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    Tire tread compound
    1.
    发明授权
    Tire tread compound 失效
    轮胎胎面复合物

    公开(公告)号：US5859133A

    公开(公告)日：1999-01-12

    申请号：US617234

    申请日：1996-03-18

    申请人： David John Zanzig ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  Paul Harry Sandstrom ,  Laurie Elizabeth Austin

    发明人： David John Zanzig ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  Paul Harry Sandstrom ,  Laurie Elizabeth Austin

    IPC分类号： B60C1/00 ,  C08L9/00 ,  C08L21/00 ,  C08L53/00 ,  C08L53/02 ,  C08F236/08 ,  C08F236/06

    CPC分类号： C08L21/00 ,  B60C1/0016 ,  C08F297/04 ,  C08L53/00 ,  C08L9/00 ,  C08L9/06

    摘要： The subject invention discloses a pneumatic tire having an outer circumferential tread wherein said tread is a sulfur-cured rubber composition comprised of (a) an isoprene-butadiene diblock rubber, said isoprene-butadiene diblock rubber being comprised of a butadiene block and an isoprene-butadiene block, wherein said butadiene block has a number average molecular weight which is within the range of about 25,000 to about 350,000, wherein said isoprene-butadiene block has a number average molecular weight which is within the range of about 25,000 to about 350,000, wherein said isoprene-butadiene diblock rubber has essentially one glass transition temperature which is within the range of about -100.degree. C. to about -70.degree. C., wherein said isoprene-butadiene diblock polymer has a Mooney ML-4 viscosity at 100.degree. C. which is within the range of about 50 to about 140, and wherein the repeat units derived from isoprene and 1,3-butadiene in the isoprene-butadiene block are in essentially random order; and (b) a second rubber selected from the group consisting of high vinyl polybutadiene rubber, styrene-isoprene-butadiene rubber, solution styrene-butadiene rubber and emulsion styrene-butadiene rubber.

    摘要翻译： 本发明公开了一种具有外周胎面的充气轮胎，其中所述胎面是由（a）异戊二烯 - 丁二烯二嵌段橡胶组成的硫固化橡胶组合物，所述异戊二烯 - 丁二烯二嵌段橡胶由丁二烯嵌段和异戊二烯 - 丁二烯嵌段，其中所述丁二烯嵌段的数均分子量在约25,000至约350,000的范围内，其中所述异戊二烯 - 丁二烯嵌段的数均分子量在约25,000至约350,000的范围内，其中 所述异戊二烯 - 丁二烯二嵌段橡胶具有在约-100℃至约-70℃范围内的基本上一个玻璃化转变温度，其中所述异戊二烯 - 丁二烯二嵌段聚合物在100℃下具有门尼ML-4粘度 ，其在约50至约140的范围内，并且其中衍生自异戊二烯和1,3-丁二烯的异戊二烯 - 丁二烯嵌段中的重复单元基本上为兰德 呃订单 和（b）选自高乙烯基聚丁二烯橡胶，苯乙烯 - 异戊二烯 - 丁二烯橡胶，溶剂苯乙烯 - 丁二烯橡胶和乳液丁苯橡胶的第二橡胶。

    Tire tread compound
    2.
    发明授权
    Tire tread compound 失效
    轮胎胎面复合

    公开(公告)号：US5686530A

    公开(公告)日：1997-11-11

    申请号：US782841

    申请日：1997-01-13

    申请人： Adel Farhan Halasa ,  David John Zanzig ,  Wen-Liang Hsu ,  Paul Harry Sandstrom ,  Laurie Elizabeth Austin

    发明人： Adel Farhan Halasa ,  David John Zanzig ,  Wen-Liang Hsu ,  Paul Harry Sandstrom ,  Laurie Elizabeth Austin

    IPC分类号： B60C1/00 ,  C08L9/00 ,  C08L21/00 ,  C08L53/00 ,  C08L53/02 ,  C08L52/03 ,  C08F297/04

    CPC分类号： C08L21/00 ,  B60C1/0016 ,  C08F297/04 ,  C08L53/00 ,  C08L9/00 ,  C08L9/06

    摘要： The subject invention discloses a pneumatic tire having an outer circumferential tread wherein said tread is a sulfur-cured rubber composition comprised of (a) an isoprene-butadiene diblock rubber, said isoprene-butadiene diblock rubber being comprised of a butadiene block and an isoprene-butadiene block, wherein said butadiene block has a number average molecular weight which is within the range of about 25,000 to about 350,000, wherein said isoprene-butadiene block has a number average molecular weight which is within the range of about 25,000 to about 350,000, wherein said isoprene-butadiene diblock rubber has essentially one glass transition temperature which is within the range of about -100.degree. C. to about -70.degree. C., wherein said isoprene-butadiene diblock polymer has a Mooney ML-4 viscosity at 100.degree. C. which is within the range of about 50 to about 140, wherein the repeat units derived from isoprene and 1,3-butadiene in the isoprene-butadiene block are in essentially random order, and wherein said isoprene-butadiene diblock polymer does not contain any blocks which are derived solely from isoprene; and (b) a second rubber selected from the group consisting of high vinyl polybutadiene rubber, styrene-isoprene-butadiene rubber, solution styrene-butadiene rubber and emulsion styrene-butadiene rubber.

    摘要翻译： 本发明公开了一种具有外周胎面的充气轮胎，其中所述胎面是由（a）异戊二烯 - 丁二烯二嵌段橡胶组成的硫固化橡胶组合物，所述异戊二烯 - 丁二烯二嵌段橡胶由丁二烯嵌段和异戊二烯 - 丁二烯嵌段，其中所述丁二烯嵌段的数均分子量在约25,000至约350,000的范围内，其中所述异戊二烯 - 丁二烯嵌段的数均分子量在约25,000至约350,000的范围内，其中 所述异戊二烯 - 丁二烯二嵌段橡胶具有基本上一个玻璃化转变温度，其在约-100℃至约-70℃的范围内，其中所述异戊二烯 - 丁二烯二嵌段聚合物在100℃下具有门尼ML-4粘度 其在约50至约140的范围内，其中衍生自异戊二烯和1,3-丁二烯在异戊二烯 - 丁二烯嵌段中的重复单元基本上是随机的 并且其中所述异戊二烯 - 丁二烯二嵌段聚合物不包含仅由异戊二烯衍生的任何嵌段; 和（b）选自高乙烯基聚丁二烯橡胶，苯乙烯 - 异戊二烯 - 丁二烯橡胶，溶剂苯乙烯 - 丁二烯橡胶和乳液丁苯橡胶的第二橡胶。

    Tire tread compositions containing asymmetrically tin-coupled polybutadiene rubber and silica coupling agent
    3.
    发明授权
    Tire tread compositions containing asymmetrically tin-coupled polybutadiene rubber and silica coupling agent 失效
    含有不对称锡偶联聚丁二烯橡胶和二氧化硅偶联剂的轮胎胎面组合物

    公开(公告)号：US6017988A

    公开(公告)日：2000-01-25

    申请号：US366236

    申请日：1999-08-03

    申请人： Edward John Blok ,  Paul Harry Sandstrom ,  Cheryl Ann Losey ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  David John Zanzig ,  John Joseph Andre Verthe

    发明人： Edward John Blok ,  Paul Harry Sandstrom ,  Cheryl Ann Losey ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  David John Zanzig ,  John Joseph Andre Verthe

    IPC分类号： B60C1/00 ,  C08C19/44 ,  C08J3/26 ,  C08K5/548 ,  C08L7/00 ,  C08L9/00 ,  C08L15/00 ,  C08L21/00 ,  C08K3/04 ,  C08K3/36

    CPC分类号： C08L15/00 ,  B60C1/0016 ,  C08C19/44 ,  C08K5/548 ,  C08L15/005 ,  C08L21/00 ,  C08L7/00 ,  C08L9/00

    摘要： This invention relates to a tire tread compound that is easily processable which can be used to improve the treadwear, rolling resistance and traction characteristics of tires. The tire tread compounds of this invention are a blend of tin-coupled polybutadiene, high vinyl polybutadiene and natural rubber. This blend of low glass transition temperature rubber and high glass transition temperature rubber is surprisingly easy to process which makes the concept of this invention commercially feasible. Thus, the tire tread compounds of this invention can be utilized in making tires having greatly improved traction characteristics and treadwear without sacrificing rolling resistance. These improved properties may be due, in part, to better interaction and compatibility with carbon black and/or silica fillers. The polybutadiene in the blend can be asymmetrical tin-coupled to further improve the cold flow characteristics of the rubber blend. Asymmetrical tin coupling in general also leads to better processability and other beneficial properties. This invention more specifically discloses a tire tread rubber composition which is comprised of (1) from about 20 phr to about 60 phr of tin-coupled polybutadiene rubber, (2) from about 20 phr to about 60 phr of a rubber selected from the group consisting of natural rubber and synthetic polyisoprene and (3) from about 5 phr to about 40 phr of high vinyl polybutadiene rubber.

    摘要翻译： 本发明涉及一种易于加工的轮胎胎面胶，其可用于改善轮胎的胎面磨损，滚动阻力和牵引特性。 本发明的轮胎胎面胶料是锡偶合的聚丁二烯，高乙烯基聚丁二烯和天然橡胶的混合物。 这种低玻璃化转变温度橡胶和高玻璃化转变温度橡胶的混合物令人惊奇地易于加工，这使得本发明的概念在商业上可行。 因此，本发明的轮胎胎面胶料可用于制造具有极大改善的牵引特性和胎面磨损的轮胎，而不会牺牲滚动阻力。 这些改进的性质可能部分是由于与炭黑和/或二氧化硅填料的更好的相互作用和相容性。 共混物中的聚丁二烯可以是不对称的锡偶联，以进一步改善橡胶共混物的冷流特性。 不对称锡偶联一般也会导致更好的加工性能和其他有益的性能。 本发明更具体地公开了一种轮胎胎面橡胶组合物，其包含（1）约20phr至约60phr的锡偶联的聚丁二烯橡胶，（2）约20phr至约60phr的选自下组的橡胶： 由天然橡胶和合成聚异戊二烯组成，（3）约5phr至约40phr的高乙烯基聚丁二烯橡胶。

    Tire tread compositions containing asymmetrically tin-coupled polybutadiene rubber
    4.
    发明授权
    Tire tread compositions containing asymmetrically tin-coupled polybutadiene rubber 失效
    含有不对称锡偶联聚丁二烯橡胶的轮胎胎面组合物

    公开(公告)号：US6084022A

    公开(公告)日：2000-07-04

    申请号：US935172

    申请日：1997-09-22

    申请人： Edward John Blok ,  Paul Harry Sandstrom ,  Cheryl Ann Losey ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  David John Zanzig ,  John Joseph Andre Verthe

    发明人： Edward John Blok ,  Paul Harry Sandstrom ,  Cheryl Ann Losey ,  Adel Farhan Halasa ,  Wen-Liang Hsu ,  David John Zanzig ,  John Joseph Andre Verthe

    IPC分类号： B60C1/00 ,  C08C19/44 ,  C08J3/26 ,  C08K5/548 ,  C08L7/00 ,  C08L9/00 ,  C08L15/00 ,  C08L21/00 ,  C08K3/36

    CPC分类号： C08L15/00 ,  B60C1/0016 ,  C08C19/44 ,  C08K5/548 ,  C08L15/005 ,  C08L21/00 ,  C08L7/00 ,  C08L9/00

    摘要： This invention relates to a tire tread compound that is easily processable which can be used to improve the treadwear, rolling resistance and traction characteristics of tires. The tire tread compounds of this invention are a blend of tin-coupled polybutadiene, high vinyl polybutadiene and natural rubber. This blend of low glass transition temperature rubber and high glass transition temperature rubber is surprisingly easy to process which makes the concept of this invention commercially feasible. Thus, the tire tread compounds of this invention can be utilized in making tires having greatly improved traction characteristics and treadwear without sacrificing rolling resistance. These improved properties may be due, in part, to better interaction and compatibility with carbon black and/or silica fillers. The polybutadiene in the blend can be asymmetrical tin-coupled to further improve the cold flow characteristics of the rubber blend. Asymmetrical tin coupling in general also leads to better processability and other beneficial properties. This invention more specifically discloses a tire tread rubber composition which is comprised of (1) from about 20 phr to about 60 phr of tin-coupled polybutadiene rubber, (2) from about 20 phr to about 60 phr of a rubber selected from the group consisting of natural rubber and synthetic polyisoprene and (3) from about 5 phr to about 40 phr of high vinyl polybutadiene rubber.

    摘要翻译： 本发明涉及一种易于加工的轮胎胎面胶，其可用于改善轮胎的胎面磨损，滚动阻力和牵引特性。 本发明的轮胎胎面胶料是锡偶合的聚丁二烯，高乙烯基聚丁二烯和天然橡胶的混合物。 这种低玻璃化转变温度橡胶和高玻璃化转变温度橡胶的混合物令人惊奇地易于加工，这使得本发明的概念在商业上可行。 因此，本发明的轮胎胎面胶料可用于制造具有极大改善的牵引特性和胎面磨损的轮胎，而不会牺牲滚动阻力。 这些改进的性质可能部分是由于与炭黑和/或二氧化硅填料的更好的相互作用和相容性。 共混物中的聚丁二烯可以是不对称的锡偶联，以进一步改善橡胶共混物的冷流特性。 不对称锡偶联一般也会导致更好的加工性能和其他有益的性能。 本发明更具体地公开了一种轮胎胎面橡胶组合物，其包含（1）约20phr至约60phr的锡偶联的聚丁二烯橡胶，（2）约20phr至约60phr的选自下组的橡胶： 由天然橡胶和合成聚异戊二烯组成，（3）约5phr至约40phr的高乙烯基聚丁二烯橡胶。

    Catalyst system for synthesizing amine functionalized rubbery polymers having a high trans microstructure
    7.
    发明授权
    Catalyst system for synthesizing amine functionalized rubbery polymers having a high trans microstructure 有权
    用于合成具有高反向显微组织的胺官能化橡胶状聚合物的催化剂体系

    公开(公告)号：US07943712B2

    公开(公告)日：2011-05-17

    申请号：US11617361

    申请日：2006-12-28

    申请人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Laurie Elizabeth Austin ,  Chad Aaron Jasiunas ,  Steven Kristofer Henning

    发明人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Laurie Elizabeth Austin ,  Chad Aaron Jasiunas ,  Steven Kristofer Henning

    IPC分类号： C08F4/50 ,  C08F2/06 ,  C07F7/08

    CPC分类号： C08F36/04 ,  C08F4/48 ,  C08F4/54

    摘要： The present invention is directed to a catalyst system for synthesizing rubbery polymers, such as polybutadiene rubber, styrene-butadiene rubber, isoprene-butadiene rubber, or styrene-isoprene-butadiene rubber, that are amine functionalized and have a high trans microstructure. The catalyst system, in one embodiment, includes (a) an organolithium amine compound, (b) a group IIa metal salt of an amino glycol or a glycol ether, (c) an organoaluminum compound, and optionally (d) an amine compound. The amine functionalized rubbery polymers can be utilized in tire tread rubbers where the rubbery polymers may provide desirable wear properties without substantially sacrificing other performance characteristic(s), e.g., traction properties.

    摘要翻译： 本发明涉及一种用于合成胺官能化并具有高反相微观结构的橡胶状聚合物如聚丁二烯橡胶，苯乙烯 - 丁二烯橡胶，异戊二烯 - 丁二烯橡胶或苯乙烯 - 异戊二烯 - 丁二烯橡胶的催化剂体系。 在一个实施方案中，催化剂体系包括（a）有机锂胺化合物，（b）氨基二醇或二醇醚的IIa族金属盐，（c）有机铝化合物和任选的（d）胺化合物。 胺官能化橡胶状聚合物可用于轮胎胎面橡胶中，其中橡胶状聚合物可提供期望的耐磨性，而基本上不会牺牲其它性能特征，例如牵引性能。

    Catalyst for synthesizing high trans polymers
    8.
    发明授权
    Catalyst for synthesizing high trans polymers 失效
    用于合成高反式聚合物的催化剂

    公开(公告)号：US07189792B2

    公开(公告)日：2007-03-13

    申请号：US11311495

    申请日：2005-12-19

    申请人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Chad Aaron Jasiunas ,  Laurie Elizabeth Austin

    发明人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Chad Aaron Jasiunas ,  Laurie Elizabeth Austin

    IPC分类号： C08F4/50 ,  C08F36/06

    CPC分类号： C08F36/06 ,  C08F4/484 ,  C08F4/52 ,  C08F4/48 ,  C08F4/50

    摘要： The process and catalyst of this invention can be utilized to synthesize homo and copolymers of conjugated diene monomers and vinyl aromatic monomers having high trans contents of greater than 60% with low melting points. These homo and copolymers of conjugated diene monomers and vinyl aromatic monomers can be utilized in tire tread and sidewall rubbers that exhibit outstanding wear and tear characteristics in the tread and excellent flexing properties in the sidewall. The rubber polymers of this invention are made utilizing an improved catalyst system. This catalyst system is comprised of (a) organo aluminum compounds, (b) organo lithium compounds, (c) a barium compound selected from barium salts of (i) di(ethylene glycol) ethyl ether, (ii) di(ethylene glycol) propyl ether, (iii) di(ethylene glycol) hexyl ether, (iv) di(N,N-dimethyl amino glycol) ethyl ether, (v) menthol and thymol in the presence of polar modifier consisting of water, alcohols, amines, thiols, phosphates and phosphites. The trans polymers and copolymers of this invention made with the above catalyst system typically have a glass transition temperature ranging from −97° C. to −40° C., a melt temperature ranging from −30° C. to +30° C., and a number average molecular weight from 20,000 to 250,000. The inclusion of such polar modifiers in the barium catalyst system results in a high styrene content in copolymerization, a high trans content, and high molecular weight. Copolymers of conjugated diolefin monomers and vinyl aromatic monomers made with the catalyst system of this invention also have a tapered macrostructure.

    摘要翻译： 本发明的方法和催化剂可用于合成共轭二烯单体和具有高反式含量大于60％的低熔点的乙烯基芳族单体的均聚物和共聚物。 共轭二烯单体和乙烯基芳族单体的这些均聚物和共聚物可以用于轮胎胎面和侧壁橡胶，其在胎面中表现出优异的耐磨性和优异的弯曲性能。 使用改进的催化剂体系制备本发明的橡胶聚合物。 该催化剂体系包括（a）有机铝化合物，（b）有机锂化合物，（c）选自（i）二（乙二醇）乙醚的钡盐，（ii）二（乙二醇） 丙基醚，（iii）二（乙二醇）己基醚，（iv）二（N，N-二甲基氨基乙二醇）乙醚，（v）薄荷醇和百里酚在由水，醇，胺， 硫醇，磷酸盐和亚磷酸盐。 用上述催化剂体系制备的本发明的反式聚合物和共聚物通常具有-97℃至-40℃的熔融温度范围为-30℃至+ 30℃的玻璃化转变温度。 ，数均分子量为20,000〜250,000。 在钡催化剂体系中包含这种极性改性剂导致共聚反应中苯乙烯含量高，反式含量高，分子量高。 用本发明的催化剂体系制得的共轭二烯烃单体和乙烯基芳族单体的共聚物也具有锥形宏观结构。

    Solution polymerization process for synthesis of styrene-butadiene or styrene-isoprene rubber
    9.
    发明授权
    Solution polymerization process for synthesis of styrene-butadiene or styrene-isoprene rubber 失效
    用于合成苯乙烯 - 丁二烯或苯乙烯 - 异戊二烯橡胶的溶液聚合方法

    公开(公告)号：US5679751A

    公开(公告)日：1997-10-21

    申请号：US599542

    申请日：1996-02-12

    申请人： Adel Farhan Halasa ,  Laurie Elizabeth Austin ,  Wen-Liang Hsu ,  Bill Bud Gross

    发明人： Adel Farhan Halasa ,  Laurie Elizabeth Austin ,  Wen-Liang Hsu ,  Bill Bud Gross

    IPC分类号： B60C1/00 ,  C08F4/46 ,  C08F4/48 ,  C08F236/10

    CPC分类号： B60C1/0016 ,  C08F236/10

    摘要： The subject invention relates to a technique for synthesizing rubbery copolymers of styrene and butadiene and/or isoprene. These rubbers exhibit an excellent combination of properties for utilization in high performance tire tread rubber compounds. The subject invention specifically discloses a process for preparing a styrene-butadiene rubber (SBR) which comprises: copolymerizing from about 30 weight percent to about 55 weight percent styrene and from about 45 weight percent to about 70 weight percent 1,3-butadiene in an alkane solvent, such as hexane, at a temperature which is within the range of about -10.degree. C. to about 150.degree. C. in the presence of (a) an alkali metal alkoxide, and (b) an organolithium compound, wherein the molar ratio of the alkali metal alkoxide to the organolithium compound is within the range of about 0.01:1 to about 1:1. The subject invention further discloses a process for preparing a rubbery copolymer of styrene and isoprene having an excellent combination of properties for use in making tire treads by a solution polymerization process which comprises: copolymerizing from about 30 weight percent to about 55 weight percent styrene and from about 45 weight percent to about 70 weight percent isoprene in an alkane solvent at a temperature which is within the range of about -10.degree. C. to about 150.degree. C. in the presence of (a) an alkali metal alkoxide, and (b) an organolithium compound, wherein the molar ratio of the alkali metal alkoxide to the organolithium compound is within the range of about 0.01:1 to about 1:1.

    摘要翻译： 本发明涉及一种合成苯乙烯和丁二烯和/或异戊二烯橡胶共聚物的技术。 这些橡胶在高性能轮胎胎面橡胶化合物中表现出优异的性能组合。 本发明具体公开了一种制备苯乙烯 - 丁二烯橡胶（SBR）的方法，其包括：以约30重量％至约55重量％的苯乙烯和约45重量％至约70重量％的1,3-丁二烯的共聚合 烷烃溶剂如己烷，在（a）碱金属醇盐存在下，在约-10℃至约150℃的温度范围内，和（b）有机锂化合物，其中， 碱金属醇盐与有机锂化合物的摩尔比在约0.01:1至约1:1的范围内。 本发明进一步公开了一种制备苯乙烯和异戊二烯的橡胶共聚物的方法，其具有通过溶液聚合方法制备轮胎胎面的优异的性能组合，其包括：共聚约30重量％至约55重量％的苯乙烯和 在（a）碱金属醇盐存在下，在约-10℃至约150℃的温度下，在烷烃溶剂中约45重量％至约70重量％的异戊二烯，和（b ）有机锂化合物，其中碱金属醇盐与有机锂化合物的摩尔比在约0.01:1至约1:1的范围内。

    Catalyst System for Synthesizing Amine Functionalized Rubbery Polymers Having a High Trans Microstructure
    10.
    发明申请
    Catalyst System for Synthesizing Amine Functionalized Rubbery Polymers Having a High Trans Microstructure 有权
    用于合成具有高转移微结构的胺官能化橡胶聚合物的催化剂体系

    公开(公告)号：US20080161518A1

    公开(公告)日：2008-07-03

    申请号：US11617361

    申请日：2006-12-28

    申请人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Laurie Elizabeth Austin ,  Chad Aaron Jasiunas ,  Steven Kristofer Henning

    发明人： Adel Farhan Halasa ,  Wen-Liang Hsu ,  Laurie Elizabeth Austin ,  Chad Aaron Jasiunas ,  Steven Kristofer Henning

    IPC分类号： C08F4/48 ,  B60C1/00 ,  C08K3/04 ,  C08K3/36

    CPC分类号： C08F36/04 ,  C08F4/48 ,  C08F4/54

    摘要： The present invention is directed to a catalyst system for synthesizing rubbery polymers, such as polybutadiene rubber, styrene-butadiene rubber, isoprene-butadiene rubber, or styrene-isoprene-butadiene rubber, that are amine functionalized and have a high trans microstructure. The catalyst system, in one embodiment, includes (a) an organolithium amine compound, (b) a group IIa metal salt of an amino glycol or a glycol ether, (c) an organoaluminum compound, and optionally (d) an amine compound. The amine functionalized rubbery polymers can be utilized in tire tread rubbers where the rubbery polymers may provide desirable wear properties without substantially sacrificing other performance characteristic(s), e.g., traction properties.

    摘要翻译： 本发明涉及一种用于合成胺官能化并具有高反相微观结构的橡胶状聚合物如聚丁二烯橡胶，苯乙烯 - 丁二烯橡胶，异戊二烯 - 丁二烯橡胶或苯乙烯 - 异戊二烯 - 丁二烯橡胶的催化剂体系。 在一个实施方案中，催化剂体系包括（a）有机锂胺化合物，（b）氨基二醇或二醇醚的IIa族金属盐，（c）有机铝化合物和任选的（d）胺化合物。 胺官能化橡胶状聚合物可用于轮胎胎面橡胶中，其中橡胶状聚合物可提供期望的耐磨性，而基本上不会牺牲其它性能特征，例如牵引性能。