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    Solid crosslinked-polymer electrolyte and use thereof
    1.
    发明授权
    Solid crosslinked-polymer electrolyte and use thereof 有权
    固体交联聚合物电解质及其用途

    公开(公告)号：US06677084B1

    公开(公告)日：2004-01-13

    申请号：US09719637

    申请日：2000-12-15

    申请人： Shouhei Matsui ,  Katsuhito Miura ,  Masato Tabuchi ,  Hiroki Higobashi

    发明人： Shouhei Matsui ,  Katsuhito Miura ,  Masato Tabuchi ,  Hiroki Higobashi

    IPC分类号： H01M1040

    CPC分类号： C08J5/20 ,  C08G65/22 ,  C08L71/02 ,  H01B1/122 ,  H01M6/181 ,  H01M10/052 ,  H01M10/054 ,  H01M10/0565 ,  H01M2300/0082 ,  C08L2666/14

    摘要： A solid polymer electrolyte containing (I) a crosslinked material obtainable by crosslinking a composition containing (i) a polyether copolymer having a weight-average molecular weight within a range from 105 to 107 and having 5 to 95 mol % of repeating unit derived from a glycidyl compound, and 95 to 5 mol % of repeating unit derived from ethylene oxide, (ii) a crosslinking agent selected from organic peroxides and azo compounds, and (iii) a crosslinking aid which is an organic compound having a carbon-carbon double bond and an imide group, (II) an electrolyte salt compound, and (III) a plasticizer, is excellent in mechanical properties and ionic conductivity.

    摘要翻译： 一种固体聚合物电解质，其含有（I）交联材料，该交联材料可通过使包含（i）重均分子量在10 5至10 7的范围内且具有5至95摩尔％ 的衍生自缩水甘油基化合物的重复单元和95〜5摩尔％的来自环氧乙烷的重复单元，（ii）选自有机过氧化物和偶氮化合物的交联剂，和（iii）交联助剂，其是具有 碳双键和酰亚胺基，（II）电解质盐化合物和（III）增塑剂，其机械性能和离子导电性优异。

    Crosslinked polymer electrolyte and use thereof
    3.
    发明授权
    Crosslinked polymer electrolyte and use thereof 有权
    交联聚合物电解质及其用途

    公开(公告)号：US08026007B2

    公开(公告)日：2011-09-27

    申请号：US10561038

    申请日：2004-06-17

    申请人： Katsuhito Miura ,  Masato Tabuchi ,  Shouhei Matsui ,  Yoshihiko Wada

    发明人： Katsuhito Miura ,  Masato Tabuchi ,  Shouhei Matsui ,  Yoshihiko Wada

    IPC分类号： H01M6/18

    CPC分类号： H01M10/0567 ,  C08G65/14 ,  C08L2205/05 ,  H01B1/122 ,  H01M6/164 ,  H01M6/168 ,  H01M6/181 ,  H01M10/052 ,  H01M10/0565 ,  H01M10/0569

    摘要： A polymer electrolyte composition characterized by comprising: (1) a crosslinked material of a polyether binary copolymer which has a main chain comprising repeating units represented by the formula (i) and crosslinking units represented by the formula (ii) and which has a weight-average molecular weight of 104 to 107, (2) an electrolyte solution comprising an aprotic organic solvent, (3) an additive, as an optical ingredient, which comprises an ether compound having an ethylene oxide unit, and (4) an electrolyte salt compound comprising a lithium salt compound. The composition is excellent in liquid retention and ionic conductivity, is usable in a wide temperature range, and has excellent electrochemical properties.

    摘要翻译： 一种聚合物电解质组合物，其特征在于包括：（1）聚醚二元共聚物的交联材料，其具有主链，其包含由式（i）表示的重复单元和由式（ⅱ）表示的交联单元， 平均分子量为104至107，（2）包含非质子有机溶剂的电解质溶液，（3）作为光学成分的添加剂，其包含具有环氧乙烷单元的醚化合物，和（4）电解质盐化合物 包含锂盐化合物。 该组合物的液体保留性和离子传导性优异，可在宽的温度范围内使用，并且具有优异的电化学性能。

    Crosslinked polymer electrolyte and use thereof
    4.
    发明申请
    Crosslinked polymer electrolyte and use thereof 有权
    交联聚合物电解质及其用途

    公开(公告)号：US20070099089A1

    公开(公告)日：2007-05-03

    申请号：US10561038

    申请日：2004-06-17

    申请人： Katsuhito Miura ,  Masato Tabuchi ,  Shouhei Matsui ,  Yoshihiko Wada

    发明人： Katsuhito Miura ,  Masato Tabuchi ,  Shouhei Matsui ,  Yoshihiko Wada

    IPC分类号： H01M10/40 ,  H01G9/025

    CPC分类号： H01M10/0567 ,  C08G65/14 ,  C08L2205/05 ,  H01B1/122 ,  H01M6/164 ,  H01M6/168 ,  H01M6/181 ,  H01M10/052 ,  H01M10/0565 ,  H01M10/0569

    摘要： A polymer electrolyte composition characterized by comprising: (1) a crosslinked material of a polyether binary copolymer which has a main chain comprising repeating units represented by the formula (i) and crosslinking units represented by the formula (ii) and which has a weight-average molecular weight of 104 to 107, (2) an electrolyte solution comprising an aprotic organic solvent, (3) an additive, as an optical ingredient, which comprises an ether compound having an ethylene oxide unit, and (4) an electrolyte salt compound comprising a lithium salt compound. The composition is excellent in liquid retention and ionic conductivity, is usable in a wide temperature range, and has excellent electrochemical properties.

    摘要翻译： 一种聚合物电解质组合物，其特征在于包括：（1）聚醚二元共聚物的交联材料，其具有主链，其包含由式（i）表示的重复单元和由式（ⅱ）表示的交联单元， 平均分子量为10 4至1​​0 7，（2）包含非质子有机溶剂的电解质溶液，（3）作为光学成分的添加剂，其包含 具有环氧乙烷单元的醚化合物，和（4）包含锂盐化合物的电解质盐化合物。 该组合物的液体保留性和离子传导性优异，可在宽的温度范围内使用，并且具有优异的电化学性能。

    Polyether copolymer and solid polymer electrolyte
    5.
    发明授权
    Polyether copolymer and solid polymer electrolyte 失效
    聚醚共聚物和固体聚合物电解质

    公开(公告)号：US06180287B2

    公开(公告)日：2001-01-30

    申请号：US09101971

    申请日：1998-07-30

    申请人： Masayoshi Watanabe ,  Katsuhito Miura ,  Masanori Yanagida ,  Hiroki Higobashi ,  Takahiro Endo

    发明人： Masayoshi Watanabe ,  Katsuhito Miura ,  Masanori Yanagida ,  Hiroki Higobashi ,  Takahiro Endo

    IPC分类号： H01M618

    CPC分类号： H01G9/025 ,  C08G59/145 ,  C08G59/22 ,  C08G65/14 ,  C08G65/22 ,  C08G65/223 ,  C08G65/24 ,  C08K5/0008 ,  C08L71/02 ,  H01M6/181 ,  H01M10/052 ,  H01M10/0565 ,  C08L71/00

    摘要： A solid polymer electrolyte obtained by blending (1) a polyether copolymer having a main chain, which is derived form ethylene oxide, and a side chain having two oligooxyethylene groups, (2) an electrolyte salt compound, and, if necessary, (3) a plasticizer which is any one of an aprotic organic solvent or a derivative or metal salt of a polyalkylene glycol having a number-average molecular weight of 200 to 5,000 or a metal salt of the derivative, is superior in ionic conductivity and also superior in processability, moldability and mechanical strength to a conventional solid electrolyte. A secondary battery is constructed by using the solid polymer electrolyte in combination with a lithium metal negative electrode and a lithium cobaltate positive electrode.

    摘要翻译： 通过共混（1）具有来自环氧乙烷的主链的聚醚共聚物和具有两个低聚氧乙烯基的侧链，（2）电解质盐化合物，以及如果需要，（3） 作为数均分子量为200〜5000的聚亚烷基二醇的非质子性有机溶剂或衍生物或金属盐或该衍生物的金属盐中的任一种的增塑剂，离子导电性优异，加工性优异 ，成型性和机械强度。 通过使用固体聚合物电解质与锂金属负极和钴酸锂正极组合来构建二次电池。

    Polyether copolymer and polymer solid electrolyte
    6.
    发明授权
    Polyether copolymer and polymer solid electrolyte 失效
    聚醚共聚物和聚合物固体电解质

    公开(公告)号：US5968681A

    公开(公告)日：1999-10-19

    申请号：US958664

    申请日：1997-10-28

    申请人： Katsuhito Miura ,  Masanori Yanagida ,  Hiroki Higobashi ,  Takahiro Endo

    发明人： Katsuhito Miura ,  Masanori Yanagida ,  Hiroki Higobashi ,  Takahiro Endo

    IPC分类号： C08G65/14 ,  C08G65/22 ,  C08L71/02 ,  H01B1/12 ,  H01M6/18 ,  H01M6/00

    CPC分类号： H01M6/181 ,  C08G65/14 ,  C08G65/22 ,  C08L71/02 ,  H01B1/122

    摘要： A polyether copolymer prepared from 5 to 95% by mol of a monomer of the formula (I), 95 to 5% by mol of a monomer of the formula (II) and 0 to 15% by mol of a monomer of the formula (III) or (IV) as a crosslinking component; the copolymer having a weight-average molecular weight within the range from 10.sup.3 to 10.sup.7 : ##STR1## The copolymer of the present invention provides a polymer solid electrolyte having such a feature that it is superior in ionic conductivity and also superior in processability, moldability, mechanical strength and flexibility to a conventional solid electrolyte.

    摘要翻译： 将由式（I）的单体为5〜95摩尔％，式（II）的单体为95〜5摩尔％和式（II）的单体为0〜15摩尔％的单体制备的聚醚共聚物， III）或（IV）作为交联组分; 该共聚物的重均分子量在103〜107的范围内。本发明的共聚物提供了具有离子导电性优异，加工性，成型性，机械强度优异的特征的高分子固体电解质， 对常规固体电解质的灵活性。

    Polyether copolymer, solid polymer electrolyte and battery
    9.
    发明授权
    Polyether copolymer, solid polymer electrolyte and battery 失效
    聚醚共聚物，固体聚合物电解质和电池

    公开(公告)号：US06201071B1

    公开(公告)日：2001-03-13

    申请号：US09242880

    申请日：1999-04-19

    申请人： Katsuhito Miura ,  Masanori Yanagida ,  Kazumasa Hinoue ,  Yoshiro Furukawa

    发明人： Katsuhito Miura ,  Masanori Yanagida ,  Kazumasa Hinoue ,  Yoshiro Furukawa

    IPC分类号： C08G6391

    CPC分类号： H01M10/052 ,  C08G65/22 ,  H01M6/181 ,  H01M10/0565

    摘要： A solid polymer electrolyte containing a polyether copolymer having a weight-average molecular weight of 104 to 107 which may optionally be cross-linked and which contains (A) 1 to 99% by mol of a repeating unit derived from a monomer represented by the formula (I):  wherein R1 represents a divalent organic group, (B) 99 to 1% by mol of a repeating unit derived from ethylene oxide, and (C) 0 to 15% by mol of a repeating unit derived from a monomer having one epoxy group and at least one reactive functional group, an electrolyte salt compound, and a plasticizer has an excellent ionic conductivity.

    摘要翻译： 一种含有重均分子量为104〜107的聚醚共聚物的固体聚合物电解质，其可以任选地交联，并且含有（A）1至99摩尔％的由式 （I）表示：其中，R1表示二价有机基团，（B）99〜1摩尔％来源于环氧乙烷的重复单元，（C）0〜15摩尔％ 环氧基和至少一个反应性官能团，电解质盐化合物和增塑剂具有优异的离子导电性。

    Polyether polymer or copolymer, monomer therefor, and process for production thereof
    10.
    发明授权
    Polyether polymer or copolymer, monomer therefor, and process for production thereof 失效
    聚醚聚合物或共聚物，其单体及其生产方法

    公开(公告)号：US4711950A

    公开(公告)日：1987-12-08

    申请号：US925270

    申请日：1986-10-31

    申请人： Katsuhito Miura ,  Tetsuya Nakata

    发明人： Katsuhito Miura ,  Tetsuya Nakata

    IPC分类号： C07D303/28 ,  C08G59/00 ,  C08G59/14 ,  C08G59/68 ,  C08G59/02 ,  C08G59/32

    CPC分类号： C08G59/00 ,  C07D303/28 ,  C08G59/145 ,  C08G59/68

    摘要： A polyether polymer or copolymer with a pendant group of the formula ##STR1## in its molecule, said polymer or copolymer consisting essentially of (1) 1 to 100 mole % of recurring units represented by the following formula (I) ##STR2## and (2) 0 to 99 mole % of at least one type of recurring units represented by the following formula (II) ##STR3## and having a reduced viscosity .eta..sub.red, determined at 45.degree. C. in its 0.1% benzene solution or at 80.degree. C. in its 0.1% monochlorobenzene solution, of at least 0.01; a process for producing thereof and novel epoxyether compound therefor.

    摘要翻译： 在其分子中具有式“IMAGE”侧基的聚醚聚合物或共聚物，所述聚合物或共聚物基本上由（1）1至100摩尔％的由下式（I）表示的重复单元组成。 ）和（2）0至99摩尔％的由下式（II）表示的至少一种类型的重复单元（II），并且具有降低的粘度等级，在45℃下测定其0.1％ 苯溶液或在其0.1％一氯苯溶液中的80℃下为至少0.01; 其制备方法和新型环氧醚化合物。