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公开(公告)号：US4547437A
公开(公告)日：1985-10-15
申请号：US657923
申请日：1984-10-05
CPC分类号： H01M8/12
摘要： A high temperature, solid electrolyte electrochemical cell is made, having a first and second electrode with solid electrolyte between them, where the electrolyte is formed by hot chemical vapor deposition, where a solid, interlayer material, which is electrically conductive, oxygen permeable, and protective of electrode material from hot metal halide vapor attack, is placed between the first electrode and the electrolyte, to protect the first electrode from the hot metal halide vapors during vapor deposition.
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公开(公告)号：US4609562A
公开(公告)日：1986-09-02
申请号：US684438
申请日：1984-12-20
CPC分类号： C23C16/455 , C04B41/5025 , C23C16/405 , C23C16/52 , H01M8/1253 , Y02E60/525 , Y02P70/56
摘要： Disclosed is an apparatus for forming a chemically vapor deposited coating on a porous substrate where oxygen from a first gaseous reactant containing a source of oxygen permeates through the pores of the substrate to react with a second gaseous reactant that is present on the other side of the substrate. The apparatus includes means for controlling the pressure and flow rate of each gaseous reactant, a manometer for measuring the difference in pressure between the gaseous reactants on each side of the substrate, and means for changing the difference in pressure between the gaseous reactants. Also disclosed is a method of detecting and closing cracks in the coating by reducing the pressure difference between the two gaseous reactants whenever the pressure difference falls suddenly after gradually rising, then again increasing the pressure difference on the two gases. The attack by the by-products of the reaction on the substrate are reduced by maintaining the flow rate of the first reactant through the pores of the substrate.
摘要翻译： 公开了一种用于在多孔基材上形成化学气相沉积涂层的装置，其中来自含有氧源的第一气态反应物的氧气渗透通过基底的孔与第二气态反应物反应，第二气态反应物存在于 基质。 该装置包括用于控制每种气体反应物的压力和流速的装置，用于测量基板每侧的气态反应物之间的压力差的压力计和用于改变气态反应物之间的压力差的装置。 还公开了每当压差在逐渐升高之后突然下降时，通过减小两种气体反应物之间的压差来检测和闭合涂层中的裂纹，然后再次增加两种气体上的压力差的方法。 通过保持第一反应物通过基底的孔的流速来降低反应副产物对基材的侵蚀。
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公开(公告)号：US4582766A
公开(公告)日：1986-04-15
申请号：US716864
申请日：1985-03-28
CPC分类号： H01M8/12 , C25B11/035 , C25B11/0405
摘要： Disclosed is a method of increasing the operating cell voltage of a solid oxide electrochemical cell having metal electrode particles in contact with an oxygen-transporting ceramic electrolyte. The metal electrode is heated with the cell, and oxygen is passed through the oxygen-transporting ceramic electrolyte to the surface of the metal electrode particles so that the metal electrode particles are oxidized to form a metal oxide layer between the metal electrode particles and the electrolyte. The metal oxide layer is then reduced to form porous metal between the metal electrode particles and the ceramic electrolyte.
摘要翻译： 公开了一种增加具有与氧输送陶瓷电解质接触的金属电极颗粒的固体氧化物电化学电池的工作电池电压的方法。 金属电极与电池一起加热，氧气通过氧传输陶瓷电解质到金属电极颗粒的表面，使得金属电极颗粒被氧化以在金属电极颗粒和电解质之间形成金属氧化物层 。 然后将金属氧化物层还原以在金属电极颗粒和陶瓷电解质之间形成多孔金属。
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4.发明授权Applying a tapered electrode on a porous ceramic support tube by masking a band inside the tube and drawing in electrode material from the outside of the tube by suction 失效通过掩蔽管内的带并通过吸力从管外吸引电极材料，将多个陶瓷支撑管上的锥形电极施加
公开(公告)号：US5073405A
公开(公告)日：1991-12-17
申请号：US641390
申请日：1991-01-15
IPC分类号： B05C3/20 , C04B41/50 , C04B41/87 , C04B41/88 , C25D17/12 , G01N27/407 , H01M4/86 , H01M4/88 , H01M8/12
CPC分类号： G01N27/4075 , B05C3/20 , C04B41/5025 , C04B41/87 , H01M4/8621 , H01M4/8846 , H01M4/8885 , H01M4/9016 , H01M8/1213 , H01M8/1226 , H01M2004/8684 , H01M2008/1293 , H01M2300/0071 , H01M2300/0074 , H01M4/9025 , H01M4/9033
摘要： An electrode is deposited on a support by providing a porous ceramic support tube (10) having an open end (14) and closed end (16); masking at least one circumferential interior band (18 and 18') inside the tube; evacuating air from the tube by an evacuation system (30), to provide a permeability gradient between the masked part (18 and 18') and unmasked part (20) of the tube; applying a liquid dispersion of solid electrode particles to the outside surface of the support tube, where liquid flows through the wall, forming a uniform coating (42) over the unmasked support part (20) and a tapered coating over the masked part (18 and 18').
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5.发明申请公开(公告)号：US20110318658A1
公开(公告)日：2011-12-29
申请号：US13069893
申请日：2011-03-23
申请人： Owen S. Taylor , Gregory E. Zymboly
发明人： Owen S. Taylor , Gregory E. Zymboly
CPC分类号： H01M8/12 , H01M8/0625 , H01M8/243 , H01M8/2457 , H01M8/247 , H01M8/2485 , Y02P70/56 , Y10T29/49108
摘要： A multi-function bundle having all of the basic support functions integrated therein can be used as a basic building block component, for example, in a fuel cell engine. The multi-function bundle is modular, easy to assemble, and able to withstand the physical and thermal shocks encountered in mobile applications. The multi-function bundle utilizes fully distributed fuel and oxidant supply systems which help to reduce temperature gradients throughout the array of fuel cells. The multi-function bundle may be comprised of a plurality of fuel cells, an oxidant supply system, a fuel supply system and a support structure which integrates the fuel cells, oxidant supply system, and fuel supply system into a single unit. The oxidant and fuel supply systems may be fully distributed. The fuel supply system may include one or more fuel feed tube assemblies which allow distributed internal fuel reformation and reduce temperature gradients throughout the array of fuel cells.
摘要翻译： 具有集成在其中的所有基本支撑功能的多功能束可用作例如燃料电池发动机中的基本构件部件。 多功能组合模块化，易于组装，并能够承受移动应用中遇到的物理和热冲击。 多功能组合使用完全分布的燃料和氧化剂供应系统，有助于降低整个燃料电池阵列的温度梯度。 多功能束可以由多个燃料电池，氧化剂供应系统，燃料供应系统和将燃料电池，氧化剂供应系统和燃料供应系统集成到单个单元中的支撑结构构成。 氧化剂和燃料供应系统可以是完全分配的。 燃料供应系统可以包括一个或多个燃料供给管组件，其允许分布式内部燃料重整并且降低整个燃料电池阵列的温度梯度。
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6.发明申请公开(公告)号：US20080233441A1
公开(公告)日：2008-09-25
申请号：US12075909
申请日：2008-03-14
申请人： Owen S. Taylor , Gregory E. Zymboly
发明人： Owen S. Taylor , Gregory E. Zymboly
CPC分类号： H01M8/12 , H01M8/0625 , H01M8/243 , H01M8/2457 , H01M8/247 , H01M8/2485 , Y02P70/56 , Y10T29/49108
摘要： A multi-function bundle having all of the basic support functions integrated therein can be used as a basic building block component, for example, in a fuel cell engine. The multi-function bundle is modular, easy to assemble, and able to withstand the physical and thermal shocks encountered in mobile applications. The multi-function bundle utilizes fully distributed fuel and oxidant supply systems which help to reduce temperature gradients throughout the array of fuel cells. The multi-function bundle may be comprised of a plurality of fuel cells, an oxidant supply system, a fuel supply system and a support structure which integrates the fuel cells, oxidant supply system, and fuel supply system into a single unit. The oxidant and fuel supply systems may be fully distributed. The fuel supply system may include one or more fuel feed tube assemblies which allow distributed internal fuel reformation and reduce temperature gradients throughout the array of fuel cells.
摘要翻译： 具有集成在其中的所有基本支撑功能的多功能束可用作例如燃料电池发动机中的基本构件部件。 多功能组合模块化，易于组装，并能够承受移动应用中遇到的物理和热冲击。 多功能组合使用完全分布的燃料和氧化剂供应系统，有助于降低整个燃料电池阵列的温度梯度。 多功能束可以由多个燃料电池，氧化剂供应系统，燃料供应系统和将燃料电池，氧化剂供应系统和燃料供应系统集成到单个单元中的支撑结构构成。 氧化剂和燃料供应系统可以是完全分配的。 燃料供应系统可以包括一个或多个燃料供给管组件，其允许分布式内部燃料重整并且降低整个燃料电池阵列的温度梯度。
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7.发明授权
公开(公告)号：US5244752A
公开(公告)日：1993-09-14
申请号：US802788
申请日：1991-12-06
申请人： Gregory E. Zymboly
发明人： Gregory E. Zymboly
CPC分类号： H01M8/243 , H01M8/1231
摘要： A generator apparatus (10) is made containing long, hollow, tubular, fuel cells containing an inner air electrode (64), an outer fuel electrode (56), and solid electrolyte (54) therebetween, placed between a fuel distribution board (29) and a board (32) which separates the combustion chamber (16) from the generating chamber (14), where each fuel cell has an insertable open end and in insertable, plugged, closed end (44), the plugged end being inserted into the fuel distribution board (29) and the open end being inserted through the separator board (32) where the plug (60) is completely within the fuel distribution board (29).
摘要翻译： 一种发电机装置（10），其包含长，中空，管状的燃料电池，其包含内部空气电极（64），外部燃料电极（56）和其间的固体电解质（54），放置在燃料分配板（29） ）和将所述燃烧室（16）与所述发生室（14）分离的板（32），其中每个燃料电池具有可插入的开口端和可插入的，封闭的封闭端（44），所述插入端插入 燃料分配板（29）和开口端插入通过分离器板（32），其中插头（60）完全在燃料分配板（29）内。
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8.发明授权High bulk self-supporting electrode with integral gas feed conduit for solid oxide fuel cells 失效用于固体氧化物燃料电池的具有整体气体供给管道的大体积自支撑电极
公开(公告)号：US4751152A
公开(公告)日：1988-06-14
申请号：US34454
申请日：1987-04-06
申请人： Gregory E. Zymboly
发明人： Gregory E. Zymboly
CPC分类号： H01M4/8626 , H01M8/1231 , H01M8/243 , H01M2008/1293 , H01M2300/0074
摘要： A porous, self-supporting, elongated electrode is made, having a closed end, an inner wall defining a gas feed conduit, and at least one other gas exit conduit within the structure, where the conduits communicate with each other near the closed end of the structure.
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公开(公告)号：US07364812B2
公开(公告)日：2008-04-29
申请号：US10804925
申请日：2004-03-19
申请人： Owen S. Taylor , Gregory E. Zymboly
发明人： Owen S. Taylor , Gregory E. Zymboly
CPC分类号： H01M8/12 , H01M8/0625 , H01M8/243 , H01M8/2457 , H01M8/247 , H01M8/2485 , Y02P70/56 , Y10T29/49108
摘要： A multi-function bundle having all of the basic support functions integrated therein can be used as a basic building block component, for example, in a fuel cell engine. The multi-function bundle is modular, easy to assemble, and able to withstand the physical and thermal shocks encountered in mobile applications. The multi-function bundle utilizes fully distributed fuel and oxidant supply systems which help to reduce temperature gradients throughout the array of fuel cells. The multi-function bundle may be comprised of a plurality of fuel cells, an oxidant supply system, a fuel supply system and a support structure which integrates the fuel cells, oxidant supply system, and fuel supply system into a single unit. The oxidant and fuel supply systems may be fully distributed. The fuel supply system may include one or more fuel feed tube assemblies which allow distributed internal fuel reformation and reduce temperature gradients throughout the array of fuel cells.
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公开(公告)号：US5273838A
公开(公告)日：1993-12-28
申请号：US957114
申请日：1992-10-07
申请人： Robert Draper , Gregory E. Zymboly
发明人： Robert Draper , Gregory E. Zymboly
CPC分类号： H01M8/243 , H01M8/0202
摘要： A fuel cell array (10) is made, containing number of tubular, elongated fuel cells (12) which are placed next to each other in rows (A, B, C, D), where each cell contains inner electrodes (14) and outer electrodes (18 and 18'), with solid electrolyte (16 and 16') between the electrodes, where the electrolyte and outer electrode are discontinuous, having two portions, and providing at least two opposed discontinuities which contain at least two oppositely opposed interconnections (20 and 20') contacting the inner electrode (14), each cell (12) having only three metallic felt electrical connectors (22) which contact surrounding cells, where each row is electrically connected to the other.
摘要翻译： 制造燃料电池阵列（10），其包含多个以行（A，B，C，D）彼此相邻放置的管状细长燃料电池（12），其中每个电池包含内电极（14）和 在电极之间具有固体电解质（16和16'）的外部电极（18和18'），其中电解质和外部电极是不连续的，具有两部分，并提供至少两个相对的不连续性，其包含至少两个相对相对的互连 （20和20'）接触内电极（14），每个电池（12）仅具有接触周围电池的三个金属毡电连接器（22），其中每排电连接到另一电极。
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