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公开(公告)号：US06486368B1
公开(公告)日：2002-11-26
申请号：US10054004
申请日：2002-01-24
IPC分类号： C07C2700
CPC分类号： C07D301/26 , C07C17/10 , C07C29/124 , C07C41/01 , C07C45/27 , Y02P20/125 , C07C19/075 , C07C47/06 , C07C31/04 , C07C43/06 , C07C43/043
摘要： Alcohols, ethers, and olefins are manufactured from alkanes by mixing an alkane and bromine in a reactor to form alkyl bromide and hydrogen bromide. The alkyl bromide only or the alkyl bromide and the hydrogen bromide are directed into contact with metal oxide to form an alcohol and/or an ether, or an olefin and metal bromide. The metal bromide is oxidized to form original metal oxide and bromine, both of which are recycled.
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公开(公告)号：US06472572B1
公开(公告)日：2002-10-29
申请号：US09886078
申请日：2001-06-20
申请人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
发明人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
IPC分类号： C07C2700
CPC分类号： C07C29/124 , C07C17/10 , C07C41/01 , C07D301/26 , Y02P20/125 , C07C19/075 , C07C31/04 , C07C43/043
摘要： Methanol and/or dimethyl ether are manufactured from methane by mixing methane and bromine in a reactor to form methyl bromide and hydrogen bromide. The methyl bromide only or the methyl bromide and the hydrogen bromide are directed into contact with metal oxide to form methanol and/or dimethyl ether and a metal bromide. The metal bromide is oxidized to form original metal oxide catalyst and bromine, both of which are recycled.
摘要翻译： 甲烷和/或二甲醚由甲烷通过在反应器中混合甲烷和溴来形成甲基溴和溴化氢。 仅甲基溴或甲基溴和溴化氢与金属氧化物接触以形成甲醇和/或二甲醚和金属溴化物。 金属溴化物被氧化形成原始的金属氧化物催化剂和溴，这两种催化剂都被再循环。
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公开(公告)号：US06462243B1
公开(公告)日：2002-10-08
申请号：US09951570
申请日：2001-09-11
申请人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
发明人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
IPC分类号： C07C2700
CPC分类号： C07C29/124 , C07C17/10 , C07C41/01 , C07D301/26 , Y02P20/125 , C07C19/075 , C07C31/04 , C07C43/043
摘要： Alcohols and/or ethers are synthesized from alkanes by mixing an alkane and bromine in a reactor to form alkyl bromide and hydrogen bromide. The alkyl bromide is directed into contact with metal oxide to form alcohol and/or ether and a metal bromide. The metal bromide is oxidized to metal oxide and bromine, both of which are recycled.
摘要翻译： 通过在反应器中混合烷烃和溴以形成烷基溴和溴化氢从烷烃合成醇和/或醚。 使烷基溴与金属氧化物接触以形成醇和/或醚和金属溴化物。 金属溴化物被氧化成金属氧化物和溴，两者都被再循环。
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4.发明授权公开(公告)号：US07148390B2
公开(公告)日：2006-12-12
申请号：US10375464
申请日：2003-02-27
CPC分类号： C07D301/26 , C07C17/10 , C07C29/124 , C07C45/27 , Y02P20/125 , C07C19/075 , C07C47/06 , C07C31/04 , C07C31/08
摘要： Alcohols, ethers, aldehydes, and olefins are manufactured from alkanes by mixing an alkane and a halogen selected from the group including chlorine, bromine, and iodine in a reactor to form alkyl halide and hydrogen halide. The alkyl halide only or the alkyl halide and the hydrogen halide are directed into contact with metal oxide to form an alcohol and/or an ether, or an olefin and metal halide. The metal halide is oxidized to form original metal oxide and halogen, both of which are recycled.
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5.发明授权Method and apparatus for synthesizing olefins, alcohols, ethers, and aldehydes 失效用于合成烯烃，醇，醚和醛的方法和装置公开(公告)号：US07161050B2
公开(公告)日：2007-01-09
申请号：US10430240
申请日：2003-08-19
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen Stucky , Peter Ford
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen Stucky , Peter Ford
CPC分类号： C07C45/27 , C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C41/16 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/043 , C07C19/07 , C07C19/075 , C07C47/06 , C07C31/08 , C07C31/125 , C07C43/04 , C07C43/06
摘要： A reactant selected from the group consisting of alkanes, alkenes, alkynes, dienes, and aromatics is reacted with a halide selected from the group including chlorine, bromine, and iodine to form a first reaction product. The first reaction product is reacted with a solid oxidizer to form a product selected from the group including olefins, alcohols, ethers, and aldehydes, and spent oxidizer. The spent oxidizer is oxidized to form the original solid oxidizer and the second reactant which are recycled.
摘要翻译： 选自烷烃，烯烃，炔烃，二烯烃和芳族化合物的反应物与选自氯，溴和碘的卤化物反应形成第一反应产物。 将第一反应产物与固体氧化剂反应以形成选自包括烯烃，醇，醚和醛的产物和废氧化剂。 废氧化剂被氧化以形成原始的固体氧化剂和再循环的第二反应物。
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公开(公告)号：US08415512B2
公开(公告)日：2013-04-09
申请号：US12904030
申请日：2010-10-13
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改善重复步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US20100121119A1
公开(公告)日：2010-05-13
申请号：US12692831
申请日：2010-01-25
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
IPC分类号： C07C17/013
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US20110034741A1
公开(公告)日：2011-02-10
申请号：US12904030
申请日：2010-10-13
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
IPC分类号： C07C17/013
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US07838708B2
公开(公告)日：2010-11-23
申请号：US12692831
申请日：2010-01-25
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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10.发明授权公开(公告)号：US06465696B1
公开(公告)日：2002-10-15
申请号：US09951739
申请日：2001-09-11
IPC分类号： C07C2700
CPC分类号： C07C29/124 , C07C17/10 , C07C41/01 , C07D301/26 , Y02P20/125 , C07C19/075 , C07C31/04 , C07C43/043
摘要： Alcohols, ethers, and olefins are manufactured from alkanes by mixing an alkane and bromine in a reactor to form alkyl bromide and hydrogen bromide. The alkyl bromide only or the alkyl bromide and the hydrogen bromide are directed into contact with metal oxide to form an alcohol and/or an ether, or an olefin and metal bromide. The metal bromide is oxidized to form original metal oxide and bromine, both of which are recycled.
摘要翻译： 通过在反应器中混合烷烃和溴以形成烷基溴和溴化氢，由烷烃制备醇，醚和烯烃。 仅将烷基溴或烷基溴和溴化氢引导与金属氧化物接触以形成醇和/或醚，或烯烃和金属溴化物。 金属溴化物被氧化以形成原始的金属氧化物和溴，这两者都被再循环。
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