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    Dental materials based on radically polymerizable macromers with antimicrobial effect
    1.
    发明申请
    Dental materials based on radically polymerizable macromers with antimicrobial effect 有权
    基于可自由基聚合的大分子单体的牙科材料具有抗菌作用

    公开(公告)号：US20070254979A1

    公开(公告)日：2007-11-01

    申请号：US11502420

    申请日：2006-08-11

    申请人： Ulrich Salz ,  Jorg Zimmermann ,  Dirk Poppe ,  Volker Rheinberger ,  Jorg Tiller ,  Christian Waschinski

    发明人： Ulrich Salz ,  Jorg Zimmermann ,  Dirk Poppe ,  Volker Rheinberger ,  Jorg Tiller ,  Christian Waschinski

    IPC分类号： A61K6/08

    CPC分类号： A61K6/0017 ,  A61K6/0023 ,  A61K6/083 ,  A61K6/09 ,  C08L33/00 ,  C08L75/16

    摘要： Dental material which contains at least one compound of the formula [PG]m-R1-Z-SP—Y—R2—[WG]p, in which m=1, 2 or 3; p=1, 2 or 3; R1=is absent, a linear or branched C1 to C20 alkylene radical which can be interrupted one or more times by O, S, NH, SiR′, CONH CONR′, COO and/or OCONH, a substituted or unsubstituted, aromatic C6 to C14 radical or a combination thereof; R2=is absent, a linear or branched C1 to C20 alkylene radical which can be interrupted one or more times by O, S, NH, SiR′, CONH CONR′, COO and/or OCONH, a substituted or unsubstituted, aromatic C6 to C14 radical or a combination thereof; PG=a radically polymerizable group; SP=a polymeric spacer which is selected from polyethylene glycol, polypropylene glycol, polyglycerol, polyalkyloxazoline, polyethyleneimine, polyacrylic acid, polymethacrylic acid, polyvinyl alcohol, polyvinyl acetate, poly-(2-hydroxyethyl)acrylate, poly-(2-hydroxyethyl)methacrylate groups, hydrophilic polypeptide groups and copolymers of the corresponding monomers; WG=antimicrobially active group; Z=is absent, O, S, an ester, amide or urethane group; Y=is absent, O, S, an ester, amide or urethane group, and which has a molecular weight of at least 1.000.

    摘要翻译： 含有至少一种式[PG] m -R 1的化合物的牙科材料-Z-SP-YR 2 - [WG] 其中m = 1,2或3; p = 1,2或3; R 1不存在，可以被O，S中断一次或多次的直链或支链C 1至C 20亚烷基 ，NH，SiR'，CONH CONR'，COO和/或OCONH，取代或未取代的芳族C 6至C 14个基团或其组合; R 2不存在，可以被O，S中断一次或多次的直链或支链C 1至C 20亚烷基 ，NH，SiR'，CONH CONR'，COO和/或OCONH，取代或未取代的芳族C 6至C 14个基团或其组合; PG =自由基聚合性基团; SP =选自聚乙二醇，聚丙二醇，聚甘油，聚烷基恶唑啉，聚乙烯亚胺，聚丙烯酸，聚甲基丙烯酸，聚乙烯醇，聚乙酸乙烯酯，聚（2-羟乙基）丙烯酸酯，聚（2-羟乙基）甲基丙烯酸酯 基团，亲水性多肽组和相应单体的共聚物; WG =抗微生物活性组; Z =不存在，O，S，酯，酰胺或氨基甲酸酯基; Y =不存在，O，S，酯，酰胺或氨基甲酸酯基，其分子量至少为1.000。

    Surface-modified fillers
    2.
    发明申请
    Surface-modified fillers 有权

    公开(公告)号：US20060247329A1

    公开(公告)日：2006-11-02

    申请号：US11292578

    申请日：2005-12-02

    申请人： Norbert Moszner ,  Simone Klapdohr ,  Ulrich Salz ,  Jorg Zimmermann ,  Volker Rheinberger

    发明人： Norbert Moszner ,  Simone Klapdohr ,  Ulrich Salz ,  Jorg Zimmermann ,  Volker Rheinberger

    IPC分类号： A61K6/08 ,  A61K6/083

    CPC分类号： A61K6/083 ,  A61K6/0017 ,  A61K6/0023 ,  A61K6/0073 ,  A61K6/093 ,  Y10T428/29 ,  C08L33/14 ,  C08L43/02 ,  C08L83/06

    摘要： Filler which is surface-modified with a compound of the formula [(PG)—R1—Z]n—SP—[Y—R2—(AG)]m, in which AG is —COOH, —P(═O)(OH)2, —O—P(═O)(OH)2, —SO2OH, —SiR3R4X, or a chelating group; R1 is a C1-C3 alkylene group or cyclopropylene group or is absent; R2 is a C1-C10 alkylene group or is absent; R3 is a C1-C8 alkyl group, chlorine or OR5; R4 is a C1-C8 alkyl group, phenyl, chlorine or OR5; R5 is a C1-C6 alkyl group; X is OR5 or chlorine; Y is O, S, CO—NH, O—CO—NH, NH—CO—NH or is absent, Y being absent if R2 is absent; Z is O, S, CO—NR6, O—CO—NH, NH—CO—NH or is absent, R6 being H or C1-C6 alkyl; PG is a radically polymerizable group of the formula in which R9 is H, C1-C3 alkyl, C1-C3 hydroxyalkyl or COOR10; R10 is H, C1-C10 alkyl, 1,6-dimethylphenyl or mesityl; R11 is H or phenyl; m is 1 or 2; n is 1, 2, 3 or 4; SP is absent or is an (n+m)-valent linear or branched aliphatic C1-C30 radical, in which the carbon chain can be interrupted by O, S, CO—NH, O—CO—NH or NH—CO—NH, an (n+m)-valent aromatic C6-C18 radical, an (n+m)-valent cycloaliphatic C3-C18 radical or an (n+m)-valent heterocyclic C3-C18 radical, where the radicals can be substituted or unsubstituted; in which, if AG is a silyl radical of the formula —SiR3R4X and PG is a vinyl group of the formula H2C═CH—, R1 and Z are not absent simultaneously.

    Dental coating materials
    4.
    发明申请
    Dental coating materials 有权
    牙科涂料

    公开(公告)号：US20050165129A1

    公开(公告)日：2005-07-28

    申请号：US10928540

    申请日：2004-08-27

    申请人： Norbert Moszner ,  Simone Klapdohr ,  Ulrich Salz ,  Jorg Zimmermann ,  Volker Rheinberger

    发明人： Norbert Moszner ,  Simone Klapdohr ,  Ulrich Salz ,  Jorg Zimmermann ,  Volker Rheinberger

    IPC分类号： A61K6/093 ,  C08F290/06 ,  C08G77/20 ,  C09D183/04 ,  A61K6/08

    CPC分类号： C09D183/04 ,  A61K6/0017 ,  Y10S522/908 ,  C08L83/16

    摘要： Polymerizable materials which contain (1) 1 to 80 wt.-% of at least one polysiloxane, (2) 0.1 to 5 wt.-% of one or more initiators for radical polymerization, (3) 0 to 60 wt.-% of radically polymerizable monomer and (4) 1 to 50 wt.-% of one or more radically polymerizable monomers which carry at least phosphonic acid group, sulphonic acid group and/or mono- or dihydrogen phosphoric acid ester group, the polysiloxane (1), the monomer (3) or both being substituted by fluorine. The materials are suitable in particular for the coating of natural or artificial teeth.

    摘要翻译： 含有（1）1至80重量％的至少一种聚硅氧烷的可聚合材料，（2）0.1至5重量％的一种或多种用于自由基聚合的引发剂，（3）0至60重量％ 可自由基聚合的单体和（4）1至50重量％的至少携带膦酸基，磺酸基和/或单或二氢磷酸酯基的一种或多种可自由基聚合的单体，聚硅氧烷（1）， 单体（3）或两者均被氟取代。 这些材料特别适用于天然或人造牙齿的涂层。

    Self-etching dental materials based on (METH) acrylamide phosphates
    6.
    发明申请
    Self-etching dental materials based on (METH) acrylamide phosphates 有权
    基于（METH）丙烯酰胺磷酸盐的自蚀牙科材料

    公开(公告)号：US20060135719A1

    公开(公告)日：2006-06-22

    申请号：US11211938

    申请日：2005-08-25

    申请人： Norbert Moszner ,  Iris Lamparth ,  Frank Zeuner ,  Ulrich Salz ,  Angela Mucke ,  Jorg Zimmermann ,  Jorg Angermann ,  Volker Rheinberger

    发明人： Norbert Moszner ,  Iris Lamparth ,  Frank Zeuner ,  Ulrich Salz ,  Angela Mucke ,  Jorg Zimmermann ,  Jorg Angermann ,  Volker Rheinberger

    IPC分类号： C08F120/54

    CPC分类号： A61K6/0017 ,  A61K6/0023 ,  A61K6/0029 ,  A61K6/083 ,  A61K6/09 ,  C08L33/26 ,  C08L33/04 ,  C08L75/04

    摘要： Polymerizable dental material, characterized in that it contains at least one (meth)acrylamide phosphate of the following general formula (I): in which R1 is H or CH3; R2 is H or a C1-C4 alkyl radical or forms together with the nitrogen atom to which it is bonded and one or more atoms which belong to R3 or R3′ a heterocyclic ring; R3, R3′ independently of each other are a linear or branched aliphatic C1-C50 radical with a valency of m+n or p+n, an aromatic C6-C18 radical with a valency of m+n or p+n, or a cycloaliphatic, araliphatic or heterocyclic C3-C18 radical with a valency of m+n or p+n, wherein the carbon chains of the radical or radicals can be interrupted by O, S, CONR4, OCONH, or form together with one or more atoms which belong to R2 and the nitrogen atom, to which the R2 is bonded a heterocyclic ring, R3′ being H if p=0, and R4 being H, C1-C10 alkyl, C6-C12 aryl, C6-C10 aralkyl or a bicylic C4-C12 radical; n is 1, 2, 3 or 4 if p=0, and is 1 or 2 if p≠0; m is 1, 2, 3 or 4; p is 0, 1, 2, 3 or 4; x is 0 or S.

    摘要翻译： 可聚合的牙科材料，其特征在于它含有至少一种下列通式（I）的（甲基）丙烯酰胺磷酸酯：其中R 1是H或CH 3; R 2是H或C 1 -C 4烷基，或与其键合的氮原子一起形成一个或多个 属于R 3或R 3'杂原子的杂原子; R 3，R 3，R 3'彼此独立地是直链或支链的脂族C 1 -C 50 - 基团 具有m + n或p + n的化合价，m + n或p + n的芳族C 6 -C 18 - 基团，或脂环族基团， 芳烷基或杂环C 3 -C 18 - 基团，其价态为m + n或p + n，其中基团或基团的碳链可以被O， S，CONR 4，OCONH，或与一个或多个属于R 2的原子和氮原子一起形成，R 2 O 2 >键合杂环，如果p = 0，则R 3'为H，R 4为H，C 1 -C 3 C 10 -C 12烷基，C 6 -C 12芳基，C 6 -C 10芳烷基或C 6 -C 12烷基 二元C 4 -C 12 - 基团; 如果p = 0，则n为1,2,3或4，如果p <0，则为1或2; m为1,2,3或4; p是0，1，2，3或4; x是0或S.

    Self-etching dental materials based on (METH) acrylamide phosphates
    7.
    发明授权
    Self-etching dental materials based on (METH) acrylamide phosphates 有权
    基于（METH）丙烯酰胺磷酸盐的自蚀牙科材料

    公开(公告)号：US07622538B2

    公开(公告)日：2009-11-24

    申请号：US11211938

    申请日：2005-08-25

    申请人： Norbert Moszner ,  Iris Lamparth ,  Frank Zeuner ,  Ulrich Salz ,  Angela Mucke ,  Jorg Zimmermann ,  Jorg Angermann ,  Volker M. Rheinberger

    发明人： Norbert Moszner ,  Iris Lamparth ,  Frank Zeuner ,  Ulrich Salz ,  Angela Mucke ,  Jorg Zimmermann ,  Jorg Angermann ,  Volker M. Rheinberger

    IPC分类号： C08F20/58 ,  C08F20/60

    CPC分类号： A61K6/0017 ,  A61K6/0023 ,  A61K6/0029 ,  A61K6/083 ,  A61K6/09 ,  C08L33/26 ,  C08L33/04 ,  C08L75/04

    摘要： Polymerizable dental material, characterized in that it contains at least one (meth)acrylamide phosphate of the following general formula (I): in which R1 is H or CH3; R2 is H or a C1-C4 alkyl radical or forms together with the nitrogen atom to which it is bonded and one or more atoms which belong to R3 or R3′ a heterocyclic ring; R3, R3′ independently of each other are a linear or branched aliphatic C1-C50 radical with a valency of m+n or p+n, an aromatic C6-C18 radical with a valency of m+n or p+n, or a cycloaliphatic, araliphatic or heterocyclic C3-C18 radical with a valency of m+n or p+n, wherein the carbon chains of the radical or radicals can be interrupted by O, S, CONR4, OCONH, or form together with one or more atoms which belong to R2 and the nitrogen atom, to which the R2 is bonded a heterocyclic ring, R3′ being H if p=0, and R4 being H, C1-C10 alkyl, C6-C12 aryl, C6-10 aralkyl or a bicylic C4-C12 radial; n is 1, 2, 3 or 4 if p=0, and is 1 or 2 if p ≠0; m is 1, 2, 3 or 4; p is 0, 1, 2, 3 or 4; x is 0 or S.

    摘要翻译： 可聚合牙科材料，其特征在于其含有至少一种下列通式（I）的（甲基）丙烯酰胺磷酸酯：其中R1是H或CH3; R2是H或C1-C4烷基或与其键合的氮原子一起形成一个或多个属于R3或R3'杂原子的原子; R 3，R 3'彼此独立地为具有m + n或p + n价的直链或支链脂族C 1 -C 50基团，价数为m + n或p + n的芳族C 6 -C 18基团或 脂环族，芳脂族或杂环C 3 -C 18基，其价态为m + n或p + n，其中基团或基团的碳链可被O，S，CONR 4，OCONH中断，或与一个或多个原子一起形成 属于R2和氮原子，R 2与杂环结合，如果p = 0，则R3'为H，R4为H，C1-C10烷基，C6-C12芳基，C6-10芳烷基或双 C4-C12径向; 如果p = 0，则n为1,2,3或4，如果p为0，则为1或2; m为1,2,3或4; p是0，1，2，3或4; x是0或S.