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    CATALYST AND CATALYST CARRIER
    1.
    发明申请
    CATALYST AND CATALYST CARRIER 有权
    催化剂和催化剂载体

    公开(公告)号：US20140100379A1

    公开(公告)日：2014-04-10

    申请号：US13648303

    申请日：2012-10-10

    Applicant: Michael A. Richard ,  John R. Lockemeyer

    Inventor： Michael A. Richard ,  John R. Lockemeyer

    IPC: B01J27/02 ,  C07D301/04

    CPC classification number: B01J27/047 ,  B01J21/04 ,  B01J23/50 ,  B01J23/66 ,  B01J27/02 ,  B01J27/055 ,  B01J35/1085 ,  B01J35/109 ,  B01J35/1095 ,  C07D301/04 ,  C07D301/10 ,  Y02P20/52

    Abstract: The carrier of the present invention includes at least 85 wt percent alpha alumina, at least 0.06 wt percent SiO2 and no more than 0.04 wt percent Na2O. The carrier has a water absorption no greater than 0.35 g/g and a ratio of water absorption (g/g) to surface area (m2/g) no greater than 0.50 g/m2. Another aspect of the invention is a catalyst for the epoxidation of olefins which comprises the above described carrier and silver dispersed thereon, where the carrier has a monomodal, bimodal or multimodal pore distribution and where the quantity of silver is between 5 and 50 wt %, relative to the weight of the catalyst. A reactor to system for the epoxidation of olefins is also disclosed.

    Abstract translation: 本发明的载体包括至少85wt％的α氧化铝，至少0.06wt％的SiO 2和不超过0.04wt％的Na 2 O. 载体的吸水率不大于0.35g / g，吸水率（g / g）与表面积（m2 / g）不大于0.50g / m 2。 本发明的另一方面是用于烯烃环氧化的催化剂，其包含分散在其上的上述载体和银，其中载体具有单峰，双峰或多峰孔分布，并且其中银的量为5至50重量％ 相对于催化剂的重量。 还公开了用于烯烃的环氧化反应器的反应器。

    PROCESS FOR FORMING A CATALYST CARRIER
    3.
    发明申请
    PROCESS FOR FORMING A CATALYST CARRIER 审中-公开
    形成催化载体的方法

    公开(公告)号：US20110077152A1

    公开(公告)日：2011-03-31

    申请号：US12915101

    申请日：2010-10-29

    Applicant: William H. Gerdes ,  Thomas Szymanski ,  Donald J. Remus ,  John R. Lockemeyer ,  Randall Clayton Yeates

    Inventor： William H. Gerdes ,  Thomas Szymanski ,  Donald J. Remus ,  John R. Lockemeyer ,  Randall Clayton Yeates

    IPC: B01J21/04

    CPC classification number: B01J21/04 ,  B01J21/12 ,  B01J23/50 ,  B01J23/66 ,  B01J23/688 ,  B01J35/023 ,  B01J35/10 ,  B01J35/1009 ,  B01J35/1038 ,  B01J35/1071 ,  B01J35/108 ,  B01J37/0009 ,  B01J37/0018 ,  B01J37/0072

    Abstract: A carrier, which comprises non-platelet alumina and/or a bond material, has a surface area of at least 1.3 m2/g, a total pore volume and a pore size distribution such that at least 80% of the total pore volume is contained in pores with diameters in the range of from 0.1 to 10 μm, and at least 80% of the pore volume contained in the pores with diameters in the range of from 0.1 to 10 μm is contained in pores with diameters in the range of from 0.3 to 10 μm, and a process for the preparation of a carrier which comprises forming a mixture comprising: a) from 50 to 95 weight percent of a first particulate α-alumina having a median particle size (d50) of from 5 to 100 μm; b) from 5 to 50 weight percent of a second particulate α-alumina having a d50 which is less than the d50 of the first particulate α-alumina and which is in the range of from 1 to 10 μm; and c) an alkaline earth metal silicate bond material; weight percent being based on the total weight of α-alumina in the mixture; and firing the mixture to form the carrier.

    Abstract translation: 包含非血小板氧化铝和/或粘合材料的载体具有至少1.3m 2 / g的表面积，总孔体积和孔径分布，使得含有总孔体积的至少80％ 在直径在0.1至10μm范围内的孔中，包含在直径在0.1至10μm范围内的直径在0.1至10μm范围内的孔中的孔体积的至少80％包含在直径范围为0.3 以及制备载体的方法，其包括形成混合物，其包含：a）50至95重量％的中值粒径（d50）为5至100μm的第一颗粒状α-氧化铝; b）5至50重量％的d50小于第一颗粒α-氧化铝的d50并且为1至10μm范围的第二颗粒状α-氧化铝; 和c）碱土金属硅酸盐粘合材料; 重量百分数是基于混合物中α-氧化铝的总重量; 并且将混合物烧制以形成载体。

    Catalyst carrier and a process for preparing the catalyst carrier
    4.
    发明授权
    Catalyst carrier and a process for preparing the catalyst carrier 有权
    催化剂载体和制备催化剂载体的方法

    公开(公告)号：US07825062B2

    公开(公告)日：2010-11-02

    申请号：US11449019

    申请日：2006-06-06

    Applicant: William H. Gerdes ,  Thomas Szymanski ,  Donald J. Remus ,  John R. Lockemeyer ,  Randall Clayton Yeates

    Inventor： William H. Gerdes ,  Thomas Szymanski ,  Donald J. Remus ,  John R. Lockemeyer ,  Randall Clayton Yeates

    IPC: B01J21/00 ,  B01J23/00 ,  B01J20/00

    CPC classification number: B01J21/04 ,  B01J21/12 ,  B01J23/50 ,  B01J23/66 ,  B01J23/688 ,  B01J35/023 ,  B01J35/10 ,  B01J35/1009 ,  B01J35/1038 ,  B01J35/1071 ,  B01J35/108 ,  B01J37/0009 ,  B01J37/0018 ,  B01J37/0072

    Abstract: A carrier, which comprises non-platelet alumina and/or a bond material, has a surface area of at least 1.3 m2/g, a total pore volume and a pore size distribution such that at least 80% of the total pore volume is contained in pores with diameters in the range of from 0.1 to 10 μm, and at least 80% of the pore volume contained in the pores with diameters in the range of from 0.1 to 10 μm is contained in pores with diameters in the range of from 0.3 to 10 μm, and a process for the preparation of a carrier which comprises forming a mixture comprising: a) from 50 to 95 weight percent of a first particulate α-alumina having a median particle size (d50) of from 5 to 100 μm; b) from 5 to 50 weight percent of a second particulate α-alumina having a d50 which is less than the d50 of the first particulate α-alumina and which is in the range of from 1 to 10 μm; and c) an alkaline earth metal silicate bond material; weight percent being based on the total weight of α-alumina in the mixture; and firing the mixture to form the carrier.

    Abstract translation: 包含非血小板氧化铝和/或粘合材料的载体具有至少1.3m 2 / g的表面积，总孔体积和孔径分布，使得含有总孔体积的至少80％ 在直径在0.1至10μm范围内的孔中，包含在直径在0.1至10μm范围内的直径在0.1至10μm范围内的孔中的孔体积的至少80％包含在直径范围为0.3 以及制备载体的方法，其包括形成混合物，其包含：a）50至95重量％的中值粒径（d50）为5至100μm的第一颗粒状α-氧化铝; b）5至50重量％的d50小于第一颗粒α-氧化铝的d50并且为1至10μm范围的第二颗粒状α-氧化铝; 和c）碱土金属硅酸盐粘合材料; 重量百分数是基于混合物中α-氧化铝的总重量; 并且将混合物烧制以形成载体。

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