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    Water-dilutable coating binder combinations which can be deposited cathodically, and their use
    1.
    发明授权
    Water-dilutable coating binder combinations which can be deposited cathodically, and their use 失效
    水可稀释的涂料粘合剂组合可以阴极沉积，以及它们的用途

    公开(公告)号：US5272188A

    公开(公告)日：1993-12-21

    申请号：US923484

    申请日：1992-08-03

    申请人： Ingo Kriessmann ,  Willibald Paar ,  Franz Holzer ,  Walter Koch

    发明人： Ingo Kriessmann ,  Willibald Paar ,  Franz Holzer ,  Walter Koch

    IPC分类号： C08F2/44 ,  C08F283/00 ,  C08F283/10 ,  C09D4/06 ,  C09D5/44 ,  C09D133/00 ,  C09D133/04 ,  C09D151/00 ,  C09D151/08 ,  C09D163/00 ,  C08K3/20 ,  C08L51/08

    CPC分类号： C09D5/4488 ,  C09D4/06

    摘要： Water-dilutable coating binder combinations which can be deposited cathodically, and based on epoxy resin-amine adducts, acrylate copolymers and crosslinking components are described. The binders are particularly suitable for formulation of water-dilutable primers and one-coat paints when deposited cathodically are described. In 3 to 30% by weight, based on the solids, of a basic epoxy resin-amine adduct (A) which is free from epoxide groups, 70 to 97% by weight of a monomer mixture (B), which consists of esters of (meth)acrylic acid which contain secondary or tertiary amino groups, of monoesters of (meth)acrylic acid with diols, of (meth)acrylic acid alkyl esters and if appropriate of aromatic vinyl monomers, is polymerized. Components (A) and (B) comprise at least 5% by weight, preferably 10 to 20% by weight, of identical aliphatic radicals having 7 to 18 carbon atoms. The baked films based on these products have a high degree of gloss and an excellent UV, washing agent, and corrosion resistance.

    摘要翻译： 描述了可以阴极沉积并基于环氧树脂 - 胺加合物，丙烯酸酯共聚物和交联组分的水可稀释涂料粘合剂组合。 粘合剂特别适用于在阴极沉积时沉积的可稀释底漆和单涂层涂料的配方。 基于固体，基于3〜30重量％的不含环氧基团的碱性环氧树脂 - 胺加合物（A），70〜97重量％的单体混合物（B），其由 （甲基）丙烯酸与二醇的单酯，（甲基）丙烯酸烷基酯和如果合适的芳族乙烯基单体的仲或叔氨基的（甲基）丙烯酸被聚合。 组分（A）和（B）包含至少5重量％，优选10至20重量％的具有7至18个碳原子的相同的脂族基团。 基于这些产品的烘烤膜具有高光泽度和优异的UV，洗涤剂和耐腐蚀性。

    Diester of phosphoric acid and monoepoxide reacted with epoxide to form product reacted with monoisocyanate
    2.
    发明授权
    Diester of phosphoric acid and monoepoxide reacted with epoxide to form product reacted with monoisocyanate 失效
    磷酸和单环氧化物的二酯与环氧化物反应形成与单异氰酸酯反应的产物

    公开(公告)号：US4992525A

    公开(公告)日：1991-02-12

    申请号：US187427

    申请日：1988-04-28

    申请人： Ingo Kriessmann ,  Willibald Paar

    发明人： Ingo Kriessmann ,  Willibald Paar

    IPC分类号： C08G59/14 ,  C08G59/30 ,  C08G59/32 ,  C08G59/56 ,  C09D5/44 ,  C09D163/00

    CPC分类号： C08G59/1488 ,  C08G59/14 ,  C08G59/56 ,  C09D5/4434

    摘要： Cationic resins based on epoxy resins which are modified through the introduction of phosphoric acid segments and the process of producing the resins are described. The reaction of the phosphoric acid is carried out in a multiple-step process whereby, in a first step, the diester is formed through reaction of ortho-phosphoric acid with 2 moles of a monoepoxy compound or through reaction of a polyphosphoric acid with n-1 moles of a monoalcohol and subsequent reaction with n+1 moles of a monoepoxy compound. The remaining acid group is reacted with a di- or polyepoxy resin. The products obtained can still contain unreacted epoxy groups. The protonable groups are introduced via the epoxy groups and/or via the hydroxy groups present or set free by opening of the oxirane ring. The binders can be combined with hardening components or may be formulated as self-crosslinking binders. The binders have excellent resistance to corrosion when stoved as electrodeposited coatings.

    摘要翻译： 描述了通过引入磷酸链段改性的基于环氧树脂的阳离子树脂和制备树脂的方法。 磷酸的反应是以多步法进行的，其中在第一步中，通过邻磷酸与2摩尔单环氧化合物的反应或通过多磷酸与正磷酸的反应形成二酯， 1摩尔一元醇，随后与n + 1摩尔单环氧化合物反应。 剩余的酸基与二环氧树脂或聚环氧树脂反应。 所得产物仍可含有未反应的环氧基。 可质子化基团通过环氧基和/或经由存在的羟基或通过开环的环氧乙烷环自由引入。 粘合剂可以与硬化组分组合，或者可以配制成自交联粘合剂。 当作为电沉积涂层被烘烤时，粘合剂具有优异的耐腐蚀性。

    Acrylate copolymer additives for aqueous cationic coating systems
    3.
    发明授权
    Acrylate copolymer additives for aqueous cationic coating systems 失效
    用于水性阳离子涂料体系的丙烯酸酯共聚物添加剂

    公开(公告)号：US5037920A

    公开(公告)日：1991-08-06

    申请号：US577124

    申请日：1990-09-04

    申请人： Ingo Kriessmann ,  Harald Rauch-Puntigam ,  Willibald Paar ,  Peter Morre

    发明人： Ingo Kriessmann ,  Harald Rauch-Puntigam ,  Willibald Paar ,  Peter Morre

    IPC分类号： C09D5/44 ,  C09D133/02 ,  C09D133/04 ,  C09D133/06

    CPC分类号： C09D5/4492

    摘要： Acrylate copolymers containing amino, hydroxyl and fluorine groups useful as additives for aqueous cationic coating systems for preventing surface flaws and for improving the adhesion of further coats, in particular of PVC-containing coating materials, are described. In addition to amino groups which can be neutralized with acids, the acrylate copolymers contain a selected quantity of hydroxyl groups originating from monoesters of (meth)acrylic acid with diols, and fluorine from esters of (meth)acrylic acid. The additives are added in a quantity from 0.5 to 5.0% by weight, calculated on solids and relative to the solids content of the binder in a coating system.

    摘要翻译： 描述了含有氨基，羟基和氟基团的丙烯酸酯共聚物，其可用作用于防止表面缺陷的水性阳离子涂层体系的添加剂，以及用于改善其它涂层，特别是含PVC涂料的粘附性。 除了可用酸中和的氨基之外，丙烯酸酯共聚物含有选自量的（甲基）丙烯酸与二醇的单酯和由（甲基）丙烯酸的酯得到的氟的羟基。 添加剂的添加量为0.5-5.0重量％，以固体计算，相对于涂料体系中粘合剂的固体含量计算。

    Aqueous binders for coatings with improved gloss
    4.
    发明授权
    Aqueous binders for coatings with improved gloss 有权
    用于具有改善光泽度的涂层的水性粘合剂

    公开(公告)号：US08546479B2

    公开(公告)日：2013-10-01

    申请号：US12293091

    申请日：2007-03-04

    申请人： Johann Billiani ,  Karl Rossmann ,  Rami-Raimund Awad ,  Thomas Fraydl ,  Ingo Kriessmann

    发明人： Johann Billiani ,  Karl Rossmann ,  Rami-Raimund Awad ,  Thomas Fraydl ,  Ingo Kriessmann

    IPC分类号： C08G18/67

    CPC分类号： C09D133/066 ,  C08F212/08 ,  C08F220/06 ,  C08F220/18

    摘要： A water-reducible mixture of (meth)acrylic copolymers having a hydroxyl number of from 40 mg/g to 250 mg/g, an acid number of from 15 mg/g to 80 mg/g, a weight average molar mass Mw from 9 kg/mol to 40 kg/mol and a glass transition temperature Tg from −40° C. to 80° C., based on polymerised monomers comprising at least one alkyl ester A of an olefinically un-saturated carboxylic acid having from 1 to 8 carbon atoms in the alkyl group, at least one hydroxy functional alkyl ester B of an olefinically unsaturated carboxylic acid, at least one aliphatic compound C that has both hydroxy and carboxyl functionalities, or which is a lactone or a cyclic lactone, at least one vinyl monomer D which does not comprise a moiety derived from an olefinically unsaturated carboxylic acid, at least one olefinically unsaturated carboxylic acid E, a process for its preparation, and a method of use thereof in the preparation of paints.

    摘要翻译： 具有羟值为40mg / g至250mg / g，酸值为15mg / g至80mg / g，重量平均摩尔质量Mw为9的（甲基）丙烯酸共聚物的水可稀释混合物 kg / mol至40kg / mol，玻璃化转变温度Tg为-40℃至80℃，基于包含至少一种具有1至8个的烯属不饱和羧酸的烷基酯A的聚合单体 烷基中的碳原子，烯属不饱和羧酸的至少一种羟基官能的烷基酯B，至少一种具有羟基和羧基官能团的脂肪族化合物C，或者是内酯或环状内酯，至少一种乙烯基 单体D，其不包含衍生自烯属不饱和羧酸的部分，至少一种烯属不饱和羧酸E，其制备方法及其在制备涂料中的用途。

    AQUEOUS BINDERS FOR COATINGS WITH IMPROVED GLOSS
    5.
    发明申请
    AQUEOUS BINDERS FOR COATINGS WITH IMPROVED GLOSS 有权
    具有改进的GLOSS的涂料的水性粘合剂

    公开(公告)号：US20090221741A1

    公开(公告)日：2009-09-03

    申请号：US12293091

    申请日：2007-03-04

    申请人： Johann Billiani ,  Karl Rossmann ,  Rami-Raimund Awad ,  Thomas Fraydl ,  Ingo Kriessmann

    发明人： Johann Billiani ,  Karl Rossmann ,  Rami-Raimund Awad ,  Thomas Fraydl ,  Ingo Kriessmann

    IPC分类号： C09D133/02

    CPC分类号： C09D133/066 ,  C08F212/08 ,  C08F220/06 ,  C08F220/18

    摘要： A water-reducible mixture of (meth)acrylic copolymers having a hydroxyl number of from 40 mg/g to 250 mg/g, an acid number of from 15 mg/g to 80 mg/g, a weight average molar mass Mw from 9 kg/mol to 40 kg/mol and a glass transition temperature Tg from −40° C. to 80° C., based on polymerised monomers comprising at least one alkyl ester A of an olefinically un-saturated carboxylic acid having from 1 to 8 carbon atoms in the alkyl group, at least one hydroxy functional alkyl ester B of an olefinically unsaturated carboxylic acid, at least one aliphatic compound C that has both hydroxy and carboxyl functionalities, or which is a lactone or a cyclic lactone, at least one vinyl monomer D which does not comprise a moiety derived from an olefinically unsaturated carboxylic acid, at least one olefinically unsaturated carboxylic acid E, a process for its preparation, and a method of use thereof in the preparation of paints.

    摘要翻译： 具有羟值为40mg / g至250mg / g，酸值为15mg / g至80mg / g，重量平均摩尔质量Mw为9的（甲基）丙烯酸共聚物的水可稀释混合物 kg / mol至40kg / mol，玻璃化转变温度Tg为-40℃至80℃，基于包含至少一种具有1至8个的烯属不饱和羧酸的烷基酯A的聚合单体 烷基中的碳原子，烯属不饱和羧酸的至少一种羟基官能的烷基酯B，至少一种具有羟基和羧基官能团的脂肪族化合物C，或者是内酯或环状内酯，至少一种乙烯基 单体D，其不包含衍生自烯属不饱和羧酸的部分，至少一种烯属不饱和羧酸E，其制备方法及其在制备涂料中的用途。

    Aqueous self-crosslinking copolymer dispersions, a process for preparing them and their use in binders for coating materials
    6.
    发明授权
    Aqueous self-crosslinking copolymer dispersions, a process for preparing them and their use in binders for coating materials 有权
    水性自交联共聚物分散体，其制备方法及其在涂料粘合剂中的应用

    公开(公告)号：US06515042B2

    公开(公告)日：2003-02-04

    申请号：US09419214

    申请日：1999-10-15

    申请人： Ingo Kriessmann ,  Rami-Raimund Awad ,  Hannelore Gsöll ,  Bernhard Hirschmann ,  Karl Rossmann

    发明人： Ingo Kriessmann ,  Rami-Raimund Awad ,  Hannelore Gsöll ,  Bernhard Hirschmann ,  Karl Rossmann

    IPC分类号： C09D15100

    CPC分类号： C08F265/06 ,  C08F257/02 ,  C09D151/00 ,  Y10S525/902

    摘要： Aqueous self-crosslinking copolymer dispersions ABC obtainable by free-radically initiated copolymerization in the first stage of a monomer mixture A comprising olefinically unsaturated monomers A1 having carbonyl groups, unsaturated carboxylic acids or monoesters of unsaturated dicarboxylic acids A2, monomers A3 selected from vinylaromatic compounds, n-butyl methacrylate and also alkyl esters of unsaturated carboxylic acids or dialkyl esters of unsaturated dicarboxylic acids, esters A4 selected from alkyl esters of unsaturated carboxylic acids of dialkyl esters of unsaturated dicarboxylic acids, and other free-radically polymerizable monomers A5, and subsequent addition of a second monomer mixture B and further polymerization in the second stage, the mixture B comprising olefinically unsaturated monomers B1 corresponding to A1, esters B2 corresponding to A4, and monomers B3 corresponding to A5, and subsequently adding compounds C having hydrazine or hydrazide groups.

    摘要翻译： 在单体混合物A的第一阶段中通过自由基引发共聚获得的水性自交联共聚物分散体ABC包含具有羰基的烯属不饱和单体A1，不饱和羧酸或不饱和二羧酸A2的单酯，选自乙烯基芳族化合物的单体A3， 甲基丙烯酸正丁酯以及不饱和羧酸的烷基酯或不饱和二羧酸的二烷基酯，选自不饱和二羧酸的二烷基酯的不饱和羧酸的烷基酯和其它可自由基聚合的单体A5的酯A4，以及随后的加成 的第二单体混合物B和在第二阶段进一步聚合，混合物B包含对应于A1的烯属不饱和单体B1，对应于A4的酯B2和对应于A5的单体B3，随后加入具有肼或酰肼基团的化合物C.

    Process for the preparation of water-dilutable coating binders based on acrylate copolymers, and their use
    8.
    发明授权
    Process for the preparation of water-dilutable coating binders based on acrylate copolymers, and their use 失效
    基于丙烯酸酯共聚物制备水可稀释涂料粘合剂的方法及其用途

    公开(公告)号：US5811484A

    公开(公告)日：1998-09-22

    申请号：US663127

    申请日：1996-06-24

    申请人： Werner Wilfinger ,  Ingo Kriessmann ,  Kurt Gossak

    发明人： Werner Wilfinger ,  Ingo Kriessmann ,  Kurt Gossak

    IPC分类号： C08G81/00 ,  B05D7/26 ,  C08F8/14 ,  C08F8/44 ,  C08G81/02 ,  C09D133/06 ,  C09D133/14 ,  C09D161/20 ,  C08L33/00

    CPC分类号： C08F8/14 ,  C08F8/44 ,  C09D133/06

    摘要： A process is disclosed for preparing water-dilutable, acrylate copolymer-based lacquer binders. A polycarboxylic component is reacted with an epoxide group-containing polyhydroxylic component, and the carboxylic groups are then at least partially neutralized. As epoxide group-containing monomers for the polyhydroxylic components, glycidyl(meth)acrylate and/or glycidylallylether are used in proportions from 0.1 to 3% by weight. Associated with cross-linking components and if required with other lacquer binders, these lacquer binders are suitable for producing water-dilutable baking enamels with a low auxiliary organic solvent content.

    摘要翻译： PCT No.PCT / AT94 / 00203 Sec。 371日期1996年6月24日 102（e）1996年6月24日PCT 1994年12月22日PCT公布。 第WO95 / 17450号公报 日期1995年6月29日公开了一种制备水可稀释丙烯酸酯共聚物基漆粘合剂的方法。 使多元羧酸成分与含环氧基的多羟基成分反应，然后将羧基至少部分中和。 作为多羟基成分的含环氧基的单体，使用0.1〜3重量％的（甲基）丙烯酸缩水甘油酯和/或缩水甘油基醚。 与交联组分相关，如果需要与其它漆粘合剂相关，这些漆粘合剂适用于生产具有低辅助有机溶剂含量的水可稀释烘烤搪瓷。