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    CATALYTIC PROCESS FOR CONTINUOUSLY GENERATING POLYOLS
    11.
    发明申请
    CATALYTIC PROCESS FOR CONTINUOUSLY GENERATING POLYOLS 有权
    用于连续生成聚合物的催化方法

    公开(公告)号：US20110313210A1

    公开(公告)日：2011-12-22

    申请号：US13193227

    申请日：2011-07-28

    申请人： Tom N. Kalnes ,  John Q. Chen ,  Joseph A. Kocal

    发明人： Tom N. Kalnes ,  John Q. Chen ,  Joseph A. Kocal

    IPC分类号： C07C31/20

    CPC分类号： C07C29/132 ,  C10G3/44 ,  C10G3/46 ,  C10G3/48 ,  C10G3/52 ,  C10G3/56 ,  C10G2300/1014 ,  Y02P20/52 ,  Y02P30/20 ,  C07C31/202 ,  C07C31/205

    摘要： A catalytic process for generating at least one polyol from a feedstock comprising cellulose is performed in a continuous manner. The process involves, contacting, continuously, hydrogen, water, and a feedstock comprising cellulose, with a catalyst to generate an effluent stream comprising at least one polyol, water, hydrogen, and at least one co-product. The water, hydrogen, and at least one co-product are separated from the effluent stream and recycled to the reaction zone. The polyol is recovered from the effluent stream.

    摘要翻译： 以包含纤维素的原料生成至少一种多元醇的催化方法是以连续方式进行的。 该方法包括使含有纤维素的氢，水和原料与催化剂连续地接触，以产生包含至少一种多元醇，水，氢和至少一种共同产物的流出物流。 将水，氢和至少一种副产物与流出物流分离并再循环至反应区。 从流出物流中回收多元醇。

    CATALYTIC PROCESS FOR CONTINUOUSLY GENERATING POLYOLS
    12.
    发明申请
    CATALYTIC PROCESS FOR CONTINUOUSLY GENERATING POLYOLS 有权

    公开(公告)号：US20110313209A1

    公开(公告)日：2011-12-22

    申请号：US13193200

    申请日：2011-07-28

    申请人： Tom N. Kalnes ,  John Q. Chen ,  Joseph A. Kocal

    发明人： Tom N. Kalnes ,  John Q. Chen ,  Joseph A. Kocal

    IPC分类号： C07C29/74

    CPC分类号： C07C29/132 ,  C07C31/20

    摘要： A catalytic process for generating at least one polyol from a feedstock comprising cellulose is performed in a continuous manner. The process involves, contacting, continuously, hydrogen, water, and a feedstock comprising cellulose, with a catalyst to generate an effluent stream comprising at least one polyol, water, hydrogen, and at least one co-product. The water, hydrogen, and at least one co-product are separated from the effluent stream and recycled to the reaction zone. The polyol is recovered from the effluent stream.

    Combination of Hydrogenation and Base Catalyzed Depolymerization for Lignin Conversion
    13.
    发明申请
    Combination of Hydrogenation and Base Catalyzed Depolymerization for Lignin Conversion 有权
    氢化和碱催化聚合用于木质素转化的组合

    公开(公告)号：US20100137663A1

    公开(公告)日：2010-06-03

    申请号：US12394892

    申请日：2009-02-27

    申请人： John Q. Chen ,  Mark B. Koch

    发明人： John Q. Chen ,  Mark B. Koch

    IPC分类号： C07C5/373

    CPC分类号： C10G1/08 ,  C10G1/002 ,  C10G1/083 ,  C10G1/086 ,  C10G3/47 ,  C10G3/48 ,  C10G3/50 ,  C10G2300/1014 ,  C10G2300/4018 ,  C10G2400/30 ,  Y02P30/20

    摘要： A process for the conversion of lignin to chemical precursors is presented. The process comprises treating the lignin to form less acidic compounds. The process includes reacting lignin with a hydrogenation catalyst under a hydrogen atmosphere to convert acidic oxygenate compounds to less acidic oxygenates or hydrocarbons. The oxygenate compounds are reacted in a dehydrogenation and deoxygenation process to remove the oxygen and to convert the cyclic hydrocarbons back to aromatic compounds.

    摘要翻译： 提出了一种将木质素转化为化学前体的方法。 该方法包括处理木质素以形成较少的酸性化合物。 该方法包括在氢气氛下使木质素与氢化催化剂反应，以将酸性含氧化合物转化为较不酸性的含氧化合物或烃。 含氧化合物在脱氢和脱氧过程中反应以除去氧并将环状碳氢化合物转化为芳族化合物。

    Selective conversion of oxygenate to propylene using moving bed technology and a hydrothermally stabilized dual-function catalyst
    17.
    发明授权
    Selective conversion of oxygenate to propylene using moving bed technology and a hydrothermally stabilized dual-function catalyst 有权
    使用移动床技术和水热稳定的双功能催化剂选择性地将含氧化合物转化为丙烯

    公开(公告)号：US07408092B2

    公开(公告)日：2008-08-05

    申请号：US10988136

    申请日：2004-11-12

    申请人： Bryan K. Glover ,  John Q. Chen ,  Peter R. Pujado ,  Bipin V. Vora

    发明人： Bryan K. Glover ,  John Q. Chen ,  Peter R. Pujado ,  Bipin V. Vora

    IPC分类号： C07C1/00

    CPC分类号： C07C11/06 ,  B01J8/082 ,  B01J8/085 ,  B01J8/12 ,  B01J2208/00274 ,  B01J2208/00283 ,  B01J2208/00292 ,  C07C1/20 ,  C07C2521/04 ,  C07C2529/40 ,  C07C2529/84 ,  C07C2529/85 ,  Y02P20/52

    摘要： The average propylene cycle selectivity of an oxygenate to propylene (OTP) process using a dual-function oxygenate conversion catalyst is substantially enhanced by the use of a combination of: 1) moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of the fixed bed technology of the prior art; 2) a hydrothermally stabilized and dual-functional catalyst system comprising a molecular sieve having dual-function capability dispersed in a phosphorus-modified alumina matrix containing labile phosphorus and/or aluminum anions; and 3) a catalyst on-stream cycle time of 400 hours or less. These provisions stabilize the catalyst against hydrothermal deactivation and hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of average propylene cycle yield near or at essentially start-of-cycle levels.

    摘要翻译： 使用双功能含氧化合物转化催化剂的含氧化合物对丙烯（OTP）方法的平均丙烯循环选择性通过使用以下组合来显着增强：1）OTP流程图的烃合成部分中的移动床反应器技术 现有技术的固定床技术的代替; 2）水热稳定和双功能催化剂体系，其包含具有分散在含有不稳定磷和/或铝阴离子的磷改性氧化铝基质中的双功能能力的分子筛; 和3）催化剂在流循环时间为400小时以下。 这些规定稳定催化剂以防止水热失活，并将催化剂上焦炭沉积物的积聚保持在基本上不降低双功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而使维持平均丙烯循环产率接近或 基本上是循环周期的水平。

    Combination of hydrogenation and base catalyzed depolymerization for lignin conversion
    18.
    发明授权
    Combination of hydrogenation and base catalyzed depolymerization for lignin conversion 有权
    加氢和碱催化解聚木质素转化的组合

    公开(公告)号：US08871989B2

    公开(公告)日：2014-10-28

    申请号：US12394892

    申请日：2009-02-27

    申请人： John Q. Chen ,  Mark B. Koch

    发明人： John Q. Chen ,  Mark B. Koch

    IPC分类号： C10G1/06 ,  C10G1/00 ,  C10G1/08

    CPC分类号： C10G1/08 ,  C10G1/002 ,  C10G1/083 ,  C10G1/086 ,  C10G3/47 ,  C10G3/48 ,  C10G3/50 ,  C10G2300/1014 ,  C10G2300/4018 ,  C10G2400/30 ,  Y02P30/20

    摘要： A process for the conversion of lignin to chemical precursors is presented. The process comprises treating the lignin to form less acidic compounds. The process includes reacting lignin with a hydrogenation catalyst under a hydrogen atmosphere to convert acidic oxygenate compounds to less acidic oxygenates or hydrocarbons. The oxygenate compounds are reacted in a dehydrogenation and deoxygenation process to remove the oxygen and to convert the cyclic hydrocarbons back to aromatic compounds.

    摘要翻译： 提出了一种将木质素转化为化学前体的方法。 该方法包括处理木质素以形成较少的酸性化合物。 该方法包括在氢气氛下使木质素与氢化催化剂反应，以将酸性含氧化合物转化为较不酸性的含氧化合物或烃。 含氧化合物在脱氢和脱氧过程中反应以除去氧并将环状碳氢化合物转化为芳族化合物。

    Process for generation of polyols from saccharide containing feedstock
    20.
    发明授权
    Process for generation of polyols from saccharide containing feedstock 有权
    从含糖原料生成多元醇的方法

    公开(公告)号：US08222463B2

    公开(公告)日：2012-07-17

    申请号：US13193072

    申请日：2011-07-28

    申请人： Tom N. Kalnes ,  Joseph A. Kocal ,  John Q. Chen

    发明人： Tom N. Kalnes ,  Joseph A. Kocal ,  John Q. Chen

    IPC分类号： C07C29/00 ,  C07C31/18

    CPC分类号： C07C29/132 ,  C07C31/20

    摘要： A process for generating at least one polyol from a feedstock comprising saccharide is performed in a continuous or batch manner. The process involves, contacting hydrogen, water, and a feedstock comprising saccharide, with a catalyst system to generate an effluent stream comprising at least one polyol and recovering the polyol from the effluent stream. The catalyst system comprises at least one metal component with an oxidation state greater than or equal to 2+.

    摘要翻译： 以包含糖的原料产生至少一种多元醇的方法以连续或间歇方式进行。 该方法涉及使氢，水和包含糖的原料与催化剂体系接触以产生包含至少一种多元醇的流出物流并从流出物流中回收多元醇。 催化剂体系包含至少一种氧化态大于或等于2+的金属组分。