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1.发明授权Transition metal complex compounds, olefin oligomerization catalysts including the compounds, and processes for producing olefin oligomers using the catalysts 有权过渡金属络合物，包括该化合物的烯烃低聚催化剂，以及使用该催化剂生产烯烃低聚物的方法公开(公告)号：US08258361B2
公开(公告)日：2012-09-04
申请号：US12452438
申请日：2008-06-27
申请人： Yasuhiko Suzuki , Shinsuke Kinoshita , Atsushi Shibahara , Naritoshi Yoshimura , Isao Hara , Tetsuya Hamada , Kazumori Kawamura , Kou Tsurugi , Yasunori Saito , Seiichi Ishii , Yasushi Nakayama , Naoto Matsukawa , Susumu Murata
发明人： Yasuhiko Suzuki , Shinsuke Kinoshita , Atsushi Shibahara , Naritoshi Yoshimura , Isao Hara , Tetsuya Hamada , Kazumori Kawamura , Kou Tsurugi , Yasunori Saito , Seiichi Ishii , Yasushi Nakayama , Naoto Matsukawa , Susumu Murata
CPC分类号： C08F10/00 , B01J31/143 , B01J31/1616 , B01J31/2243 , B01J2231/122 , B01J2231/20 , B01J2531/46 , B01J2531/62 , C07C2/32 , C07C251/24 , C07C2521/08 , C07C2521/16 , C07C2531/14 , C07C2531/22 , C07F7/003 , C08F110/02 , C07C11/107 , C08F4/64048 , C08F2500/02 , C08F4/64124 , C08F4/6931 , C08F4/64117 , C08F4/02
摘要： The invention provides transition metal complex compounds, high-activity olefin oligomerization catalysts containing the compounds, and olefin oligomerization processes using the catalysts.A transition metal complex compound [A] according to the invention is represented by Formula (I) or Formula (I′) below. An olefin oligomerization catalyst includes the transition metal complex compound [A]. In an olefin oligomerization process of the invention, an olefin is oligomerized in the presence of the catalyst.
摘要翻译： 本发明提供了过渡金属络合物，含有这些化合物的高活性烯烃低聚催化剂和使用该催化剂的烯烃低聚方法。 根据本发明的过渡金属络合物[A]由下式（I）或式（I'）表示。 烯烃低聚催化剂包括过渡金属络合物[A]。 在本发明的烯烃低聚方法中，烯烃在催化剂存在下被低聚。
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2.发明申请TRANSITION METAL COMPLEX COMPOUNDS, OLEFIN OLIGOMERIZATION CATALYSTS INCLUDING THE COMPOUNDS, AND PROCESSES FOR PRODUCING OLEFIN OLIGOMERS USING THE CATALYSTS 有权过渡金属复合化合物，包括该化合物的烯烃低聚催化剂，以及使用催化剂生产烯烃低聚物的方法公开(公告)号：US20110082325A1
公开(公告)日：2011-04-07
申请号：US12452438
申请日：2008-06-27
申请人： Yasuhiko Suzuki , Shinsuke Kinoshita , Atsushi Shibahara , Naritoshi Yoshimura , Isao Hara , Tetsuya Hamada , Kazumori Kawamura , Kou Tsurugi , Yasunori Saito , Seiichi Ishii , Yasushi Nakayama , Naoto Matsukawa , Susumu Murata
发明人： Yasuhiko Suzuki , Shinsuke Kinoshita , Atsushi Shibahara , Naritoshi Yoshimura , Isao Hara , Tetsuya Hamada , Kazumori Kawamura , Kou Tsurugi , Yasunori Saito , Seiichi Ishii , Yasushi Nakayama , Naoto Matsukawa , Susumu Murata
CPC分类号： C08F10/00 , B01J31/143 , B01J31/1616 , B01J31/2243 , B01J2231/122 , B01J2231/20 , B01J2531/46 , B01J2531/62 , C07C2/32 , C07C251/24 , C07C2521/08 , C07C2521/16 , C07C2531/14 , C07C2531/22 , C07F7/003 , C08F110/02 , C07C11/107 , C08F4/64048 , C08F2500/02 , C08F4/64124 , C08F4/6931 , C08F4/64117 , C08F4/02
摘要： The invention provides transition metal complex compounds, high-activity olefin oligomerization catalysts containing the compounds, and olefin oligomerization processes using the catalysts.A transition metal complex compound [A] according to the invention is represented by Formula (I) or Formula (I′) below. An olefin oligomerization catalyst includes the transition metal complex compound [A]. In an olefin oligomerization process of the invention, an olefin is oligomerized in the presence of the catalyst.
摘要翻译： 本发明提供了过渡金属络合物，含有这些化合物的高活性烯烃低聚催化剂和使用该催化剂的烯烃低聚方法。 根据本发明的过渡金属络合物[A]由下式（I）或式（I'）表示。 烯烃低聚催化剂包括过渡金属络合物[A]。 在本发明的烯烃低聚方法中，烯烃在催化剂存在下被低聚。
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3.发明授权Method for producing unsaturated carboxylic acid-modified vinyl alcohol polymer, and gas barrier film or gas barrier laminate using the same 有权不饱和羧酸改性乙烯醇聚合物的制造方法以及使用该乙烯醇聚合物的阻气性膜或阻气性层叠体公开(公告)号：US08809490B2
公开(公告)日：2014-08-19
申请号：US12302993
申请日：2007-05-31
申请人： Kou Tsurugi , Yoshihisa Inoue , Isao Hara , Hiroyoshi Watanabe , Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura
发明人： Kou Tsurugi , Yoshihisa Inoue , Isao Hara , Hiroyoshi Watanabe , Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura
摘要： A method for producing a solution containing at least an unsaturated carboxylic acid-modified vinyl alcohol polymer is characterized by reacting a vinyl alcohol polymer and an unsaturated carboxylic acid compound in the presence of an acid catalyst soluble in the reaction system or a solid acid catalyst, and a gas barrier film is obtained by using the same. An example thereof is a method for producing a solution (A) containing an unsaturated carboxylic acid-modified vinyl alcohol polymer (b), the method comprising following two steps of: (1) a reaction step in which the unsaturated carboxylic acid-modified vinyl alcohol polymer (b) is formed by reacting a vinyl alcohol polymer and an unsaturated carboxylic acid compound (a) in the presence of an acid catalyst soluble in the reaction system; and (2) an ion exchange step in which at least the acid catalyst of acidic compounds is removed by an anion exchange resin.
摘要翻译： 至少含有不饱和羧酸改性的乙烯醇聚合物的溶液的制造方法的特征在于，在可溶于反应体系的酸催化剂或固体酸催化剂的存在下使乙烯醇聚合物与不饱和羧酸化合物反应， 并且通过使用它们获得阻气膜。 其实例是制备含有不饱和羧酸改性的乙烯醇聚合物（b）的溶液（A）的方法，该方法包括以下两个步骤：（1）反应步骤，其中不饱和羧酸改性乙烯醇聚合物 醇聚合物（b）通过乙烯醇聚合物和不饱和羧酸化合物（a）在可溶于反应体系的酸催化剂存在下反应形成; 和（2）离子交换步骤，至少酸性化合物的酸催化剂通过阴离子交换树脂除去。
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4.发明申请METHOD FOR PRODUCING UNSATURATED CARBOXYLIC ACID-MODIFIED VINYL ALCOHOL POLYMER, AND GAS BARRIER FILM OR GAS BARRIER LAMINATE USING THE SAME 有权用于生产不饱和羧酸改性的乙烯醇聚合物的方法，以及使用其的气体阻隔膜或气体阻挡层压板公开(公告)号：US20090324836A1
公开(公告)日：2009-12-31
申请号：US12302993
申请日：2007-05-31
申请人： Kou Tsurugi , Yoshihisa Inoue , Isao Hara , Hiroyoshi Watanabe , Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura
发明人： Kou Tsurugi , Yoshihisa Inoue , Isao Hara , Hiroyoshi Watanabe , Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura
IPC分类号： B05D3/10 , C08F220/06 , C08K5/09
摘要： The present invention provides an industrially advantageous method for producing an unsaturated carboxylic acid-modified vinyl alcohol polymer, and a gas barrier film obtained by using the same. In summary of the present invention, the present invention is a method for producing a solution containing at least an unsaturated carboxylic acid-modified vinyl alcohol polymer characterized by reacting a vinyl alcohol polymer and an unsaturated carboxylic acid compound in the presence of an acid catalyst soluble in the reaction system or a solid acid catalyst, and a gas barrier film obtained by using the same, and an example of a representative constitution thereof is a method for producing a solution (A) containing an unsaturated carboxylic acid-modified vinyl alcohol polymer (b), the method comprising following two steps of: (1) a reaction step in which the unsaturated carboxylic acid-modified vinyl alcohol polymer (b) is formed by reacting a vinyl alcohol polymer and an unsaturated carboxylic acid compound (a) in the presence of an acid catalyst soluble in the reaction system; and (2) an ion exchange step in which at least the acid catalyst of acidic compounds is removed by an anion exchange resin.
摘要翻译： 本发明提供了用于制备不饱和羧酸改性的乙烯醇聚合物的工业上有利的方法，以及通过使用它们得到的阻气膜。 本发明概述本发明是一种生产含有至少不饱和羧酸改性的乙烯醇聚合物的溶液的方法，其特征在于在酸催化剂可溶的存在下使乙烯醇聚合物与不饱和羧酸化合物反应 在反应体系或固体酸催化剂中使用的气体阻隔膜，其代表性构成的实施例是含有不饱和羧酸改性乙烯醇系聚合物（A）的溶液（A）的制造方法， b），该方法包括以下两个步骤：（1）反应步骤，其中不饱和羧酸改性的乙烯醇聚合物（b）通过乙烯醇聚合物和不饱和羧酸化合物（a）在 存在可溶于反应体系的酸催化剂; 和（2）离子交换步骤，至少酸性化合物的酸催化剂通过阴离子交换树脂除去。
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5.发明授权Gas barrier film, gas barrier laminate and method for manufacturing film or laminate 有权气体阻隔膜，阻气性层压体以及薄膜或层压体的制造方法公开(公告)号：US08097345B2
公开(公告)日：2012-01-17
申请号：US12065395
申请日：2006-08-30
申请人： Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura , Yoshihisa Inoue , Kou Tsurugi , Nobuhiro Tanabe , Yoshihiro Yamamoto
发明人： Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura , Yoshihisa Inoue , Kou Tsurugi , Nobuhiro Tanabe , Yoshihiro Yamamoto
CPC分类号： C08F261/04 , B32B27/08 , C08L29/04 , C08L33/02 , C08L51/003 , C09D129/04 , C09D151/003 , Y10T428/31855 , C08L2666/04 , C08L2666/02
摘要： Disclosed is an excellent gas barrier laminate whose gas-barrier property has little dependency on temperature and which hardly causes fracture even when the laminate is stretched. A gas barrier film comprising a polymer (A) of an unsaturated carboxylic acid compound monovalent metal salt (a), wherein the polymer (A) contains a modified vinyl alcohol polymer (B); a gas barrier laminate comprising a base layer and the gas barrier film formed on at least one surface of the base layer; and a method for production of a gas barrier laminate comprising the steps of: coating a solution of an unsaturated carboxylic acid compound monovalent metal salt (a) having a polymerization degree less than 20 on at least one surface of a base layer, wherein the solution contains a modified vinyl alcohol polymer (B); performing the polymerization to form a layer of the polymer (A) of the unsaturated carboxylic acid compound monovalent metal salt (a) containing the modified vinyl alcohol polymer (B).
摘要翻译： 公开了一种优异的阻气性层压体，其气体阻隔性对温度几乎没有依赖性，即使在层叠体被拉伸时也难以引起断裂。 一种阻气膜，其包含不饱和羧酸化合物一价金属盐（a）的聚合物（A），其中所述聚合物（A）含有改性乙烯醇聚合物（B）; 阻气层压板，其包含形成在所述基层的至少一个表面上的基底层和所述阻气膜; 和阻气性层压体的制造方法，其特征在于，在基层的至少一个表面上涂布聚合度小于20的不饱和羧酸化合物一价金属盐（a）的溶液， 含有改性乙烯醇聚合物（B）; 进行聚合以形成含有改性乙烯醇聚合物（B）的不饱和羧酸化合物一价金属盐（a）的聚合物（A）的层。
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6.发明申请GAS BARRIER FILM, GAS BARRIER LAMINATE AND METHOD FOR MANUFACTURING FILM OR LAMINATE 有权气体阻隔膜，气体阻隔层压板及制造薄膜或层压体的方法公开(公告)号：US20090269592A1
公开(公告)日：2009-10-29
申请号：US12065395
申请日：2006-08-30
申请人： Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura , Yoshihisa Inoue , Kou Tsurugi , Nobuhiro Tanabe , Yoshihiro Yamamoto
发明人： Tomoyoshi Hakamata , Akira Nomoto , Osamu Nakamura , Yoshihisa Inoue , Kou Tsurugi , Nobuhiro Tanabe , Yoshihiro Yamamoto
CPC分类号： C08F261/04 , B32B27/08 , C08L29/04 , C08L33/02 , C08L51/003 , C09D129/04 , C09D151/003 , Y10T428/31855 , C08L2666/04 , C08L2666/02
摘要： Disclosed is an excellent gas barrier laminate whose gas-barrier property has little dependency on temperature and which hardly causes fracture even when the laminate is stretched. A gas barrier film comprising a polymer (A) of an unsaturated carboxylic acid compound monovalent metal salt (a), wherein the polymer (A) contains a modified vinyl alcohol polymer (B); a gas barrier laminate comprising a base layer and the gas barrier film formed on at least one surface of the base layer; and a method for production of a gas barrier laminate comprising the steps of: coating a solution of an unsaturated carboxylic acid compound monovalent metal salt (a) having a polymerization degree less than 20 on at least one surface of a base layer, wherein the solution contains a modified vinyl alcohol polymer (B); performing the polymerizaton to form a layer of the polymer (A) of the unsaturated carboxylic acid compound monovalent metal salt (a) containing the modified vinyl alcohol polymer (B).
摘要翻译： 公开了一种优异的阻气性层压体，其气体阻隔性对温度几乎没有依赖性，即使在层叠体被拉伸时也难以引起断裂。 一种阻气膜，其包含不饱和羧酸化合物一价金属盐（a）的聚合物（A），其中所述聚合物（A）含有改性乙烯醇聚合物（B）; 阻气层压板，其包含形成在所述基层的至少一个表面上的基底层和所述阻气膜; 和阻气性层压体的制造方法，其特征在于，在基层的至少一个表面上涂布聚合度小于20的不饱和羧酸化合物一价金属盐（a）的溶液， 含有改性乙烯醇聚合物（B）; 进行聚合以形成含有改性乙烯醇聚合物（B）的不饱和羧酸化合物一价金属盐（a）的聚合物（A）的层。
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