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    Catalyst carrier and a process for preparing the catalyst carrier
    1.
    发明申请
    Catalyst carrier and a process for preparing the catalyst carrier 有权
    催化剂载体和制备催化剂载体的方法

    公开(公告)号：US20060281631A1

    公开(公告)日：2006-12-14

    申请号：US11449019

    申请日：2006-06-06

    申请人： William Gerdes ,  Thomas Szymanski ,  Donald Remus ,  John Lockemeyer ,  Randall Yeates

    发明人： William Gerdes ,  Thomas Szymanski ,  Donald Remus ,  John Lockemeyer ,  Randall Yeates

    IPC分类号： B01J21/12

    CPC分类号： B01J21/04 ,  B01J21/12 ,  B01J23/50 ,  B01J23/66 ,  B01J23/688 ,  B01J35/023 ,  B01J35/10 ,  B01J35/1009 ,  B01J35/1038 ,  B01J35/1071 ,  B01J35/108 ,  B01J37/0009 ,  B01J37/0018 ,  B01J37/0072

    摘要： A carrier, which comprises non-platelet alumina and/or a bond material, has a surface area of at least 1.3 m2/g, a total pore volume and a pore size distribution such that at least 80% of the total pore volume is contained in pores with diameters in the range of from 0.1 to 10 μm, and at least 80% of the pore volume contained in the pores with diameters in the range of from 0.1 to 10 μm is contained in pores with diameters in the range of from 0.3 to 10 μm, and a process for the preparation of a carrier which comprises forming a mixture comprising: a) from 50 to 95 weight percent of a first particulate α-alumina having a median particle size (d50) of from 5 to 100 μm; b) from 5 to 50 weight percent of a second particulate α-alumina having a d50 which is less than the d50 of the first particulate α-alumina and which is in the range of from 1 to 10 μm; and c) an alkaline earth metal silicate bond material; weight percent being based on the total weight of α-alumina in the mixture; and firing the mixture to form the carrier.

    摘要翻译： 包括非血小板氧化铝和/或粘合材料的载体具有至少1.3m 2 / g的表面积，总孔体积和孔径分布，使得至少80 总细孔容积的百分比包含在直径在0.1-10μm范围内的孔中，并且包含在直径在0.1-10μm范围内的孔中的孔体积的至少80％包含在孔中 直径在0.3-10μm范围内，以及一种制备载体的方法，该方法包括形成混合物，该混合物包含：a）50至95重量％的中等颗粒尺寸（d 5〜100μm的50％ b）5至50重量％的第二颗粒α-氧化铝，其具有小于第一颗粒α-氧化铝的d 50 O 3，其为 范围从1到10 mum; 和c）碱土金属硅酸盐粘合材料; 重量百分比基于混合物中α-氧化铝的总重量; 并且将混合物烧制以形成载体。

    CATALYST AND PROCESS USING THE CATALYST
    2.
    发明申请
    CATALYST AND PROCESS USING THE CATALYST 审中-公开
    催化剂和使用催化剂的方法

    公开(公告)号：US20070184973A1

    公开(公告)日：2007-08-09

    申请号：US11734516

    申请日：2007-04-12

    申请人： John LOCKEMEYER ,  Randall Yeates ,  Thomas Szymanski ,  Donald Remus ,  William Gerdes

    发明人： John LOCKEMEYER ,  Randall Yeates ,  Thomas Szymanski ,  Donald Remus ,  William Gerdes

    IPC分类号： B01J27/24 ,  B01J27/25 ,  B01J21/02 ,  B01J27/00 ,  B01J27/198 ,  B01J27/188 ,  B01J27/06 ,  B01J23/50

    CPC分类号： B01J23/50 ,  B01J21/04 ,  B01J21/12 ,  B01J23/66 ,  B01J23/688 ,  B01J35/10 ,  B01J35/1009 ,  B01J35/1038 ,  B01J35/1042 ,  B01J35/108 ,  B01J37/0018 ,  B01J37/0201 ,  C07C29/106 ,  C07C213/04 ,  C07D301/10 ,  C07C31/20

    摘要： A catalyst which comprises a carrier and silver deposited on the carrier, which carrier has a surface area of at least 1 m2/g, and a pore size distribution such that pores with diameters in the range of from 0.2 to 10 μm represent at least 70% of the total pore volume and such pores together provide a pore volume of at least 0.27 ml/g, relative to the weight of the carrier; a process for the preparation of a catalyst which process comprises depositing silver on a carrier, wherein the carrier has been obtained by a method which comprises forming a mixture comprising: a) from 50 to 90% w of a first particulate α-alumina having an average particle size (d50) of from more than 10 up to 100 μm; and b) from 10 to 50% w of a second particulate α-alumina having an average particle size (d50) of from 1 to 10 μm; % w being based on the total weight of α-alumina in the mixture; and shaping the mixture into formed bodies and firing the formed bodies to form the carrier, and a process for the epoxidation of an olefin, which process comprises reacting an olefin with oxygen in the presence of a said catalyst.

    摘要翻译： 一种催化剂，其包含沉积在载体上的载体和银，该载体具有至少1m 2 / g的表面积，并且孔径分布使得孔直径在 0.2至10um表示总孔体积的至少70％，并且这些孔一起相对于载体的重量提供至少0.27ml / g的孔体积; 一种制备催化剂的方法，该方法包括在载体上沉积银，其中载体已经通过包括形成混合物的方法获得，所述方法包括：a）50-90％w的第一颗粒α-氧化铝，其具有 大于10至100μm的平均粒度（d <50％）; 和b）10至50％w的平均粒度（d <50％）为1-10μm的第二颗粒状α-氧化铝; ％w基于混合物中α-氧化铝的总重量; 并将混合物成型为成形体并焙烧成形体以形成载体，以及烯烃环氧化方法，该方法包括在所述催化剂存在下使烯烃与氧气反应。

    Process for the production of an olefin oxide, a 1,2-diol, a 1,2-diol ether, or an alkanolamine
    6.
    发明申请
    Process for the production of an olefin oxide, a 1,2-diol, a 1,2-diol ether, or an alkanolamine 有权

    公开(公告)号：US20060009647A1

    公开(公告)日：2006-01-12

    申请号：US11154143

    申请日：2005-06-16

    申请人： Randall Yeates ,  Leonid Rubinstein

    发明人： Randall Yeates ,  Leonid Rubinstein

    IPC分类号： C07D301/10

    CPC分类号： C07D301/10

    摘要： A process is provided for the epoxidation of an olefin comprising the steps of: contacting a feed comprising an olefin and oxygen with a catalyst comprising a silver component deposited on a fluoride-mineralized carrier; and producing a product mix comprising an olefin oxide, wherein the partial pressure of olefin oxide in the product mix is greater than about 60 kPa. A process is provided for the epoxidation of an olefin comprising the steps of: contacting a feed comprising an olefin and oxygen with a catalyst comprising a silver component and a high-selectivity dopant deposited on a fluoride-mineralized carrier; and producing a product mix comprising an olefin oxide, wherein the partial pressure of olefin oxide in the product mix is greater than about 20 kPa.