , B01J35/1047 , B01J35/1066 , B01J35/108 , C07C5/05 , C07C5/09 , C07C15/107 , C07C2521/04 , C07C2523/44 , C07C2523/58 , C07C11/02
摘要： A process and catalyst are presented for the selective hydrogenation of branched diolefins and acetylenes to olefins. The process uses a catalyst having large pores, and a minimal amount of micropores. The catalyst is designed to have minimal diffusional resistance through the large pores, and to minimize the hydrogenation of olefins to paraffins.
摘要翻译： 提出了一种方法和催化剂，用于将支链二烯烃和炔烃选择性氢化成烯烃。 该方法使用具有大孔的催化剂和最少量的微孔。 该催化剂被设计为具有通过大孔的最小扩散阻力，并使烯烃氢化至链烷烃最小化。
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59.发明授权Preparing a light-olefin containing product stream from an oxygenate-containing feed steam using reactors directing a flow of a fluidized dual-function catalyst system 有权使用引导流化双功能催化剂体系流的反应器从含氧化合物的进料蒸汽制备含轻烯烃的产物流公开(公告)号：US08735639B2
公开(公告)日：2014-05-27
申请号：US12755632
申请日：2010-04-07
CPC分类号： C07C11/06 , C07C1/20 , C07C4/06 , C07C2529/40 , C07C2529/85
摘要： The present process provides a method for converting an oxygenate-containing feed stream to an olefin-containing product stream. The method includes: (1) providing a first fluidized catalytic reactor for converting methanol to propylene, the first reactor having a fluidized catalyst system comprising a first catalyst and a second catalyst; (2) providing a second fluidized catalytic reactor communicating with the first fluidized catalytic reactor for cracking heavy olefins having four carbon atoms or greater into propylene, the second reactor having the fluidized catalyst system; (3) providing an oxygenate containing feed to the first reactor; and (4) fluidizing the catalyst system with the oxygenate containing feed.
摘要翻译： 本发明方法提供了将含氧化合物的进料流转化为含烯烃的产物流的方法。 该方法包括：（1）提供用于将甲醇转化为丙烯的第一流化催化反应器，所述第一反应器具有包含第一催化剂和第二催化剂的流化催化剂体系; （2）提供与第一流化催化反应器连通的第二流化催化反应器，用于将具有四个或更多碳原子的重质烯烃裂解成丙烯，第二反应器具有流化催化剂体系; （3）向第一反应器提供含氧化合物进料; 和（4）用含氧化合物进料使催化剂体系流化。
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公开(公告)号：US08603399B2
公开(公告)日：2013-12-10
申请号：US12571841
申请日：2009-10-01
IPC分类号： B01J8/18
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： An improved processing system of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. The system further comprises acid gas removal means to remove acid gases from the cracked product gas and that the olefin cracking reactor is a moving bed reactor.
摘要翻译： 含氧化合物原料的改进处理系统，用于提高轻质烯烃的生产或产率。 这种处理涉及含氧化合物转化为烯烃并随后开裂较重的烯烃，其中使用普通的压缩机将来自每个反应器的产物的至少一部分在压力下升高，然后被送至共同的产物分馏和回收段。 该系统还包括从裂化产物气体除去酸性气体的酸性气体去除装置，并且烯烃裂解反应器是移动床反应器。
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