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公开(公告)号：US20070155999A1
公开(公告)日：2007-07-05
申请号：US11322412
申请日：2005-12-30
申请人： Peter Pujado , Bipin Vora , John Senetar , Lawrence Miller
发明人： Peter Pujado , Bipin Vora , John Senetar , Lawrence Miller
CPC分类号： C07C1/20 , C07C11/02 , C07C29/151 , C07C41/01 , C10G2300/4081 , C10G2400/20 , C10G2400/22 , C07C31/04 , C07C43/043
摘要： Improved processing for the production of light olefins via oxygenate conversion processing is provided. Synthesis gas conversion such as to produce an effluent including at least methanol can be integrated with oxygenate conversion processing such as to produce an oxygenate conversion reactor effluent including at least light olefins and dimethyl ether. At least a portion of the oxygenate conversion reactor effluent can be contacted with such produced methanol to effect recovery of dimethyl ether from the oxygenate conversion reactor effluent.
摘要翻译： 提供了通过含氧化合物转化处理生产轻质烯烃的改进方法。 合成气转化如产生至少包含甲醇的流出物可与含氧化合物转化处理结合，以产生包含至少轻烯烃和二甲醚的含氧化合物转化反应器流出物。 含氧化合物转化反应器流出物的至少一部分可以与这样产生的甲醇接触以从含氧化合物转化反应器流出物中回收二甲醚。
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公开(公告)号：US20080039667A1
公开(公告)日：2008-02-14
申请号：US11874448
申请日：2007-10-18
申请人： Bipin Vora , Peter Pujado
发明人： Bipin Vora , Peter Pujado
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C4/06 , C07C2529/035 , C07C2529/40 , C07C2529/86 , Y02P30/42 , C07C11/06 , C07C11/04
摘要： The present invention relates to a process for the production of light weight olefins comprising olefins having from 2 to 3 carbon atoms per molecule from an oxygenate feedstock. The process comprises passing the oxygenate feedstock to an oxygenate conversion zone containing a metal aluminophosphate catalyst to produce a light weight olefin stream. A propylene stream and/or mixed butylene is fractionated from said light weight olefin stream and a medium weight C4 to C7 stream is cracked in a separate olefin cracking reactor to enhance the yield of ethylene and propylene products.
摘要翻译： 本发明涉及一种生产轻质烯烃的方法，其包含每分子含有2-3个碳原子的含氧原料。 该方法包括使含氧化合物原料通入含有金属磷酸铝催化剂的含氧化合物转化区以产生轻质烯烃物流。 将丙烯料流和/或混合的丁烯从所述轻质烯烃料流中分馏，并将中等重量C 4至C 7 H 2流在单独的烯烃裂解反应器中裂化以增强 乙烯和丙烯产品的产率。
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3.发明申请Selective conversion of oxygenate to propylene using moving bed technology and a hydrothermally stabilized dual-function catalyst 有权使用移动床技术和水热稳定的双功能催化剂选择性地将含氧化合物转化为丙烯公开(公告)号：US20060106270A1
公开(公告)日：2006-05-18
申请号：US10988136
申请日：2004-11-12
申请人： Bryan Glover , John Chen , Peter Pujado , Bipin Vora
发明人： Bryan Glover , John Chen , Peter Pujado , Bipin Vora
IPC分类号： C07C1/00
CPC分类号： C07C11/06 , B01J8/082 , B01J8/085 , B01J8/12 , B01J2208/00274 , B01J2208/00283 , B01J2208/00292 , C07C1/20 , C07C2521/04 , C07C2529/40 , C07C2529/84 , C07C2529/85 , Y02P20/52
摘要： The average propylene cycle selectivity of an oxygenate to propylene (OTP) process using a dual-function oxygenate conversion catalyst is substantially enhanced by the use of a combination of: 1) moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of the fixed bed technology of the prior art; 2) a hydrothermally stabilized and dual-functional catalyst system comprising a molecular sieve having dual-function capability dispersed in a phosphorus-modified alumina matrix containing labile phosphorus and/or aluminum anions; and 3) a catalyst on-stream cycle time of 400 hours or less. These provisions stabilize the catalyst against hydrothermal deactivation and hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of average propylene cycle yield near or at essentially start-of-cycle levels.
摘要翻译： 使用双功能含氧化合物转化催化剂的含氧化合物对丙烯（OTP）方法的平均丙烯循环选择性通过使用以下组合来显着增强：1）OTP流程图的烃合成部分中的移动床反应器技术 现有技术的固定床技术的代替; 2）水热稳定和双功能催化剂体系，其包含具有分散在含有不稳定磷和/或铝阴离子的磷改性氧化铝基质中的双功能能力的分子筛; 和3）催化剂在流循环时间为400小时以下。 这些规定稳定催化剂以防止水热失活，并将催化剂上焦炭沉积物的积聚保持在基本上不降低双功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而使维持平均丙烯循环产率接近或 基本上是循环周期的水平。
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公开(公告)号：US20070203380A1
公开(公告)日：2007-08-30
申请号：US11322897
申请日：2005-12-30
申请人： Bipin Vora , Peter Pujado
发明人： Bipin Vora , Peter Pujado
CPC分类号： C07C1/20 , C07C11/02 , C07C29/151 , C07C41/01 , C07C41/09 , C10G2300/1022 , C10G2300/4081 , C10G2400/20 , C07C31/04 , C07C43/043
摘要： Improved processing for the production of light olefins is provided involving synthesis gas conversion to form an effluent including product dimethyl ether, subsequent separation of the product dimethyl ether and conversion thereof to the desired light olefins. The synthesis gas conversion effluent may also desirably include methanol and at least a portion of such methanol may be employed to effect the separation of the product dimethyl ether.
摘要翻译： 提供了用于生产轻质烯烃的改进方法，包括合成气转化以形成包含产物二甲醚的流出物，随后分离产物二甲醚并将其转化成所需的轻质烯烃。 合成气转化流出物还可以理想地包括甲醇，并且可以使用至少一部分这种甲醇来实现产物二甲醚的分离。
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公开(公告)号：US20050080307A1
公开(公告)日：2005-04-14
申请号：US10951359
申请日：2004-09-28
申请人： Timur Voskoboynikov , Michael Quick , Peter Pujado , Bipin Vora
发明人： Timur Voskoboynikov , Michael Quick , Peter Pujado , Bipin Vora
IPC分类号： B01J29/035 , B01J29/40 , C07C4/06 , C07C4/02
CPC分类号： B01J29/035 , B01J29/40 , B01J2229/42 , C07C4/06 , Y02P20/52 , C07C11/04 , C07C11/06
摘要： The present invention comprises a process for producing propylene comprising the steps of contacting an olefin feed containing between about 40 and about 80 wt-% olefins and between about 20 and about 60 wt-% olefins and aromatics with a spherical catalyst to form a cracked product, the catalyst comprising about 30 to about 80 wt-% of a crystalline zeolite, the reaction conditions including a temperature from about 500° to 650° C., a hydrocarbon partial pressure of 70 to 280 kPa (10 to 40 psia), a liquid hourly space velocity in the range of 5 to 40 hr−1 and wherein propylene comprises at least 90 mol-% of the total C3 products.
摘要翻译： 本发明包括一种生产丙烯的方法，包括以下步骤：将含有约40至约80重量％的烯烃和约20至约60重量％的烯烃和芳族化合物的烯烃进料与球形催化剂接触以形成裂化产物 ，催化剂包含约30至约80重量％的结晶沸石，反应条件包括约500℃至650℃的温度，70至280kPa（10至40psia）的烃分压， 在5至40小时-1的范围内的液时空速，其中丙烯包含总C3产物的至少90摩尔％。
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公开(公告)号：US20060247481A1
公开(公告)日：2006-11-02
申请号：US11457889
申请日：2006-07-17
IPC分类号： C07C2/02
摘要： The present invention comprises a process for removal of oxygenates from a paraffin-rich or olefin-rich paraffin stream which comprises passing a feed stream, comprising one or more C10 to C15 feed paraffins or C10 to C15 olefin-rich paraffin stream and one or more oxygenates through an adsorbent bed comprising one or more adsorbents selected from silica gel, activated alumina and sodium x zeolites to remove essentially all of said oxygenates; and recovering said paraffins. A second adsorbent bed may be employed to more thoroughly remove these oxygenates.
摘要翻译： 本发明包括从富含链烷烃或富烯烃的石蜡流中除去含氧化合物的方法，该方法包括将含有一个或多个C 10的进料流通入C 15 通过吸附床将含有一种或多种选自硅胶，活性氧化铝和吸附剂的吸附剂的烷烃或C 10向富含C 15的富烯烃链烷烃流和一种或多种含氧化合物进料， 钠x沸石以除去基本上所有的含氧化合物; 并回收所述石蜡。 可以使用第二吸附剂床来更彻底地除去这些含氧化合物。
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公开(公告)号：US20050033101A1
公开(公告)日：2005-02-10
申请号：US10939797
申请日：2004-09-13
IPC分类号： B01J21/04 , B01J23/58 , B01J23/62 , B01J35/00 , B01J35/10 , B01J37/00 , B01J37/02 , C07B61/00 , C07C5/32 , C07C11/06 , C07C5/333
CPC分类号： C07C5/325 , B01J21/04 , B01J23/58 , B01J23/62 , B01J23/626 , B01J35/002 , B01J35/0026 , B01J35/1014 , B01J35/1019 , B01J37/0072 , B01J37/0207 , C07C2523/62
摘要： A hydrocarbon dehydrogenation process utilizing a novel catalyst composite. The catalyst composite comprises a Group VIII noble metal component, a Group IA or IIA metal component, and a component selected from the group consisting of tin, germanium, lead, indium, gallium, thallium, or mixtures thereof, all on an alumina support comprising essentially theta-alumina, having a surface area from about 50 to about 120 m2/g, an apparent bulk density of at 0.5 g/cm3 and a mole ratio of the Group IA or IIA metal component to the component selected from the group consisting of tin, germanium, lead, indium, gallium, thallium or mixtures thereof greater than about 16.
摘要翻译： 一种利用新型催化剂复合材料的烃脱氢方法。 所述催化剂复合材料包括VIII族贵金属组分，IA族或IIA族金属组分，以及选自锡，锗，铅，铟，镓，铊或其混合物的组分，全部在氧化铝载体上，包含 基本上是θ-氧化铝，其表面积为约50至约120m 2 / g，表观堆积密度为0.5g / cm 3，IA或IIA族金属组分与组分的摩尔比 选自锡，锗，铅，铟，镓，铊或大于约16的混合物。
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公开(公告)号：US20070264176A1
公开(公告)日：2007-11-15
申请号：US11828433
申请日：2007-07-26
申请人： Douglas Stewart , Joseph Zimmermann , Angelo Furfaro , Bipin Vora
发明人： Douglas Stewart , Joseph Zimmermann , Angelo Furfaro , Bipin Vora
IPC分类号： B01J7/02
摘要： The present invention relates to a process and apparatus for the production of light olefins comprising olefins having from 2 to 3 carbon atoms per molecule from a feedstock containing heavier olefins. An intermediate cut from a fractionation column is used as olefinic feed to an olefin cracking process preferably after undergoing selective hydrogenation of diolefins. In one embodiment, a liquid side draw from a fractionation column is selectively hydrogenated and then returned to the fractionation column from which a vapor side draw containing olefins is cracked in the olefin cracking reactor.
摘要翻译： 本发明涉及一种用于生产轻质烯烃的方法和设备，其包含每分子含有2至3个碳原子的烯烃，其含有较重的烯烃的原料。 来自分馏塔的中间馏分用作烯烃裂化方法的烯烃进料，优选在进行二烯烃的选择性氢化之后。 在一个实施方案中，从分馏塔抽出的液体侧被选择性氢化，然后返回到在烯烃裂解反应器中含有烯烃的蒸汽侧馏分从其分馏的分馏塔。
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9.发明申请公开(公告)号：US20060135832A1
公开(公告)日：2006-06-22
申请号：US11014049
申请日：2004-12-16
申请人： Bipin Vora , Charles Luebke , Jill Meister , Michael Schultz , Dale Shields
发明人： Bipin Vora , Charles Luebke , Jill Meister , Michael Schultz , Dale Shields
摘要： In an oligomerization process comprising at least two oligomerization reactors, at least portions of product streams from two reactors are separated in the same separator vessel. In an embodiment, a liquid product stream from the first oligomerization reactor is fed to a fractionation column and a side cut from the fractionation column feeds the second oligomerization reactor.
摘要翻译： 在包含至少两个低聚反应器的低聚方法中，来自两个反应器的至少部分产物流在相同的分离器容器中分离。 在一个实施方案中，将来自第一低聚反应器的液体产物流进料至分馏塔，并且从分馏塔切出的一侧进料第二低聚反应器。
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