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    Hydrothermally stable catalyst and its use in catalytic cracking
    5.
    发明授权
    Hydrothermally stable catalyst and its use in catalytic cracking 失效
    水热稳定催化剂及其在催化裂化中的应用

    公开(公告)号：US07615143B2

    公开(公告)日：2009-11-10

    申请号：US10903152

    申请日：2004-07-30

    申请人： Tan-Jen Chen ,  Paul F. Keusenkothen ,  J. Jason Wu ,  John Scott Buchanan ,  Guang Cao ,  Larry L. Iaccino ,  David L. Stern ,  Matthew J. Vincent

    发明人： Tan-Jen Chen ,  Paul F. Keusenkothen ,  J. Jason Wu ,  John Scott Buchanan ,  Guang Cao ,  Larry L. Iaccino ,  David L. Stern ,  Matthew J. Vincent

    IPC分类号： C10G11/05

    CPC分类号： C10G11/05 ,  C10G2400/20

    摘要： There is provided a catalyst composition having improved hydrothermal stability for the catalytic cracking of a hydrocarbon feedstock to selectively produce propylene. The catalyst composition comprises a first crystalline molecular sieve selected from the group consisting of IM-5, MWW, ITH, FER, MFS, AEL, and AFO and an effective amount of a stabilization metal (copper, zirconium, or mixtures thereof) exchanged into the molecular sieve. The catalyst finds application in the cracking of naphtha and heavy hydrocarbon feedstocks. When used in the catalytic cracking of heavier hydrocarbon feedstocks, the catalyst composition preferably comprises a second molecular sieve having a pore size that is greater than the pore size of the first molecular sieve. The process is carried out by contacting a feedstock containing hydrocarbons having at least 4 carbon atoms is contacted, under catalytic cracking conditions, with the catalyst composition.

    摘要翻译： 提供了一种具有改进的水热稳定性用于烃原料的催化裂化以选择性地生产丙烯的催化剂组合物。 催化剂组合物包含选自由IM-5，MWW，ITH，FER，MFS，AEL和AFO组成的组的第一结晶分子筛和有效量的稳定金属（铜，锆或其混合物）交换成 分子筛。 该催化剂可用于石脑油和重质烃原料的裂解。 当用于较重烃原料的催化裂化时，催化剂组合物优选包含具有大于第一分子筛孔径的孔径的第二分子筛。 该方法通过使含有至少4个碳原子的烃的原料在催化裂化条件下与催化剂组合物接触来进行。

    Production of alkylated aromatic hydrocarbons from methane
    6.
    发明授权
    Production of alkylated aromatic hydrocarbons from methane 有权
    从甲烷生产烷基化芳烃

    公开(公告)号：US08138384B2

    公开(公告)日：2012-03-20

    申请号：US11792324

    申请日：2005-12-02

    申请人： Larry L. Iaccino ,  Elizabeth L. Stavens ,  Gary D. Mohr ,  Matthew J. Vincent

    发明人： Larry L. Iaccino ,  Elizabeth L. Stavens ,  Gary D. Mohr ,  Matthew J. Vincent

    IPC分类号： C07C15/00

    CPC分类号： C07C2/66 ,  C07C2/76 ,  Y10S585/943 ,  C07C15/02

    摘要： In a process for converting methane to alkylated aromatic hydrocarbons, a feed containing methane is contacted with a dehydrocyclization catalyst under conditions effective to convert said methane to aromatic hydrocarbons and produce a first effluent stream comprising aromatic hydrocarbons and hydrogen. At least a portion of said aromatic hydrocarbon from said first effluent stream is then contacted with an alkylating agent under conditions effective to alkylate said aromatic hydrocarbon and produce an alkylated aromatic hydrocarbon having more alkyl side chains than said aromatic hydrocarbon prior to the alkylating.

    摘要翻译： 在将甲烷转化为烷基化芳烃的方法中，将甲烷的进料与脱氢环化催化剂在有效地将所述甲烷转化为芳烃并产生包含芳族烃和氢的第一流出物流的条件下接触。 然后使来自所述第一流出物流的所述芳烃的至少一部分与烷基化剂在有效使所述芳族烃烷基化的条件下接触，并在烷基化之前产生具有比所述芳烃更多的烷基侧链的烷基化芳族烃。

    Production of aromatic hydrocarbons from methane
    7.
    发明授权
    Production of aromatic hydrocarbons from methane 有权
    从甲烷生产芳烃

    公开(公告)号：US07759535B2

    公开(公告)日：2010-07-20

    申请号：US11792359

    申请日：2005-12-02

    申请人： Larry L. Iaccino ,  Xiaobing Feng ,  Matthew J. Vincent ,  Elizabeth L. Stavens

    发明人： Larry L. Iaccino ,  Xiaobing Feng ,  Matthew J. Vincent ,  Elizabeth L. Stavens

    IPC分类号： C07C2/78

    CPC分类号： C07C2/76 ,  Y10S585/943 ,  C07C15/02

    摘要： In a process for converting methane to higher hydrocarbons including aromatic hydrocarbons, a feed containing methane is contacted with a dehydrocyclization catalyst under conditions effective to convert said methane to aromatic hydrocarbons and produce a first effluent stream comprising aromatic hydrocarbons and hydrogen, wherein said first effluent stream comprises at least 5 wt % more aromatic hydrocarbons than said feed. At least part of the hydrogen from said first effluent stream is then reacted with an oxygen-containing species, such as carbon dioxide, to produce a second effluent stream having a reduced hydrogen content compared with said first effluent stream.

    摘要翻译： 在将甲烷转化为包括芳烃的高级烃的方法中，含有甲烷的进料在有效地将所述甲烷转化为芳烃并产生包含芳族烃和氢的第一流出物流的条件下与脱氢环化催化剂接触，其中所述第一流出物流 包含比所述进料多至少5重量％的芳烃。 然后使来自所述第一流出物流的氢的至少一部分与含氧物质如二氧化碳反应，以产生与所述第一流出物流相比具有降低的氢含量的第二流出物流。

    Process for methane conversion
    8.
    发明授权
    Process for methane conversion 有权
    甲烷转化工艺

    公开(公告)号：US07781636B2

    公开(公告)日：2010-08-24

    申请号：US11732039

    申请日：2007-04-02

    申请人： Larry L. Iaccino ,  Neeraj Sangar ,  Elizabeth L. Stavens ,  Matthew J. Vincent

    发明人： Larry L. Iaccino ,  Neeraj Sangar ,  Elizabeth L. Stavens ,  Matthew J. Vincent

    IPC分类号： C07C2/78

    CPC分类号： C07C2/76 ,  C10G50/00 ,  C10G2300/1025 ,  C10G2400/30 ,  Y02P20/52 ,  Y10S585/943 ,  C07C15/02 ,  C07C15/04

    摘要： A process for converting methane to higher hydrocarbon(s) including aromatic hydrocarbon(s) in a reaction zone comprises providing to a hydrocarbon feedstock containing methane and a catalytic particulate material to the reaction zone and contacting the catalytic particulate material and the hydrocarbon feedstock in a substantially countercurrent fashion in the reaction zone, while operating the reaction zone under reaction conditions sufficient to convert at least a portion of said methane to a first effluent having said higher hydrocarbon(s).

    摘要翻译： 在反应区中将甲烷转化为高级烃（包括芳族烃）的方法包括向反应区提供含有甲烷和催化颗粒物质的烃原料，并使催化颗粒材料和烃原料接触 同时在足以将至少一部分甲烷转化为具有所述较高烃的第一流出物的反应条件下操作反应区。

    Use of isotopic analysis for determination of aromatic hydrocarbons produced from methane
    9.
    发明授权
    Use of isotopic analysis for determination of aromatic hydrocarbons produced from methane 有权
    使用同位素分析测定甲烷产生的芳烃

    公开(公告)号：US07754930B2

    公开(公告)日：2010-07-13

    申请号：US11805868

    申请日：2007-05-24

    申请人： Larry L. Iaccino

    发明人： Larry L. Iaccino

    IPC分类号： C07C13/00

    CPC分类号： C07C2/66 ,  C07C2/76 ,  Y10S585/941 ,  C07C15/08 ,  C07C15/04

    摘要： Benzene and xylene are described having a unique distribution of deuterium and 13C such that δ(deuterium) for each of the benzene and xylene is less than −250 and δ(13C) for the benzene is greater than −36 and for xylene is less than −24, wherein δ(deuterium)=(R′sample/R′standard−1)×1000 where R′sample is the ratio of deuterium to hydrogen in the benzene/xylene; and R′standard is the ratio of the natural abundance of deuterium to the natural abundance of hydrogen; and wherein δ(13C)=(R″sample/R″standard−1)×1000 where R″sample is the ratio of 13C to 12C in the benzene/xylene; and R″standard is the ratio of the natural abundance of 13C to the natural abundance of 12C.

    摘要翻译： 描述苯和二甲苯具有氘和13C的独特分布，使得苯和二甲苯中的每一个的δ（氘）小于-250，苯的δ（13℃）大于-36，并且对于二甲苯小于 -24，其中δ（氘）=（R'sample / R'standard-1）×1000其中R'示例是苯/二甲苯中氘与氢的比例; R'standard是氘的天然丰度与氢的天然丰度之比; 其中δ（13C）=（R“样品/ R”标准-1）×1000其中R“样品是苯/二甲苯中13C至12C的比例; 而R“标准是13C的天然丰度与12C的天然丰度之比。

    Production of Aromatics from Aliphatics
    10.
    发明申请
    Production of Aromatics from Aliphatics 有权
    从芳烃生产芳烃

    公开(公告)号：US20090030253A1

    公开(公告)日：2009-01-29

    申请号：US12166153

    申请日：2008-07-01

    申请人： Teng Xu ,  Kenneth R. Clem ,  Jeremy J. Patt ,  J. Scott Buchanan ,  Larry L. Iaccino

    发明人： Teng Xu ,  Kenneth R. Clem ,  Jeremy J. Patt ,  J. Scott Buchanan ,  Larry L. Iaccino

    IPC分类号： C07C2/00

    CPC分类号： C07C2/76 ,  C07C15/02

    摘要： In a process for converting a low carbon number aliphatic hydrocarbon to higher hydrocarbons including aromatic hydrocarbons, a feed containing the aliphatic hydrocarbon is contacted with a dehydrocyclization catalyst under conditions effective to convert the aliphatic hydrocarbon to aromatic hydrocarbons and produce an effluent stream comprising aromatic hydrocarbons and hydrogen. The dehydrocyclization catalyst comprises a metal or metal compound and a molecular sieve wherein the ratio of the amount of any Bronsted acid sites in the catalyst to the amount of said metal in the catalyst is less than 0.4 mol/mol of said metal.

    摘要翻译： 在将低碳数脂肪族烃转化成包括芳烃的高级烃的方法中，将含有脂族烃的进料与脱氢环化催化剂在有效将脂肪烃转化为芳族烃并产生包含芳族烃的流出物流的条件下接触， 氢。 脱氢环化催化剂包括金属或金属化合物和分子筛，其中催化剂中任何布朗斯台德酸位点的量与催化剂中所述金属的量的比例小于所述金属的0.4mol / mol。