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    Seal Structures for Solid Oxide Fuel Cell Devices
    1.
    发明申请
    Seal Structures for Solid Oxide Fuel Cell Devices 审中-公开
    固体氧化物燃料电池装置的密封结构

    公开(公告)号：US20100297534A1

    公开(公告)日：2010-11-25

    申请号：US12864149

    申请日：2009-01-27

    申请人： Thomas Dale Ketcham ,  John Stephen Rosettie ,  Dell Joseph St. Julien ,  Sujanto Widjaja

    发明人： Thomas Dale Ketcham ,  John Stephen Rosettie ,  Dell Joseph St. Julien ,  Sujanto Widjaja

    IPC分类号： H01M2/08 ,  H01M8/00

    CPC分类号： H01M8/0273 ,  H01M2008/1293 ,  Y02P70/56

    摘要： Disclosed are seals and seal structures for use in electrochemical devices such as solid oxide fuel cell devices. Exemplary seal structures are configured such that at least a portion of the interface between the seal and electrolyte sheet deviates from planarity by extending either (i) upwardly and inwardly (ii) or downwardly and inwardly, toward the active portion of the electrolyte sheet surface where one or more device electrodes are deposited. By angling the seal portion of the electrolyte sheet, the sharpness of any resulting bends or deformations that may occur during use can be reduced, thus reducing the likelihood of any cracks forming in the typically high stress regions of the electrolyte sheet. Further, preferably at least a portion of the electrolyte sheet contacting the seal composition, the seal-electrolyte interface may deviate from planarity by at least 0.1 mm from the seal-electrolyte interface, where the deviation from planarity extends normal to the seal or inwardly toward the active surface region of the electrolyte sheet. Also disclosed are methods for manufacturing the inventive seal structures and electrochemical device assemblies comprising same.

    摘要翻译： 公开了用于电化学装置例如固体氧化物燃料电池装置的密封件和密封结构。 示例性的密封结构被配置成使得密封和电解质片之间的界面的至少一部分通过（i）向上和向内（ii）或向下和向内延伸朝向电解质片表面的有效部分而偏离平面度， 沉积一个或多个器件电极。 通过使电解质片的密封部分倾斜，可以减少在使用期间可能发生的任何所得到的弯曲或变形的锐度，从而降低在电解质片的典型高应力区域中形成任何裂纹的可能性。 此外，优选地，与密封组合物接触的电解质片的至少一部分，密封 - 电解质界面可能偏离与密封电解质界面至少0.1mm的平面度，其中平面度的偏离垂直于密封或向内朝向 电解质片的活性表面区域。 还公开了用于制造本发明的密封结构的方法和包括其的电化学装置组件。

    GLASS-CERAMIC SEALS FOR USE IN SOLID OXIDE FUEL CELLS
    4.
    发明申请
    GLASS-CERAMIC SEALS FOR USE IN SOLID OXIDE FUEL CELLS 有权
    用于固体氧化物燃料电池的玻璃 - 陶瓷密封

    公开(公告)号：US20090075802A1

    公开(公告)日：2009-03-19

    申请号：US12273022

    申请日：2008-11-18

    申请人： Michael Edward Badding ,  Sasha Marjanovic ,  Linda Ruth Pinckney ,  Dell Joseph St. Julien

    发明人： Michael Edward Badding ,  Sasha Marjanovic ,  Linda Ruth Pinckney ,  Dell Joseph St. Julien

    IPC分类号： C03C10/04 ,  C03C8/00

    CPC分类号： C03C8/24 ,  C03C3/087 ,  C03C3/097 ,  C03C10/0036 ,  C03C27/00 ,  C03C29/00 ,  H01M8/0282 ,  H01M2008/1293

    摘要： The invention is directed to highly crystalline, frit-sintered glass-ceramic materials and seals made using them that are suitable for solid oxide fuel cell applications. The seals have a coefficient of thermal expansion in the range of 70-130×10−7° C., preferably 85-115×10−7° C. The glass-ceramic materials have a crystalline component and a glass component, the crystalline component being >50% of the glass-ceramic and the glass component being 75%. Regarding the crystalline component only, >50% of the crystals in the crystalline component of the glass-ceramic has a structure selected from the structural groups represented by walstromite, cyclowollastonite, μ-(Ca,Sr)SiO3, kalsilite, kaliophilite and wollastonite (the primary crystalline phase) and the remaining

    摘要翻译： 本发明涉及高度结晶的烧结玻璃陶瓷材料和使用它们制造的适用于固体氧化物燃料电池应用的密封件。 密封件的热膨胀系数为70-130×10-7℃，优选为85-115×10-7℃。玻璃 - 陶瓷材料具有结晶成分和玻璃成分，结晶成分> 50 玻璃陶瓷和玻璃组分的％为<50％。 在一个优选实施方案中，结晶组分> 75％。 关于结晶成分，玻璃 - 陶瓷的结晶成分中的> 50％的结晶具有选自由硬质铁矿，环状硅灰石，mu-（Ca，Sr）SiO 3，硅酸镁，闪锌矿和硅灰石（ 主结晶相），剩余的<50％的结晶成分是至少一个第二结晶相。 通常，本发明的玻璃陶瓷可用作金属对金属，金属对陶瓷和陶瓷到陶瓷密封剂。