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公开(公告)号：US08686208B2
公开(公告)日：2014-04-01
申请号：US13457493
申请日：2012-04-27
IPC分类号： C07C1/207
CPC分类号： B01J29/08 , B01J27/24 , B01J29/082 , B01J29/084 , B01J29/085 , B01J29/12 , B01J29/14 , B01J29/16 , B01J29/18 , B01J29/7007 , B01J29/83 , B01J29/85 , B01J2229/183 , B01J2229/186 , B01J2229/38 , C07C2/864 , C07C2/865 , C07C2/867 , C07C2521/02 , C07C2521/06 , C07C2523/04 , C07C2523/08 , C07C2523/12 , C07C2523/34 , C07C2523/50 , C07C2523/72 , C07C2523/745 , C07C2523/75 , C07C2529/08 , C07C2529/70 , C07C2529/83 , C07C2529/85 , C07C15/46
摘要： A process for making styrene including providing a C1 source to a reactor containing a catalyst and reacting toluene with the C1 source in the presence of the catalyst to form a product stream comprising ethylbenzene and styrene. The C1 source can be selected from the group of methanol, formaldehyde, formalin, trioxane, methylformcel, paraformaldehyde, methylal, dimethyl ether, and combinations thereof, and wherein the catalyst contains a nitrogen-substituted zeolite.
摘要翻译： 一种制备苯乙烯的方法，包括在含有催化剂的反应器中提供C1源，并在催化剂存在下使甲苯与C1源反应，形成包含乙苯和苯乙烯的产物流。 C1源可以选自甲醇，甲醛，福尔马林，三恶烷，甲基甲缩醛，多聚甲醛，甲缩醛，二甲醚及其组合，其中催化剂含有氮取代的沸石。
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公开(公告)号：US20120296142A1
公开(公告)日：2012-11-22
申请号：US13457512
申请日：2012-04-27
IPC分类号： C07C2/88 , B01J29/076 , B01J37/00 , B01J29/04
CPC分类号： B01J29/061 , B01J2229/38 , C07C2/864 , C07C2529/70 , C07C15/073 , C07C15/46
摘要： A process for making styrene including providing toluene, a co-feed, and a C1 source to a reactor containing a catalyst having a total number of acid sites and reacting toluene with the C1 source in the presence of the catalyst and the co-feed to form a product stream containing ethylbenzene and styrene where the co-feed removes at least a portion of the total number of acid sites on the catalyst. The co-feed can be selected from the group of ammonia, primary amines, and secondary amines, and combinations thereof. The C1 source can be selected from methanol, formaldehyde, formalin, trioxane, methylformcel, paraformaldehyde, methylal, dimethyl ether, and combinations thereof.
摘要翻译： 一种制备苯乙烯的方法，包括将甲苯，共同进料和C1源提供到含有总酸值位点的催化剂的反应器中，并在催化剂存在下使甲苯与C1源反应，共同进料至 形成含有乙苯和苯乙烯的产物流，其中共同进料除去催化剂上总酸数的至少一部分。 共进料可以选自氨，伯胺和仲胺，以及它们的组合。 C1源可以选自甲醇，甲醛，福尔马林，三恶烷，甲基甲缩醛，多聚甲醛，甲缩醛，二甲醚及其组合。
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33.发明申请公开(公告)号：US20120296132A1
公开(公告)日：2012-11-22
申请号：US13457510
申请日：2012-04-27
IPC分类号： C07C2/88
CPC分类号： C07C2/862 , C07C2529/70 , C07C15/073 , C07C15/46
摘要： A process for making styrene including reacting toluene with a C1 source in the presence of a catalyst and a co-feed including at least one oxidizing agent in a reactor to form a product stream including ethylbenzene and styrene and, optionally, at least one de-oxidized oxidizing agent.
摘要翻译： 一种制备苯乙烯的方法，包括在催化剂存在下使甲苯与C1源反应，并在反应器中包含至少一种氧化剂的共进料，以形成包含乙苯和苯乙烯的产物流， 氧化氧化剂。
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34.发明申请公开(公告)号：US20120108873A1
公开(公告)日：2012-05-03
申请号：US12938453
申请日：2010-11-03
CPC分类号： C07C2/867 , B01J29/068 , B01J29/072 , B01J29/084 , B01J35/002 , B01J35/006 , B01J37/0246 , B82Y30/00 , C07C2/864 , C07C2/865 , C07C2529/06 , C07C2529/72 , C07C2529/78 , C07C15/46
摘要： A method of making a catalyst containing nanosize zeolite particles supported on a support material is disclosed. A process for making styrene or ethylbenzene by reacting toluene with a C1 source over a catalyst containing nanosize zeolite particles supported on a support material is disclosed.
摘要翻译： 公开了一种制备包含负载在载体材料上的纳米尺寸沸石颗粒的催化剂的方法。 公开了一种通过使甲苯与C1源在含有负载在载体材料上的纳米尺寸沸石颗粒的催化剂上反应制备苯乙烯或乙苯的方法。
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公开(公告)号：US20110257454A1
公开(公告)日：2011-10-20
申请号：US12938449
申请日：2010-11-03
CPC分类号： B01J29/061 , B01J29/082 , B01J29/087 , B01J29/103 , B01J29/143 , B01J29/163 , B01J2229/18 , B01J2229/37 , B01J2229/38 , C07C2/862 , C07C2/864 , C07C2/867 , C07C2529/06 , C07C2529/08 , C07C15/46 , C07C15/073
摘要： A method is disclosed of preparing a catalyst including providing a substrate and a first solution containing at least one promoter, contacting the substrate with the solution to obtain a catalyst containing at least one promoter, wherein the contacting of the substrate with the solution subjects the substrate to the addition of at least one promoter.
摘要翻译： 公开了一种制备催化剂的方法，包括提供基材和含有至少一种助催化剂的第一溶液，使基材与溶液接触以获得含有至少一种助催化剂的催化剂，其中基材与溶液的接触使基材 至少加入一种启动子。
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公开(公告)号：US20110257453A1
公开(公告)日：2011-10-20
申请号：US12763233
申请日：2010-04-20
CPC分类号： C07C2/84 , B01J8/02 , B01J8/18 , B01J19/02 , B01J23/002 , B01J23/02 , B01J23/34 , B01J37/0201 , B01J37/031 , B01J2219/00006 , B01J2219/0209 , B01J2219/0218 , B01J2219/025 , B01J2523/00 , C07C2/64 , C07C5/327 , C07C2521/10 , C07C2523/02 , C07C2523/30 , C07C2523/34 , Y02P20/52 , B01J2523/12 , B01J2523/22 , B01J2523/69 , B01J2523/72 , C07C15/46
摘要： A method for the oxidative coupling of hydrocarbons includes providing an oxidative catalyst inside a reactor and carrying out the oxidative coupling reaction under a set of reaction conditions. The reactor surfaces that contact the reactants and products do not provide a significant detrimental catalyzing effect. In an embodiment the reactor contains an inert lining or a portion of the reactor inner surface is treated to reduce the detrimental catalytic effects. In an embodiment the reactor contains a lining that includes an oxidative catalyst.
摘要翻译： 烃的氧化偶合的方法包括在反应器内提供氧化催化剂，并在一组反应条件下进行氧化偶联反应。 与反应物和产物接触的反应器表面不会产生显着的不利的催化作用。 在一个实施方案中，反应器包含惰性衬里或处理反应器内表面的一部分以减少有害的催化作用。 在一个实施方案中，反应器含有包含氧化催化剂的衬里。
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公开(公告)号：US20100331593A1
公开(公告)日：2010-12-30
申请号：US12494138
申请日：2009-06-29
IPC分类号： C07C15/46
CPC分类号： C07C2/84 , C07C2521/00 , C07C2521/10 , C07C2523/00 , C07C2523/02 , C07C2523/10 , C07C2523/36 , C07C15/073 , C07C15/46
摘要： A method for the oxidative coupling of hydrocarbons, such as the oxidative coupling of methane to toluene, includes providing an oxidative catalyst inside a reactor, and carrying out the oxidative coupling reaction under a set of reaction conditions. The oxidative catalyst includes (A) at least one element selected from the group consisting of the Lanthanoid group, Mg, Ca, and the elements of Group 4 of the periodic table (Ti, Zr, and Hf); (B) at least one element selected from the group consisting of the Group 1 elements of Li, Na, K, Rb, Cs, and the elements of Group 3 (including La and Ac) and Groups 5-15 of the periodic table; (C) at least one element selected from the group consisting of the Group 1 elements of Li, Na, K, Rb, Cs, and the elements Ca, Sr, and Ba; and (D) oxygen.
摘要翻译： 烃的氧化偶合的方法，例如甲烷氧化偶联甲苯，包括在反应器内提供氧化催化剂，并在一组反应条件下进行氧化偶联反应。 氧化催化剂包括（A）选自镧系元素，Mg，Ca和元素周期表第4族元素（Ti，Zr和Hf）中的至少一种元素; （B）选自Li，Na，K，Rb，Cs的第1族元素和第3族元素（包括La和Ac）和元素周期表第5-15族中的至少一种元素; （C）选自Li，Na，K，Rb，Cs族元素和元素Ca，Sr和Ba中的至少一种元素; 和（D）氧气。
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