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    Catalyst for oxygenate synthesis and method for manufacturing same, device for manufacturing oxygenate, and method for manufacturing oxygenate
    1.
    发明授权
    Catalyst for oxygenate synthesis and method for manufacturing same, device for manufacturing oxygenate, and method for manufacturing oxygenate 有权
    含氧化合物合成催化剂及其制造方法，含氧化合物的制造装置以及含氧化合物的制造方法

    公开(公告)号：US09272267B2

    公开(公告)日：2016-03-01

    申请号：US14237427

    申请日：2012-08-22

    申请人： Toshihito Miyama

    发明人： Toshihito Miyama

    IPC分类号： B01J31/00 ,  B01J23/00 ,  B01J23/656 ,  C07C29/158 ,  C07C45/49 ,  B01J37/02 ,  B01J21/14

    CPC分类号： B01J23/6562 ,  B01J21/14 ,  B01J37/02 ,  B01J37/0207 ,  B01J37/0242 ,  C07C29/158 ,  C07C45/49 ,  Y02E50/18 ,  Y02P20/52 ,  C07C31/08 ,  C07C47/06

    摘要： The present invention relates to a catalyst for oxygenate synthesis for synthesizing an oxygenate from a mixed gas containing hydrogen and carbon monoxide, the catalyst for oxygenate synthesis containing: a component (A): rhodium, a component (B): manganese, a component (C): an alkali metal, and a component (D): a component (D1), component (D2) or component (D3), wherein the component (D1) is one or more substances selected from the group consisting of titanium, vanadium and chromium, the component (D2) is an element belonging to group 13 of the periodic table, and the component (D3) is one or more substances selected from the group consisting of magnesium and lanthanoids. According to the present invention, an oxygenate can be synthesized efficiently from a mixed gas containing hydrogen and carbon monoxide.

    摘要翻译： 本发明涉及一种用于从含氢和一氧化碳的混合气体中合成含氧化合物的含氧化合物催化剂，含氧合成催化剂含有：组分（A）：铑，组分（B）：锰，组分（ C）：碱金属和组分（D）：组分（D1），组分（D2）或组分（D3），其中组分（D1）是一种或多种选自钛，钒 和组分（D2）是属于周期表第13族的元素，组分（D3）是一种或多种选自镁和镧系元素的物质。 根据本发明，可以从含有氢和一氧化碳的混合气体中有效地合成含氧化合物。

    Proton conductive film, process for producing the same, and fuel cell employing the proton-conductive film
    3.
    发明申请
    Proton conductive film, process for producing the same, and fuel cell employing the proton-conductive film 审中-公开
    质子导电膜，其制造方法和使用质子传导膜的燃料电池

    公开(公告)号：US20060219981A1

    公开(公告)日：2006-10-05

    申请号：US10554222

    申请日：2004-04-23

    申请人： Toshihito Miyama ,  Toshiya Sugimoto ,  Shigeki Nomura

    发明人： Toshihito Miyama ,  Toshiya Sugimoto ,  Shigeki Nomura

    IPC分类号： H01B1/12

    CPC分类号： H01B1/122 ,  H01M8/0289 ,  H01M8/1037 ,  H01M8/1067 ,  H01M8/1074 ,  Y02P70/56

    摘要： It is intended to provide a proton conducting membrane which is excellent in heat resistance, dimensional stability, fuel barrier properties, flexibility, etc. and exhibits an excellent protonic conductivity even at high temperatures, a method of producing same and a fuel cell which can operate stably at high temperatures, the proton conducting membrane of the present invention comprises a support filled with a proton conducting structure (β) comprising an acid-containing structure containing an acid group, which support being made of an organic-inorganic composite structure (α) having a crosslinked structure formed by a metal-oxygen bond and an open-cell structure having internally-formed pores connected continuously to each other by the crosslinked structure, and the use of this proton conducting membrane makes it possible to obtain a fuel cell having an excellent performance.

    摘要翻译： 本发明提供一种耐热性，尺寸稳定性，燃料阻隔性，柔软性等优异的质子传导膜，即使在高温下也表现出优异的质子传导性，其制造方法和能够操作的燃料电池 稳定地在高温下，本发明的质子传导膜包括填充有质子传导结构（β）的载体，该质子传导结构（β）包含含有酸基团的含酸结构，其支持由有机 - 无机复合结构（α） 具有通过金属 - 氧键形成的交联结构和具有通过交联结构彼此连续连接的内部形成的孔的开孔结构，并且通过使用该质子传导膜，可以获得具有 出色表现。

    PROTON CONDUCTING MEMBRANE, MEMBRANE-ELECTRODE ASSEMBLY, AND POLYMER ELECTROLYTE FUEL CELL
    4.
    发明申请
    PROTON CONDUCTING MEMBRANE, MEMBRANE-ELECTRODE ASSEMBLY, AND POLYMER ELECTROLYTE FUEL CELL 审中-公开
    原子导电膜，膜电极组件和聚合物电解质燃料电池

    公开(公告)号：US20100119908A1

    公开(公告)日：2010-05-13

    申请号：US12529637

    申请日：2008-02-29

    申请人： Hideyasu Nakajima ,  Toshihito Miyama ,  Yoshiharu Konno ,  Masashi Kanoh

    发明人： Hideyasu Nakajima ,  Toshihito Miyama ,  Yoshiharu Konno ,  Masashi Kanoh

    IPC分类号： H01M8/10

    CPC分类号： C08F220/60 ,  C08F220/38 ,  C08F222/1006 ,  C08F222/385 ,  C08G77/28 ,  C08J5/2256 ,  C08J2383/04 ,  H01B1/122 ,  H01M8/1027 ,  H01M8/1037 ,  H01M2300/0082

    摘要： A proton conducting membrane, a membrane-electrode assembly, and a polymer electrolyte fuel cell, which can realize high impact resistance and high polar solvent resistance as well as high proton conductivity, at the same time, can improve adhesion to an electrode, and can improve power generation performance, are provided. A proton conducting membrane includes a silicon-oxygen bonding structure (A) containing a cross-linked structure formed by a silicon-oxygen bond, and an acid group-containing structure (B) covalently bonded to a silane compound and containing an acid group, which are coupled to each other by a silicon—oxygen bond, wherein the acid group-containing structure (B) includes a structure in which a silane compound (α) having a polymerizable unsaturated double bond and an acid group-containing compound (β) having an acid group and a polymerizable unsaturated double bond are covalently bonded to each other.

    摘要翻译： 能够同时实现高耐冲击性和高极性耐溶剂性以及高质子传导性的质子传导膜，膜 - 电极组件和聚合物电解质燃料电池可以提高对电极的粘附性，并且可以 提高发电性能。 质子传导膜包括含有由硅 - 氧键形成的交联结构的硅 - 氧键合结构（A）和与硅烷化合物共价键合并含有酸基的含酸基的结构（B） 它们通过硅 - 氧键彼此耦合，其中含酸基的结构（B）包括其中具有可聚合不饱和双键的硅烷化合物（α）和含酸基的化合物（＆bgr; ）具有酸基和可聚合不饱和双键共价键合。

    MEMBRANE-ELECTRODE JUNCTION AGENT, PROTON CONDUCTING MEMBRANE HAVING JUNCTION LAYER, MEMBRANE-ELECTRODE ASSEMBLY, POLYMER ELECTROLYTE FUEL CELL, AND MANUFACTURING METHOD OF THE MEMBRANE-ELECTRODE ASSEMBLY
    5.
    发明申请
    MEMBRANE-ELECTRODE JUNCTION AGENT, PROTON CONDUCTING MEMBRANE HAVING JUNCTION LAYER, MEMBRANE-ELECTRODE ASSEMBLY, POLYMER ELECTROLYTE FUEL CELL, AND MANUFACTURING METHOD OF THE MEMBRANE-ELECTRODE ASSEMBLY 有权
    膜电极接合剂，具有结层的导电膜，膜电极组件，聚合物电解质燃料电池和膜电极组件的制造方法

    公开(公告)号：US20100047659A1

    公开(公告)日：2010-02-25

    申请号：US12531242

    申请日：2008-03-12

    申请人： Toshihito Miyama ,  Yoshiharu Konno ,  Hideyasu Nakajima ,  Masashi Kanoh

    发明人： Toshihito Miyama ,  Yoshiharu Konno ,  Hideyasu Nakajima ,  Masashi Kanoh

    IPC分类号： H01M8/10 ,  B05D5/12

    CPC分类号： H01M8/0297 ,  H01M8/0258 ,  H01M8/1004 ,  H01M8/241 ,  Y02P70/56

    摘要： A membrane-electrode junction agent, a proton conducting membrane having a junction layer, a membrane-electrode assembly, a polymer electrolyte fuel cell, and a manufacturing method of the membrane-electrode assembly, which enhance the power generation performance, realize the high fuel barrier property, and are capable of enhancing the joint strength between the membrane and the electrodes, is provided. A membrane-electrode junction agent that joins a proton conducting membrane and electrodes arranged on both surfaces of the proton conducting membrane to each other, the membrane-electrode junction agent including: a cross-linked compound (X) having a silicon-oxygen bond; a polymer material (Y) containing an acid group; and a hydrophilic resin (Z) containing no acid group.

    摘要翻译： 膜 - 电极接合剂，具有接合层的质子传导膜，膜 - 电极组件，聚合物电解质燃料电池和增强发电性能的膜 - 电极组件的制造方法，实现高燃料 并且能够提高膜与电极之间的接合强度。 一种膜 - 电极接合剂，其将质子传导膜和布置在质子传导膜的两个表面上的电极彼此连接，所述膜 - 电极接合剂包括：具有硅 - 氧键的交联化合物（X）; 含有酸基的聚合物材料（Y） 和不含酸基的亲水性树脂（Z）。

    Proton conductive film, method for producing the same, and fuel cell using same
    6.
    发明申请
    Proton conductive film, method for producing the same, and fuel cell using same 有权
    质子导电膜，其制造方法和使用其的燃料电池

    公开(公告)号：US20060141313A1

    公开(公告)日：2006-06-29

    申请号：US10559082

    申请日：2004-06-10

    申请人： Shigeki Nomura ,  Toshihito Miyama

    发明人： Shigeki Nomura ,  Toshihito Miyama

    IPC分类号： H01M8/10 ,  C08J5/22

    CPC分类号： C08J5/2256 ,  C08J2383/04 ,  H01B1/122 ,  H01M8/1027 ,  H01M8/1037 ,  H01M8/1072 ,  H01M2300/0068 ,  Y02P70/56

    摘要： An object of the present invention is to solve the problems with conventional polymer electrolyte fuel cells and provide a proton conducting membrane which exhibits an excellent heat resistance and an excellent protonic conductivity and a high dimensional stability even at high temperatures, a method for producing the same and a fuel cell using the same. The proton conducting membrane of the present invention is a proton conducting membrane having particles 1 comprising a metal-oxygen crosslinked structure and the particles 1 have an acid group such as sulfonic acid group incorporated in the surface thereof and form a continuity. The gap 2 between the particles is communicated from the main surface to the opposite surface of the proton conducting membrane to form a proton conducting channel.

    摘要翻译： 本发明的目的是解决现有的高分子电解质燃料电池的问题，提供即使在高温下也显示优异的耐热性，优异的质子传导性和高尺寸稳定性的质子传导膜，其制造方法 和使用该燃料电池的燃料电池。 本发明的质子传导膜是具有包含金属 - 氧交联结构的颗粒1的质子传导膜，并且颗粒1具有结合在其表面中的酸基如磺酸基并形成连续性。 颗粒之间的间隙2从质子传导膜的主表面传递到相对表面，以形成质子传导通道。

    Proton conductive film, method for producing the same, and fuel cell using same
    7.
    发明授权
    Proton conductive film, method for producing the same, and fuel cell using same 有权
    质子导电膜，其制造方法和使用其的燃料电池

    公开(公告)号：US07829237B2

    公开(公告)日：2010-11-09

    申请号：US10559082

    申请日：2004-06-10

    申请人： Shigeki Nomura ,  Toshihito Miyama

    发明人： Shigeki Nomura ,  Toshihito Miyama

    IPC分类号： H01M6/14 ,  H01M6/18 ,  C08G77/22 ,  C08G77/60

    CPC分类号： C08J5/2256 ,  C08J2383/04 ,  H01B1/122 ,  H01M8/1027 ,  H01M8/1037 ,  H01M8/1072 ,  H01M2300/0068 ,  Y02P70/56

    摘要： An object of the present invention is to solve the problems with conventional polymer electrolyte fuel cells and provide a proton conducting membrane which exhibits an excellent heat resistance and an excellent protonic conductivity and a high dimensional stability even at high temperatures, a method for producing the same and a fuel cell using the same.The proton conducting membrane of the present invention is a proton conducting membrane having particles 1 comprising a metal-oxygen crosslinked structure and the particles 1 have an acid group such as sulfonic acid group incorporated in the surface thereof and form a continuity. The gap 2 between the particles is communicated from the main surface to the opposite surface of the proton conducting membrane to form a proton conducting channel.

    摘要翻译： 本发明的目的是解决现有的高分子电解质燃料电池的问题，提供即使在高温下也显示优异的耐热性，优异的质子传导性和高尺寸稳定性的质子传导膜，其制造方法 和使用该燃料电池的燃料电池。 本发明的质子传导膜是具有包含金属 - 氧交联结构的颗粒1的质子传导膜，并且颗粒1具有结合在其表面中的酸基如磺酸基并形成连续性。 颗粒之间的间隙2从质子传导膜的主表面传递到相对表面，以形成质子传导通道。

    CATALYST FOR OXYGENATE SYNTHESIS AND METHOD FOR MANUFACTURING SAME, DEVICE FOR MANUFACTURING OXYGENATE, AND METHOD FOR MANUFACTURING OXYGENATE
    8.
    发明申请
    CATALYST FOR OXYGENATE SYNTHESIS AND METHOD FOR MANUFACTURING SAME, DEVICE FOR MANUFACTURING OXYGENATE, AND METHOD FOR MANUFACTURING OXYGENATE 有权
    用于氧化合成的催化剂及其制造方法，用于制造氧化剂的装置以及制造氧化剂的方法

    公开(公告)号：US20140187654A1

    公开(公告)日：2014-07-03

    申请号：US14237427

    申请日：2012-08-22

    申请人： Toshihito Miyama

    发明人： Toshihito Miyama

    IPC分类号： B01J23/656 ,  C07C29/158

    CPC分类号： B01J23/6562 ,  B01J21/14 ,  B01J37/02 ,  B01J37/0207 ,  B01J37/0242 ,  C07C29/158 ,  C07C45/49 ,  Y02E50/18 ,  Y02P20/52 ,  C07C31/08 ,  C07C47/06

    摘要： The present invention relates to a catalyst for oxygenate synthesis for synthesizing an oxygenate from a mixed gas containing hydrogen and carbon monoxide, the catalyst for oxygenate synthesis containing: a component (A): rhodium, a component (B): manganese, a component (C): an alkali metal, and a component (D): a component (D1), component (D2) or component (D3), wherein the component (D1) is one or more substances selected from the group consisting of titanium, vanadium and chromium, the component (D2) is an element belonging to group 13 of the periodic table, and the component (D3) is one or more substances selected from the group consisting of magnesium and lanthanoids. According to the present invention, an oxygenate can be synthesized efficiently from a mixed gas containing hydrogen and carbon monoxide.

    摘要翻译： 本发明涉及一种用于从含氢和一氧化碳的混合气合成含氧化合物的含氧化合物催化剂，含氧合成催化剂含有：组分（A）：铑，组分（B）：锰，组分（ C）：碱金属和组分（D）：组分（D1），组分（D2）或组分（D3），其中组分（D1）是一种或多种选自钛，钒 和组分（D2）是属于周期表第13族的元素，组分（D3）是一种或多种选自镁和镧系元素的物质。 根据本发明，可以从含有氢和一氧化碳的混合气体中有效地合成含氧化合物。