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    Production of diisopropylbenzene
    5.
    发明授权
    Production of diisopropylbenzene 有权
    生产二异丙基苯

    公开(公告)号：US06933419B2

    公开(公告)日：2005-08-23

    申请号：US09844051

    申请日：2001-04-27

    申请人： William A. Weber ,  Walter R. Cade ,  Francis S. Bryan ,  Jose Guadalupe Santiesteban

    发明人： William A. Weber ,  Walter R. Cade ,  Francis S. Bryan ,  Jose Guadalupe Santiesteban

    IPC分类号： C07B61/00 ,  C07C6/12 ,  C07C15/02 ,  C07C15/12

    CPC分类号： C07C6/123 ,  C07C2529/08 ,  C07C2529/18 ,  C07C2529/70 ,  C07C15/02

    摘要： A process for the disproportionation of cumene is disclosed which comprises the step of contacting a feed containing cumene, under disproportionation conditions, with a catalyst comprising a molecular sieve, preferably TEA-mordenite. The contacting step disproportionates at least part of the cumene in the feed to provide a disproportionation effluent containing benzene and a mixture of diisopropylbenzene isomers. The effluent is then recovered and contains, prior to any separation step, less 1% of ortho-diisopropylbenzene by weight of the total diisopropylbenzene content of said effluent, less than 1 wt % of n-propylbenzene, less than 5 wt % of triisopropylbenzenes and less than 5 wt % of disproportionation products other than benzene and diisopropylbenzenes.

    摘要翻译： 公开了异丙苯歧化的方法，其包括在歧化条件下使含有枯烯的进料与包含分子筛，优选TEA丝光沸石的催化剂接触的步骤。 接触步骤歧化进料中的异丙基苯的至少一部分，以提供含有苯和二异丙基苯异构体的混合物的歧化流出物。 然后回收流出物，并且在任何分离步骤之前，包含按所述流出物的总二异丙苯含量的重量计小于1重量％的邻二异丙基苯，小于1重量％的正丙基苯，小于5重量％的三异丙基苯和 除苯和二异丙基苯以外的歧化产物少于5重量％。

    Partially decomposed catalyst and hydrocarbon oxidation processes using the same
    9.
    发明授权
    Partially decomposed catalyst and hydrocarbon oxidation processes using the same 有权
    部分分解的催化剂和烃氧化方法使用它们

    公开(公告)号：US07718564B2

    公开(公告)日：2010-05-18

    申请号：US11434717

    申请日：2006-05-16

    申请人： Jihad Mohammed Dakka ,  Sabato Miseo ,  Stuart Leon Soled ,  Jose Guadalupe Santiesteban ,  Joseph Ernest Baumgartner ,  Michiel Christian Alexander Van Vliet ,  Roger Arthur Sheldon

    发明人： Jihad Mohammed Dakka ,  Sabato Miseo ,  Stuart Leon Soled ,  Jose Guadalupe Santiesteban ,  Joseph Ernest Baumgartner ,  Michiel Christian Alexander Van Vliet ,  Roger Arthur Sheldon

    IPC分类号： B01J23/72 ,  B01J23/755 ,  B01J31/00 ,  B01J27/24

    CPC分类号： B01J31/2243 ,  B01J23/76 ,  B01J2231/70 ,  B01J2531/16 ,  B01J2531/847 ,  C07C68/00 ,  C07C69/96

    摘要： The present invention is related to a hydrocarbon oxidation process. The process comprises bringing one or more hydrocarbons into contact with a source of oxygen in the presence of a radical initiator and a catalyst. The catalyst comprises an organic metal complex located on a catalyst support, and is obtained by partial decomposition of the organic metal complex. For example, the process can be used to produce dimethyl carbonate from dimethoxy methane. The invention is also related to a partially decomposed catalyst that comprises a silica support and an organic metal complex, wherein at least 5% of the organic compound remains in the catalyst. The organic metal complex comprises an organic compound and a metal-based compound wherein the metal is selected from copper, nickel, and combinations thereof. The invention is also related to a process for manufacturing of a catalyst comprising mixing L-arginine, a Cu-based compound, water, and optionally another metal-based compound to form a solution; impregnating the solution onto a silica support to form a catalyst precursor; and partially decomposing the L-arginine to form the catalyst so that at least 5% of L-arginine remains in the catalyst.

    摘要翻译： 本发明涉及烃氧化方法。 该方法包括在自由基引发剂和催化剂的存在下使一种或多种烃与氧源接触。 催化剂包含位于催化剂载体上的有机金属络合物，并通过有机金属络合物的部分分解获得。 例如，该方法可用于从二甲氧基甲烷生产碳酸二甲酯。 本发明还涉及包含二氧化硅载体和有机金属络合物的部分分解的催化剂，其中至少5％的有机化合物保留在催化剂中。 有机金属络合物包括有机化合物和金属基化合物，其中金属选自铜，镍及其组合。 本发明还涉及制造催化剂的方法，其包括将L-精氨酸，Cu基化合物，水和任选的其它金属类化合物混合以形成溶液; 将溶液浸渍到二氧化硅载体上以形成催化剂前体; 并部分分解L-精氨酸以形成催化剂，使得至少5％的L-精氨酸保留在催化剂中。