公开(公告)号：US20160060516A1

公开(公告)日：2016-03-03

申请号：US14781132

申请日：2014-03-28

Applicant: UBE INDUSTRIES, LTD.

Inventor： Mao Sumino ,  Kazuki Iwashita ,  Takuma Sakai ,  Masataka Fujinaga ,  Shinsuke Jida

IPC: C09K11/77

CPC classification number: C09K11/7734 ,  C01B21/06

Abstract: An oxynitride phosphor powder has a fluorescence peak wavelength of 610 to 625 nm and also has higher external quantum efficiency than the conventional one. The oxynitride phosphor powder includes an α-type SiAlON and aluminum nitride, represented by the compositional formula: Cax1Eux2Si12−(y+z)Al(y+z)OzN16−z wherein x1, x2, y, z fulfill the following formulae: 1.60≦x1+x2≦2.90, 0.18≦x2/x1≦0.70, 4.0≦y≦6.5, 0.0≦z≦1.0. The powder can additionally contain Li in an amount of 50 to 10000 ppm. The content of the aluminum nitride may be more than 0 mass % to less than 33 mass %.

Abstract translation: 氮氧化物荧光体粉末的荧光峰值波长为610〜625nm，外部量子效率高于常规荧光粉。 氧氮化物荧光体粉末包括由以下组成式表示的α型SiAlON和氮化铝：Cax1Eux2Si12-（y + z）Al（y + z）OzN16-z其中x1，x2，y，z满足下列公式：1.60 ＆nlE; x1 + x2＆nlE; 2.90,0.18＆nlE; x2 / x1＆nlE; 0.70,4.0＆nlE; y＆nlE; 6.5,0.0＆nlE; z＆nlE; 1.0。 该粉末还可以含有50〜10000ppm的Li。 氮化铝的含量可以大于0质量％至小于33质量％。

公开(公告)号：US20160024379A1

公开(公告)日：2016-01-28

申请号：US14773443

申请日：2014-03-07

Applicant: Ube Industries, Ltd.

Inventor： Kazuki Iwashita ,  Mao Sumino ,  Takayuki Ueda ,  Masataka Fujinaga ,  Shinsuke Jida

IPC: C09K11/77

CPC classification number: C09K11/7734 ,  C04B35/58 ,  C04B35/581 ,  C04B35/584 ,  C04B2235/3852 ,  C04B2235/3865 ,  C04B2235/3873 ,  C04B2235/5409 ,  C04B2235/5436 ,  C09K11/0883 ,  C09K11/7728

Abstract: A nitride phosphor includes a (Ca,Sr)AlSiN3:Eu phosphor, of which the chemical composition can be controlled easily and which has excellent fluorescent properties. A method produces a nitride phosphor represented by the formula: (Ca1-x1-x2Srx1Eux2)aAlbSicN2a/3+b+4/3c (wherein 0.49

Abstract translation: 氮化物荧光体包括（Ca，Sr）AlSiN 3：Eu荧光体，其化学组成可以容易地控制并且具有优异的荧光性能。 一种方法产生由下式（Ca1-x1-x2Srx1Eux2）aAlbSicN2a / 3 + b + 4 / 3c（其中0.49

公开(公告)号：US20140158858A1

公开(公告)日：2014-06-12

申请号：US13927716

申请日：2013-06-26

Applicant: Ube Industries, Ltd.

Inventor： Takeshi Yamao ,  Takayuki Fujii ,  Shinsuke Jida

IPC: B29C33/60 ,  B29C33/38

CPC classification number: B29C33/60 ,  B29C33/38 ,  C01B21/068 ,  C01B21/0687 ,  C01B33/02 ,  C01P2004/03 ,  C01P2004/61 ,  C01P2004/62 ,  C01P2006/22 ,  C01P2006/80 ,  C30B11/002 ,  C30B29/06 ,  Y10T428/2982

Abstract: Provided are a polycrystalline silicon ingot casting mold and a method for producing a polycrystalline silicon ingot casting mold, with which high-quality silicon ingots can be obtained at high yields by minimizing sticking with the surfaces of the silicon ingot casting mold, and losses and damages that occur when solidified silicon ingot is released from the mold. The method for producing a polycrystalline silicon ingot casting mold having a release layer, including: forming a slurry by mixing a silicon nitride powder with water, coating the surface of the mold with the slurry, and heating the mold at 400 to 800° C. in an atmosphere containing oxygen, after coating the slurry.

Abstract translation: 提供一种多晶硅锭铸造模具和多晶硅锭铸造模具的制造方法，通过使硅锭铸造模具的表面最小化而能以高产率获得高质量的硅锭，以及损失和损坏 当固化的硅锭从模具中释放出现时。 一种具有脱模层的多晶硅锭铸造模具的制造方法，其特征在于，包括：通过将氮化硅粉末与水混合形成浆料，用所述浆料涂布所述模具的表面，并在400〜800℃下加热所述模具。 在包含氧气的气氛中，涂覆浆料后。

公开(公告)号：US10399854B2

公开(公告)日：2019-09-03

申请号：US15318005

申请日：2015-06-16

Applicant: Ube Industries, Ltd.

Inventor： Takeshi Yamao ,  Michio Honda ,  Shinsuke Jida

IPC: C01B21/068 ,  C04B35/584 ,  C04B35/626 ,  H05K1/02 ,  H05K1/03

Abstract: A silicon nitride powder having a specific surface area of 4.0 to 9.0 m2/g, a β phase proportion of less than 40 mass %, and an oxygen content of 0.20 to 0.95 mass %, wherein a frequency distribution curve obtained by measuring a volume-based particle size distribution by a laser diffraction scattering method has two peaks, peak tops of the peaks are present respectively at 0.4 to 0.7 μm and 1.5 to 3.0 μm, a ratio of frequencies of the peak tops ((frequency of the peak top in a particle diameter range of 0.4 to 0.7 μm)/(frequency of the peak top in a particle diameter range of 1.5 to 3.0 μm)) is 0.5 to 1.5, and a ratio D50/DBET (μm/μm) of a median diameter D50 (μm) determined by the measurement of particle size distribution to a specific surface area-equivalent diameter DBET (μm) calculated from the specific surface area is 3.5 or more.

公开(公告)号：US09758720B2

公开(公告)日：2017-09-12

申请号：US14350929

申请日：2012-10-12

Applicant: Ube Industries, Ltd.

Inventor： Masataka Fujinaga ,  Takayuki Ueda ,  Takuma Sakai ,  Shinsuke Jida

IPC: C09K11/77 ,  C01B21/082 ,  C09K11/08 ,  H05B33/14 ,  H01L33/50

CPC classification number: C09K11/7728 ,  C01B21/0821 ,  C01B21/0826 ,  C01P2002/54 ,  C01P2002/72 ,  C01P2002/77 ,  C01P2002/84 ,  C01P2004/03 ,  C01P2004/04 ,  C01P2004/62 ,  C01P2006/12 ,  C09K11/0883 ,  C09K11/7734 ,  H01L33/502 ,  H05B33/14

Abstract: An oxynitride phosphor powder contains α-SiAlON and aluminum nitride, obtained by mixing a silicon source, an aluminum source, a calcium source, and a europium source to produce a composition represented by a compositional formula: Cax1Eux2Si12−(y+z)Al(y+z)OzN16−z (wherein x1, x2, y and z are 0

公开(公告)号：US09708533B2

公开(公告)日：2017-07-18

申请号：US14436224

申请日：2013-10-17

Applicant: Ube Industries, Ltd.

Inventor： Kazuki Iwashita ,  Takuma Sakai ,  Takayuki Ueda ,  Masataka Fujinaga ,  Shinsuke Jida ,  Masataka Yamanaga ,  Yuki Nagao ,  Takafumi Kawano

IPC: C09K11/64 ,  H01L33/50 ,  C09K11/77 ,  F21V9/16 ,  C04B35/597 ,  C04B35/626 ,  C09K11/08 ,  C04B35/645 ,  F21K9/64

CPC classification number: C09K11/7734 ,  C04B35/597 ,  C04B35/6265 ,  C04B35/645 ,  C04B2235/3852 ,  C04B2235/3865 ,  C04B2235/3873 ,  C04B2235/3895 ,  C04B2235/5409 ,  C04B2235/77 ,  C04B2235/80 ,  C09K11/0883 ,  F21K9/64 ,  F21V9/30 ,  H01L33/502

Abstract: A method of manufacturing a wavelength conversion member including a polycrystalline ceramics includes mixing a substance serving as a silicon source, a substance serving as an aluminum source, a substance serving as a calcium source, and a substance serving as a europium source; firing the obtained mixture to obtain an oxynitride phosphor powder; then sintering the oxynitride phosphor powder in an inert atmosphere to obtain the polycrystalline ceramics, characterized in that the sintered oxynitride phosphor powder has a composition (excluding oxygen) represented by the Formula: Cax1Eux2Si12-(y+z)Al(y+z)OzN16-z (in the Formula, x1, x2, y, and z are values such that 0

公开(公告)号：US20170174515A1

公开(公告)日：2017-06-22

申请号：US15118115

申请日：2015-02-09

Applicant: Ube Industries, Ltd.

Inventor： Takeshi Yamao ,  Michio Honda ,  Shinsuke Jida

IPC: C01B21/068 ,  B22C3/00 ,  C09D1/00

CPC classification number: C01B21/068 ,  B22C3/00 ,  B22C9/02 ,  B22C9/061 ,  B22D7/005 ,  C01B21/0685 ,  C01P2002/02 ,  C01P2004/04 ,  C01P2006/12 ,  C01P2006/80 ,  C09D1/00 ,  C10M103/00 ,  C10M2201/1006 ,  C10N2240/58 ,  C10N2270/00

Abstract: A silicon nitride powder to be used in a slurry for forming a mold release layer of a polycrystalline silicon casting mold, wherein the specific surface area thereof is 5-50 m2/g, the proportion of amorphous silicon nitride is 1.0-25.0 mass %, and the oxygen content is 0.6-2.5 mass %. A silicon nitride powder slurry for use in mold release material and capable of forming, on a polycrystalline silicon casting mold, a mold release layer which exhibits favorable mold release properties and exhibits favorable adhesion to the casting mold after casting the polycrystalline silicon ingot, and a method for producing the same. A silicon nitride powder for mold release material, a silicon nitride powder for a slurry use for obtaining the silicon nitride powder slurry for use in the mold release material, and a method for producing the same. A polycrystalline silicon casting mold which exhibits favorable mold release properties of a polycrystalline silicon ingot; and method for producing the same.

公开(公告)号：US20170107109A1

公开(公告)日：2017-04-20

申请号：US15318005

申请日：2015-06-16

Applicant: Ube Industries, Ltd.

Inventor： Takeshi Yamao ,  Michio Honda ,  Shinsuke Jida

IPC: C01B21/068 ,  H05K1/03 ,  H05K1/02 ,  C04B35/584

CPC classification number: C01B21/068 ,  C01P2004/61 ,  C01P2004/62 ,  C01P2006/12 ,  C04B35/584 ,  C04B35/626 ,  C04B2235/3882 ,  H05K1/0201 ,  H05K1/0306

Abstract: A silicon nitride powder having a specific surface area of 4.0 to 9.0 m2/g, a β phase proportion of less than 40 mass %, and an oxygen content of 0.20 to 0.95 mass %, wherein a frequency distribution curve obtained by measuring a volume-based particle size distribution by a laser diffraction scattering method has two peaks, peak tops of the peaks are present respectively at 0.4 to 0.7 μm and 1.5 to 3.0 μm, a ratio of frequencies of the peak tops ((frequency of the peak top in a particle diameter range of 0.4 to 0.7 μm)/(frequency of the peak top in a particle diameter range of 1.5 to 3.0 μm)) is 0.5 to 1.5, and a ratio D50/DBET (μm/μm) of a median diameter D50 (μm) determined by the measurement of particle size distribution to a specific surface area-equivalent diameter DBET (μm) calculated from the specific surface area is 3.5 or more.

公开(公告)号：US08973888B2

公开(公告)日：2015-03-10

申请号：US13927716

申请日：2013-06-26

Applicant: Ube Industries, Ltd.

Inventor： Takeshi Yamao ,  Takayuki Fujii ,  Shinsuke Jida

IPC: B29C33/38 ,  C01B21/068 ,  B29C33/60 ,  C01B33/02 ,  C30B11/00 ,  C30B29/06

CPC classification number: B29C33/60 ,  B29C33/38 ,  C01B21/068 ,  C01B21/0687 ,  C01B33/02 ,  C01P2004/03 ,  C01P2004/61 ,  C01P2004/62 ,  C01P2006/22 ,  C01P2006/80 ,  C30B11/002 ,  C30B29/06 ,  Y10T428/2982

Abstract: Provided are a polycrystalline silicon ingot casting mold and a method for producing a polycrystalline silicon ingot casting mold, with which high-quality silicon ingots can be obtained at high yields by minimizing sticking with the surfaces of the silicon ingot casting mold, and losses and damages that occur when solidified silicon ingot is released from the mold. The method for producing a polycrystalline silicon ingot casting mold having a release layer, including: forming a slurry by mixing a silicon nitride powder with water, coating the surface of the mold with the slurry, and heating the mold at 400 to 800° C. in an atmosphere containing oxygen, after coating the slurry.

Abstract translation: 提供一种多晶硅锭铸造模具和多晶硅锭铸造模具的制造方法，通过使硅锭铸造模具的表面最小化而能以高产率获得高质量的硅锭，以及损失和损坏 当固化的硅锭从模具中释放出现时。 一种具有脱模层的多晶硅锭铸造模具的制造方法，其特征在于，包括：通过将氮化硅粉末与水混合形成浆料，用所述浆料涂布所述模具的表面，并在400〜800℃下加热所述模具。 在包含氧气的气氛中，涂覆浆料后。