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公开(公告)号：US07767870B2
公开(公告)日：2010-08-03
申请号：US11216652
申请日：2005-08-31
申请人： Rutton D. Patel , Arun K. Sharma , E. Nicholas Jones , James H. Beech, Jr. , Richard E. Walter , Donald F. Shaw , Kenneth R. Clem , Nicolas P. Coute
发明人： Rutton D. Patel , Arun K. Sharma , E. Nicholas Jones , James H. Beech, Jr. , Richard E. Walter , Donald F. Shaw , Kenneth R. Clem , Nicolas P. Coute
CPC分类号： B01J8/1827 , B01D45/12 , B01J8/0055 , B01J8/0065 , B01J8/1809 , B01J8/1872 , B01J8/26 , B01J8/28 , B01J8/34 , B01J8/388 , B01J2208/0069 , C07C1/20 , C07C2529/85 , C10G11/18 , C10G31/10 , C07C11/02
摘要： A gas-solids reaction system with termination devices to connect a riser with one or more separation devices. The termination devices have a radius of curvature that is at least 1.0 times as great as the diameter of the conduit forming the termination device. The termination devices can be openly or closely coupled to the separation devices.
摘要翻译： 一种具有终端装置的气体 - 固体反应系统，用于将提升管与一个或多个分离装置连接。 端接装置的曲率半径至少是形成端接装置的导管的直径的1.0倍。 终端设备可以公开地或紧密地耦合到分离设备。
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2.发明授权Method of circulating catalyst between a catalyst regenerator and an external catalyst cooler 有权在催化剂再生器和外部催化剂冷却器之间循环催化剂的方法公开(公告)号：US07906697B2
公开(公告)日：2011-03-15
申请号：US12059717
申请日：2008-03-31
申请人： James H. Beech, Jr. , Chunshe Cao , Michael P. Nicoletti , James R. Lattner , Jesse F. Goellner , Rutton D. Patel , Timothy M. Healy
发明人： James H. Beech, Jr. , Chunshe Cao , Michael P. Nicoletti , James R. Lattner , Jesse F. Goellner , Rutton D. Patel , Timothy M. Healy
IPC分类号： C07C2/04
CPC分类号： C07C1/20 , B01J29/90 , B01J38/30 , B01J38/32 , C07C2529/40 , C07C2529/70 , C07C2529/83 , C07C2529/85 , C10G3/49 , C10G3/62 , C10G2300/802 , C10G2400/20 , Y02P20/584 , Y02P30/20 , C07C11/02
摘要： This invention relates to efficiently regenerating catalyst particles by minimizing the formation of localized “hot spots” and “cold spots” in a regeneration zone. Specifically this invention relates to a method for controlling regenerator temperature in an oxygenates-to-olefins system, comprising the steps of: contacting an oxygenate feed in a reactor with a catalytically effective amount of molecular sieve-containing catalyst under conditions effective for converting said oxygenate to a product containing light olefins and forming a coked catalyst; contacting a portion of the coked catalyst in a regenerator, having a catalyst bed height (Hc), an inlet height (Hi), and an outlet height (Ho), with an oxygen-containing regeneration medium under conditions effective to at least partially regenerate the coked catalyst; and conducting a portion of the catalyst from the regenerator to a catalyst cooler to form a cooled catalyst portion, wherein Ho is greater than Hi.
摘要翻译： 本发明涉及通过最小化再生区中局部“热点”和“冷点”的形成来有效地再生催化剂颗粒。 具体地说，本发明涉及一种用于控制含氧化合物至烯烃体系中的再生器温度的方法，其包括以下步骤：在有效转化所述含氧化合物的条件下使反应器中的含氧化合物进料与催化有效量的含分子筛催化剂接触 涉及含有轻质烯烃并形成焦化催化剂的产品; 在具有催化剂床高度（Hc），入口高度（Hi）和出口高度（Ho））的再生器中使一部分焦化催化剂与含氧再生介质在有效至少部分再生的条件下接触 焦化催化剂; 并将催化剂的一部分从再生器导入催化剂冷却器以形成冷却的催化剂部分，其中Ho大于Hi。
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3.发明授权Fluidizing a population of catalyst particles having a low catalyst fines content 有权流化具有低催化剂细粉含量的催化剂颗粒群公开(公告)号：US08097216B2
公开(公告)日：2012-01-17
申请号：US12898069
申请日：2010-10-05
CPC分类号： C10G3/62 , B01J8/0055 , B01J8/1809 , B01J8/28 , B01J8/34 , B01J2208/00168 , B01J2208/00495 , B01J2208/00752 , B01J2208/00761 , B01J2208/0084 , B01J2208/00884 , C10G3/49 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/20
摘要： A process and apparatus for fluidizing a population of catalyst particles having a low catalyst fines content includes a fluidized bed reactor which includes a plurality of catalyst particles in the reactor wherein the catalyst particles having a d2 value of greater than about 40 microns. The catalyst particles are contacted with a fluidizing medium under conditions to fluidize the particles, the reactor includes a continuous reaction zone and separation zone and the fluidized of the catalyst particles are situated within the reaction and both the reaction zone and the separation zone include obstructing members which obstruct the flow of particles such that the catalyst particles can be maintained at an axial gas Peclet number from about 10 to about 20.
摘要翻译： 用于流化具有低催化剂细粉含量的催化剂颗粒群的方法和设备包括流化床反应器，其在反应器中包括多个催化剂颗粒，其中催化剂颗粒的d2值大于约40微米。 催化剂颗粒在流化颗粒的条件下与流化介质接触，反应器包括连续反应区和分离区，催化剂颗粒的流化位于反应中，反应区和分离区都包括阻挡构件 这阻碍了颗粒的流动，使得催化剂颗粒可以保持在约10至约20的轴向气体佩克莱数。
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公开(公告)号：US07329309B2
公开(公告)日：2008-02-12
申请号：US11134913
申请日：2005-05-23
申请人： Jeffrey S. Smith , James H. Beech, Jr. , Nicolas P. Coute , Jesse F. Goellner , Kenneth Ray Clem
发明人： Jeffrey S. Smith , James H. Beech, Jr. , Nicolas P. Coute , Jesse F. Goellner , Kenneth Ray Clem
IPC分类号： B01D45/01
CPC分类号： F23J15/027 , B01D45/16 , B04C5/081 , B04C5/26
摘要： A multi-stage gas-solids separator is configured so that the higher density (solids) output flows of two or more of the separator stages are merged together. The multi-stage separator is preferably composed of cyclone separators, with the diplegs of at least two of the cyclone separator stages merged together.
摘要翻译： 多级气 - 固分离器被构造成使得两个或更多个分离器级的较高密度（固体）输出流合并在一起。 多级分离器优选由旋风分离器组成，其中至少两个旋风分离器级的叶片合并在一起。
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5.发明授权Fluidizing a population of catalyst particles having a low catalyst fines content 有权流化具有低催化剂细粉含量的催化剂颗粒群公开(公告)号：US07829030B2
公开(公告)日：2010-11-09
申请号：US11143390
申请日：2005-06-02
IPC分类号： C07C1/00 , B01J8/18 , B01J27/182
CPC分类号： C10G3/62 , B01J8/0055 , B01J8/1809 , B01J8/28 , B01J8/34 , B01J2208/00168 , B01J2208/00495 , B01J2208/00752 , B01J2208/00761 , B01J2208/0084 , B01J2208/00884 , C10G3/49 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/20
摘要： The present invention relates to processes for fluidizing a population of catalyst particles that are depleted of catalyst fines. In one embodiment, the process includes providing a plurality of catalyst particles in the reactor, wherein the catalyst particles have a d2 value of greater than about 40 microns. The catalyst particles are contacted with a fluidizing medium under conditions effective to cause the catalyst particles to behave in a fluidized manner and form a fluidized bed. The particles are contacted with one or more primary obstructing members while in the fluidized bed. By fluidizing the catalyst particles in this manner, the catalyst particles can be maintained at an axial gas Peclet number of from about 10 to about 20.
摘要翻译： 本发明涉及流化催化剂细粒的催化剂颗粒群的方法。 在一个实施方案中，该方法包括在反应器中提供多个催化剂颗粒，其中催化剂颗粒具有大于约40微米的d2值。 在有效地使催化剂颗粒以流化方式表现并形成流化床的条件下，催化剂颗粒与流化介质接触。 颗粒在流化床中与一个或多个主要阻塞构件接触。 通过以这种方式使催化剂颗粒流化，催化剂颗粒可以保持在约10至约20的轴向气体Peclet数。
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公开(公告)号：US07309383B2
公开(公告)日：2007-12-18
申请号：US10948984
申请日：2004-09-23
CPC分类号： C10G3/62 , C10G3/49 , C10G3/57 , C10G2300/4093 , C10G2400/20 , Y10S585/91 , Y10S585/911
摘要： Catalyst losses are prevented in riser reactor systems by using a low inlet velocity for the first cyclone separator in each multi-stage cyclone separator in the reactor. Catalyst particles not separated from the product output flow in an oxygenate-to-olefin reactor are also recaptured by cooling the product output flow and passing the flow through an electrostatic precipitator.
摘要翻译： 通过在反应器中的每个多级旋风分离器中使用低入口速度用于第一旋风分离器，在提升管反应器系统中防止催化剂损失。 通过冷却产物输出流量并使流过静电除尘器也可以重新捕获在含氧化合物至烯烃反应器中未与产物输出流分离的催化剂颗粒。
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公开(公告)号：US07687675B2
公开(公告)日：2010-03-30
申请号：US11385288
申请日：2006-03-21
申请人： Teng Xu , Stephen N. Vaughn , Kenneth R. Clem , James H. Beech, Jr. , Peter Nicholas Loezos , Richard B. Hall , Jesse Frederick Goellner
发明人： Teng Xu , Stephen N. Vaughn , Kenneth R. Clem , James H. Beech, Jr. , Peter Nicholas Loezos , Richard B. Hall , Jesse Frederick Goellner
CPC分类号： B01J29/90 , B01J29/85 , B01J38/12 , B01J38/38 , C10G3/45 , C10G3/49 , C10G3/62 , C10G2300/4006 , C10G2300/708 , C10G2300/802 , C10G2300/805 , C10G2400/20 , Y02P30/20 , Y10S502/514
摘要： This invention is directed to methods of converting oxygenates to olefin products. The methods provided include steps for protecting against deactivation of active molecular sieve catalysts during the conversion process. In particular, the invention provides for methods of regenerating coked catalyst to minimize catalyst deactivation due to contact with moisture.
摘要翻译： 本发明涉及将含氧化合物转化成烯烃产物的方法。 所提供的方法包括在转化过程中防止活性分子筛催化剂失活的步骤。 特别地，本发明提供了再生焦化催化剂以使由于与水分接触导致的催化剂失活最小化的方法。
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公开(公告)号：US07619128B2
公开(公告)日：2009-11-17
申请号：US11089965
申请日：2005-03-25
CPC分类号： B01J29/90 , B01J29/85 , B01J38/12 , B01J38/38 , C10G3/45 , C10G3/49 , C10G3/62 , C10G2300/4006 , C10G2300/708 , C10G2300/802 , C10G2300/805 , C10G2400/20 , Y02P30/20 , Y10S502/514
摘要： This invention is directed to methods of converting oxygenates to olefin products. The methods provided include steps for protecting against deactivation of active molecular sieve catalysts during the conversion process. In particular, the invention provides for methods of regenerating coked catalyst to minimize catalyst deactivation due to contact with moisture.
摘要翻译： 本发明涉及将含氧化合物转化成烯烃产物的方法。 所提供的方法包括在转化过程中防止活性分子筛催化剂失活的步骤。 特别地，本发明提供了再生焦化催化剂以使由于与水分接触导致的催化剂失活最小化的方法。
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公开(公告)号：US07452838B2
公开(公告)日：2008-11-18
申请号：US11070607
申请日：2005-03-02
IPC分类号： B01J20/34
摘要： This invention relates to efficiently regenerating catalyst particles by minimizing the formation of localized “hot spots” and “cold spots” in a regeneration zone. In one embodiment, the invention includes mixing spent catalyst from a reactor and cold catalyst from a catalyst cooler in a mixing zone and directing the mixed catalyst to the regeneration zone in a fluidized manner with a fluidizing medium. In the regeneration zone, the mixed catalyst contacts an oxygen-containing regeneration medium under conditions effective to regenerate the spent catalyst contained therein.
摘要翻译： 本发明涉及通过最小化再生区中局部“热点”和“冷点”的形成来有效地再生催化剂颗粒。 在一个实施方案中，本发明包括将来自反应器的废催化剂和来自混合区域中的催化剂冷却器的冷催化剂混合并将流化介质以流化方式引导至再生区。 在再生区中，混合催化剂在有效地再生其中所含的废催化剂的条件下与含氧再生介质接触。
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公开(公告)号：US07223714B2
公开(公告)日：2007-05-29
申请号：US10981269
申请日：2004-11-04
IPC分类号： B01J27/182
CPC分类号： B01J8/18 , B01J8/0015 , B01J8/02 , B01J2208/00548 , B01J2208/00752 , B01J2208/00769 , C07C1/20 , C10G3/49 , C10G3/62 , C10G2300/708 , C10G2400/20 , Y02P30/20 , C07C11/02
摘要： The invention is directed to methods of transfering catalyst particles into and within reaction systems. The reaction systems are those that use catalysts that comprise molecular sieves, particularly metalloaluminophosphate molecular sieves, especially metalloaluminophosphate molecular sieves which are susceptible to loss of catalytic activity due to contact with water molecules. The transfer methods provide appropriate mechanisms for transporting catalyst into and within a reactor to protect against loss of catalytic activity that can occur due to contact with water molecules.
摘要翻译： 本发明涉及将催化剂颗粒转移到反应体系内和在反应体系内的方法。 反应体系是使用包含分子筛的催化剂，特别是金属铝磷酸盐分子筛，特别是金属铝磷酸盐分子筛，它们由于与水分子接触而易于损失催化活性。 转移方法提供用于将催化剂输送到反应器内部和内部的适当机制，以防止由于与水分子接触而可能发生的催化活性的损失。
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