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1.发明授权Proton conductors which are thermally stable over a wide range and have good proton conductivities 失效在宽范围内热稳定且具有良好质子电导率的质子导体公开(公告)号：US06264857B1
公开(公告)日：2001-07-24
申请号：US09242036
申请日：1999-07-02
申请人： Klaus-Dieter Kreuer , Annette Fuchs , Joachim Maier , Georg Frank , Thomas Soczka-Guth , Joachim Clauss
发明人： Klaus-Dieter Kreuer , Annette Fuchs , Joachim Maier , Georg Frank , Thomas Soczka-Guth , Joachim Clauss
IPC分类号： H01B100
CPC分类号： C25B13/04 , H01M2/1653 , H01M8/0289 , H01M8/08 , H01M10/02
摘要： Proton conductors comprising from 1 to 99% by weight of an acid and from 99 to 1% by weight of a nonaqueous amphoteric material which are thermally stable from −50° C. to 400° C. and have a proton conductivity of ≧10−5 S/cm. The invention further relates to membranes comprising the proton conductors of the invention, processes for preparing the membranes and their use in electrochromic cells, secondary batteries and electrochromic displays.
摘要翻译： 包含1至99重量％的酸和99至1重量％的非水性两性材料的质子导体，其在-50℃至400℃下热稳定且质子传导率≥10 -5 S / cm。 本发明还涉及包含本发明的质子导体的膜，制备膜的方法及其在电致变色电池，二次电池和电致变色显示器中的应用。
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2.发明授权Alkaline single ion conductors with high conductivity and transference number and methods for preparing the same 有权具有高导电性和转移次数的碱性单离子导体及其制备方法公开(公告)号：US09299501B2
公开(公告)日：2016-03-29
申请号：US13882535
申请日：2011-11-02
IPC分类号： H01M8/10 , H01G9/035 , H01B1/12 , H01M10/0565 , H01M10/0568 , H01M10/0569
CPC分类号： H01G9/035 , H01B1/122 , H01M8/1018 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M2300/0082
摘要： A method of producing an alkaline single ion conductor with high conductivity includes: a) providing a hydrocarbon oligomer or polymer having immobilized acidic substituent groups selected from the group consisting of a sulfonic acid group, sulfamide group, a phosphonic acid group, or a carboxy group, in its alkaline ion form wherein at least a part of the acidic protons of the substituent groups have been exchanged against alkali cations, and b) solvating the hydrocarbon oligomer or polymer of step a) in an aprotic polar solvent for a sufficient time to effect a solvent uptake of at least 5% by weight and to obtain a solvated product, wherein the molar ratio of solvent/alkaline cation is 1:1 to 10,000:1, and which solvated product has a conductivity of at least 10−5 S/cm at room temperature (24° C.).
摘要翻译： 制备具有高导电性的碱性单离子导体的方法包括：a）提供具有选自磺酸基，磺酰胺基，膦酸基或羧基的固定的酸性取代基的烃低聚物或聚合物 以其碱性离子形式，其中取代基的至少一部分酸性质子已经被碱金属阳离子交换，和b）将非极性极性溶剂中的步骤a）的烃低聚物或聚合物溶剂足够的时间来实现 溶剂吸收量为至少5重量％，并获得溶剂化产物，其中溶剂/碱性阳离子的摩尔比为1:1至10,000:1，并且该溶剂化产物具有至少10 -5 S / 室温（24℃）。
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3.发明申请ALKALINE SINGLE ION CONDUCTORS WITH HIGH CONDUCTIVITY AND TRANSFERENCE NUMBER AND METHODS FOR PREPARING THE SAME 有权具有高电导率和转移数的碱性单离子导体及其制备方法公开(公告)号：US20130216936A1
公开(公告)日：2013-08-22
申请号：US13882535
申请日：2011-11-02
IPC分类号： H01G9/035 , H01M8/10 , H01M10/0565
CPC分类号： H01G9/035 , H01B1/122 , H01M8/1018 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M2300/0082
摘要： A method of producing an alkaline single ion conductor with high conductivity includes: a) providing a hydrocarbon oligomer or polymer having immobilized acidic substituent groups selected from the group consisting of a sulfonic acid group, sulfamide group, a phosphonic acid group, or a carboxy group, in its alkaline ion form wherein at least a part of the acidic protons of the substituent groups have been exchanged against alkali cations, and b) solvating the hydro-carbon oligomer or polymer of step a) in an aprotic polar solvent for a sufficient time to effect a solvent uptake of at least 5% by weight and to obtain a solvated product, wherein the molar ratio of solvent/alkaline cation is 1:1 to 10,000:1, and which solvated product has a conductivity of at least 10−5 S/cm at room temperature (24° C.).
摘要翻译： 制备具有高导电性的碱性单离子导体的方法包括：a）提供具有选自磺酸基，磺酰胺基，膦酸基或羧基的固定的酸性取代基的烃低聚物或聚合物 以其碱性离子形式，其中取代基的至少一部分酸性质子已经被碱金属阳离子交换，和b）将非氢化极性溶剂中的步骤a）的氢碳低聚物或聚合物溶剂足够的时间 以使溶剂吸收至少为5重量％，并获得溶剂化产物，其中溶剂/碱性阳离子的摩尔比为1:1至10,000:1，并且该溶剂化产物的导电率至少为10-5 在室温（24℃）下S / cm。
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4.发明申请Sulfonated Poly(Arylenes) as Hydrolytically and Thermo-Oxidatively Stable Polymers 有权磺化聚（亚芳基）作为水解和热氧化稳定的聚合物公开(公告)号：US20080207781A1
公开(公告)日：2008-08-28
申请号：US11885904
申请日：2006-03-07
CPC分类号： C08G75/20 , C08J5/2256 , C08J2381/06 , C08L81/06 , C08L2666/02
摘要： Hydrolytically and thermo-oxidatively stable sulfonated polyarylenes include the structural element —X—Ar(SO3M)n-Y—. The aromatic ring carrying the sulfonic acid group is substituted exclusively by electron-acceptor bridge groups X and Y and, if applicable, by other non-electron-donor substituents. Their synthesis and application are also included.
摘要翻译： 水解和热氧化稳定的磺化聚芳烯包括结构单元-X-Ar（SO 3 M）N - Y - 。 携带磺酸基团的芳环仅被电子受体桥基团X和Y取代，并且如果适用，被其它非电子给体取代基取代。 它们的合成和应用也包括在内。
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5.发明授权Sulfonated poly(arylenes) as hydrolytically and thermo-oxidatively stable polymers 有权磺化聚（亚芳基）作为水解和热氧化稳定的聚合物公开(公告)号：US08349993B2
公开(公告)日：2013-01-08
申请号：US11885904
申请日：2006-03-07
IPC分类号： C08G75/00
CPC分类号： C08G75/20 , C08J5/2256 , C08J2381/06 , C08L81/06 , C08L2666/02
摘要： Hydrolytically and thermo-oxidatively stable sulfonated polyarylenes include the structural element —X—Ar(SO3M)n-Y—. The aromatic ring carrying the sulfonic acid group is substituted exclusively by electron-acceptor bridge groups X and Y and, if applicable, by other non-electron-donor substituents. Their synthesis and application are also included.
摘要翻译： 水解和热氧化稳定的磺化聚芳烯包括结构单元-X-Ar（SO3M）n-Y-。 携带磺酸基团的芳环仅被电子受体桥基团X和Y取代，并且如果适用，被其它非电子给体取代基取代。 它们的合成和应用也包括在内。
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公开(公告)号：US08164881B2
公开(公告)日：2012-04-24
申请号：US12302758
申请日：2007-05-25
申请人： Yong-Sheng Hu , Yu-Guo Guo , Lizhen Fan , Joachim Maier , Philipp Adelhelm , Bernd Smarsly , Markus Antonietti
发明人： Yong-Sheng Hu , Yu-Guo Guo , Lizhen Fan , Joachim Maier , Philipp Adelhelm , Bernd Smarsly , Markus Antonietti
IPC分类号： H01G9/00
CPC分类号： H01G11/26 , C01B32/05 , H01G11/24 , H01G11/32 , H01G11/34 , H01G11/48 , H01G11/86 , H01M4/04 , H01M4/583 , H01M4/587 , H01M10/0525 , Y02E60/13 , Y10T428/24998 , Y10T428/249981
摘要： An extremely high-performance polyaniline electrode was prepared by potentiostatic deposition of aniline on hierarchically porous carbon monolith (HPCM), which was carbonized from mesophase pitch. A capacitance value of 2200 F g−1 of polyaniline was obtained at a power density of 0.47 kW kg−1 and an energy density of 300 Wh kg−1. This active material deposited on HPCM also has an advantageous high stability. These superior advantages can be attributed to the backbone role of HPCM. This method also has the advantages of not introducing any binder, thus contributing to the increase of ionic conductivity and power density. High specific capacitance, high power and energy density, high stability, and low cost of active material make it very promising for supercapacitors.
摘要翻译： 通过在分层多孔碳整料（HPCM）上静电沉积苯胺制备了极高性能的聚苯胺电极，其由中间相沥青碳化。 在功率密度为0.47 kW kg-1，能量密度为300 Wh kg-1时，得到聚苯胺的2200 F g-1的电容值。 沉积在HPCM上的这种活性材料也具有有利的高稳定性。 这些优势可以归功于HPCM的骨干作用。 该方法还具有不引入任何粘合剂的优点，因此有助于提高离子电导率和功率密度。 高比电容，高功率和能量密度，高稳定性和低成本的活性材料使其非常有前途的超级电容器。
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7.发明申请NON-AQUEOUS ELECTROLYTE AND A BATTERY, A SUPERCAPACITOR, AN ELECTROCHROMIC DEVICE AND A SOLAR CELL INCLUDING SUCH AN ELECTROLYTE 审中-公开非水电解质和电池，超级电容器，电致发光器件和包括这种电解质的太阳能电池公开(公告)号：US20100239916A1
公开(公告)日：2010-09-23
申请号：US12748649
申请日：2010-03-29
CPC分类号： H01M6/181 , G02F1/1525 , H01M6/168 , H01M6/22 , H01M10/0525 , H01M10/0565 , H01M10/0567 , H01M2300/0085 , H01M2300/0091
摘要： A non-aqueous electrolyte including at least one ionically conducting salt, especially a lithium salt, a non-aqueous, anhydrous solvent for the ionically conductive salt, and at least one oxide in a particulate form, said oxide being selected such that it is not soluble in said solvent and such that it is water-free. The electrolyte can be used in a primary or secondary lithium battery, in a supercapacitor, in an electro-chromic display or in a solar cell.
摘要翻译： 包括至少一种离子导电盐，特别是锂盐，用于离子导电盐的非水性无水溶剂和至少一种颗粒形式的氧化物的非水电解质，所述氧化物选择为不是 溶于所述溶剂，使其不含水。 电解质可用于一次或二次锂电池，超级电容器，电显示器或太阳能电池中。
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8.发明申请Novel electrodes for li-based electrochemical energy storage devices and a li-based electrochemical storage device 审中-公开用于锂基电化学储能装置的新型电极和基于锂的电化学存储装置公开(公告)号：US20060035148A1
公开(公告)日：2006-02-16
申请号：US10527638
申请日：2003-09-11
申请人： Palani Balaya , Hong Li , Joachim Maier
发明人： Palani Balaya , Hong Li , Joachim Maier
CPC分类号： H01M4/485 , H01M4/622 , H01M4/624 , H01M10/052 , H01M2004/021 , H01M2300/0082 , H01M2300/0085
摘要： The description relates to the use of at least one transition metal halide with a binder, e.g. at least one of PVDF, PTFE, PAN and ETDM and optionally with at least one conductive additive such as carbon black, graphite, metal powder and metal fibres as an electrode in an Li-based electrochemical energy storage device. Further electrode materials are also described based on ruthenium oxide, molybdenum oxide, a nano-composite composed of transition metal and lithium fluoride or lithium oxide clusters with a typical grain size of 1-10 mm.
摘要翻译： 该描述涉及至少一种过渡金属卤化物与粘合剂的使用，例如， PVDF，PTFE，PAN和ETDM中的至少一种，并且任选地具有至少一种导电添加剂，例如在基于Li的电化学能量存储装置中作为电极的炭黑，石墨，金属粉末和金属纤维。 还描述了另外的电极材料，其基于氧化钌，氧化钼，由过渡金属和具有1-10mm典型晶粒尺寸的氟化锂或氧化锂簇组成的纳米复合物。
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9.发明申请Material, In Particular For Use In Electrochemical Cells Or Supercapacitors And A Method Of Making Such A Material 审中-公开材料，特别用于电化学电池或超级电容器和制造这种材料的方法公开(公告)号：US20100117033A1
公开(公告)日：2010-05-13
申请号：US12529535
申请日：2007-03-05
申请人： Yu-Guo Guo , Yong-Sheng Hu , Joachim Maier
发明人： Yu-Guo Guo , Yong-Sheng Hu , Joachim Maier
CPC分类号： H01M4/5825 , H01G9/2027 , H01G11/24 , H01G11/46 , H01M4/136 , H01M4/366 , H01M4/8605 , H01M10/052 , H01M2004/021 , Y02E10/542 , Y02E60/122 , Y02E60/13
摘要： A material in particular for use in electrochemical cells or supercapacitors comprises a poorly conducting active material of relatively low conductivity having regular or irregular passages having average cross-sectional dimensions generally in the size range from 5 μm to 200 nm and interconnected mesopores having average cross-sectional dimensions in the size range from 2 to 50 nm. The active material is covered with a network of an electronically conductive metal oxide of relatively high conductivity extending into said mesopores. Also claimed is a method of manufacturing such a material.
摘要翻译： 特别是用于电化学电池或超级电容器的材料包括具有通常具有5μm至200nm尺寸范围内的平均截面尺寸的规则或不规则通道的导电性较差的活性材料，并且具有平均截面尺寸的互连中孔， 尺寸范围为2至50nm。 活性材料被延伸到所述介孔中的相对高导电性的电子导电金属氧化物的网络覆盖。 还要求保护的是制造这种材料的方法。
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公开(公告)号：US20100008021A1
公开(公告)日：2010-01-14
申请号：US12302758
申请日：2007-05-25
申请人： Yong-Sheng Hu , Yu-Guo Guo , Lizhen Fan , Joachim Maier , Philipp Adelhelm , Bernd Smarsly , Markus Antonietti
发明人： Yong-Sheng Hu , Yu-Guo Guo , Lizhen Fan , Joachim Maier , Philipp Adelhelm , Bernd Smarsly , Markus Antonietti
CPC分类号： H01G11/26 , C01B32/05 , H01G11/24 , H01G11/32 , H01G11/34 , H01G11/48 , H01G11/86 , H01M4/04 , H01M4/583 , H01M4/587 , H01M10/0525 , Y02E60/13 , Y10T428/24998 , Y10T428/249981
摘要： An extremely high-performance polyaniline electrode was prepared by potentiostatic deposition of aniline on hierarchically porous carbon monolith (HPCM), which was carbonized from mesophase pitch. A capacitance value of 2200 F g−1 of polyaniline was obtained at a power density of 0.47 kW kg−1 and an energy density of 300 Wh kg−1. This active material deposited on HPCM also has an advantageous high stability. These superior advantages can be attributed to the backbone role of HPCM. This method also has the advantages of not introducing any binder, thus contributing to the increase of ionic conductivity and power density. High specific capacitance, high power and energy density, high stability, and low cost of active material make it very promising for supercapacitors.
摘要翻译： 通过在分层多孔碳整料（HPCM）上静电沉积苯胺制备了极高性能的聚苯胺电极，其由中间相沥青碳化。 在功率密度为0.47 kW kg-1，能量密度为300 Wh kg-1时，得到聚苯胺的2200 F g-1的电容值。 沉积在HPCM上的这种活性材料也具有有利的高稳定性。 这些优势可以归功于HPCM的骨干作用。 该方法还具有不引入任何粘合剂的优点，因此有助于提高离子电导率和功率密度。 高比电容，高功率和能量密度，高稳定性和低成本的活性材料使其非常有前途的超级电容器。
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