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    Fluidized bed process for upgrading diene-containing light olefins
    71.
    发明授权
    Fluidized bed process for upgrading diene-containing light olefins 失效
    用于升级含二烯烃的轻质烯烃的流化床方法

    公开(公告)号：US4855521A

    公开(公告)日：1989-08-08

    申请号：US186526

    申请日：1988-04-27

    申请人： Amos A. Avidan ,  Fritz A. Smith ,  Samuel A. Tabak

    发明人： Amos A. Avidan ,  Fritz A. Smith ,  Samuel A. Tabak

    IPC分类号： C07C2/00

    CPC分类号： C07C2/00 ,  C07C2529/40

    摘要： An improved fluidized bed process for upgrading olefinic hydrocarbon feedstock by contacting the feedstock with acidic siliceous zeolite conversion catalyst particles at elevated temperature under exothermic conditions to produce heavier hydrocarbons including gasoline range hydrocarbons. The improvement comprises maintaining a turbulent fluidized bed of catalyst particles by flowing hydrocarbon-containing vapor upwardly through said bed at less than transport velocity; and introducing liquid olefinic feedstock comprising at least one C.sub.4 -C.sub.6 diene component into the fluidized catalyst bed in a lower portion thereof by rapidly atomizing and vaporizing the liquid feedstock, thus converting feedstock to heavier hydrocarbon without substantial thermal diene degradation thereof prior to contacting conversion catalyst particles in the fluidized bed. A predominantly liquid product is recovered containing C.sub.4 -C.sub.9 hydrocarbons rich in olefins and aromatics.

    摘要翻译： 改进的流化床方法，用于通过使原料与酸性硅沸石转化催化剂颗粒在升高的温度下在放热条件下接触以产生包含汽油范围烃的较重的烃来提纯烯烃原料。 改进包括通过以低于运输速度将含烃蒸汽向上流动穿过所述床来维持催化剂颗粒的湍流流化床; 并且通过使液体原料快速雾化并使其加热，将包含至少一种C 4 -C 6二烯组分的液体烯烃原料引入到其下部的流化催化剂床中，从而将原料转化为较重的烃，而在转化催化剂 流化床中的颗粒。 回收含有富含烯烃和芳族化合物的C4-C9烃的主要液体产物。

    Upgrading diene-containing light olefins in a fluidized bed reactor
    72.
    发明授权
    Upgrading diene-containing light olefins in a fluidized bed reactor 失效
    在流化床反应器中升级含二烯的轻质烯烃

    公开(公告)号：US4778661A

    公开(公告)日：1988-10-18

    申请号：US6408

    申请日：1987-01-23

    申请人： Amos A. Avidan ,  Fritz A. Smith ,  Samuel A. Tabak

    发明人： Amos A. Avidan ,  Fritz A. Smith ,  Samuel A. Tabak

    IPC分类号： C07C2/00 ,  B01J8/24

    CPC分类号： C07C2/00 ,  C07C2529/40

    摘要： An improved fluidized bed process for upgrading olefinic hydrocarbon feedstock by contacting the feedstock with acidic siliceous zeolite conversion catalyst particles at elevated temperature under exothermic conditions to produce heavier hydrocarbons including gasoline range hydrocarbons. The improvement comprises maintaining a turbulent fluidized bed of catalyst particles by flowing hydrocarbon-containing vapor upwardly through said bed at less than transport velocity; and introducing liquid olefinic feedstock comprising at least one C.sub.4 -C.sub.6 diene component into the fluidized catalyst bed in a lower portion thereof by rapidly atomizing and vaporizing the liquid feedstock, thus converting feedstock to heavier hydrocarbon without substantial thermal diene degradation thereof prior to contacting conversion catalyst particles in the fluidized bed. Reaction severity conditions may be maintained by controlling catalyst acidity, reaction temperature and reactant contact time to produce reaction efluent containing propane and propene in the ratio of about 0.2:1 to 200:1. A predominantly liquid product is recovered containing C.sub.4 -C.sub.9 hydrocarbons rich in olefins and aromatics.

    摘要翻译： 改进的流化床方法，用于通过使原料与酸性硅沸石转化催化剂颗粒在升高的温度下在放热条件下接触以产生包含汽油范围烃的较重烃来提纯烯烃原料。 改进包括通过以低于运输速度将含烃蒸汽向上流动穿过所述床来维持催化剂颗粒的湍流流化床; 并通过快速雾化和蒸发液体原料将包含至少一种C 4 -C 6二烯组分的液体烯烃原料引入到其下部的流化催化剂床中，从而在接触转化催化剂之前将原料转化成较重的烃，而不会发生相当的热二烯降解 流化床中的颗粒。 可以通过控制催化剂酸度，反应温度和反应物接触时间来维持反应强度条件，以产生约0.2:1至200:1的丙烷和丙烯的反应液。 回收含有富含烯烃和芳族化合物的C4-C9烃的主要液体产物。

    Integration of paraffin dehydrogenation with MOGD to minimize compression and gas plant separation
    73.
    发明授权
    Integration of paraffin dehydrogenation with MOGD to minimize compression and gas plant separation 失效
    石蜡脱氢与MOGD的整合使压缩和气体分离最小化

    公开(公告)号：US4749820A

    公开(公告)日：1988-06-07

    申请号：US650594

    申请日：1984-09-14

    申请人： James C. Kuo ,  Samuel A. Tabak

    发明人： James C. Kuo ,  Samuel A. Tabak

    IPC分类号： C07C11/02 ,  C10G50/00 ,  C07C5/00 ,  C07C1/00

    CPC分类号： C10G50/00 ,  C07C11/02 ,  Y02P30/48

    摘要： Disclosed is a method and apparatus for producing gasoline and distillate grade products which employs integrating catalytic (or thermal) dehydrogenation of paraffins with MOGD to minimize interstage compression and gas plant separation cost. The process cascades the product from a low temperature propane or butane dehydrogenation zone into a first catalytic reactor zone which operates at low pressure and contains zeolite oligomerization catalysts, where the low molecular weight olefins are reacted to primarily gasoline range materials. These gasoline range materials can then be pressurized to the pressure required for reacting to distillate in a second catalytic reactor zone operating at high pressure and containing zeolite oligomerization catalyst. The first catalytic reactor zone also acts to remove the olefins from the dehydrogenation reactor effluent to allow recycle of the unreacted paraffins.

    摘要翻译： 公开了用于生产汽油和馏出物级产物的方法和装置，其采用将链烷烃的催化（或热）脱氢与MOGD整合，以最小化级间压缩和气体分离成本。 该方法将产物从低温丙烷或丁烷脱氢区级联到在低压下操作并含有沸石低聚催化剂的第一催化反应器区，其中低分子量烯烃主要与汽油范围材料反应。 然后可以将这些汽油范围的材料加压至在高压下操作并含有沸石低聚催化剂的第二催化反应器区域中与馏出物反应所需的压力。 第一催化反应器区还用于从脱氢反应器流出物中除去烯烃以允许未反应的链烷烃的再循环。

    Catalytic process for oligomerizing ethene
    74.
    发明授权
    Catalytic process for oligomerizing ethene 失效
    催化乙烯齐聚的方法

    公开(公告)号：US4717782A

    公开(公告)日：1988-01-05

    申请号：US893522

    申请日：1986-08-05

    申请人： William E. Garwood ,  John D. Kushnerick ,  Samuel A. Tabak

    发明人： William E. Garwood ,  John D. Kushnerick ,  Samuel A. Tabak

    IPC分类号： C07C2/12 ,  C07C2/02

    CPC分类号： C07C2/12 ,  C07C2529/46 ,  Y02P20/52

    摘要： A continuous catalytic process for converting ethene-rich olefinic feedstock containing reducing gas to heavier liquid hydrocarbon product, comprising the steps ofcontacting the ethene-rich feedstock at elevated temperature in a catalytic reaction zone with a zeolite catalyst comprising a nickel-ethene oligomerization component and a shape-selective medium pore acid zeolite oligomerization component to convert at least a portion of the lower olefinic components to heavier olefinic hydrocarbons; andfeeding water with the feedstock in sufficient amount to prevent substantial reduction of the nickel component.

    摘要翻译： 一种用于将含有还原气体的富含烯烃的烯烃原料转化为较重液体烃产物的连续催化方法，包括以下步骤：使催化反应区中升温的富含乙烯的原料与包含镍 - 乙烯低聚组分的沸石催化剂和 形状选择性中孔酸性沸石低聚组分，将至少一部分较低级烯烃组分转化成较重的烯烃; 并用足够量的原料给予原料以防止镍组分的显着减少。

    Multi-stage system for converting oxygenates to liquid hydrocarbons with aliphatic recycle
    75.
    发明授权
    Multi-stage system for converting oxygenates to liquid hydrocarbons with aliphatic recycle 失效
    将含氧化合物转化为具有脂肪族循环的液体烃的多级系统

    公开(公告)号：US4689205A

    公开(公告)日：1987-08-25

    申请号：US824473

    申请日：1986-01-31

    申请人： Ronald M. Gould ,  Samuel A. Tabak

    发明人： Ronald M. Gould ,  Samuel A. Tabak

    IPC分类号： C07C1/20 ,  C10G3/00 ,  C10G50/00

    CPC分类号： C07C1/20 ,  C10G3/49 ,  C10G3/57 ,  C10G50/00 ,  B01J2208/00265 ,  C07C2529/40 ,  C10G2300/4081 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/20 ,  Y02P20/582 ,  Y02P30/20

    摘要： An apparatus for converting oxygenated feedstock, such as methanol, dimethyl ether or the like, to liquid hydrocarbons. In the primary catalyst stage the feedstock is contacted with a fluidized zeolite catalyst to produce C.sub.2 -C.sub.4 olefins and C.sub.5.sup.+ hydrocarbons. In a secondary catalytic stage with oligomerization catalyst comprising medium-pore shape selective acidic zeolite at increased pressure converts C.sub.3.sup.+ olefins to gasoline and/or distillate liquids. A portion of the recovered gasoline stream is recycled to the fluidized bed at a point above the bed stratum corresponding to substantially complete oxygenate conversion.

    摘要翻译： 将含氧原料如甲醇，二甲醚等转化为液体烃的装置。 在主要催化剂阶段，原料与流化沸石催化剂接触以产生C 2 -C 4烯烃和C 5+烃。 在具有增压压力的中孔形选择性酸性沸石的低聚催化剂的二次催化阶段中，将C3 +烯烃转化成汽油和/或馏出液。 回收的汽油流的一部分在床层上方的点上再循环到流化床，对应于基本上完全的含氧化合物转化。

    Multistage process for converting oxygenates to liquid hydrocarbons with aliphatic recycle
    77.
    发明授权
    Multistage process for converting oxygenates to liquid hydrocarbons with aliphatic recycle 失效
    将含氧化合物转化为具有脂肪族循环的液体烃的多阶段过程

    公开(公告)号：US4579999A

    公开(公告)日：1986-04-01

    申请号：US733994

    申请日：1985-05-14

    申请人： Ronald M. Gould ,  Samuel A. Tabak

    发明人： Ronald M. Gould ,  Samuel A. Tabak

    IPC分类号： C07C1/20 ,  C10G3/00 ,  C10G50/00

    CPC分类号： C10G50/00 ,  C07C1/20 ,  C10G3/49 ,  B01J2208/00265 ,  C07C2529/40 ,  C10G2300/4081 ,  C10G2400/02 ,  C10G2400/20 ,  Y02P20/582 ,  Y02P20/584 ,  Y02P30/20

    摘要： A process for converting oxygenated feedstock, such as methanol, dimethyl ether or the like, to liquid hydrocarbons.In the primary catalyst stage the feedstock is contacted with zeolite catalyst to produce C.sub.2 -C.sub.4 olefins and C.sub.5.sup.+ hydrocarbons.In a secondary catalytic stage with oligomerization catalyst comprising medium-pore shape selective acidic zeolite at increased pressure converts C.sub.3.sup.+ olefins to gasoline and/or distillate liquids.The improvement is a technique for recovering lower alkene for recycle to the primary catalytic stage.

    摘要翻译： 将氧化原料如甲醇，二甲醚等转化成液体烃的方法。 在初级催化剂阶段，原料与沸石催化剂接触以产生C 2 -C 4烯烃和C 5+烃。 在具有增压压力的中孔形选择性酸性沸石的低聚催化剂的二次催化阶段中，将C3 +烯烃转化成汽油和/或馏出液。 该改进是用于回收低级烯烃以再循环到初级催化级的技术。

    Process for dewaxing middle distillates
    79.
    发明授权
    Process for dewaxing middle distillates 失效
    脱蜡中间馏分的方法

    公开(公告)号：US4483760A

    公开(公告)日：1984-11-20

    申请号：US509828

    申请日：1983-06-30

    申请人： Samuel A. Tabak ,  Robert E. Holland

    发明人： Samuel A. Tabak ,  Robert E. Holland

    IPC分类号： C10G45/64 ,  C10G65/04 ,  C10G69/10

    CPC分类号： C10G45/64 ,  C10G65/043

    摘要： A process is provided for catalytically dewaxing a middle distillate with a ZSM-5 type catalyst. In this process the olefinic by-product is separated and catalytically converted to additional fuel oil and gasoline of good quality.

    摘要翻译： 提供了一种使用ZSM-5型催化剂催化脱蜡中间馏分的方法。 在这个过程中，烯烃副产物被分离并催化转化成额外的燃料油和质量好的汽油。