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公开(公告)号：US08957274B2
公开(公告)日：2015-02-17
申请号：US13000401
申请日：2009-06-24
IPC分类号： C07C1/20 , C07C1/24 , C07C1/26 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J38/12 , C07C1/32
CPC分类号： C07C1/20 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J38/12 , B01J2229/16 , B01J2229/18 , B01J2229/36 , B01J2229/37 , C07C1/26 , C07C1/322 , C07C2/864 , C07C4/06 , C07C2529/40 , Y02P20/584 , Y02P30/42 , C07C15/02 , C07C11/02
摘要： The present invention relates to a process to make light olefins and aromatics, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising: a0) providing a first portion and a second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock, a) providing a catalyst comprising zeolitic molecular sieves containing at least 10 membered ring pore openings or larger in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone; c) contacting the first portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction and the second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction and oxygen-containing, halogenide-containing or sulphur-containing organic feedstock to light olefins and aromatics.
摘要翻译： 本发明涉及一种在组合的XTO-OC方法中由含氧，含卤素或含硫有机原料制备轻质烯烃和芳族化合物的方法，包括：a0）提供第一部分和第二部分 所述含氧，含卤素或含硫有机原料，a）提供包含在其微孔结构中含有至少10元环孔孔或更大的沸石分子筛的催化剂，b）提供XTO反应区，OC反应 区域和催化剂再生区，所述催化剂在三个区域中循环，使得至少一部分再生催化剂通过OC反应区，OC反应区中的至少一部分催化剂通过XTO 反应区和XTO反应区中的至少一部分催化剂通入再生区; c）在有效地转化至少一部分原料以形成包含轻质烯烃的XTO反应器流出物的条件下，将XTO反应器中的含氧卤化物或含硫有机原料的第一部分与催化剂接触， 重质烃馏分; d）从所述重质烃馏分中分离出所述轻质烯烃; e）在OC反应器中将所述重质烃部分和第二部分所述含氧卤化物或含硫有机原料与所述催化剂接触，所述条件有效地将至少一部分所述重质烃部分和氧 - 含有卤化物或含硫有机原料至轻质烯烃和芳族化合物。
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12.发明申请公开(公告)号：US20130046122A1
公开(公告)日：2013-02-21
申请号：US13513892
申请日：2010-12-15
IPC分类号： C07C5/02
CPC分类号： C10G51/04 , C10G9/002 , C10G69/06 , C10G2300/807 , C10G2400/20 , C10G2400/26
摘要： The present invention is method for debottlenecking an existing steam cracker unit of which the operation is modified from high severity to low severity operation, having a cracking zone and a fractionation zone, said fractionation zone comprising a gasoline stripper, a de-methaniser (I), a de-ethaniser (I) a de-propaniser (I) and a de-butaniser (I), said de-propaniser (I) receiving product from the bottom of the de-ethaniser (I) and optionally product from the bottom of the gasoline stripper (I), wherein said debottlenecking method comprises the steps of: a) adding a selective hydrogenation unit (II), b) adding a cracking reactor (II) comprising a catalyst selective towards light olefins in the outlet, c) adding a re-run column and a de-propaniser (II), d) sending a part or all of the bottoms stream of the gasoline stripper (I) to the selective hydrogenation unit (II) and subsequently to the cracking reactor (II) at conditions effective to produce an outlet with an olefin content of lower molecular weight than that of the inlet, e) sending a part of the bottoms stream of the de-ethaniser (I) to the de-propaniser (II), such as, not to overload the de-propaniser (I) f) optionally sending a part or all of the overhead raw C4 fraction of the de-butaniser (I) to the selective hydrogenation unit (II), g) sending the cracking reactor (II) outlet to the re-run column to produce a C6+ bottom stream and a C1-C5 overhead, sending said overhead to the de-propaniser (II) to produce a C1-C3 overhead and a C4+ bottom stream recycled in whole or in part to the selective hydrogenation unit (II), optionally withdrawing a part of said C4+ bottom stream.
摘要翻译： 本发明是用于对现有的蒸汽裂解装置进行脱瓶的方法，其中操作由高严重度到低严重度操作改变，具有裂化区和分馏区，所述分馏区包含汽提汽提塔，脱甲烷反应器（I） （I）脱乙烷醇（I）和脱丁烷（I）的脱乙烷醇（I），脱丙烷（I）从脱乙烷醚（I）的底部接收产物，并且任选地从底部产物 其中所述脱瓶方法包括以下步骤：a）加入选择性氢化单元（II），b）在出口中加入包含对轻质烯烃选择性的催化剂的裂解反应器（II），c） 加入一个再运行的塔和一个脱丙烷醚（II），d）将汽油汽提塔（I）的一部分或全部塔底物流送到选择性加氢单元（II），然后送到裂解反应器（II） 在有效产生烯烃含量为l的出口的条件下 e）将脱乙烷醚（I）的一部分底部物流送到去岐化器（II），例如不会使去岐化剂（I）过载f） 任选地将脱丁烷（I）的部分或全部原料C4馏分送入选择性氢化单元（II），g）将裂解反应器（II）出口送至再运行塔以产生C6 +底 将所述开销发送到去推进器（II）以产生C1-C3塔顶馏出物，以及将全部或部分再循环到选择性加氢装置（II）的C4 +塔底馏分，任选地将部分 的所述C4 +底部流。
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公开(公告)号：US20110166303A1
公开(公告)日：2011-07-07
申请号：US13000364
申请日：2009-06-24
CPC分类号： C07C1/22 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J37/10 , B01J38/12 , B01J2229/16 , B01J2229/186 , B01J2229/36 , C07C1/20 , C07C1/26 , C07C1/322 , C07C4/06 , C07C2529/40 , C10G3/44 , C10G3/49 , C10G3/62 , C10G9/00 , C10G55/04 , C10G2400/20 , Y02P20/584 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： The present invention relates to a process to make light olefins, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising:a) providing a catalyst comprising zeolitic molecular sieves containing 10 member and larger channels in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone; c) contacting said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction to light olefins.
摘要翻译： 本发明涉及一种在组合的XTO-OC方法中由含氧的含卤化物或含硫有机原料制备轻质烯烃的方法，包括：a）提供包含含10个成员的沸石分子筛和 在其微孔结构中较大的通道，b）提供XTO反应区，OC反应区和催化剂再生区，所述催化剂在三个区中循环，使得至少一部分再生催化剂通过OC反应区 ，将OC反应区中的至少一部分催化剂通入XTO反应区，并将XTO反应区中的至少一部分催化剂通入再生区; c）在有效地转化至少一部分原料以形成包含轻质烯烃和重质烃部分的XTO反应器流出物的条件下，将XTO反应器中的含氧卤化物或含硫有机原料与催化剂接触 ; d）从所述重质烃馏分中分离出所述轻质烯烃; e）使OC反应器中的所述重质烃馏分与催化剂在有效将至少一部分所述重质烃馏分转化为轻质烯烃的条件下接触。
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14.发明授权
公开(公告)号：US5591324A
公开(公告)日：1997-01-07
申请号：US446901
申请日：1995-05-17
IPC分类号： B01J29/48 , B01J29/06 , C07B61/00 , C10G35/04 , C10G35/095 , C10G45/12 , C10G47/20 , C10G61/04 , C10G45/04
CPC分类号： B01J29/061 , C10G35/095 , C10G47/20 , C10G61/04
摘要： A hydroconversion catalyst composition includes a catalytically active matrix having a surface area of between about 50 m.sup.2 /g to about 290 m.sup.2 /g, a silicious molecular sieve support medium distributed through the matrix and having a surface area of between about 250 m.sup.2 /g to about 1200 m.sup.2 /g and a catalytically active phase supported on the support medium and including a first metal selected from group IIIA of the periodic table of elements and a second metal selected from group VIB of the periodic table of elements. The matrix preferably further includes aluminum, gallium, cobalt, molybdenum, and phosphorus.
摘要翻译： 加氢转化催化剂组合物包括表面积为约50m 2 / g至约290m 2 / g的催化活性基质，分布在基质中的硅分子筛载体介质，其表面积为约250m 2 / g至 约1200m 2 / g的催化活性相和负载在载体介质上的催化活性相，并且包含选自元素周期表的IIIA族的第一种金属和选自元素周期表的VIB族的第二种金属。 该基质优选还包括铝，镓，钴，钼和磷。
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公开(公告)号：US4795548A
公开(公告)日：1989-01-03
申请号：US923190
申请日：1986-10-27
摘要： A process for the production of anode grade coke from a hydrocarbon feed characterized by high levels of sulfur and metals comprises subjecting a vacuum resid to a fluidized bed coking process so as to produce gas, distillates, coke and a residual bottom stream, filtering the residual stream so as to remove solids and thereafter coking the filtered stream.
摘要翻译： 由烃类进料生产阳极级焦炭的方法，其特征在于高含量的硫和金属包括将真空渣油经受流化床焦化过程，以产生气体，馏出物，焦炭和残余底部流，过滤残留物 流以除去固体，然后焦化过滤的流。
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