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公开(公告)号：US07838708B2
公开(公告)日：2010-11-23
申请号：US12692831
申请日：2010-01-25
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US20100121119A1
公开(公告)日：2010-05-13
申请号：US12692831
申请日：2010-01-25
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Breed , Michael F. Doherty
IPC分类号： C07C17/013
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US20110034741A1
公开(公告)日：2011-02-10
申请号：US12904030
申请日：2010-10-13
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
IPC分类号： C07C17/013
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改性步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US08415512B2
公开(公告)日：2013-04-09
申请号：US12904030
申请日：2010-10-13
申请人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
发明人： Jeffrey H. Sherman , Eric W. McFarland , Michael J. Weiss , Ivan Marc Lorkovic , Leroy E. Laverman , Shouli Sun , Dieter J. Schaefer , Galen D. Stucky , Peter C. Ford , Philip Grosso , Ashley W. Rreed , Michael F. Doherty
CPC分类号： C07C1/30 , C07C17/10 , C07C29/124 , C07C29/58 , C07C45/27 , C07C2521/02 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/04 , C07C2523/06 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/80 , C07C2527/128 , C07C2527/133 , C07D301/26 , Y02P20/582 , C07C19/075 , C07C19/043 , C07C19/07 , C07C47/06 , C07C41/01 , C07C43/04 , C07C31/02
摘要： Improvements in previously disclosed methods of and apparatuses for converting alkanes, alkenes, and aromatics to olefins, alcohols, ethers, and aldehydes includes: safety improvements, use of alternative feedstocks, process simplification, improvements to the halogenation step, improvements to the reproportionation step, improvements to the solid oxide reaction, improvements to solid oxide regeneration, improvements in separations, maintenance, start-up, shut-down, and materials of construction.
摘要翻译： 将烷烃，烯烃和芳族化合物转化为烯烃，醇，醚和醛的先前公开的方法和装置的改进包括：安全性改进，替代原料的使用，工艺简化，改进卤化步骤，改善重复步骤， 固体氧化物反应的改进，固体氧化物再生的改进，分离改进，维护，启动，停机和施工材料。
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公开(公告)号：US06472572B1
公开(公告)日：2002-10-29
申请号：US09886078
申请日：2001-06-20
申请人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
发明人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
IPC分类号： C07C2700
CPC分类号： C07C29/124 , C07C17/10 , C07C41/01 , C07D301/26 , Y02P20/125 , C07C19/075 , C07C31/04 , C07C43/043
摘要： Methanol and/or dimethyl ether are manufactured from methane by mixing methane and bromine in a reactor to form methyl bromide and hydrogen bromide. The methyl bromide only or the methyl bromide and the hydrogen bromide are directed into contact with metal oxide to form methanol and/or dimethyl ether and a metal bromide. The metal bromide is oxidized to form original metal oxide catalyst and bromine, both of which are recycled.
摘要翻译： 甲烷和/或二甲醚由甲烷通过在反应器中混合甲烷和溴来形成甲基溴和溴化氢。 仅甲基溴或甲基溴和溴化氢与金属氧化物接触以形成甲醇和/或二甲醚和金属溴化物。 金属溴化物被氧化形成原始的金属氧化物催化剂和溴，这两种催化剂都被再循环。
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公开(公告)号：US06462243B1
公开(公告)日：2002-10-08
申请号：US09951570
申请日：2001-09-11
申请人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
发明人： Xiao Ping Zhou , Ivan Marc Lorkovic , Galen D. Stucky , Peter C. Ford , Jeffrey H. Sherman , Philip Grosso
IPC分类号： C07C2700
CPC分类号： C07C29/124 , C07C17/10 , C07C41/01 , C07D301/26 , Y02P20/125 , C07C19/075 , C07C31/04 , C07C43/043
摘要： Alcohols and/or ethers are synthesized from alkanes by mixing an alkane and bromine in a reactor to form alkyl bromide and hydrogen bromide. The alkyl bromide is directed into contact with metal oxide to form alcohol and/or ether and a metal bromide. The metal bromide is oxidized to metal oxide and bromine, both of which are recycled.
摘要翻译： 通过在反应器中混合烷烃和溴以形成烷基溴和溴化氢从烷烃合成醇和/或醚。 使烷基溴与金属氧化物接触以形成醇和/或醚和金属溴化物。 金属溴化物被氧化成金属氧化物和溴，两者都被再循环。
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公开(公告)号：US06214176B1
公开(公告)日：2001-04-10
申请号：US09479114
申请日：2000-01-07
IPC分类号： C07C2900
CPC分类号： C07C29/48 , B01F2003/04858 , B01F2215/0431 , B01J8/009 , B01J10/007 , B01J12/007 , B01J19/123 , B01J19/127 , B01J19/2415 , B01J19/2475 , B01J35/002 , B01J35/004 , B01J2219/00081 , B01J2219/00139 , B01J2219/00162 , B01J2219/00189 , B01J2219/0869 , B01J2219/0877 , B01J2219/0884 , B01J2219/0892 , C01B3/38 , C01B2203/0233 , C01B2203/1035 , C01B2203/1041 , C01B2203/1241 , C07C29/00 , C12C11/02 , Y02P20/52 , C07C31/04 , C07C31/08 , C07C31/10
摘要： In a method of and apparatus for manufacturing methanol and higher alcohols from natural gas a catalytic area is formed on the exterior of a gas permeable partition. Natural gas is maintained on the interior of the gas permeable partition at predetermined pressure. Relative movement between the gas permeable partition and the water forms sub-micron sized bubbles of natural gas. Electromagnetic radiation is directed onto the catalytic surface to form hydroxyl radicals from the water. Methyl, ethyl, and propyl ions from the natural gas combine with the hydroxyl ions to form methanol, ethanol, and propanol.
摘要翻译： 在从天然气制造甲醇和高级醇的方法和装置中，在透气性隔板的外部形成催化区域。 天然气以预定压力保持在透气隔板的内部。 透气隔板与水之间的相对运动形成亚微米级的天然气气泡。 电磁辐射被引导到催化表面上以从水中形成羟基自由基。 来自天然气的甲基，乙基和丙基离子与羟基离子结合形成甲醇，乙醇和丙醇。
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公开(公告)号：US07847139B2
公开(公告)日：2010-12-07
申请号：US12217311
申请日：2008-07-02
IPC分类号： C07C1/00
CPC分类号： C07C1/26 , C07C2521/10 , C07C2523/02 , C07C2529/18 , C07C2529/40 , Y10S585/935 , Y10S585/943
摘要： A method of synthesizing hydrocarbons from smaller hydrocarbons includes the steps of hydrocarbon halogenation, simultaneous oligomerization and hydrogen halide neutralization, and product recovery, with a metal-oxygen cataloreactant used to facilitate carbon-carbon coupling. Treatment with air or oxygen liberates halogen and regenerates the cataloreactant.
摘要翻译： 从较小的烃合成烃的方法包括烃卤化，同时低聚和卤化氢中和以及用于促进碳 - 碳偶联的金属 - 氧催化反应物的产物回收步骤。 用空气或氧气处理释放卤素并再生催化反应物。
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公开(公告)号：US20080269534A1
公开(公告)日：2008-10-30
申请号：US12217311
申请日：2008-07-02
IPC分类号： C07C2/00
CPC分类号： C07C1/26 , C07C2521/10 , C07C2523/02 , C07C2529/18 , C07C2529/40 , Y10S585/935 , Y10S585/943
摘要： A method of synthesizing hydrocarbons from smaller hydrocarbons includes the steps of hydrocarbon halogenation, simultaneous oligomerization and hydrogen halide neutralization, and product recovery, with a metal-oxygen cataloreactant used to facilitate carbon-carbon coupling. Treatment with air or oxygen liberates halogen and regenerates the cataloreactant.
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10.发明授权公开(公告)号：US06713655B2
公开(公告)日：2004-03-30
申请号：US10365087
申请日：2003-02-12
申请人： Aysen Yilmaz , Gurkan Atinc Yilmaz , Ivan M. Lorkovic , Galen D. Stucky , Peter C. Ford , Eric McFarland , Jeffrey H. Sherman
发明人： Aysen Yilmaz , Gurkan Atinc Yilmaz , Ivan M. Lorkovic , Galen D. Stucky , Peter C. Ford , Eric McFarland , Jeffrey H. Sherman
IPC分类号： C07C4500
CPC分类号： C07D301/26 , C07C17/10 , C07C29/124 , C07C45/27 , Y02P20/125 , C07C19/075 , C07C47/06 , C07C31/04 , C07C31/08
摘要： Alcohols, ethers, aldehydes, and olefins are manufactured from alkanes by mixing an alkane and a halogen selected from the group including chlorine, bromine, and iodine in a reactor to form alkyl halide and hydrogen halide. The alkyl halide only or the alkyl halide and the hydrogen halide are directed into contact with metal oxide to form an alcohol and/or an ether, or an olefin and metal halide. The metal halide is oxidized to form original metal oxide and halogen, both of which are recycled.
摘要翻译： 醇，醚，醛和烯烃是由烷烃和反应器中的烷烃和选自氯，溴和碘的卤素混合形成烷基卤和卤化氢制成的。 仅将烷基卤化物或烷基卤化物和卤化氢引导与金属氧化物接触以形成醇和/或醚，或烯烃和金属卤化物。 金属卤化物被氧化以形成原始的金属氧化物和卤素，这两者都被再循环。
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