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公开(公告)号：US08513361B2
公开(公告)日：2013-08-20
申请号：US12808943
申请日：2008-12-29
申请人： Xiaorong Wang , Yuan-Yong Yan
发明人： Xiaorong Wang , Yuan-Yong Yan
IPC分类号： C08L53/02
CPC分类号： C08G81/021 , C08F8/00 , C08F297/04
摘要： This disclosure relates to a block interpolymer comprising at least one diene block and at least one butyl block, wherein the at least one butyl block comprises residue from a functionalizing agent on at least one end adjacent to the diene block(s). The disclosure also relates to methods of making such block interpolymers. Also disclosed is a rubber composition comprising: (a) a block interpolymer comprising at least one diene block and at least one butyl block, and (b) a filler, wherein said at least one butyl block comprises residue from a functionalizing agent on at least one end adjacent to said diene block(s).
摘要翻译： 本公开内容涉及包含至少一个二烯嵌段和至少一个丁基嵌段的嵌段互聚物，其中所述至少一个丁基嵌段包含在与二烯嵌段相邻的至少一个末端的官能化试剂的残基。 本公开还涉及制备这种嵌段互聚物的方法。 还公开了一种橡胶组合物，其包含：（a）包含至少一个二烯嵌段和至少一个丁基嵌段的嵌段互聚物，和（b）填料，其中所述至少一个丁基嵌段至少包含官能化试剂的残基 一端与所述二烯嵌段相邻。
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公开(公告)号：US20120232223A1
公开(公告)日：2012-09-13
申请号：US13509419
申请日：2010-11-08
申请人： Yuan-Yong Yan
发明人： Yuan-Yong Yan
IPC分类号： C08F8/34
摘要： A method for providing a polymer having terminal functionality that includes at least one sulfur atom and at least one silicon or tin atom involves reacting a terminally active polymer with a cyclic compound that includes in its ring structure at least one Si or Sn atom and at least one S atom, optionally at adjacent positions of the ring structure.
摘要翻译： 提供具有包含至少一个硫原子和至少一个硅或锡原子的末端官能团的聚合物的方法包括使末端活性聚合物与环状化合物反应，所述环状化合物在其环结构中包括至少一个Si或Sn原子，并且至少 一个S原子，任选地在环结构的相邻位置。
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公开(公告)号：US08227562B2
公开(公告)日：2012-07-24
申请号：US12922611
申请日：2009-03-15
申请人： Yuan-Yong Yan , Michael W. Hayes
发明人： Yuan-Yong Yan , Michael W. Hayes
CPC分类号： C08C19/44 , C08F8/00 , C08L15/00 , C08L19/006 , C08F12/08
摘要： A polymer includes at a terminus a cyclic amine radical bonded to the polymer through a ring nitrogen atom. The polymer can be provided by using a lithiated version of the cyclic amine to initiate polymerization of one or more ethylenically unsaturated monomers. The polymer can be used in the production in a variety of vulcanizates.
摘要翻译： 聚合物在末端包括通过环氮原子键合到聚合物上的环胺自由基。 聚合物可以通过使用锂化型环胺来引发一种或多种烯属不饱和单体的聚合来提供。 该聚合物可用于生产各种硫化橡胶。
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公开(公告)号：US20120136113A1
公开(公告)日：2012-05-31
申请号：US13381331
申请日：2010-06-30
申请人： Yuan-Yong Yan , Zenquan Qin , Xiao-Dong Pan
发明人： Yuan-Yong Yan , Zenquan Qin , Xiao-Dong Pan
CPC分类号： C08F2/38 , C08C19/44 , C08F236/10 , C08L7/00 , C08L15/00 , C08F4/545 , C08L2666/08
摘要： A functionalized polymer includes the reaction product of a reactive polymer and a compound that includes an aryl group having at least one directly bonded OGp substituent, where Gp is a protecting group, and a substituent (Q) which is free of active hydrogen atoms and which is, or connects to the aryl group through, a moiety that includes a carbon-to-nitrogen multiple bond. The polymer can be provided from a solution that includes one or more types of ethylenically unsaturated monomers which include at least one type of polyene, particularly one or more conjugated dienes in certain embodiments. An active terminus of the resulting reactive polymer can react with the Q substituent of the compound so as to provide a polymer having as a terminal functionality the radical of a compound that includes an aryl group having at least one directly bonded OGp substituent.
摘要翻译： 官能化聚合物包括反应性聚合物和包括具有至少一个直接键合的OGp取代基的芳基的化合物的反应产物，其中Gp是保护基，和不含活性氢原子的取代基（Q），其中 是或通过包含碳 - 氮多键的部分连接到芳基。 聚合物可以由包括一种或多种类型的烯键式不饱和单体的溶液提供，所述烯属不饱和单体在某些实施方案中包括至少一种类型的多烯，特别是一种或多种共轭二烯。 所得反应性聚合物的活性末端可与化合物的Q取代基反应，从而提供具有包含具有至少一个直接键合的OGp取代基的芳基的化合物基团作为末端官能团的聚合物。
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公开(公告)号：US20120130009A1
公开(公告)日：2012-05-24
申请号：US13381345
申请日：2010-06-30
申请人： Zengquan Qin , Yuan-Yong Yan , Xiao-Dong Pan
发明人： Zengquan Qin , Yuan-Yong Yan , Xiao-Dong Pan
IPC分类号： C08L25/10 , C08F8/00 , C07C39/15 , C08F236/10
摘要： Vulcanizates with desirable properties can be obtained from compounds incorporating polymers that include hydroxyl group-containing diphenylethylene-type functionalities. The functionalities can be incorporated by using any or all of appropriate initiators, monomers and optional terminating compounds. Such polymers exhibit excellent interactivity with both conventional and non-conventional fillers.
摘要翻译： 具有所需性质的硫化剂可以从包含含羟基的二苯基乙烯型官能团的聚合物的化合物中获得。 可以通过使用任何或所有合适的引发剂，单体和任选的终止化合物来掺入官能团。 这些聚合物与常规和非常规填料都具有优异的相互作用。
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公开(公告)号：US20120059113A1
公开(公告)日：2012-03-08
申请号：US13207694
申请日：2011-08-11
申请人： Xiao-Dong Pan , Zengquan Qin , Yuan-Yong Yan , Jessica Kurasch
发明人： Xiao-Dong Pan , Zengquan Qin , Yuan-Yong Yan , Jessica Kurasch
摘要： Vulcanizates with desirable properties can be obtained from compositions incorporating polymers that include hydroxyl group-containing aryl functionalities, silica or other particulate filler(s) that contain or include oxides of silicon and a compound that includes multiple hydroxyl groups. The compound can act to disrupt the interactivity of the functionalities and the particulate filler particles during processing of the composition, thereby facilitating processing of the composition.
摘要翻译： 具有期望性质的硫化橡胶可以从包含含羟基芳基官能团的聚合物的组合物，二氧化硅或其中包含或包括硅的氧化物和包括多个羟基的化合物的其它颗粒填料获得。 该组合物可以在组合物加工期间起作用以破坏功能性和颗粒填料颗粒的相互作用，从而有助于组合物的加工。
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57.发明授权Enhancing interactivity between amine-functionalized polymers and particulate fillers 有权增强胺官能化聚合物和颗粒填料之间的交互性公开(公告)号：US07928159B2
公开(公告)日：2011-04-19
申请号：US11920669
申请日：2006-05-26
申请人： Yuan-Yong Yan
发明人： Yuan-Yong Yan
CPC分类号： C08C19/44 , C08J5/04 , C08J2321/00 , C08K3/013
摘要： A process for providing interaction between particulate filler and a functionalized polymer involves a composition that includes at least three components: (1) a polymer that includes a functional group including an acidic cation of a primary or secondary amine functionality, (2) a material including a functionality capable of reacting with the acidic cation, and (3) particulate filler. The amine functionality from (1) is allowed to interact with (3) after being neutralized by the action of the acid-reactive functionality from (2). The process is useful in the formation of vulcanizates and articles made therefrom.
摘要翻译： 提供颗粒填料与官能化聚合物之间的相互作用的方法涉及包含至少三种组分的组合物：（1）包含官能团的聚合物，其包括伯胺或仲胺官能团的酸性阳离子，（2）包括 能够与酸性阳离子反应的官能团，和（3）颗粒填料。 （2）的酸反应性官能团的作用被中和后，允许（1）的胺官能团与（3）相互作用。 该方法可用于形成由其制成的硫化橡胶和制品。
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公开(公告)号：US20100120976A1
公开(公告)日：2010-05-13
申请号：US11995947
申请日：2006-07-19
申请人： Yuan-Yong Yan
发明人： Yuan-Yong Yan
摘要： A functionalized polymer includes a polymer chain and, bonded thereto, an functional group having the general formula —NHAR1 where A is an oxygen atom, a sulfinyl (thionyl) group, a sulfonyl group, a quaternary phosphonium group, or a secondary amino group and where R1 is a hydrogen atom or a moiety of the general formula —CH2Z where Z is H or a substituted or unsubstituted aryl, alkyl, alkenyl, alkenaryl, aralkenyl, alkaryl, or aralkyl group. The material can be the reaction product of a living polymer and a compound that includes protected imine functionality. The functional group can interact with particulate filler such as, e.g., carbon black.
摘要翻译： 官能化聚合物包括聚合物链，并且键合有具有通式-NHAR 1的官能团，其中A是氧原子，亚磺酰基（亚硫酰基）基团，磺酰基基团，季鏻基团或仲氨基，和 其中R 1是氢原子或通式-CH 2 Z的部分，其中Z是H或取代或未取代的芳基，烷基，烯基，烯芳基，芳烯基，烷芳基或芳烷基。 该材料可以是活性聚合物和包含受保护的亚胺官能团的化合物的反应产物。 官能团可以与颗粒填料例如炭黑相互作用。
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公开(公告)号：US07335712B2
公开(公告)日：2008-02-26
申请号：US11111615
申请日：2005-04-21
IPC分类号： C08F4/44
摘要： This invention relates to siloxy-functionalized polymers having the silicon of the siloxy group directly bonded to the end of a polymer chain through one or more carbon atoms, processes of producing the polymers, and initiators used to prepare the polymers. The polymers may be rubbery polymers, such as butadiene-styrene polymers, which are commonly used in tires.
摘要翻译： 本发明涉及具有硅烷氧基的硅通过一个或多个碳原子直接键合到聚合物链末端的甲硅烷氧基官能化聚合物，制备聚合物的方法和用于制备聚合物的引发剂。 聚合物可以是通常用于轮胎中的橡胶状聚合物，例如丁二烯 - 苯乙烯聚合物。
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公开(公告)号：US20070078232A1
公开(公告)日：2007-04-05
申请号：US11542836
申请日：2006-10-04
申请人： Yuan-Yong Yan
发明人： Yuan-Yong Yan
IPC分类号： C08F8/30
CPC分类号： C08L9/06 , C08C19/22 , C08C19/25 , C08C19/44 , C08F2/06 , C08F4/08 , C08F8/30 , C08F8/32 , C08F8/42 , C08F212/08 , C08F236/06 , C08F236/10 , C08K3/013 , C08K3/0033 , C08L15/00
摘要： A macromolecule includes a functional group including imine functionality bonded to a polymer chain. Where desired, the functional group also can contain additional (e.g., amine and/or silane) functionality. The material can be provided by reacting a polymer including carbonyl functionality with a compound including a primary amino group. The functional group can interact with particulate filler such as, e.g., carbon black and silica.
摘要翻译： 大分子包括键合到聚合物链上的亚胺官能团的官能团。 如果需要，官能团还可以含有另外的（例如胺和/或硅烷）官能团。 可以通过使包括羰基官能团的聚合物与包含伯氨基的化合物反应来提供该材料。 官能团可以与颗粒填料例如炭黑和二氧化硅相互作用。
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