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    Cured product of a modified multiplex ethylene copolymer
    1.
    发明授权
    Cured product of a modified multiplex ethylene copolymer 失效
    改性多元乙烯共聚物的固化产物

    公开(公告)号：US5252675A

    公开(公告)日：1993-10-12

    申请号：US797986

    申请日：1991-11-26

    申请人： Yoshihiro Moteki ,  Toshiyuki Iwashita ,  Hitoshi Funada ,  Naotoshi Watanabe

    发明人： Yoshihiro Moteki ,  Toshiyuki Iwashita ,  Hitoshi Funada ,  Naotoshi Watanabe

    IPC分类号： C08F8/14 ,  C08F8/32 ,  C08F210/02 ,  C08F8/00

    CPC分类号： C08F210/02 ,  C08F8/14 ,  C08F8/32 ,  C08F2810/20 ,  C08F2810/30

    摘要： Disclosed is a multiplex ethylene copolymer comprising (a) 50 to 94.8 mole % of units derived from ethylene, which are represented by the following formula (I):--CH.sub.2 --CH.sub.2 -- (I)(b) 5 to 45 mole % of units derived from a monomer selected from alkyl acrylates, alkyl methacrylates, vinyl carboxylates and isopropenyl carboxylates, which are represented by the following formula (II): ##STR1## wherein R.sub.1 stands for a hydrogen atom or a methyl group, and X is ##STR2## (in which R.sub.2 and R.sub.3 stand for an alkyl group having 1 to 10 carbon atoms),and (c) 0.2 to 5 mole % of units derived from a monomer having a radical-polymerizable ethylenic double bond and at least one carbon-to-carbon double bond which is different from a double bond of an aromatic nucleus. This ethylene copolymer can be easily cured, and the cured copolymer is a rubber having excellent oil resistance and heat resistance. This multiplex ethylene copolymer can be obtained by copolymerizing a monomer forming the units (a) with a monomer forming the units (b) and (c') a monomer having a radical-polymerizable ethylenic double bond and an acid anhydride group, a carboxyl group and/or an epoxy group, and modifying the obtained copolymer with a low-molecular-weight modifier selected from unsaturated amines and unsaturated alcohols having at least one carbon-to-carbon double bond different from a double bond of an aromatic nucleus (when a radical-polymerizable monomer having an epoxy group is used, the low-molecular-weight modifier may be an unsaturated carboxylic acid having at least one carbon-to-carbon double bond different from a double bond of an aromatic nucleus).

    摘要翻译： 公开了一种多元乙烯共聚物，其包含（a）50至94.8摩尔％的由乙烯衍生的单元，其由下式（I）表示：-CH 2 -CH 2 - （I）（b）5至45摩尔％的单元 衍生自由下式（II）表示的丙烯酸烷基酯，甲基丙烯酸烷基酯，羧酸乙烯酯和异丙烯基羧酸酯的单体：其中R1代表氢原子或甲基，X是 （其中R2和R3代表具有1-10个碳原子的烷基），和（c）0.2-5摩尔％的衍生自具有可自由基聚合的烯属双键和至少一个碳的单体的单元 碳双键，其与芳香核的双键不同。 该乙烯共聚物可以容易地固化，并且固化的共聚物是具有优异的耐油性和耐热性的橡胶。 这种多元乙烯共聚物可以通过使形成单元（a）的单体与形成单元（b）和（c'）的单体共聚而获得，该单体具有可自由基聚合的烯属双键和酸酐基的单体，羧基 和/或环氧基，并且用选自不同于芳族核的双键的至少一个碳 - 碳双键的不饱和胺和不饱和醇的低分子量改性剂改性所得共聚物（当a 使用具有环氧基的可自由基聚合的单体，低分子量改性剂可以是具有至少一个与芳香核的双键不同的碳 - 碳双键的不饱和羧酸）。

    Multiplex ethylene copolymer, process for preparation thereof and cured product thereof
    2.
    发明授权
    Multiplex ethylene copolymer, process for preparation thereof and cured product thereof 失效
    复合乙烯共聚物，其制备方法和其固化产物

    公开(公告)号：US5093429A

    公开(公告)日：1992-03-03

    申请号：US480382

    申请日：1990-02-15

    申请人： Yoshihiro Moteki ,  Toshiyuki Iwashita ,  Hitoshi Funada ,  Naotoshi Watanabe

    发明人： Yoshihiro Moteki ,  Toshiyuki Iwashita ,  Hitoshi Funada ,  Naotoshi Watanabe

    IPC分类号： C08F8/00 ,  C08F8/14 ,  C08F8/32 ,  C08F210/02

    CPC分类号： C08F210/02 ,  C08F8/14 ,  C08F8/32 ,  C08F2810/20 ,  C08F2810/30

    摘要： Disclosed is a multiplex ethylene coplymer comprising (a) 50 to 94.8 mole % of units derived from ethylene, which are represented by the following formula (I):--CH.sub.2 --CH.sub.2 -- (I)(b) 5 to 45 mole % of units derived from a monomer selected from alkyl acrylates, alkyl methacrylates, vinyl carboxylates and isopropenyl carboxylates, which are represented by the following formula (II): ##STR1## wherein R.sub.1 stands for a hydrogen atom or a methyl group, and X is ##STR2## in which R.sub.2 and R.sub.3 stand for an alkyl group having 1 to 10 carbon atoms), and (c) 0.2 to 5 mole % of units derived from a monomer having a radical-polymerizable ethylenic double bond and at least one carbon-to-carbon double bond which is different from a double bond of an aromatic nucleus. This ethylene copolymer can be easily cured, and the cured copolymer is a rubber having excellent oil resistance and heat resistance.This multiplex ethylene copolymer can be obtained by copolymerizing a monomer forming the units (a) with a monomer forming the units (b) and (c') a monomer having a radical-polymerizable ethylenic double bond and an acid anhydride group, a carboxyl group and/or an epoxy group, and modifying the obtained copolymer with a low-molecular-weight modifier selected from unsaturated amines and unsaturated alcohols having at least one carbon-to-carbon double bond different from a double bond of an aromatic nucleus (when a radical-polymerizable monomer having an epoxy group is used, the low-molecular-weight modifier may be an unsaturated carboxylic acid having at least one carbon-to-carbon double bond different from a double bond of an aromatic nucleus).

    摘要翻译： 公开了一种多元乙烯共聚物，其包含（a）50至94.8摩尔％的衍生自乙烯的单元，其由下式（I）表示：-CH 2 -CH 2 - （I）（b）5至45摩尔％的单元 衍生自由下式（II）表示的丙烯酸烷基酯，甲基丙烯酸烷基酯，羧酸乙烯酯和异丙烯基羧酸酯的单体：其中R1代表氢原子或甲基，X是 其中R 2和R 3代表具有1至10个碳原子的烷基），和（c）0.2至5摩尔％的衍生自具有自由基聚合性烯键式双键的单体和至少一种碳 - 与芳香族核的双键不同的碳 - 碳双键。 该乙烯共聚物可以容易地固化，并且固化的共聚物是具有优异的耐油性和耐热性的橡胶。 这种多元乙烯共聚物可以通过使形成单元（a）的单体与形成单元（b）和（c'）的单体共聚而获得，该单体具有可自由基聚合的烯属双键和酸酐基的单体，羧基 和/或环氧基，并且用选自不同于芳族核的双键的至少一个碳 - 碳双键的不饱和胺和不饱和醇的低分子量改性剂改性所得共聚物（当a 使用具有环氧基的可自由基聚合的单体，低分子量改性剂可以是具有至少一个与芳香核的双键不同的碳 - 碳双键的不饱和羧酸）。

    Polypropylene resin composition
    4.
    发明申请
    Polypropylene resin composition 审中-公开
    聚丙烯树脂组合物

    公开(公告)号：US20090203816A1

    公开(公告)日：2009-08-13

    申请号：US12291630

    申请日：2008-11-12

    申请人： Toshiyuki Iwashita

    发明人： Toshiyuki Iwashita

    IPC分类号： C08K5/00 ,  C08L23/12 ,  C08F8/00

    CPC分类号： C08K5/057 ,  C08F8/50 ,  C08F110/06 ,  C08F210/06 ,  C08F2800/20 ,  C08F2810/10 ,  C08J3/28 ,  C08J2323/10 ,  C08K3/22 ,  C08K3/2279 ,  C08K5/0091 ,  C08K5/14 ,  C08L23/10 ,  C08L2205/02 ,  C08L2666/04 ,  C08F2500/12 ,  C08F2500/11 ,  C08F2500/17 ,  C08F210/16 ,  C08F110/02

    摘要： A polypropylene resin composition comprising (A) 99.8 to 80 weight parts of a polypropylene resin having a melt flow rate of 0.1 to 50 g/10 min and (B) 0.2 to 20 weight parts of an olefin copolymer rubber having an intrinsic viscosity [η] of 0.5 to 4.0 dl/g and/or a polyethylene resin having a density of 0.895 to 0.945 g/cc and a melt flow rate of 0.05 to 15 g/10 min, which have undergone an ionization ray-irradiation treatment and/or a treatment of adding 0.05 to 5 weight parts of an organic peroxide to 100 weight parts of the aforesaid polypropylene resin composition comprising (A) and (B) and then melting.

    摘要翻译： 一种聚丙烯树脂组合物，其包含（A）99.8〜80重量份熔体流动速率为0.1〜50g / 10分钟的聚丙烯树脂，（B）0.2〜20重量份的特性粘度[η ]为0.5〜4.0dl / g，和/或密度为0.895〜0.945g / cc，熔体流动速率为0.05〜15g / 10min的聚乙烯树脂，其经过电离射线照射处理和/或 在100重量份上述包含（A）和（B）的聚丙烯树脂组合物中然后熔融的情况下，加入0.05〜5重量份有机过氧化物的处理。

    Polyropylene resin compositions
    6.
    发明申请
    Polyropylene resin compositions 审中-公开
    聚丙烯树脂组合物

    公开(公告)号：US20080076865A1

    公开(公告)日：2008-03-27

    申请号：US11903621

    申请日：2007-09-24

    申请人： Toshiyuki Iwashita

    发明人： Toshiyuki Iwashita

    IPC分类号： C08K3/22 ,  C08L23/12

    CPC分类号： C08K5/057 ,  C08F8/50 ,  C08F2810/10 ,  C08K3/22 ,  C08K3/2279 ,  C08K5/0091 ,  C08K5/14 ,  C08L23/10 ,  C08L2023/42 ,  C08L2205/02 ,  C08L2666/04 ,  C08F110/06

    摘要： A polypropylene resin composition containing (A) a polypropylene resin treatment product obtained by adding from (0.05) to (5) weight parts of an organic peroxide to (100) weight parts of a polypropylene resin with a melt flow rate of from (0.1) to (50) g/10 min and carrying out a melt treatment and (B) from (0.01) to (2) weight parts of an oxide of the group (2) or (12) metal of the periodic table or a metal alkoxide of defined formula to (100) weight parts of a resin content of the above polypropylene resin treatment product.

    摘要翻译： 一种聚丙烯树脂组合物，其含有（A）通过从（0.05）〜（5）重量份的有机过氧化物加入（100）重量份熔体流动速率为（0.1）的聚丙烯树脂得到​​的聚丙烯树脂处理产物， 至（50）g / 10分钟，进行熔融处理，（B）从（0.01）至（2）重量份的元素周期表第（2）或（12）族金属的氧化物或金属醇盐 （100）重量份上述聚丙烯树脂处理产物的树脂含量。

    Polypropylene resin composition
    7.
    发明申请
    Polypropylene resin composition 审中-公开
    聚丙烯树脂组合物

    公开(公告)号：US20050119380A1

    公开(公告)日：2005-06-02

    申请号：US10502102

    申请日：2003-01-16

    申请人： Toshiyuki Iwashita

    发明人： Toshiyuki Iwashita

    IPC分类号： C08J3/28 ,  C08K3/18 ,  C08K3/22 ,  C08K5/00 ,  C08K5/057 ,  C08L23/10 ,  C08L23/12 ,  C08L23/16 ,  C08L23/26 ,  C08L53/00 ,  C08L53/02 ,  C08L1/00

    CPC分类号： C08L23/16 ,  C08K3/22 ,  C08K5/0083 ,  C08K5/057 ,  C08L23/10 ,  C08L53/00 ,  C08L53/02 ,  C08L53/025 ,  C08L2205/02 ,  C08L2666/06 ,  C08L2666/04

    摘要： A polypropylene composition comprising (C) one or more compound(s) selected from the group consisting of oxides of the group 2 or the group 12 metals of the periodic table and metal alkoxides, added in an amount of from 0.01 to 2 weight parts to 100 weight parts of a resin component prepared by subjecting 100 weight parts of a resin component comprising (A) from 10 to less than 80 weight parts of a polypropylene component having a melt flow rate of from 0.1 to 300 g/10 min and (B) from 90 to more than 20 weight parts of an olefin copolymer rubber component having an intrinsic viscosity [η] of from 0.5 to 5.0 dl/g to a treatment of irradiating with an ionizing radiation and/or a melt treatment after adding from 0.05 to 5 weight parts of an organic peroxide.

    摘要翻译： 一种聚丙烯组合物，其包含（C）一种或多种选自元素周期表第2族或第12族金属的氧化物和金属醇盐的化合物，其添加量为0.01至2重量份， 将100重量份的树脂成分（100重量份）由（A）10〜80重量份的熔体流动速率为0.1〜300g / 10分钟的聚丙烯成分和（B ）从90至大于20重量份的特性粘度η为0.5-5.0dl / g的烯烃共聚物橡胶组分，用于在从0.05至0.5重量份之间添加电离辐射和/或熔融处理 5重量份有机过氧化物。

    Polypropylene resin composition
    8.
    发明授权
    Polypropylene resin composition 失效
    聚丙烯树脂组合物

    公开(公告)号：US07470727B2

    公开(公告)日：2008-12-30

    申请号：US10478347

    申请日：2002-05-21

    申请人： Toshiyuki Iwashita

    发明人： Toshiyuki Iwashita

    IPC分类号： C08J3/28 ,  C08L23/12

    CPC分类号： C08K5/057 ,  C08F8/50 ,  C08F110/06 ,  C08F210/06 ,  C08F2800/20 ,  C08F2810/10 ,  C08J3/28 ,  C08J2323/10 ,  C08K3/22 ,  C08K3/2279 ,  C08K5/0091 ,  C08K5/14 ,  C08L23/10 ,  C08L2205/02 ,  C08L2666/04 ,  C08F2500/12 ,  C08F2500/11 ,  C08F2500/17 ,  C08F210/16 ,  C08F110/02

    摘要： A polypropylene resin composition comprising (A) 99.8 to 80 weight parts of a polypropylene resin having a melt flow rate of 0.1 to 50 g/10 min and (B) 0.2 to 20 weight parts of an olefin copolymer rubber having an intrinsic viscosity [η] of 0.5 to 4.0 dl/g and/or a polyethylene resin having a density of 0.895 to 0.945 g/cc and a melt flow rate of 0.05 to 15 g/10 min, which have undergone an ionization ray-irradiation treatment and/or a treatment of adding 0.05 to 5 weight parts of an organic peroxide to 100 weight parts of the aforesaid polypropylene resin composition comprising (A) and (B) and then melting.

    摘要翻译： 一种聚丙烯树脂组合物，其包含（A）99.8〜80重量份熔体流动速率为0.1〜50g / 10分钟的聚丙烯树脂，（B）0.2〜20重量份的特性粘度[η ]为0.5〜4.0dl / g，和/或密度为0.895〜0.945g / cc，熔体流动速率为0.05〜15g / 10min的聚乙烯树脂，其经过电离射线照射处理和/或 在100重量份上述包含（A）和（B）的聚丙烯树脂组合物中然后熔融的情况下，加入0.05〜5重量份有机过氧化物的处理。