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    A PROCESS FOR THE SYNTHETIC GENERATION OF METHANE
    1.
    发明授权
    A PROCESS FOR THE SYNTHETIC GENERATION OF METHANE 有权
    方法甲烷合成法生产

    公开(公告)号：EP1751078B1

    公开(公告)日：2011-01-12

    申请号：EP05701134.8

    申请日：2005-01-24

    申请人： PAUL SCHERRER INSTITUT

    发明人： SEEMANN, Martin ,  BIOLLAZ, Serge ,  STUCKI, Samuel

    IPC分类号： C07C1/10 ,  C07C1/04 ,  C07C9/04

    CPC分类号： C07C1/046 ,  C07C1/043 ,  C07C2523/755 ,  C07C9/04

    摘要： The present invention discloses a process for the synthetic generation of methane from a feed gas mixture comprising carbon monoxide, hydrogen and water vapour and optionally aromatic hydrocarbons; said process comprising the steps of: a) bringing the feed gas mixture in contact with a fluidized bed catalyst having catalyst particles which comprise as catalytic active component a metal and/or a metal compound or a mixture thereof under the circumstances of: b) an elevated temperature in the range of 250 to 500°C; c) a feed gas pressure in the range of 0.8 to 70 bar; d) a gas hourly space velocity of 1000 to 50000 h-1; and e) a concentration of H2/CO in the initial gas mixture in the range of 0.25 to 5. The afore-mentioned process allows to catalytically convert hydrogen and carbon monoxide effectively in a fluidized bed catalytic reactor which avoids a rapid deactivation of the catalyst material and therefore delivers a high activity of the catalytic active components in the process. Both thermochemical reactions, the endothermic reformation of higher hydrocarbons, i.e. aromatic hydrocarbons, and the exothermic methane generation, proceed simultaneously within the fluidized be catalytic reactor, leading to an overall enhanced thermal efficiency of the conversion process.

    Process for the production of methane
    7.
    发明公开
    Process for the production of methane 失效
    维尔法赫尔·赫尔斯滕

    公开(公告)号：EP0086538A1

    公开(公告)日：1983-08-24

    申请号：EP83200208.3

    申请日：1983-02-09

    申请人： VEG-GASINSTITUUT N.V.

    发明人： Kuijpers, Eugène Gérard Marie, Dr. ,  Geus, John Wilhelm ,  Bottelberghs, Pierre Henri, Dr.

    IPC分类号： C07C9/04 ,  C07C1/04 ,  C07C1/10 ,  B01J23/74

    CPC分类号： C07C1/046 ,  B01J23/755 ,  C07C1/0425 ,  C07C1/0445 ,  C07C1/10 ,  C07C2521/04 ,  C07C2521/08 ,  C07C2521/10 ,  C07C2523/755 ,  C07C9/04

    摘要： A process for the preparation of methane from gas mixtures containing hydrogen and/or steam and at least 5% by volume of carbonmonoxide by means of a nickel catalyst, which contains on a thermally stable oxidic carrier metallic nickel particles as an active catalyst component, in which the metallic nickel particles are chemically bonded to the thermally stable carrier. The chemical bond between the metallic nickel particles and the carrier is preferably provided by an interfacial layer different from the oxidic carrier, which layer consists of a compound containing oxygen and at feast one member selected from the group consisting of nickel and the carrier base element or elements.

    摘要翻译： 一种由包含氢和/或蒸汽的气体混合物和至少5体积％的一氧化碳的甲烷制备方法，其中镍催化剂在热稳定的氧化载体上含有作为活性催化剂组分的金属镍颗粒， 金属镍颗粒化学键合到热稳定载体上。 金属镍颗粒和载体之间的化学键优选由不同于氧化载体的界面层提供，该层由包含氧的化合物和选自镍和载体基础元素的至少一种构成， 元素。