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    Palladium-containing catalyst and method for producing same
    5.
    发明授权
    Palladium-containing catalyst and method for producing same 有权
    含钯催化剂及其制造方法

    公开(公告)号：US07446223B2

    公开(公告)日：2008-11-04

    申请号：US11628214

    申请日：2005-06-02

    申请人： Wataru Ninomiya ,  Yoshiyuki Himeno ,  Yuji Fujimori

    发明人： Wataru Ninomiya ,  Yoshiyuki Himeno ,  Yuji Fujimori

    IPC分类号： C07C51/14 ,  C07C51/16 ,  C07C45/34

    CPC分类号： B01J37/0203 ,  B01J21/08 ,  B01J21/18 ,  B01J23/44 ,  B01J27/0576 ,  B01J37/0205 ,  B01J37/16 ,  C07C45/34 ,  C07C45/35 ,  C07C45/36 ,  C07C51/252 ,  C07C47/21 ,  C07C47/22 ,  C07C47/232 ,  C07C57/04

    摘要： The present invention provides: a palladium-containing catalyst which is used for highly selectively or highly productively producing an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an olefin or in that way producing an α,β-unsaturated carboxylic acid from an α,β-unsaturated aldehyde; a method for producing the catalyst; and a method for highly selectively or highly productively producing an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an olefin or in that way producing an α,β-unsaturated carboxylic acid from an α,β-unsaturated aldehyde. In particular, the present invention resides in a palladium-containing catalyst comprising 0.001 to 0.40 mole of tellurium metal to 1.0 mole of palladium metal. This catalyst can be preferably produced by a method having a step of reducing a compound containing palladium atom in its oxidized state and tellurium atom in its oxidized state by a reducing agent.

    摘要翻译： 本发明提供：一种含钯催化剂，其用于从烯烃高度选择性或高产率地生产α，β-不饱和醛和α，β-不饱和羧酸，或以这种方式产生α，β-不饱和的 羧酸从α，β-不饱和醛; 催化剂的制造方法; 以及用于从烯烃高度选择性地或高效地生产α，β-不饱和醛和α，β-不饱和羧酸的方法，或以这种方式从α，β-不饱和醛生产α，β-不饱和羧酸的方法 。 特别地，本发明涉及一种含钯催化剂，其包含0.001至0.40摩尔的碲金属至1.0摩尔的钯金属。 该催化剂可以优选通过还原剂还原含有氧化态的钯原子的化合物和其氧化态的碲原子的方法来制造。

    Palladium-Containing Catalyst and Method for Producing Same
    6.
    发明申请
    Palladium-Containing Catalyst and Method for Producing Same 有权
    含钯催化剂及其制造方法

    公开(公告)号：US20070238903A1

    公开(公告)日：2007-10-11

    申请号：US11628214

    申请日：2005-06-02

    申请人： Wataru Ninomiya ,  Yoshiyuki Himeno ,  Yuji Fujimori

    发明人： Wataru Ninomiya ,  Yoshiyuki Himeno ,  Yuji Fujimori

    IPC分类号： B01J23/44 ,  C07C409/00

    CPC分类号： B01J37/0203 ,  B01J21/08 ,  B01J21/18 ,  B01J23/44 ,  B01J27/0576 ,  B01J37/0205 ,  B01J37/16 ,  C07C45/34 ,  C07C45/35 ,  C07C45/36 ,  C07C51/252 ,  C07C47/21 ,  C07C47/22 ,  C07C47/232 ,  C07C57/04

    摘要： The present invention provides: a palladium-containing catalyst which is used for highly selectively or highly productively producing an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an olefin or in that way producing an α,β-unsaturated carboxylic acid from an α,β-unsaturated aldehyde; a method for producing the catalyst; and a method for highly selectively or highly productively producing an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an olefin or in that way producing an α,β-unsaturated carboxylic acid from an α,β-unsaturated aldehyde. In particular, the present invention resides in a palladium-containing catalyst comprising 0.001 to 0.40 mole of tellurium metal to 1.0 mole of palladium metal. This catalyst can be preferably produced by a method having a step of reducing a compound containing palladium atom in its oxidized state and tellurium atom in its oxidized state by a reducing agent.

    摘要翻译： 本发明提供：一种含钯催化剂，其用于从烯烃高度选择性或高产率地生产α，β-不饱和醛和α，β-不饱和羧酸，或以这种方式产生α，β-不饱和的 羧酸从α，β-不饱和醛; 催化剂的制造方法; 以及用于从烯烃高度选择性地或高效地生产α，β-不饱和醛和α，β-不饱和羧酸的方法，或以这种方式从α，β-不饱和醛生产α，β-不饱和羧酸的方法 。 特别地，本发明涉及一种含钯催化剂，其包含0.001至0.40摩尔的碲金属至1.0摩尔的钯金属。 该催化剂可以优选通过还原剂还原含有氧化态的钯原子的化合物和其氧化态的碲原子的方法来制造。

    Method for producing at least one of α, β-unsaturated aldehyde and α, β-unsaturated carboxylic acid
    7.
    发明授权
    Method for producing at least one of α, β-unsaturated aldehyde and α, β-unsaturated carboxylic acid 有权
    生产α，β-不饱和醛和α，β-不饱和羧酸中的至少一种的方法

    公开(公告)号：US08173838B2

    公开(公告)日：2012-05-08

    申请号：US12443994

    申请日：2006-10-03

    申请人： Akio Takeda ,  Yuji Fujimori ,  Seiichi Kawato

    发明人： Akio Takeda ,  Yuji Fujimori ,  Seiichi Kawato

    IPC分类号： C07C51/16 ,  C07C45/00

    CPC分类号： C07C45/38 ,  C07C51/235 ,  C07C47/22 ,  C07C57/04

    摘要： Disclosed is a method for producing at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an alcohol in a liquid phase through a simple process. Namely, at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid is produced by dehydrating and oxidizing an alcohol in a liquid phase at 110 to 250° C. in the presence of molecular oxygen and a noble metal-containing catalyst. Alternatively, at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid is produced by dehydrating and oxidizing an alcohol in a liquid phase in the presence of molecular oxygen, a noble metal-containing catalyst, and an acidic substance.

    摘要翻译： 公开了通过简单的方法从液相中生产α，β-不饱和醛和α，β-不饱和羧酸中的至少一种的方法。 即，α-和β-不饱和醛和α，β-不饱和羧酸中的至少一种是通过在分子氧存在下在110-250℃下在液相中脱水和氧化来制备的， 含贵金属的催化剂。 或者，α，β-不饱和醛和α，β-不饱和羧酸中的至少一种是通过在分子氧，含贵金属的催化剂存在下在液相中脱水和氧化来制备的， 和酸性物质。

    METHOD FOR PRODUCING AT LEAST ONE OF ALPHA, BETA-UNSATURATED ALDEHYDE AND ALPHA, BETA-UNSATURATED CARBOXYLIC ACID
    8.
    发明申请
    METHOD FOR PRODUCING AT LEAST ONE OF ALPHA, BETA-UNSATURATED ALDEHYDE AND ALPHA, BETA-UNSATURATED CARBOXYLIC ACID 有权
    用于生产至少一种ALPHA，不饱和二硫代氨基甲酸酯和ALPHA，β-不饱和羧酸的方法

    公开(公告)号：US20100094045A1

    公开(公告)日：2010-04-15

    申请号：US12443994

    申请日：2006-10-03

    申请人： Akio Takeda ,  Yuji Fujimori ,  Seiichi Kawato

    发明人： Akio Takeda ,  Yuji Fujimori ,  Seiichi Kawato

    IPC分类号： C07C51/235 ,  C07C45/38

    CPC分类号： C07C45/38 ,  C07C51/235 ,  C07C47/22 ,  C07C57/04

    摘要： Disclosed is a method for producing at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid from an alcohol in a liquid phase through a simple process. Namely, at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid is produced by dehydrating and oxidizing an alcohol in a liquid phase at 110 to 250° C. in the presence of molecular oxygen and a noble metal-containing catalyst. Alternatively, at least one of an α,β-unsaturated aldehyde and an α,β-unsaturated carboxylic acid is produced by dehydrating and oxidizing an alcohol in a liquid phase in the presence of molecular oxygen, a noble metal-containing catalyst, and an acidic substance.

    摘要翻译： 公开了通过简单的方法从液相中生产α，β-不饱和醛和α，β-不饱和羧酸中的至少一种的方法。 即，α-和β-不饱和醛和α，β-不饱和羧酸中的至少一种是通过在分子氧存在下在110-250℃下在液相中脱水和氧化来制备的， 含贵金属的催化剂。 或者，α，β-不饱和醛和α，β-不饱和羧酸中的至少一种是通过在分子氧，含贵金属的催化剂存在下在液相中脱水和氧化来制备的， 和酸性物质。

    PROCESS FOR PRODUCING ALPHA, BETA-UNSATURATED CARBOXYLIC ACID
    9.
    发明申请
    PROCESS FOR PRODUCING ALPHA, BETA-UNSATURATED CARBOXYLIC ACID 有权
    生产ALPHA，不饱和羧酸的方法

    公开(公告)号：US20090182170A1

    公开(公告)日：2009-07-16

    申请号：US11815907

    申请日：2006-02-08

    申请人： Atsushi Koizumi ,  Kazunori Matake ,  Toshihiko Fukuda ,  Yuji Fujimori

    发明人： Atsushi Koizumi ,  Kazunori Matake ,  Toshihiko Fukuda ,  Yuji Fujimori

    IPC分类号： C07C51/00

    CPC分类号： C07C51/087 ,  C07C51/252 ,  C07C57/04

    摘要： Disclosed is a method for enhancing a yield of an α,β-unsaturated carboxylic acid obtained by liquid-phase oxidation reaction of an olefin or an α,β-unsaturated aldehyde. In particular, there is provided a method for producing an α,β-unsaturated carboxylic acid, wherein the method includes the step of carrying out oxidation reaction of an olefin or an α,β-unsaturated aldehyde in a liquid phase to obtain a reaction mixture containing an α,β-unsaturated carboxylic acid and an α,β-unsaturated carboxylic acid anhydride and the step of bringing the α,β-unsaturated carboxylic acid anhydride into contact with an alcohol or water to obtain an α,β-unsaturated carboxylic acid resulting from decomposition of the α,β-unsaturated carboxylic acid anhydride.

    摘要翻译： 公开了一种提高通过烯烃或α，β-不饱和醛的液相氧化反应获得的α，β-不饱和羧酸的收率的方法。 特别地，提供了一种制备α，β-不饱和羧酸的方法，其中该方法包括在液相中进行烯烃或α，β-不饱和醛的氧化反应以获得反应混合物的步骤 含有α，β-不饱和羧酸和α，β-不饱和羧酸酐，以及使α，β-不饱和羧酸酐与醇或水接触以获得α，β-不饱和羧酸的步骤 由α，β-不饱和羧酸酐的分解产生。

    Photoelectric conversion element
    10.
    发明授权
    Photoelectric conversion element 失效
    光电转换元件

    公开(公告)号：US06683244B2

    公开(公告)日：2004-01-27

    申请号：US10002112

    申请日：2001-12-05

    申请人： Yuji Fujimori ,  Tsutomu Miyamoto

    发明人： Yuji Fujimori ,  Tsutomu Miyamoto

    IPC分类号： H01L5120

    CPC分类号： H01G9/2031 ,  H01L51/0084 ,  H01L51/4226 ,  Y02E10/542 ,  Y02E10/549

    摘要： A solar cell including a first electrode, a second electrode arranged opposite to the first electrode, an electron transport layer arranged between the first electrode and the second electrode, a dye layer D which is in contact with the electron transport layer, a hole transport layer arranged between the electron transport layer and the second electrode and being in contact with the dye layer D, and a barrier layer, and these elements are provided on a substrate. The barrier layer prevents or suppresses short-circuit between the first electrode and the hole transport layer. The porosity of the barrier layer is made smaller than that of the electron transport layer. The barrier layer is formed into a film-like shape and arranged between the first electrode and the electron transport layer. The solar cell can accomplish excellent photoelectric conversion efficiency by the provision of such a barrier layer.

    摘要翻译： 一种太阳能电池，包括第一电极，与第一电极相对布置的第二电极，布置在第一电极和第二电极之间的电子传输层，与电子传输层接触的染料层D，空穴传输层 布置在电子传输层和第二电极之间并且与染料层D接触，并且阻挡层，并且这些元件设置在基板上。 阻挡层防止或抑制第一电极和空穴传输层之间的短路。 阻挡层的孔隙率比电子传输层的孔隙度小。 阻挡层形成为膜状，并配置在第一电极和电子输送层之间。 太阳能电池可以通过设置这样的阻挡层来实现优异的光电转换效率。