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公开(公告)号：US06521562B1
公开(公告)日：2003-02-18
申请号：US09672469
申请日：2000-09-28
申请人： Kenneth R. Clem , Luc R. M. Martens , Stephen N. Vaughn , Paul R. Stafford , John W. Kress , Machteld M. Mertens
发明人： Kenneth R. Clem , Luc R. M. Martens , Stephen N. Vaughn , Paul R. Stafford , John W. Kress , Machteld M. Mertens
IPC分类号： B01J27182
CPC分类号： B01J37/0009 , B01J29/04 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/48 , C10G3/49 , C10G2400/20 , Y02P30/20
摘要： A method of making a molecular sieve catalyst by preparing a catalyst slurry containing molecular sieve, binder and a matrix material and directing the slurry to a forming unit. The catalyst slurry is prepared by using a microfiltration process whereby the molecular sieve is washed and concentrated from a preparation medium without having to isolate the molecular sieve in a dry or semi-dry form. The catalyst is used to make ethylene and propylene from an oxygenate.
摘要翻译： 一种通过制备含有分子筛，粘合剂和基质材料并将浆料引导至成形单元的催化剂浆料制备分子筛催化剂的方法。 通过使用微滤方法制备催化剂浆料，其中分子筛从制备介质中洗涤和浓缩，而不必分离干燥或半干燥形式的分子筛。 催化剂用于从含氧化合物制备乙烯和丙烯。
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2.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US07541508B2
公开(公告)日：2009-06-02
申请号：US11640559
申请日：2006-12-18
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： C07C1/00
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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3.发明授权Molecular-sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和在转化过程中的应用公开(公告)号：US07301065B2
公开(公告)日：2007-11-27
申请号：US10893642
申请日：2004-07-16
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： C07C1/20
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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4.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US07160831B2
公开(公告)日：2007-01-09
申请号：US10178374
申请日：2002-06-24
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： B01J29/06
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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5.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 失效分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US06787501B2
公开(公告)日：2004-09-07
申请号：US10178578
申请日：2002-06-24
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R. M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： B01J2906
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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6.发明申请Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US20080269436A1
公开(公告)日：2008-10-30
申请号：US11640559
申请日：2006-12-18
申请人： Stephen N. Vaughn , Yun-feng Chang , Luc R.M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
发明人： Stephen N. Vaughn , Yun-feng Chang , Luc R.M. Martens , Kenneth R. Clem , Machteld M. Mertens , Albert E. Schweizer
IPC分类号： C08F2/00
CPC分类号： C10G3/49 , B01J29/83 , B01J29/84 , B01J29/85 , B01J37/0009 , B01J37/0045 , B01J2229/12 , B01J2229/14 , B01J2229/24 , B01J2229/34 , B01J2229/42 , C07C1/20 , C07C7/04 , C07C7/08 , C07C2529/85 , C08F10/00 , C08F110/02 , C08F110/06 , C10G2400/20 , C10G2400/22 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/02 , C07C11/04 , C08F4/12 , C08F4/16 , C08F4/025 , C08F4/005
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to making a formulated molecular sieve catalyst composition from a slurry of formulation composition of a synthesized molecular sieve that has not been fully dried, a binder and an optional matrix material. In a more preferred embodiment, the weight ratio of the binder to the molecular sieve and/or the solid content of the slurry is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及从尚未完全干燥的合成分子筛的配方组合物的浆料，粘合剂和任选的基质材料制备配制的分子筛催化剂组合物。 在更优选的实施方案中，控制粘合剂与分子筛的重量比和/或浆料的固体含量，以提供改进的耐磨性催化剂组合物，特别可用于生产烯烃的转化方法 乙烯和/或丙烯，优选含有氧化合物的原料。
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7.发明授权Molecular sieve catalyst composition, its making and use in conversion process 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US07271123B2
公开(公告)日：2007-09-18
申请号：US10178455
申请日：2002-06-24
IPC分类号： B01J29/04 , B01J27/182
CPC分类号： B01J37/0009 , B01J29/85 , B01J35/10 , B01J35/1019 , B01J35/1023 , B01J37/0045 , B01J2229/42 , C07C1/20 , C07C2529/85 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a molecular sieve catalyst composition of a molecular sieve, a binder and a matrix material, wherein the weight ratio of the binder to the molecular sieve is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及分子筛，粘合剂和基质材料的分子筛催化剂组合物，其中控制粘合剂与分子筛的重量比以提供改进的耐磨性催化剂组合物，特别适用于 用于从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。
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8.发明授权Molecular sieve catalyst compositions, its making and use in conversion processes 有权分子筛催化剂组合物，其制备和用于转化过程公开(公告)号：US07214844B2
公开(公告)日：2007-05-08
申请号：US11039294
申请日：2005-01-20
申请人： Yun-feng Chang , Stephen N. Vaughn , Luc R. M. Martens , Joseph E. Baumgartner , Stuart L. Soled , Kenneth R. Clem
发明人： Yun-feng Chang , Stephen N. Vaughn , Luc R. M. Martens , Joseph E. Baumgartner , Stuart L. Soled , Kenneth R. Clem
IPC分类号： C07C1/00
CPC分类号： B01J37/10 , B01J29/85 , B01J35/10 , B01J37/0009 , B01J37/0045 , B01J2229/36 , B01J2229/42 , C07C1/20 , C07C11/02 , C07C11/04 , C07C11/06 , C07C2529/00 , C07C2529/85 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P20/52 , Y02P30/42
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a making a molecular sieve catalyst composition by forming a slurry by combining a molecular sieve, a binder and a matrix material, wherein the slurry has a pH, above or below the isoelectric point of the molecular sieve. The catalyst composition has improved attrition resistance, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及通过组合分子筛，粘合剂和基质材料形成浆料来制备分子筛催化剂组合物，其中所述浆料具有高于或低于分子筛等电点的pH。 催化剂组合物具有改善的耐磨性，特别适用于从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。
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9.发明授权Molecular sieve catalyst composition, its making and use in conversion processes 有权分子筛催化剂组成，其制备和用途在转化过程中公开(公告)号：US06872680B2
公开(公告)日：2005-03-29
申请号：US10178518
申请日：2002-06-24
申请人： Yun-feng Chang , Stephen N. Vaughn , Luc R. M. Martens , Joseph E. Baumgartner , Stuart L. Soled , Kenneth R. Clem
发明人： Yun-feng Chang , Stephen N. Vaughn , Luc R. M. Martens , Joseph E. Baumgartner , Stuart L. Soled , Kenneth R. Clem
IPC分类号： B01J29/85 , B01J35/10 , B01J37/00 , B01J37/10 , C07C1/20 , C07C11/02 , C07C11/04 , C07C11/06 , C10G3/00 , B01J29/06
CPC分类号： B01J37/10 , B01J29/85 , B01J35/10 , B01J37/0009 , B01J37/0045 , B01J2229/36 , B01J2229/42 , C07C1/20 , C07C11/02 , C07C11/04 , C07C11/06 , C07C2529/00 , C07C2529/85 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P20/52 , Y02P30/42
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a making a molecular sieve catalyst composition by forming a slurry by combining a molecular sieve, a binder and a matrix material, wherein the slurry has a pH, above or below the isoelectric point of the molecular sieve. The catalyst composition has improved attrition resistance, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译： 本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。 特别地，本发明涉及通过组合分子筛，粘合剂和基质材料形成浆料来制备分子筛催化剂组合物，其中所述浆料具有高于或低于分子筛等电点的pH。 催化剂组合物具有改善的耐磨性，特别适用于从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。
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公开(公告)号：US07071136B2
公开(公告)日：2006-07-04
申请号：US10442586
申请日：2003-05-21
IPC分类号： B01J29/06
CPC分类号： B01J37/0045 , B01J29/06 , B01J29/85 , C07C1/20 , C07C2529/83 , C07C2529/85 , C10G2400/20 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： This invention is directed to a hardened molecular sieve catalyst composition, a method of making the composition and a method of using the composition. The catalyst composition is made by mixing together molecular sieve, liquid, and an effective hardening amount of a dried molecular sieve catalyst to form a slurry. The slurry is dried, and then calcined to form the hardened molecular sieve catalyst composition. The hardened molecular sieve catalyst is highly attrition resistant.
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