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公开(公告)号：US20230227741A1
公开(公告)日：2023-07-20
申请号：US18175798
申请日：2023-02-28
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
IPC分类号： C10J3/48 , C10J3/46 , C10K1/00 , C10K3/00 , C10G2/00 , C10K1/10 , C10K1/12 , C10K1/08 , C10K1/16 , C01B3/12 , C10K3/02 , C10K3/04
CPC分类号： C10J3/48 , C01B3/12 , C10G2/30 , C10J3/463 , C10K1/003 , C10K1/004 , C10K1/12 , C10K1/16 , C10K1/085 , C10K1/102 , C10K3/04 , C10K3/005 , C10K3/026 , C10J2300/092 , C10J2300/0909 , C10J2300/0946 , C10J2300/0976 , C10J2300/1612 , C10J2300/1659 , C10J2300/1687 , C10J2300/1838 , C10J2300/1892
摘要： A process for the manufacture of a useful product from carbonaceous feedstock of fluctuating compositional characteristics, the process comprising the steps of: continuously providing the carbonaceous feedstock of fluctuating compositional characteristics to a gasification zone; gasifying the carbonaceous feedstock in the gasification zone to obtain raw synthesis gas; sequentially removing ammoniacal, sulphurous and carbon dioxide impurities from the raw synthesis gas to form desulphurised gas and recovering carbon dioxide in substantially pure form; converting at least a portion of the desulphurised synthesis gas to a useful product. Despite having selected a more energy intensive sub-process i.e. physical absorption for removal of acid gas impurities, the overall power requirement of the facility is lower on account of lower steam requirements and thereby leading to a decrease in the carbon intensity score for the facility.
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公开(公告)号：US11578281B2
公开(公告)日：2023-02-14
申请号：US17203706
申请日：2021-03-16
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu , Ashish Gupta
摘要： A process for the manufacture of a useful product from carbonaceous feedstock of fluctuating compositional characteristics, comprising the steps of: continuously providing the carbonaceous feedstock of fluctuating compositional characteristics to a gasification zone; gasifying the carbonaceous feedstock in the gasification zone to obtain raw synthesis gas; recovering at least part of the raw synthesis gas from the gasification zone and supplying at least part of the recovered raw synthesis gas to a partial oxidation zone; equilibrating the H2:CO ratio of the raw synthesis gas in the partial oxidation zone to obtain equilibrated synthesis gas; recovering at least part of the equilibrated synthesis gas from the partial oxidation zone and treating the gas to remove impurities and generate a fine synthesis gas; and converting the optionally adjusted fine synthesis gas into the useful product in a further chemical reaction requiring a usage ratio.
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公开(公告)号：US20230392090A1
公开(公告)日：2023-12-07
申请号：US18249843
申请日：2021-10-21
CPC分类号： C10K3/005 , C10J2300/1846 , C10G2/30 , C10J3/84 , C10K1/004 , C10K1/005 , C10K3/006 , C01B2203/0233 , C01B2203/0244 , C01B2203/025 , C01B2203/0415 , C01B2203/0485 , C01B2203/049 , C01B2203/0495 , C01B2203/061 , C01B2203/062 , C01B2203/068 , C01B2203/1058 , C01B2203/1223 , C01B2203/141 , C01B2203/1241 , C01B2203/127 , C10G2400/08 , C10G2400/04 , C10J2300/092 , C10J2300/0946 , C10J2300/0959 , C10J2300/0976 , C10J2300/1618 , C10J2300/1659 , C10J2300/1665 , C10J2300/1668 , C10J2300/1838 , C01B3/38
摘要： The present invention provides a process for the manufacture of a useful product from synthesis gas having a desired hydrogen to carbon monoxide molar ratio comprising: gasifying a first carbonaceous feedstock comprising waste materials and/or biomass in a gasification zone to produce a first synthesis gas; optionally partially oxidising the first synthesis gas in a partial oxidation zone to generate oxidised synthesis gas; reforming a second carbonaceous feedstock to produce a second synthesis gas, the second synthesis gas having a different hydrogen to carbon ratio from that of the first raw synthesis gas; combining at least a portion of the first synthesis gas and at least a portion of the second synthesis gas in an amount to achieve the desired hydrogen to carbon molar ratio and to generate a combined synthesis gas and subjecting at least part of the combined synthesis gas to a conversion process effective to produce the useful product. The reforming step enables the conventional water gas shift reaction to be dispensed with.
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公开(公告)号：US11618860B2
公开(公告)日：2023-04-04
申请号：US17224744
申请日：2021-04-07
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
摘要： The present invention provides a process for the manufacture of a useful product from carbonaceous feedstock of fluctuating compositional characteristics, the process comprising the steps of: continuously providing the carbonaceous feedstock of fluctuating compositional characteristics to a gasification zone; gasifying the carbonaceous feedstock in the gasification zone to obtain raw synthesis gas; sequentially removing ammoniacal, sulphurous and carbon dioxide impurities from the raw synthesis gas to form desulphurised gas and recovering carbon dioxide in substantially pure form; converting at least a portion of the desulphurised synthesis gas to a useful product. Despite having selected a more energy intensive sub-process i.e. physical absorption for removal of acid gas impurities, the overall power requirement of the facility is lower on account of lower steam requirements and thereby leading to a decrease in the carbon intensity score for the facility.
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公开(公告)号：US12116538B2
公开(公告)日：2024-10-15
申请号：US17318328
申请日：2021-05-12
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
CPC分类号： C10J3/86 , C01B3/36 , C01B3/48 , C10J3/463 , C10J3/60 , C10J3/721 , C10J3/723 , C10J3/82 , C10J2300/0909 , C10J2300/0916 , C10J2300/0946 , C10J2300/1215 , C10J2300/1606 , C10J2300/1612 , C10J2300/1643 , C10J2300/1659 , C10J2300/1687 , C10J2300/1807 , C10J2300/1846 , C10J2300/1853
摘要： A process for the manufacture of one or more useful products comprises: gasifying a carbonaceous feedstock comprising waste materials and/or biomass in a gasification zone to generate a raw synthesis gas; supplying at least a portion of the raw synthesis gas to a clean-up zone to remove contaminants and provide a clean synthesis gas; supplying the clean synthesis gas to a first further reaction train to generate at least one first useful product and a tailgas; and diverting selectively on demand a portion of at least one of the carbonaceous feedstock, the clean synthesis gas, the tailgas and the light gas fraction to heat or power generation within the process, in response to external factors to control the carbon intensity of the overall process and enable GHG emission savings.
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公开(公告)号：US20210317375A1
公开(公告)日：2021-10-14
申请号：US17224744
申请日：2021-04-07
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
摘要： The present invention provides a process for the manufacture of a useful product from carbonaceous feedstock of fluctuating compositional characteristics, the process comprising the steps of: continuously providing the carbonaceous feedstock of fluctuating compositional characteristics to a gasification zone; gasifying the carbonaceous feedstock in the gasification zone to obtain raw synthesis gas; sequentially removing ammoniacal, sulphurous and carbon dioxide impurities from the raw synthesis gas to form desulphurised gas and recovering carbon dioxide in substantially pure form; converting at least a portion of the desulphurised synthesis gas to a useful product. Despite having selected a more energy intensive sub-process i.e. physical absorption for removal of acid gas impurities, the overall power requirement of the facility is lower on account of lower steam requirements and thereby leading to a decrease in the carbon intensity score for the facility.
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公开(公告)号：US11905478B2
公开(公告)日：2024-02-20
申请号：US18175798
申请日：2023-02-28
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
IPC分类号： C10K1/00 , C01B32/50 , C01B3/56 , C10G2/00 , C10G65/12 , C10K1/10 , C10K1/32 , C10K3/04 , C10G1/00 , C10J3/00 , C10K1/08 , C10K3/00 , C01B3/12 , C10J3/46 , C10J3/48 , C10K1/12 , C10K1/16 , C10K3/02
CPC分类号： C10K1/004 , C01B3/12 , C01B3/56 , C01B32/50 , C10G1/002 , C10G2/30 , C10G65/12 , C10J3/00 , C10J3/463 , C10J3/48 , C10K1/002 , C10K1/003 , C10K1/005 , C10K1/08 , C10K1/085 , C10K1/10 , C10K1/102 , C10K1/12 , C10K1/16 , C10K1/32 , C10K3/005 , C10K3/026 , C10K3/04 , C01B2203/0283 , C01B2203/0425 , C01B2203/0485 , C01B2203/062 , C01B2203/0894 , C01B2203/1211 , C01B2203/146 , C01B2203/148 , C01B2203/86 , C10G2300/1003 , C10G2300/1014 , C10G2300/1022 , C10G2300/405 , C10G2400/04 , C10G2400/08 , C10J2300/092 , C10J2300/0909 , C10J2300/0946 , C10J2300/0976 , C10J2300/1612 , C10J2300/1659 , C10J2300/1687 , C10J2300/1838 , C10J2300/1892
摘要： A process for the manufacture of a useful product from carbonaceous feedstock of fluctuating compositional characteristics, the process comprising the steps of: continuously providing the carbonaceous feedstock of fluctuating compositional characteristics to a gasification zone; gasifying the carbonaceous feedstock in the gasification zone to obtain raw synthesis gas; sequentially removing ammoniacal, sulphurous and carbon dioxide impurities from the raw synthesis gas to form desulphurised gas and recovering carbon dioxide in substantially pure form; converting at least a portion of the desulphurised synthesis gas to a useful product. Despite having selected a more energy intensive sub-process i.e. physical absorption for removal of acid gas impurities, the overall power requirement of the facility is lower on account of lower steam requirements and thereby leading to a decrease in the carbon intensity score for the facility.
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公开(公告)号：US11834614B2
公开(公告)日：2023-12-05
申请号：US17506240
申请日：2021-10-20
CPC分类号： C10G2/30 , C01B3/40 , C10J3/00 , C10K1/004 , C10K1/005 , C01B2203/0233 , C01B2203/0244 , C01B2203/061 , C01B2203/062 , C01B2203/068 , C01B2203/1058 , C01B2203/1223 , C01B2203/1229 , C01B2203/1241 , C10G2400/04 , C10G2400/08 , C10J2300/092 , C10J2300/0946 , C10J2300/1618 , C10J2300/1659 , C10J2300/1665 , C10J2300/1668 , C10J2300/1846
摘要： A process for the manufacture of a useful product from synthesis gas having a desired hydrogen to carbon monoxide molar ratio comprises gasifying a first carbonaceous feedstock comprising waste materials and/or biomass in a gasification zone to produce a first synthesis gas; optionally partially oxidising the first synthesis gas in a partial oxidation zone to generate oxidised synthesis gas; reforming a second carbonaceous feedstock to produce a second synthesis gas, the second synthesis gas having a different hydrogen to carbon ratio from that of the first raw synthesis gas; combining at least a portion of the first synthesis gas and at least a portion of the second synthesis gas in an amount to achieve the desired hydrogen to carbon molar ratio and to generate a combined synthesis gas and subjecting at least part of the combined synthesis gas to a conversion process effective to produce the useful product.
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公开(公告)号：US20210355392A1
公开(公告)日：2021-11-18
申请号：US17318328
申请日：2021-05-12
发明人： Ivan Philip Greager , Roger Allen Harris , Neil Alexander King , Soumitra R. Deshmukh , Zheyan Qiu
摘要： A process for the manufacture of one or more useful products comprises: gasifying a carbonaceous feedstock comprising waste materials and/or biomass in a gasification zone to generate a raw synthesis gas; supplying at least a portion of the raw synthesis gas to a clean-up zone to remove contaminants and provide a clean synthesis gas; supplying the clean synthesis gas to a first further reaction train to generate at least one first useful product and a tailgas; and diverting selectively on demand a portion of at least one of the carbonaceous feedstock, the clean synthesis gas, the tailgas and the light gas fraction to heat or power generation within the process, in response to external factors to control the carbon intensity of the overall process and enable GHG emission savings.
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公开(公告)号：US11173483B2
公开(公告)日：2021-11-16
申请号：US16892490
申请日：2020-06-04
摘要： A catalyst is regenerated by an inventive process using a heat exchange fluid such as superheated steam to remove heat during the process relying on efficient heat transfer (e.g., enabled by the microchannel reactor construction) in comparison with prior art heat exchange relying on a phase change, e.g. between water and (partial or complete vaporization) steam, allows simplification of the protocols to enable transition at higher temperatures between steps which translates in reduced duration of the regeneration process and avoids potential water hammering risks.
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