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    Method and apparatus for regenerating catalyst during oxygenates to olefins reaction
    3.
    发明授权
    Method and apparatus for regenerating catalyst during oxygenates to olefins reaction 有权
    在含氧化合物到烯烃反应过程中再生催化剂的方法和装置

    公开(公告)号：US08178741B2

    公开(公告)日：2012-05-15

    申请号：US12793340

    申请日：2010-06-03

    申请人： Chunshe J. Cao ,  James H. Beech, Jr. ,  Michael P. Nicoletti ,  Thomas H. Colle ,  Teng Xu ,  Stephen N. Vaughn

    发明人： Chunshe J. Cao ,  James H. Beech, Jr. ,  Michael P. Nicoletti ,  Thomas H. Colle ,  Teng Xu ,  Stephen N. Vaughn

    IPC分类号： C07C1/00 ,  B01J20/34 ,  B01J19/00

    CPC分类号： B01J38/02 ,  B01J29/90 ,  B01J38/32 ,  C07C1/20 ,  C07C2529/85 ,  Y02P20/584 ,  C07C11/02

    摘要： Disclosed herein is a method of recovery of the activity of a molecular sieve catalyst following use of the catalyst in an OTO conversion process. This is achieved by a regeneration apparatus and a method of regenerating a molecular sieve catalyst, comprising two stages. In a pretreatment stage, the catalyst is pretreated under pretreatment conditions by heating the catalyst to a temperature of between 320° C. to 700° C. in an oxygen depleted medium for a residence time of between 1 minute to two hours; and, in a regeneration stage, the catalyst is regenerated under regeneration conditions by heating the catalyst at a temperature of between 200° C. to 700° C. in an oxidizing medium for a residence time of between 1 to 60 minutes.

    摘要翻译： 本文公开了在OTO转化方法中使用催化剂后回收分子筛催化剂的活性的方法。 这是通过再生装置和再生分子筛催化剂的方法实现的，包括两个阶段。 在预处理阶段，催化剂在预处理条件下通过将催化剂在耗氧贫乏的介质中在320℃至700℃之间的温度下进行预处理，停留时间为1分钟至2小时; 并且在再生阶段，催化剂在再生条件下通过在氧化介质中在200℃至700℃的温度下加热催化剂，停留时间为1至60分钟而再生。

    Method And Apparatus For Regenerating Catalyst During Oxygenates To Olefins Reaction
    4.
    发明申请
    Method And Apparatus For Regenerating Catalyst During Oxygenates To Olefins Reaction 有权
    氧化催化剂再生催化剂对烯烃反应的方法与装置

    公开(公告)号：US20110021857A1

    公开(公告)日：2011-01-27

    申请号：US12793340

    申请日：2010-06-03

    申请人： Chunshe J. Cao ,  James H. Beech, JR. ,  Michael P. Nicoletti ,  Thomas H. Colle ,  Teng Xu ,  Stephen N. Vaughn

    发明人： Chunshe J. Cao ,  James H. Beech, JR. ,  Michael P. Nicoletti ,  Thomas H. Colle ,  Teng Xu ,  Stephen N. Vaughn

    IPC分类号： C07C1/00 ,  B01J20/34 ,  B01J19/00

    CPC分类号： B01J38/02 ,  B01J29/90 ,  B01J38/32 ,  C07C1/20 ,  C07C2529/85 ,  Y02P20/584 ,  C07C11/02

    摘要： Disclosed herein is a method of recovery of the activity of a molecular sieve catalyst following use of the catalyst in an OTO conversion process. This is achieved by a regeneration apparatus and a method of regenerating a molecular sieve catalyst, comprising two stages. In a pretreatment stage, the catalyst is pretreated under pretreatment conditions by heating the catalyst to a temperature of between 320° C. to 700° C. in an oxygen depleted medium for a residence time of between 1 minute to two hours; and, in a regeneration stage, the catalyst is regenerated under regeneration conditions by heating the catalyst at a temperature of between 200° C. to 700° C. in an oxidizing medium for a residence time of between 1 to 60 minutes.

    摘要翻译： 本文公开了在OTO转化方法中使用催化剂后回收分子筛催化剂的活性的方法。 这是通过再生装置和再生分子筛催化剂的方法实现的，包括两个阶段。 在预处理阶段，催化剂在预处理条件下通过将催化剂在耗氧贫乏的介质中在320℃至700℃之间的温度下进行预处理，停留时间为1分钟至2小时; 并且在再生阶段，催化剂在再生条件下通过在氧化介质中在200℃至700℃的温度下加热催化剂，停留时间为1至60分钟而再生。

    Oxygenate to olefin process
    9.
    发明授权
    Oxygenate to olefin process 有权
    氧化烯到烯烃工艺

    公开(公告)号：US06965057B2

    公开(公告)日：2005-11-15

    申请号：US10807818

    申请日：2004-03-24

    申请人： James H. Beech, Jr. ,  Cor F. Van Egmond ,  Teng Xu ,  James R. Lattner

    发明人： James H. Beech, Jr. ,  Cor F. Van Egmond ,  Teng Xu ,  James R. Lattner

    IPC分类号： B01J20/34 ,  B01J38/30 ,  B01J38/32 ,  C07C1/00 ,  C07C1/20 ,  C07C1/207 ,  C10G3/00

    CPC分类号： C07C1/20 ,  B01J38/30 ,  B01J38/32 ,  C10G3/49 ,  C10G3/62 ,  C10G2300/4093 ,  C10G2300/708 ,  C10G2300/802 ,  C10G2300/805 ,  C10G2400/20 ,  Y02P20/584 ,  Y02P30/42 ,  C07C11/02

    摘要： The invention relates to a process for converting an oxygenate feedstock into an olefin product stream comprising (a) contacting an oxygenate feedstock with a molecular sieve catalyst in a reactor under conditions effective to convert the feedstock into an olefin product stream and to form carbonaceous deposits on the catalyst; (b) contacting at least a portion of the catalyst having said carbonaceous deposits with an oxygen containing gas under conditions effective to obtain a regenerated catalyst having a reduced carbonaceous deposit level and having an increased molecular oxygen content; (c) removing at least 60% by volume of said molecular oxygen from the regenerated catalyst based upon the total volume of molecular oxygen; (d) returning said regenerated catalyst to said reactor; and (e) repeating steps (a)–(d).

    摘要翻译： 本发明涉及一种将含氧化合物原料转化成烯烃产物流的方法，该方法包括（a）在有效将原料转化成烯烃产物流并形成碳质沉积物的条件下，使反应器中的含氧化合物原料与分子筛催化剂接触 催化剂; （b）在有效获得具有降低的碳沉积物水平并且具有增加的分子氧含量的再生催化剂的条件下使至少一部分具有所述碳质沉积物的催化剂与含氧气体接触; （c）基于分子氧的总体积从再生催化剂中除去至少60体积％的所述分子氧; （d）将所述再生催化剂返回到所述反应器; 和（e）重复步骤（a） - （d）。