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公开(公告)号：US07241716B2
公开(公告)日：2007-07-10
申请号：US10704741
申请日：2003-11-10
IPC分类号： B01J27/182 , B01J27/00
CPC分类号： C10G3/49 , B01J29/84 , B01J29/85 , B01J2229/24 , C07C1/20 , C07C209/16 , C07C2529/85 , C10G3/48 , C10G2300/802 , C10G2300/805 , C10G2400/20 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/06 , C07C211/04
摘要： Metalloaluminophosphate molecular sieves and metalloaluminophosphate molecular sieve catalyst particles are protecting from degradation by water by maintaining said molecular sieves or catalysts in contact with a liquid mixture of alcohol and water, the mixture of alcohol and water containing from 45 wt % to 99.8 wt % alcohol. The metalloaluminophosphate molecular sieves and metalloaluminophosphate molecular sieve catalyst particles which have been protected in such fashion catalyze the conversion of feedstocks to hydrocarbons.
摘要翻译： 金属铝磷酸盐分子筛和金属铝磷酸盐分子筛催化剂颗粒通过保持所述分子筛或催化剂与醇和水的液体混合物（含有45重量％至99.8重量％的醇的水和水的混合物）接触来防止水分降解。 以这种方式被保护的金属铝磷酸盐分子筛和金属铝磷酸盐分子筛催化剂颗粒催化原料转化为烃。
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公开(公告)号：US06936566B2
公开(公告)日：2005-08-30
申请号：US10395421
申请日：2003-03-24
申请人： Filip Mees , Etienne Vansant , Kun Wang , Richard B. Hall , Marcel Johannes Janssen , Luc Roger Marc Martens , An Verberckmoes , Guang Cao
发明人： Filip Mees , Etienne Vansant , Kun Wang , Richard B. Hall , Marcel Johannes Janssen , Luc Roger Marc Martens , An Verberckmoes , Guang Cao
CPC分类号： B01J37/0209 , B01J29/84 , B01J29/85 , B01J2229/14 , B01J2229/30 , C07C1/20 , C07C2531/14 , C10G3/49 , C10G3/62 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/04 , C07C11/06
摘要： The invention is directed to a method for modifying a microporous metalloaluminophosphate molecular sieve, the method comprising the steps of a) introducing a compound containing at least one M-X group within the cages of said microporous molecular sieve; and b) reacting said compound containing at least one M-X group with the acid groups located in the cages of the molecular sieve, wherein the compound containing at least one M-X group is selected from the group consisting of compounds of formula MX3, compounds of formula M2X6, and mixtures thereof, M being a metal belonging to Group 13 of the Periodic Table, and each X independently being a hydrogen or halogen atom. Preferably, X is a hydrogen atom. The present invention also relates to modified metalloaluminophosphate molecular sieves, preferably modified silicoaluminophosphate molecular sieves, as well as to the use of these modified molecular sieves in catalytic processes, such as processes for the conversion of oxygenated hydrocarbon feedstocks.
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公开(公告)号：US5783321A
公开(公告)日：1998-07-21
申请号：US351351
申请日：1995-05-15
IPC分类号： B01J29/04 , B01J29/06 , B01J29/40 , C01B37/02 , C01B39/04 , C01B39/06 , C01B39/08 , C01B39/38 , C01B39/40 , C01B33/34
CPC分类号： C01B39/082 , B01J29/04 , C01B39/38 , C01B39/40 , Y10S423/22
摘要： Crystalline tectosilicate ZSM-5 zeolite may be prepared which comprise substantially needle-shaped agglomerates. Tectosilicate ZSM-5 zeolite having a .sup.29 Si NMR spectrum having at least three peaks indicates the presence of Si atoms in the structure having 0, 1 or 2 T-atoms as nearest neighbors.
摘要翻译： PCT No.PCT / EP93 / 01404 Sec。 371日期1995年5月15日 102（e）日期1995年5月15日PCT提交1994年6月4日PCT公布。 公开号WO93 / 25476 日期1993年12月23日可以制备晶体硅酸锌ZSM-5沸石，其包含基本上针状的附聚物。 具有至少三个峰的29Si NMR光谱的表面硅酸盐ZSM-5沸石表示在具有0,1或2个T原子的结构中存在Si原子作为最近邻。
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公开(公告)号：US20120010426A1
公开(公告)日：2012-01-12
申请号：US13239004
申请日：2011-09-21
申请人： Raphael F. Caers , Eddy Theophile Van Driessche , Hubertus J. Beckers , Luc Roger Marc Martens , Georges Marie Mathys , John Richard Shutt
发明人： Raphael F. Caers , Eddy Theophile Van Driessche , Hubertus J. Beckers , Luc Roger Marc Martens , Georges Marie Mathys , John Richard Shutt
IPC分类号： C07C69/003 , C07C31/125 , C07C53/126 , C07C47/02
CPC分类号： C07C29/141 , C07C29/175 , C07C31/125 , C07C45/50 , C07C47/02 , C07C53/126 , C07C69/003 , C07C69/22 , C07C69/80
摘要： Mixed butene streams containing butene-1 and isobutylene and optionally butene-2 are hydroformylated under conditions that hydroformylates all the monomers to yield a mixture of valeraldehydes
摘要翻译： 含有丁烯-1和异丁烯和任选的丁烯-2的混合丁烯流在加氢甲酰化所有单体以产生戊醛混合物的条件下加氢甲酰化
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公开(公告)号：US07582802B2
公开(公告)日：2009-09-01
申请号：US10591306
申请日：2005-01-28
申请人： Raphael Frans Caers , Hubertus Joseph Beckers , Eddy Theophyle Andrea Van Driessche , Luc Roger Marc Martens , John Stephen Godsmark , John Richard Shutt
发明人： Raphael Frans Caers , Hubertus Joseph Beckers , Eddy Theophyle Andrea Van Driessche , Luc Roger Marc Martens , John Stephen Godsmark , John Richard Shutt
IPC分类号： C07C45/50
CPC分类号： C07C51/252 , C07C2/66 , C07C45/50 , C07C253/00 , Y02P20/582 , Y02P30/20 , C07C15/085 , C07C57/04 , C07C255/16 , C07C47/02
摘要： Propylene streams obtained by the conversion of oxygenates to olefins are used as feeds for hydroformylation. The streams may contain measurable amounts of dimethyl ether without adversely impacting the hydroformylation.
摘要翻译： 通过将含氧化合物转化为烯烃获得的丙烯流用作加氢甲酰化的进料。 流可以含有可测量的二甲醚，而不会不利地影响加氢甲酰化。
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16.发明授权Catalyst having a zeolitic core and zeolitic layer and the use of the catalyst for olefin oligomerization 失效具有沸石芯和沸石层的催化剂以及催化剂用于烯烃低聚的催化剂公开(公告)号：US06300536B1
公开(公告)日：2001-10-09
申请号：US09436485
申请日：1999-11-08
IPC分类号： C07C202
CPC分类号： C07C2/12 , B01J29/04 , B01J35/0006 , C07C2529/06 , C07C2529/70 , C07C2529/80
摘要： A molecular sieve comprising a core having deposited thereon a surface layer, wherein the core is a zeolite containing silicon and at least one element selected from gallium and iron and the surface layer has a higher Si:Al ratio than that of the silicon:selected element ratio of the core, provides for lower branching in olefin oligomerization products.
摘要翻译： 一种分子筛，其包含在其上沉积有表面层的芯，其中所述芯是含有硅的沸石和选自镓和铁的至少一种元素，并且所述表面层具有比所述硅选择元素更高的Si：Al比率 芯的比例，提供烯烃低聚产物中的较低支化。
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公开(公告)号：US5866096A
公开(公告)日：1999-02-02
申请号：US353427
申请日：1994-12-09
CPC分类号： B01J29/7042 , B01J29/04 , B01J29/80 , C01B39/48 , Y10S423/35
摘要： ZSM-22 zeolite which is particularly pure and whose synthesis does not require the synthesis mixture to be stirred can be produced by the addition to the synthesis mixture of a small quantity e.g. 1000 ppm, of preformed ZSM-22 zeolite seed crystals.
摘要翻译： ZSM-22沸石是特别纯的，其合成不需要合成混合物进行搅拌的方法，可以通过加入到少量的合成混合物中来制备。 1000ppm的预制ZSM-22沸石晶种。
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公开(公告)号：US20120253059A1
公开(公告)日：2012-10-04
申请号：US13439231
申请日：2012-04-04
申请人： Raphael F. Caers , Eddy Theophile Van Driessche , Hubertus J. Beckers , Luc Roger Marc Martens , Georges Marie Mathys , John Richard Shutt
发明人： Raphael F. Caers , Eddy Theophile Van Driessche , Hubertus J. Beckers , Luc Roger Marc Martens , Georges Marie Mathys , John Richard Shutt
CPC分类号： C07C29/141 , C07C29/175 , C07C31/125 , C07C45/50 , C07C47/02 , C07C53/126 , C07C69/003 , C07C69/22 , C07C69/80
摘要： Mixed butene streams containing butene-1 and isobutylene and optionally butene-2 are hydroformylated under conditions that hydroformylates all the monomers to yield a mixture of valeraldehydes. Higher temperatures and/or longer residence times and/or higher partial pressure of carbon monoxide than in conventional processes are used to ensure hydroformylation of all the monomers.
摘要翻译： 在加氢甲酰化所有单体以产生戊醛混合物的条件下，将含有丁烯-1和异丁烯和任选的丁烯-2的混合丁烯流加氢甲酰化。 使用比常规方法更高的温度和/或更长的停留时间和/或更高的一氧化碳分压来确保所有单体的加氢甲酰化。
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公开(公告)号：US07495142B2
公开(公告)日：2009-02-24
申请号：US11818496
申请日：2007-06-14
IPC分类号： C07C1/00
CPC分类号： C10G3/49 , B01J29/84 , B01J29/85 , B01J2229/24 , C07C1/20 , C07C209/16 , C07C2529/85 , C10G3/48 , C10G2300/802 , C10G2300/805 , C10G2400/20 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/06 , C07C211/04
摘要： Metalloaluminophosphate molecular sieves and metalloaluminophosphate molecular sieve catalyst particles are protecting from degradation by water by maintaining said molecular sieves or catalysts in contact with a liquid mixture of alcohol and water, the mixture of alcohol and water containing from 45 wt % to 99.8 wt % alcohol. The metalloaluminophosphate molecular sieves and metalloaluminophosphate molecular sieve catalyst particles which have been protected in such fashion catalyze the conversion of feedstocks to hydrocarbons.
摘要翻译： 金属铝磷酸盐分子筛和金属铝磷酸盐分子筛催化剂颗粒通过保持所述分子筛或催化剂与醇和水的液体混合物（含有45重量％至99.8重量％的醇的水和水的混合物）接触来防止水分降解。 以这种方式被保护的金属铝磷酸盐分子筛和金属铝磷酸盐分子筛催化剂颗粒催化原料转化为烃。
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公开(公告)号：US06906233B2
公开(公告)日：2005-06-14
申请号：US10317425
申请日：2002-12-12
申请人： Filip Mees , Etienne Vansant , Kun Wang , Richard B. Hall , Marcel Johannes Janssen , Luc Roger Marc Martens , An Amandine Verberckmoes , Guang Cao
发明人： Filip Mees , Etienne Vansant , Kun Wang , Richard B. Hall , Marcel Johannes Janssen , Luc Roger Marc Martens , An Amandine Verberckmoes , Guang Cao
CPC分类号： B01J37/0209 , B01J29/84 , B01J29/85 , B01J2229/14 , B01J2229/30 , C07C1/20 , C07C2531/14 , C10G3/49 , C10G3/62 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/04 , C07C11/06
摘要： The invention is directed to a method for modifying a microporous metalloaluminophosphate molecular sieve, the method comprising the steps of a) introducing a compound containing at least one M-X group within the cages of said microporous molecular sieve; and b) reacting said compound containing at least one M-X group with the acid groups located in the cages of the molecular sieve, wherein the compound containing at least one M-X group is selected from the group consisting of compounds of formula MX3, compounds of formula M2X6, and mixtures thereof, M being a metal belonging to Group 13 of the Periodic Table, and each X independently being a hydrogen or halogen atom. Preferably, X is a hydrogen atom. The present invention also relates to modified metalloaluminophosphate molecular sieves, preferably modified silicoaluminophosphate molecular sieves, as well as to the use of these modified molecular sieves in catalytic processes, such as processes for the conversion of oxygenated hydrocarbon feedstocks.
摘要翻译： 本发明涉及一种改性微孔金属铝磷酸盐分子筛的方法，该方法包括以下步骤：a）将含有至少一个M-X基团的化合物引入所述微孔分子筛的笼中; 和b）使含有至少一个MX基团的化合物与位于分子筛网笼中的酸基反应，其中含有至少一个MX基团的化合物选自式MX 3化合物， / SUB，式M 2 X 6的化合物及其混合物，M是属于周期表第13族的金属，并且每个X独立地为氢 或卤素原子。 优选地，X是氢原子。 本发明还涉及改性的金属铝磷酸盐分子筛，优选改性的硅铝磷酸盐分子筛，以及这些改性分子筛在催化方法中的用途，例如转化含氧烃原料的方法。
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