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公开(公告)号：US09333484B2
公开(公告)日：2016-05-10
申请号：US14089055
申请日：2013-11-25
申请人： David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
发明人： David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
CPC分类号： B01J20/3085 , B01D53/02 , B01D53/62 , B01D2253/202 , B01D2257/504 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/3064 , B01J20/3078 , C08G77/26 , C08L83/08 , Y02C10/04 , Y02C10/06 , Y02C10/08 , Y02P20/152
摘要： Methods are provided for synthesizing novel types of self-assembled siloxanes, such as polysiloxanes, with a sufficiently high density of amine functional groups to be useful for CO2 capture and release processes. Additionally, it has been unexpectedly found that some self-assembled polysiloxanes can be used for high temperature adsorption of CO2.
摘要翻译： 提供了用于合成新类型的自组装硅氧烷（例如聚硅氧烷）的方法，其具有足够高密度的胺官能团以用于CO 2捕获和释放过程。 另外，意外地发现一些自组装聚硅氧烷可用于高温吸附二氧化碳。
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公开(公告)号：US20140186246A1
公开(公告)日：2014-07-03
申请号：US14089055
申请日：2013-11-25
申请人： David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
发明人： David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
CPC分类号： B01J20/3085 , B01D53/02 , B01D53/62 , B01D2253/202 , B01D2257/504 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/3064 , B01J20/3078 , C08G77/26 , C08L83/08 , Y02C10/04 , Y02C10/06 , Y02C10/08 , Y02P20/152
摘要： Methods are provided for synthesizing novel types of self-assembled siloxanes, such as polysiloxanes, with a sufficiently high density of amine functional groups to be useful for CO2 capture and release processes. Additionally, it has been unexpectedly found that some self-assembled polysiloxanes can be used for high temperature adsorption of CO2.
摘要翻译： 提供了用于合成新类型的自组装硅氧烷（例如聚硅氧烷）的方法，其具有足够高密度的胺官能团以用于CO 2捕获和释放过程。 另外，意外地发现一些自组装聚硅氧烷可用于高温吸附二氧化碳。
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3.发明申请Epoxy-Amine Acid Gas Adsorption-Desorption Polymers and Oligomers, Processes for Preparing Same, and Uses Thereof 有权环氧 - 胺酸气体吸附 - 解吸聚合物和低聚物，制备方法及其用途公开(公告)号：US20120160097A1
公开(公告)日：2012-06-28
申请号：US13332576
申请日：2011-12-21
CPC分类号： B01J20/262 , B01D53/02 , B01D2253/202 , B01D2253/311 , B01D2257/504 , B01J20/267 , B01J20/28069 , Y02C10/04 , Y02C10/08
摘要： This disclosure involves an adsorption-desorption material, e.g., crosslinked epoxy-amine material having an Mw from about 500 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles CO2 per gram of crosslinked material, and/or linear epoxy-amine material having an Mw from about 160 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles CO2 per gram of linear material. This disclosure also involves processes for preparing the crosslinked epoxy-amine materials and linear epoxy-amine materials, as well as selective removal of CO2 and/or other acid gases from a gaseous stream using the epoxy-amine materials.
摘要翻译： 该公开内容涉及吸附 - 解吸材料，例如具有约500至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积和CO 2吸附容量的交联的环氧胺材料 每克交联材料至少约0.2毫摩尔二氧化碳，和/或具有约160至约1×10 6 Mw的直链环氧胺材料，总孔体积为约0.2cc / g至约2.0cc / g， 和每克线性材料至少约0.2毫摩尔二氧化碳的CO2吸附容量。 本公开还涉及制备交联的环氧胺材料和线性环氧胺材料的方法，以及使用环氧胺材料从气流中选择性除去CO 2和/或其它酸性气体。
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4.发明授权公开(公告)号：US09610533B2
公开(公告)日：2017-04-04
申请号：US14791772
申请日：2015-07-06
IPC分类号： C07C211/13 , C07C211/14 , C08J9/00 , B01J20/26 , B01J20/28 , B01J20/30 , C08G73/00 , C08G73/02 , B01D53/02 , B01D53/62 , C08J9/26 , C08J9/28 , B01J20/34 , B01D53/40 , C07C211/53 , C08J9/14
CPC分类号： B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
摘要： An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having a weight average molecular weight of from about 500 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material, and linear organo-amine polymeric materials having a weight average molecular weight of from about 160 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material. This disclosure also relates in part to processes for preparing the crosslinked organo-amine materials and linear organo-amine materials. This disclosure further relates in part to the selective removal of CO2 and/or other acid gases from a gaseous stream containing one or more of these gases using the adsorption-desorption materials.
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5.发明授权Organo-amine acid gas adsorption-desorption polymers, processes for preparing same, and uses thereof 有权有机胺酸性气体吸附 - 解吸聚合物，其制备方法及其应用公开(公告)号：US09115260B2
公开(公告)日：2015-08-25
申请号：US13332500
申请日：2011-12-21
IPC分类号： C07C211/48 , C07C211/50 , C07C211/49 , B01J20/26 , B01J20/22 , B01J20/28 , C08J9/26 , B01D53/02 , B01D53/62 , C08G73/02 , B01J20/30 , B01J20/34
CPC分类号： B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
摘要： An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having an Mw from about 500 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles adsorbed CO2 per gram of adsorption-desorption material, and linear organo-amine polymeric materials having an Mw from about 160 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles adsorbed CO2 per gram of adsorption-desorption material. This disclosure also relates to processes for preparing the crosslinked and linear organo-amine materials, as well as to selective removal of CO2 and/or other acid gases from a gaseous stream using the adsorption-desorption materials.
摘要翻译： 一种吸附 - 解吸材料，特别是具有约500至约1×10 6 M w，约0.2cc / g至约2.0cc / g的总孔容积和在约0.2cc / g至约2.0cc / g的吸附能力的交联的有机 - 胺聚合物材料 每克吸附 - 解吸材料吸收最少约0.2毫摩尔的二氧化碳，和约160至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积的线性有机胺聚合物， 并且每克吸附 - 解吸材料吸附能力为至少约0.2毫摩尔吸附二氧化碳。 本公开还涉及制备交联和线性有机胺材料的方法，以及使用吸附 - 解吸材料从气流中选择性除去CO 2和/或其它酸性气体。
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6.发明申请Organo-Amine Acid Gas Adsorption-Desorption Polymers, Processes for Preparing Same, and Uses Thereof 有权有机胺酸气吸附解吸聚合物，其制备方法及用途公开(公告)号：US20120164043A1
公开(公告)日：2012-06-28
申请号：US13332500
申请日：2011-12-21
CPC分类号： B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
摘要： An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having an Mw from about 500 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles adsorbed CO2 per gram of adsorption-desorption material, and linear organo-amine polymeric materials having an Mw from about 160 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles adsorbed CO2 per gram of adsorption-desorption material. This disclosure also relates to processes for preparing the crosslinked and linear organo-amine materials, as well as to selective removal of CO2 and/or other acid gases from a gaseous stream using the adsorption-desorption materials.
摘要翻译： 一种吸附 - 解吸材料，特别是具有约500至约1×10 6 M w，约0.2cc / g至约2.0cc / g的总孔容积和在约0.2cc / g至约2.0cc / g的吸附能力的交联的有机 - 胺聚合物材料 每克吸附 - 解吸材料吸收最少约0.2毫摩尔的二氧化碳，和约160至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积的线性有机胺聚合物， 并且每克吸附 - 解吸材料吸附能力为至少约0.2毫摩尔吸附二氧化碳。 本公开还涉及制备交联和线性有机胺材料的方法，以及使用吸附 - 解吸材料从气流中选择性除去CO 2和/或其它酸性气体。
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7.发明授权Organo-amine acid gas adsorption-desorption polymers, processes for preparing same, and uses thereof 有权有机胺酸性气体吸附 - 解吸聚合物，其制备方法及其应用公开(公告)号：US09533248B2
公开(公告)日：2017-01-03
申请号：US14791800
申请日：2015-07-06
IPC分类号： C08L79/00 , C07C209/06 , B01J20/22 , B01J20/26 , B01D53/02 , B01D53/62 , C08G73/02 , C08J9/26 , C08J9/28 , B01J20/28 , B01J20/30 , B01J20/34 , C08G73/00 , B01D53/40 , C07C211/53 , C08J9/14
CPC分类号： B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
摘要： An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having a weight average molecular weight of from about 500 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material, and linear organo-amine polymeric materials having a weight average molecular weight of from about 160 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material. This disclosure also relates in part to processes for preparing the crosslinked organo-amine materials and linear organo-amine materials. This disclosure further relates in part to the selective removal of CO2 and/or other acid gases from a gaseous stream containing one or more of these gases using the adsorption-desorption materials.
摘要翻译： 吸附解吸材料，特别是重均分子量为约500至约1×10 6的交联有机胺聚合物材料，总孔体积为约0.2立方厘米每克（cc / g）至约 2.0cc / g，每克吸附 - 解吸材料吸附至少约0.2毫摩尔二氧化碳的吸附能力，重均分子量为约160至约1×106的线性有机胺聚合物， 总孔体积为约0.2立方厘米每克（cc / g）至约2.0cc / g，吸附能力为每克吸附 - 解吸材料吸附至少约0.2毫摩尔二氧化碳。 本公开还部分涉及制备交联的有机胺材料和线性有机胺材料的方法。 本公开还部分地涉及使用吸附 - 解吸材料从含有一种或多种这些气体的气流中选择性除去CO 2和/或其它酸性气体。
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8.发明申请ORGANO-AMINE ACID GAS ADSORPTION-DESORPTION POLYMERS, PROCESSES FOR PREPARING SAME, AND USES THEREOF 有权有机酸酸气体吸收分解聚合物，其制备方法及其用途公开(公告)号：US20150307661A1
公开(公告)日：2015-10-29
申请号：US14791772
申请日：2015-07-06
IPC分类号： C08G73/02 , C07C211/53 , B01D53/02
CPC分类号： B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
摘要： An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having a weight average molecular weight of from about 500 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material, and linear organo-amine polymeric materials having a weight average molecular weight of from about 160 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material. This disclosure also relates in part to processes for preparing the crosslinked organo-amine materials and linear organo-amine materials. This disclosure further relates in part to the selective removal of CO2 and/or other acid gases from a gaseous stream containing one or more of these gases using the adsorption-desorption materials.
摘要翻译： 吸附解吸材料，特别是重均分子量为约500至约1×10 6的交联有机胺聚合物材料，总孔体积为约0.2立方厘米每克（cc / g）至约 2.0cc / g，每克吸附 - 解吸材料吸附至少约0.2毫摩尔二氧化碳的吸附能力，重均分子量为约160至约1×106的线性有机胺聚合物， 总孔体积为约0.2立方厘米每克（cc / g）至约2.0cc / g，吸附能力为每克吸附 - 解吸材料吸附至少约0.2毫摩尔二氧化碳。 本公开还部分涉及制备交联的有机胺材料和线性有机胺材料的方法。 本公开还部分地涉及使用吸附 - 解吸材料从含有一种或多种这些气体的气流中选择性除去CO 2和/或其它酸性气体。
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9.发明授权Epoxy-amine acid gas adsorption-desorption polymers and oligomers, processes for preparing same, and uses thereof 有权环氧胺酸性气体吸附 - 解吸聚合物和低聚物，其制备方法及其应用公开(公告)号：US08557027B2
公开(公告)日：2013-10-15
申请号：US13332576
申请日：2011-12-21
CPC分类号： B01J20/262 , B01D53/02 , B01D2253/202 , B01D2253/311 , B01D2257/504 , B01J20/267 , B01J20/28069 , Y02C10/04 , Y02C10/08
摘要： This disclosure involves an adsorption-desorption material, e.g., crosslinked epoxy-amine material having an Mw from about 500 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles CO2 per gram of crosslinked material, and/or linear epoxy-amine material having an Mw from about 160 to about 1×106, a total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles CO2 per gram of linear material. This disclosure also involves processes for preparing the crosslinked epoxy-amine materials and linear epoxy-amine materials, as well as selective removal of CO2 and/or other acid gases from a gaseous stream using the epoxy-amine materials.
摘要翻译： 该公开内容涉及吸附 - 解吸材料，例如具有约500至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积和CO 2吸附容量的交联的环氧胺材料 每克交联材料至少约0.2毫摩尔二氧化碳，和/或具有约160至约1×10 6 Mw的直链环氧胺材料，总孔体积为约0.2cc / g至约2.0cc / g， 和每克线性材料至少约0.2毫摩尔二氧化碳的CO2吸附容量。 本公开还涉及制备交联的环氧胺材料和线性环氧胺材料的方法，以及使用环氧胺材料从气流中选择性除去CO 2和/或其它酸性气体。
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10.发明申请Polyvinyl-Amine Acid Gas Adsorption-Desorption Polymers, Processes for Preparing Same, and Uses Thereof 有权聚乙烯基胺酸气体吸附 - 解吸聚合物，其制备方法及其用途公开(公告)号：US20120164045A1
公开(公告)日：2012-06-28
申请号：US13332560
申请日：2011-12-21
IPC分类号： B01D53/02 , B01D53/047 , C08J9/228 , C08G61/12
CPC分类号： C08J9/28 , B01D53/02 , B01D53/0462 , B01D53/047 , B01D53/62 , B01D2253/202 , B01D2253/311 , B01D2257/304 , B01D2257/504 , C08J9/26 , C08J2201/026 , C08J2201/0502 , C08J2339/02 , Y02C10/04 , Y02C10/08 , Y02P20/152
摘要： This disclosure involves an adsorption-desorption material, e.g., crosslinked polyvinyl-amine material having an Mw from about 500 to about 1×106, total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles per gram of crosslinked material, and/or linear polyvinyl-amine material having an Mw from about 160 to about 1×106, total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles per gram of linear material. This disclosure also involves processes for preparing the crosslinked polyvinyl-amine materials and linear polyvinyl-amine materials, as well as selective removal of CO2 and/or other acid gases from a gaseous stream using the polyvinyl-amine materials.
摘要翻译： 该公开内容涉及吸附 - 解吸材料，例如具有约500至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积的交联聚乙烯胺材料和CO 2吸附容量 至少约0.2毫摩尔/克交联材料，和/或Mw为约160至约1×10 6，总孔体积为约0.2cc / g至约2.0cc / g的直链聚乙烯胺材料，以及CO 2 至少约0.2毫摩尔每克线性材料的吸附容量。 本公开还涉及制备交联聚乙烯胺材料和线性聚乙烯胺材料的方法，以及使用聚乙烯基胺材料从气流中选择性除去CO 2和/或其它酸性气体。
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