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    Ethane conversion process
    2.
    发明授权
    Ethane conversion process 失效
    乙烷转化过程

    公开(公告)号：US4260839A

    公开(公告)日：1981-04-07

    申请号：US57924

    申请日：1979-07-16

    申请人： Nai Y. Chen ,  Werner O. Haag ,  Tracy J. Huang

    发明人： Nai Y. Chen ,  Werner O. Haag ,  Tracy J. Huang

    IPC分类号： C07C2/00 ,  C07C4/00 ,  C07C9/04 ,  B01J29/30 ,  C07C2/12 ,  C07C6/10

    CPC分类号： C07C2/00 ,  C07C4/00 ,  C07C2529/40 ,  C07C2529/50 ,  C07C2529/65 ,  C07C2529/70 ,  Y10S208/02

    摘要： A process for effecting an endothermic and an exothermic reaction, under conversion conditions, in a single reaction zone wherein ethane is endothermically converted to C.sub.3 + hydrocarbons, and wherein an unconverted portion of ethane is simultaneously exothermically hydrogenated to methane in the presence of a catalyst system comprising a crystalline aluminosilicate zeolite having a uniform structure characterized by pores, the major dimension of which is less than 6 Angstroms and ZSM-5 type aluminosilicate zeolite, containing a minor amount of Zn in combination with a Group VIII noble metal or a Group IB metal, the exothermic reaction providing sufficient heat to maintain the reaction zone at a temperature capable of sustaining the endothermic reaction.

    摘要翻译： 在转化条件下在单一反应区中进行吸热和放热反应的方法，其中乙烷吸热转化为C 3+烃，并且其中未转化部分的乙烷在催化剂体系存在下同时放热氢化成甲烷，所述催化剂体系包含 具有均匀结构的结晶硅铝酸盐沸石，其主要尺寸小于6埃，ZSM-5型硅铝酸盐沸石，其含有少量的Zn与VIII族贵金属或IB族金属组合， 放热反应提供足够的热量以将反应区保持在能够维持吸热反应的温度。

    Lubricant production process
    3.
    发明授权
    Lubricant production process 失效
    润滑油生产过程

    公开(公告)号：US4919788A

    公开(公告)日：1990-04-24

    申请号：US260857

    申请日：1988-10-21

    申请人： Nai Y. Chen ,  William E. Garwood ,  Tracy J. Huang ,  Quang N. Le ,  Stephen S. Wong

    发明人： Nai Y. Chen ,  William E. Garwood ,  Tracy J. Huang ,  Quang N. Le ,  Stephen S. Wong

    IPC分类号： C10G45/64 ,  C10G65/04 ,  C10G67/04

    CPC分类号： C10G67/04 ,  C10G45/64 ,  C10G65/043

    摘要： A process for producing lubricant oils of low pour point and high viscosity index by first carrying out a partial dewaxing of a lubricant base stock in an initial catalytic dewaxing operation, followed by a selective dewaxing step. The initial catalytic dewaxing step is carried out using a large pore, high silica zeolite dewaxing catalyst such as high silica Y or zeolite beta which dewaxes by isomerizing the waxy components of the base stock to less waxy brance chain isoparaffins but the severity of the operation is controlled so as to effect only a partial removal of the waxy components. Further removal of the waxy components is effected during the subsequent dewaxing step which is selective for the removal of the more waxy n-paraffin components, leaving the branched chain isoparaffins which contribute to a high VI in the product. The selective dewaxing step may be either a solvent, e.g. MEK dewaxing operation or a catalytic dewaxing using a highly shape selective zeolite such as ZSM-22 or ZSM-23. The severity of the initial catalytic dewaxing operation may be controlled so as to effect a net increase in the content of isoparaffins and because of the selective nature of the solvent dewaxing step, this increased isoparaffins concentration may be retained, producing a product of high VI. The pour point of the feedstock is preferably reduced during the initial catalytic dewaxing step to a value which is no lower than 10.degree. F. and preferably no lower than 20.degree. F., above the target pour point for the products. Generally, this will entail a reduction of at least 10.degree. F. and preferably at least 20.degree. F. in the pour point of the feed.

    摘要翻译： 首先在初始催化脱蜡操作中进行润滑剂原料的部分脱蜡，然后进行选择性脱蜡步骤，生产低倾点和高粘度指数的润滑油的方法。 初始催化脱蜡步骤使用大孔，高二氧化硅沸石脱蜡催化剂如高二氧化硅Y或沸石β进行，该脱蜡通过使基础油料的蜡质组分异构化成较少的蜡状分支链异链烷烃，但操作的严重性是 被控制以仅影响蜡组分的部分去除。 在随后的脱蜡步骤中进一步除去蜡状组分，该脱蜡步骤选择性地除去更多的蜡状正链烷烃组分，留下有助于产物中高VI的支链异链烷烃。 选择性脱蜡步骤可以是溶剂，例如 MEK脱蜡操作或使用ZSM-22或ZSM-23等高选择性沸石的催化脱蜡。 可以控制初始催化脱蜡操作的严重性，以便实现异链烷烃含量的净增加，并且由于溶剂脱蜡步骤的选择性，可以保留这种增加的异链烷烃浓度，从而产生高VI的产物。 原料的倾点优选在初始催化脱蜡步骤期间降低至不低于产物的目标倾点的10°F，优选不低于20°F的值。 通常，这将导致在进料的倾点下降至少10°F，优选至少降低20°F。

    Process for producing alkyl aromatic compounds
    4.
    发明授权
    Process for producing alkyl aromatic compounds 失效
    烷基芳族化合物的制备方法

    公开(公告)号：US4409412A

    公开(公告)日：1983-10-11

    申请号：US423337

    申请日：1982-09-24

    申请人： Werner O. Haag ,  Tracy J. Huang

    发明人： Werner O. Haag ,  Tracy J. Huang

    IPC分类号： C07C2/86

    CPC分类号： C07C2/862 ,  C07C2529/40 ,  C07C2529/44 ,  C07C2529/46

    摘要： A process for alkylating aromatic compounds wherein the product aromatics are provided with one or more alkyl groups possessing at least two carbon atoms is disclosed wherein starting aromatic compound(s) and an alkylating atent which is a mixture of hydrogen and/or a hydrogen-containing substance which provides hydrogen under process conditions and a carbon oxide, e.g., a mixture of syngas (hydrogen and carbon monoxide) are reacted at elevated temperature in the presence of an activated catalyst containing metal values selected from the group consisting of iron, cobalt, ruthenium, manganese, rhodium and osmium, and a zeolite having a constraint index of 12 or less, e.g., ZSM-5. The alkylated aromatics can be dealkylated by known and conventional means to provide olefin and the dealkylated aromatics can be recycled to the alkylation zone.

    摘要翻译： 公开了一种芳族化合物的烷基化方法，其中产物芳族化合物具有一个或多个具有至少两个碳原子的烷基，其中起始芳族化合物和烷基化剂是氢和/或含氢的混合物 在工艺条件下提供氢的物质和碳氧化物，例如合成气（氢气和一氧化碳）的混合物在升高的温度下在活性催化剂存在下反应，所述催化剂含有选自铁，钴，钌的金属值 ，锰，铑和锇以及具有12或更小约束指数的沸石，例如ZSM-5。 烷基化芳族化合物可以通过已知和常规方法脱烷基化以提供烯烃，并且脱烷基化的芳族化合物可以再循环到烷基化区。

    Conversion of ketones over metal-containing zeolite catalysts
    5.
    发明授权
    Conversion of ketones over metal-containing zeolite catalysts 失效
    酮与含金属的沸石催化剂的转化

    公开(公告)号：US4339606A

    公开(公告)日：1982-07-13

    申请号：US232074

    申请日：1981-02-06

    申请人： Tracy J. Huang ,  Werner O. Haag

    发明人： Tracy J. Huang ,  Werner O. Haag

    IPC分类号： C07C45/73 ,  C07C45/45

    CPC分类号： C07C45/73

    摘要： Ketones are converted in one step to saturated dimeric ketones by passing them over a zeolite having a silica to alumina ratio of at least 12 and a Constraint Index of from 1 to 12 and containing a Group VIII metal.

    摘要翻译： 将酮通过使它们通过二氧化硅与氧化铝之比至少为12且约束指数为1至12并含有第Ⅷ族金属的沸石而在一个步骤中转化成饱和二聚酮。

    Conversion of synthesis gas to hydrocarbon mixtures
    6.
    发明授权
    Conversion of synthesis gas to hydrocarbon mixtures 失效
    将合成气转化为烃混合物

    公开(公告)号：US4157338A

    公开(公告)日：1979-06-05

    申请号：US883970

    申请日：1978-03-06

    申请人： Werner O. Haag ,  Tracy J. Huang

    发明人： Werner O. Haag ,  Tracy J. Huang

    IPC分类号： C07C1/04

    CPC分类号： C07C1/0455 ,  C07C2529/068

    摘要： A mixture of carbon monoxide and hydrogen is contacted with a mixture comprising an element selected from the group consisting of ruthenium, rhodium and osmium carbon monoxide reduction catalyst and a crystalline alumino-silicate providing a pore dimension greater than about 5 Angstroms and a constraint index in the range of 1 to 12 to produce hydrocarbon mixtures useful in forming gasoline boiling range products, aromatic rich hydrocarbons, and chemical intermediates.

    摘要翻译： 将一氧化碳和氢气的混合物与包含选自钌，铑和锇一氧化碳还原催化剂的元素的混合物和提供孔尺寸大于约5埃的结晶铝硅酸盐接触，并且约束指数 范围为1至12，以产生可用于形成汽油沸点产物，富含芳烃的化学中间体的烃混合物。

    Conversion of synthesis gas to hydrocarbon mixtures utilizing dual reactors
    7.
    发明授权
    Conversion of synthesis gas to hydrocarbon mixtures utilizing dual reactors 失效
    使用双重反应器将合成气转化为烃混合物

    公开(公告)号：US4159995A

    公开(公告)日：1979-07-03

    申请号：US826487

    申请日：1977-08-22

    申请人： Werner O. Haag ,  Tracy J. Huang

    发明人： Werner O. Haag ,  Tracy J. Huang

    IPC分类号： C07C1/04

    CPC分类号： C07C1/0485 ,  C07C2523/04 ,  C07C2523/745 ,  C07C2523/78 ,  Y10S585/943

    摘要： A gaseous mixture of carbon monoxide and hydrogen is contacted in a first reactor with an iron Fischer-Tropsch catalyst such as potassium promoted iron under special conditions and the total products from said contact are then converted in a second reactor containing HZSM-5 to obtain either a highly olefinic or highly aromatic product depending on reaction conditions.

    摘要翻译： 一氧化碳和氢气的气体混合物在特殊条件下在第一反应器中与铁费 - 托催化剂如促进铁的铁接触，然后将所述接触物的总产物在含有HZSM-5的第二反应器中转化，以获得 高度烯烃或高度芳族的产物，这取决于反应条件。

    Conversion of olefinic naphtha
    8.
    发明授权
    Conversion of olefinic naphtha 失效
    烯烃石脑油的转化

    公开(公告)号：US4097367A

    公开(公告)日：1978-06-27

    申请号：US818632

    申请日：1977-07-25

    申请人： Werner O. Haag ,  Tracy J. Huang

    发明人： Werner O. Haag ,  Tracy J. Huang

    IPC分类号： C07C5/373 ,  B01J29/00 ,  B01J29/70 ,  B01J29/74 ,  C07B61/00 ,  C07C1/00 ,  C07C2/76 ,  C07C15/02 ,  C07C67/00 ,  C10G35/06 ,  C10G35/095 ,  C10G45/04 ,  C10G45/10 ,  C10G45/54

    CPC分类号： C10G35/095 ,  B01J29/7049 ,  B01J29/74

    摘要： High severity catalytic conversion of olefinic naphthas which contain diolefins is conducted over special catalysts to yield a product stream which contains little or no non-aromatics boiling in the range of benzene, toluene and xylene. The catalysts are combinations of zinc and a metal of Groups I B and VIII of the Periodic Table with a crystalline aluminosilicate zeolite having a silica/alumina ratio greater than 12 and a constraint index not less than one nor greater than 12.

    摘要翻译： 含有二烯烃的烯烃石脑油的高度苛刻度催化转化是通过特殊的催化剂进行的，以产生在苯，甲苯和二甲苯范围内很少或没有非芳族化合物沸腾的产物流。 催化剂是锌和元素周期表ⅠB和Ⅷ族金属与二氧化硅/氧化铝比大于12的结晶硅铝酸盐沸石和约束指数不小于1或不超过12的组合。