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    Supercapacitor with a meso-porous nano graphene electrode
    1.
    发明申请
    Supercapacitor with a meso-porous nano graphene electrode 有权
    具有中孔多孔纳米石墨烯电极的超级电容器

    公开(公告)号：US20120026643A1

    公开(公告)日：2012-02-02

    申请号：US12804911

    申请日：2010-08-02

    申请人： Zhenning Yu ,  David Neff ,  Chen-guang Liu ,  Bor Z. Jang ,  Aruna Zhamu

    发明人： Zhenning Yu ,  David Neff ,  Chen-guang Liu ,  Bor Z. Jang ,  Aruna Zhamu

    IPC分类号： H01G9/00

    CPC分类号： H01G11/36 ,  H01G11/02 ,  H01G11/04 ,  H01G11/24 ,  H01G11/38 ,  H01G11/46 ,  Y02E60/13

    摘要： A supercapacitor comprising a two electrodes, a porous separator disposed between the two electrodes, and an ionic liquid electrolyte in physical contact with the two electrodes, wherein at least one of the two electrodes comprises a meso-porous structure being formed of a plurality of nano graphene platelets and multiple pores having a pore size in the range of 2 nm and 25 nm, wherein the graphene platelets are not spacer-modified or surface-modified platelets. Preferably, the graphene platelets are curved, not flat-shaped. The pores are accessible to ionic liquid molecules, enabling the formation of large amounts of electric double layer charges in a supercapacitor, which exhibits an exceptionally high specific capacitance and high energy density.

    摘要翻译： 一种超级电容器，包括两个电极，设置在所述两个电极之间的多孔隔离体和与所述两个电极物理接触的离子液体电解质，其中所述两个电极中的至少一个包括由多个纳米颗粒形成的中孔多孔结构 石墨烯血小板和孔径在2nm和25nm范围内的多个孔，其中石墨烯血小板不是间隔子改性的或表面改性的血小板。 优选地，石墨烯片晶是弯曲的，不是平坦的。 离子液体分子可以获得孔隙，使得能够在超级电容器中形成大量的双电层电荷，其表现出非常高的比电容和高能量密度。

    Supercapacitor with a meso-porous nano graphene electrode
    2.
    发明授权
    Supercapacitor with a meso-porous nano graphene electrode 有权
    具有中孔多孔纳米石墨烯电极的超级电容器

    公开(公告)号：US09053870B2

    公开(公告)日：2015-06-09

    申请号：US12804911

    申请日：2010-08-02

    申请人： Zhenning Yu ,  David Neff ,  Chen-guang Liu ,  Bor Z. Jang ,  Aruna Zhamu

    发明人： Zhenning Yu ,  David Neff ,  Chen-guang Liu ,  Bor Z. Jang ,  Aruna Zhamu

    IPC分类号： H01G11/36 ,  H01G11/02 ,  H01G11/04 ,  H01G11/46 ,  H01G11/38 ,  H01G11/24

    CPC分类号： H01G11/36 ,  H01G11/02 ,  H01G11/04 ,  H01G11/24 ,  H01G11/38 ,  H01G11/46 ,  Y02E60/13

    摘要： A supercapacitor comprising a two electrodes, a porous separator disposed between the two electrodes, and an ionic liquid electrolyte in physical contact with the two electrodes, wherein at least one of the two electrodes comprises a meso-porous structure being formed of a plurality of nano graphene platelets and multiple pores having a pore size in the range of 2 nm and 25 nm, wherein the graphene platelets are not spacer-modified or surface-modified platelets. Preferably, the graphene platelets are curved, not flat-shaped. The pores are accessible to ionic liquid molecules, enabling the formation of large amounts of electric double layer charges in a supercapacitor, which exhibits an exceptionally high specific capacitance and high energy density.

    摘要翻译： 一种超级电容器，包括两个电极，设置在所述两个电极之间的多孔隔离体和与所述两个电极物理接触的离子液体电解质，其中所述两个电极中的至少一个包括由多个纳米颗粒形成的中孔多孔结构 石墨烯血小板和孔径在2nm和25nm范围内的多个孔，其中石墨烯血小板不是间隔子改性的或表面改性的血小板。 优选地，石墨烯片晶是弯曲的，不是平坦的。 离子液体分子可以获得孔隙，使得能够在超级电容器中形成大量的双电层电荷，其表现出非常高的比电容和高能量密度。

    Spacer-modified graphene electrode for supercapacitor
    3.
    发明授权
    Spacer-modified graphene electrode for supercapacitor 有权
    用于超级电容器的间隔改性石墨烯电极

    公开(公告)号：US08947854B2

    公开(公告)日：2015-02-03

    申请号：US13573844

    申请日：2012-10-09

    申请人： Aruna Zhamu ,  Zhenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    发明人： Aruna Zhamu ,  Zhenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    IPC分类号： H01G9/00 ,  H01G11/36 ,  B82Y30/00

    CPC分类号： H01G11/36 ,  B82Y30/00 ,  B82Y40/00 ,  H01G11/32 ,  Y02E60/13 ,  Y02T10/7022 ,  Y10S977/734 ,  Y10S977/932 ,  Y10S977/948

    摘要： A spacer-modified nano graphene platelet electrode, comprising: (a) multiple nano graphene platelets or sheets having an average thickness smaller than 10 nm; and (b) discrete, non-metallic nano-scaled particles that are disposed between two graphene platelets or sheets to serve as a spacer. In such a spacer-modified graphene electrode, large amounts of electrolyte-accessible pores are formed, enabling the formation of large amounts of electric double layer charges in a supercapacitor, which exhibits an exceptionally high specific capacitance.

    摘要翻译： 一种间隔物改性的纳米石墨烯片晶电极，包括：（a）平均厚度小于10nm的多个纳米石墨烯片晶或片; 和（b）分散的非金属纳米级粒子，其设置在两个石墨烯片晶片之间以用作间隔物。 在这种间隔物改性的石墨烯电极中，形成大量的电解质可接近的孔，使得能够在超级电容器中形成大量的双电层电荷，这表现出特别高的比电容。

    Spacer-modified graphene electrode for supercapacitor
    4.
    发明申请
    Spacer-modified graphene electrode for supercapacitor 有权
    用于超级电容器的间隔改性石墨烯电极

    公开(公告)号：US20140098461A1

    公开(公告)日：2014-04-10

    申请号：US13573844

    申请日：2012-10-09

    申请人： Aruna Zhamu ,  Zhenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    发明人： Aruna Zhamu ,  Zhenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    IPC分类号： H01G11/36

    CPC分类号： H01G11/36 ,  B82Y30/00 ,  B82Y40/00 ,  H01G11/32 ,  Y02E60/13 ,  Y02T10/7022 ,  Y10S977/734 ,  Y10S977/932 ,  Y10S977/948

    摘要： A spacer-modified nano graphene platelet electrode, comprising: (a) multiple nano graphene platelets or sheets having an average thickness smaller than 10 nm; and (b) discrete, non-metallic nano-scaled particles that are disposed between two graphene platelets or sheets to serve as a spacer. In such a spacer-modified graphene electrode, large amounts of electrolyte-accessible pores are formed, enabling the formation of large amounts of electric double layer charges in a supercapacitor, which exhibits an exceptionally high specific capacitance.

    摘要翻译： 一种间隔物改性的纳米石墨烯片晶电极，包括：（a）平均厚度小于10nm的多个纳米石墨烯片晶或片; 和（b）分散的非金属纳米级粒子，其设置在两个石墨烯片晶片之间以用作间隔物。 在这种间隔物改性的石墨烯电极中，形成大量的电解质可接近的孔，使得能够在超级电容器中形成大量的双电层电荷，这表现出特别高的比电容。

    Partially and fully surface-enabled metal ion-exchanging energy storage devices
    8.
    发明申请
    Partially and fully surface-enabled metal ion-exchanging energy storage devices 有权
    部分和完全表面使能的金属离子交换储能装置

    公开(公告)号：US20120171574A1

    公开(公告)日：2012-07-05

    申请号：US12930294

    申请日：2011-01-03

    申请人： Aruna Zhamu ,  ChenGuang Liu ,  David Neff ,  Bor Z. Jang ,  Zhenning Yu

    发明人： Aruna Zhamu ,  ChenGuang Liu ,  David Neff ,  Bor Z. Jang ,  Zhenning Yu

    IPC分类号： H01M10/02 ,  H01M10/05 ,  B82Y30/00

    CPC分类号： H01M10/054 ,  B82Y30/00 ,  B82Y40/00 ,  H01M4/13 ,  H01M4/364 ,  H01M4/38 ,  H01M4/386 ,  H01M4/387 ,  H01M4/583 ,  H01M4/60 ,  H01M4/602 ,  H01M10/05 ,  H01M10/0565 ,  H01M10/0566 ,  H01M2004/021 ,  H01M2300/0025 ,  H01M2300/0085 ,  Y02E60/122 ,  Y02E60/13 ,  Y02T10/7011 ,  Y02T10/7022

    摘要： A surface-enabled, metal ion-exchanging battery device comprising a cathode, an anode, a porous separator, and a metal ion-containing electrolyte, wherein the metal ion is selected from (A) non-Li alkali metals; (B) alkaline-earth metals; (C) transition metals; (D) other metals such as aluminum (Al); or (E) a combination thereof; and wherein at least one of the electrodes contains therein a metal ion source prior to the first charge or discharge cycle of the device and at least the cathode comprises a functional material or nano-structured material having a metal ion-capturing functional group or metal ion-storing surface in direct contact with said electrolyte, and wherein the operation of the battery device does not involve the introduction of oxygen from outside the device and does not involve the formation of a metal oxide, metal sulfide, metal selenide, metal telluride, metal hydroxide, or metal-halogen compound. This energy storage device has a power density significantly higher than that of a lithium-ion battery and an energy density dramatically higher than that of a supercapacitor.

    摘要翻译： 一种表面使能的金属离子交换电池装置，包括阴极，阳极，多孔隔膜和含金属离子的电解质，其中所述金属离子选自（A）非Li碱金属; （B）碱土金属; （C）过渡金属; （D）其他金属如铝（Al）; 或（E）其组合; 并且其中所述电极中的至少一个在所述器件的第一充电或放电循环之前包含金属离子源，并且至少所述阴极包括具有金属离子捕获官能团或金属离子的功能材料或纳米结构材料 并且其中电池装置的操作不涉及从装置外部引入氧气，并且不涉及形成金属氧化物，金属硫化物，金属硒化物，金属碲化物，金属 氢氧化物或金属卤素化合物。 该能量存储装置的功率密度显着高于锂离子电池的功率密度，能量密度显着高于超级电容器。

    Continuous process for producing spacer-modified nano Graphene electrodes for supercapacitors
    9.
    发明申请
    Continuous process for producing spacer-modified nano Graphene electrodes for supercapacitors 有权
    用于制造用于超级电容器的间隔改性纳米石墨烯电极的连续工艺

    公开(公告)号：US20110165321A1

    公开(公告)日：2011-07-07

    申请号：US12655744

    申请日：2010-01-07

    申请人： Aruna Zhamu ,  Zenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    发明人： Aruna Zhamu ,  Zenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    IPC分类号： B05D5/12

    CPC分类号： H01G9/058 ,  B82Y30/00 ,  B82Y40/00 ,  C01B32/194 ,  C01B2204/04 ,  C01B2204/32 ,  H01G11/36 ,  H01G11/46 ,  Y02E60/13

    摘要： A specific embodiment of the present invention is a process for continuously producing a porous solid film of spacer-modified nano graphene platelets for supercapacitor electrode applications. This process comprises: (a) dissolving a precursor material in a solvent to form a precursor solution and dispersing multiple nano graphene platelets into the solution to form a suspension; (b) continuously delivering and forming the suspension into a layer of solid film composed of precursor material-coated graphene platelets overlapping one another, and removing the solvent from the solid film (e.g., analogous to a paper-making, mat-making, or web-making procedure); (c) continuously converting the precursor material into nodules bonded to surfaces of graphene platelets to form a porous solid film composed of spacer-modified graphene platelets; and (d) continuously collecting the porous solid film on a collector (e.g., a winding roller). The roll of porous solid film (mat, paper, or web) can then be cut into pieces for used as supercapacitor electrodes.

    摘要翻译： 本发明的具体实施方案是连续制备用于超级电容器电极应用的间隔物改性的纳米石墨烯片晶的多孔固体膜的方法。 该方法包括：（a）将前体材料溶解在溶剂中以形成前体溶液并将多个纳米石墨烯片晶分散到溶液中以形成悬浮液; （b）将悬浮液连续输送并形成为由彼此重叠的前体材料涂覆的石墨烯片晶组成的固体膜层，以及从固体膜中除去溶剂（例如，类似于造纸，制毡或 网络制作程序）; （c）将前体材料连续转化为结合到石墨烯片晶表面的结节，以形成由间隔改性石墨烯片晶组成的多孔固体膜; 和（d）在收集器（例如卷绕辊）上连续收集多孔固体膜。 然后可以将多孔固体膜（垫，纸或网）卷切成片以用作超级电容器电极。

    Spacer-modified nano graphene electrodes for supercapacitors
    10.
    发明授权
    Spacer-modified nano graphene electrodes for supercapacitors 有权
    用于超级电容器的间隔改性纳米石墨烯电极

    公开(公告)号：US08315039B2

    公开(公告)日：2012-11-20

    申请号：US12655247

    申请日：2009-12-28

    申请人： Aruna Zhamu ,  Zenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    发明人： Aruna Zhamu ,  Zenning Yu ,  Chen-guang Liu ,  Bor Z. Jang

    IPC分类号： H01G9/00

    CPC分类号： H01G11/24 ,  B82Y30/00 ,  B82Y40/00 ,  C01B32/19 ,  C01B32/192 ,  C01B32/194 ,  C01B2204/02 ,  C01B2204/04 ,  C01B2204/32 ,  H01G11/36 ,  H01G11/46 ,  Y02E60/13 ,  Y10T428/24802

    摘要： A surface-modified nano graphene platelet (NGP), comprising: (a) a nano graphene platelet having a thickness smaller than 10 nm; and (b) discrete, non-continuous, and non-metallic bumps or nodules bonded to a surface of the graphene platelet to serve as a spacer. When multiple surface-modified NGP sheets are stacked together to form an electrode, large numbers of electrolyte-accessible pores are formed, enabling the formation of large amounts of double layer charges in a supercapacitor, which exhibits an exceptionally high specific capacitance.

    摘要翻译： 一种表面改性的纳米石墨烯血小板（NGP），包括：（a）厚度小于10nm的纳米石墨烯血小板; 和（b）结合到石墨烯薄片的表面上的离散的，非连续的和非金属的凸起或结节用作间隔物。 当多个表面改性的NGP片堆叠在一起以形成电极时，形成大量的电解质可接近的孔，使得能够在超级电容器中形成大量的双层电荷，这表现出特别高的比电容。