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31.发明授权Method for preparing SSZ-26/33 zeolites using novel structure directing agents 有权使用新型结构导向剂制备SSZ-26/33沸石的方法公开(公告)号：US07648694B2
公开(公告)日：2010-01-19
申请号：US12249770
申请日：2008-10-10
申请人： Allen W. Burton, Jr.
发明人： Allen W. Burton, Jr.
CPC分类号： C01B39/48 , B01J29/70 , B01J29/86 , B01J37/0009 , C01B39/12
摘要： The present invention is directed to a process for preparing zeolites belonging to the SSZ-26/33 family of zeolites using novel nitrogen-based structure directing agents. The process for preparing the SSZ-26/33 family of zeolites involves using a structure directing agent selected from the group consisting of 1,5-bis(N,N-dimethylcyclohexylammonium)pentane dications, 1,4-bis(N-cyclohexylpiperidinium)butane dications and 1,4-bis(N-cyclopentylpiperidinium)butane dications.
摘要翻译： 本发明涉及使用新型氮基结构导向剂制备属于SSZ-26/33沸石族沸石的方法。 制备SSZ-26/33沸石系列的方法涉及使用选自1,5-双（N，N-二甲基环己基铵）戊烷二异氰酸酯，1,4-双（N-环己基哌啶鎓） 丁烷和1,4-双（N-环戊基哌啶鎓）丁烷偶联剂。
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公开(公告)号：US08679451B2
公开(公告)日：2014-03-25
申请号：US12622680
申请日：2009-11-20
CPC分类号： C01B39/42 , C07C5/2708 , C07C2523/42 , C07C2523/44 , C07C2529/70 , C07C9/16 , C07C9/00
摘要： An aluminosilicate ZSM-12 may be prepared de novo in a small crystalline form from a reaction mixture containing a source of silica and a source of alumina. A small crystalline form of aluminosilicate ZSM-12 may also be prepared from a small crystalline form of borosilicate ZSM-12 by replacement of boron in the borosilicate ZSM-12 framework with aluminum. The aluminosilicate ZSM-12 is useful as an isomerization selective catalyst in processes such as isomerization dewaxing hydrocarbon feedstocks.
摘要翻译： 铝硅酸盐ZSM-12可以从含有二氧化硅源和氧化铝源的反应混合物中以小结晶形式从头制备。 也可以通过用硼替代硼硅酸盐ZSM-12骨架中的硼，由小晶体形式的硼硅酸盐ZSM-12制备小晶体的硅酸铝ZSM-12。 铝硅酸盐ZSM-12可用作异构化选择性催化剂，例如异构化脱蜡烃原料。
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33.发明授权N-paraffin selective hydroconversion process using borosilicate ZSM-48 molecular sieves 有权使用硼硅酸盐ZSM-48分子筛的N-链烷烃选择性加氢转化方法公开(公告)号：US08212099B2
公开(公告)日：2012-07-03
申请号：US12612820
申请日：2009-11-05
申请人： Allen W. Burton, Jr.
发明人： Allen W. Burton, Jr.
IPC分类号： C07C4/06
CPC分类号： C10G47/16 , B01J29/703 , B01J29/86 , B01J35/002 , B01J35/023 , B01J37/0201 , B01J2229/186 , C10G47/18 , C10G2300/1081 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2300/4025
摘要： The present invention is directed to processes using a borosilicate ZSM-48 as a catalyst for the selective hydroconversion of heavy normal paraffins into lighter normal paraffin products, with minimal formation of isoparaffins. The borosilicate ZSM-48 molecular sieve has a mole ratio of between 40 and 400 of silicon oxide to boron oxide, synthesized using novel structure directing agents.
摘要翻译： 本发明涉及使用硼硅酸盐ZSM-48作为催化剂的重质正链烷烃选择性加氢转化为更轻质的正链烷烃产物，同时形成异链烷烃的方法。 硼硅酸盐ZSM-48分子筛的氧化硅与氧化硼的摩尔比为40〜400，采用新型结构导向剂合成。
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34.发明授权Process for isomerizing a hydrocarbonaceous feedstock using aluminosilicate ZSM-12 有权使用硅铝酸盐ZSM-12异构化含烃原料的方法公开(公告)号：US08101811B2
公开(公告)日：2012-01-24
申请号：US12622669
申请日：2009-11-20
CPC分类号： B01J29/7469 , B01J29/7034 , B01J29/86 , C01B39/42 , C07C5/2708 , C07C2523/42 , C07C2523/44 , C07C2523/46 , C07C2523/755 , C07C2529/70 , C07C2529/86 , C10G45/64 , C10G2300/1037 , C10G2300/4018 , C07C9/16 , C07C9/00
摘要： An aluminosilicate ZSM-12 may be prepared de novo in a small crystalline form from a reaction mixture containing a source of silica and a source of alumina A small crystalline form of aluminosilicate ZSM-12 may also be prepared from a small crystalline form of borosilicate ZSM-12 by replacement of boron in the borosilicate ZSM-12 framework with aluminum. The aluminosilicate ZSM-12 is useful as an isomerization selective catalyst in processes such as isomerization dewaxing hydrocarbon feedstocks.
摘要翻译： 铝硅酸盐ZSM-12可以从含有二氧化硅源和氧化铝源的反应混合物中以小结晶形式重新制备。也可以从小晶体形式的硼硅酸盐ZSM制备铝硅酸盐ZSM-12的小结晶形式 -12通过用硼替代硼硅酸盐ZSM-12框架中的硼。 铝硅酸盐ZSM-12可用作异构化选择性催化剂，例如异构化脱蜡烃原料。
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35.发明授权Process for preparing MTT zeolites using N,N,N,N′,N′,N′-hexamethyl-propane-1,3-diammonium dication structure directing agent 有权使用N，N，N，N'，N'，N'-六甲基丙烷-1,3-二铵双键结构导向剂制备MTT沸石的方法公开(公告)号：US07682600B2
公开(公告)日：2010-03-23
申请号：US11565812
申请日：2006-12-01
申请人： Allen W. Burton, Jr.
发明人： Allen W. Burton, Jr.
IPC分类号： C01B39/04
CPC分类号： C01B39/48 , C01B39/12 , Y10S423/36
摘要： The present invention rebates to a process for preparing zeolites having the MTT framework topology defined by the connectivity of the tetrahedral atoms in the zeolite, such as zeolites SSZ-32 and ZSM-23, using an N,N,N,N′,N′,N′-hexamethyl-propane-1,3-diammonium dication as a structure directing agent.
摘要翻译： 本发明涉及制备具有由沸石中四面体原子如沸石SSZ-32和ZSM-23的连通性使用N，N，N，N'，N '，N'-六甲基 - 丙烷-1,3-二铵二水合作为结构导向剂。
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公开(公告)号：US08142757B2
公开(公告)日：2012-03-27
申请号：US12612824
申请日：2009-11-05
申请人： Allen W. Burton, Jr.
发明人： Allen W. Burton, Jr.
摘要： The present invention is directed to a borosilicate ZSM-48 molecular sieve having a mole ratio of between 40 and 400 of silicon oxide to boron oxide, synthesized using novel structure directing agents. Also disclosed are processes using a borosilicate ZSM-48 as a catalyst for the selective hydroconversion of heavy normal paraffins into lighter normal paraffin products, with minimal formation of isoparaffins.
摘要翻译： 本发明涉及使用新型结构导向剂合成的氧化硅与氧化硼的摩尔比在40和400之间的硼硅酸盐ZSM-48分子筛。 还公开了使用硼硅酸盐ZSM-48作为催化剂的重质正链烷烃选择性加氢转化为更轻的正链烷烃产物，同时形成异链烷烃的方法。
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公开(公告)号：US07943674B1
公开(公告)日：2011-05-17
申请号：US12622972
申请日：2009-11-20
申请人： Charles L. Kibby , Kandaswamy Jothimurugesan , Tapan K. Das , Robert J. Saxton , Allen W. Burton, Jr.
发明人： Charles L. Kibby , Kandaswamy Jothimurugesan , Tapan K. Das , Robert J. Saxton , Allen W. Burton, Jr.
IPC分类号： C07C27/00
CPC分类号： B01J29/7469 , B01J29/7669 , B01J2229/42 , C07C1/0435 , C07C2529/46 , C10G2/332 , C10G2/334 , C10G2300/1022 , C10G2300/4006 , C10G2300/4012 , C10G2300/703 , C07C9/00
摘要： A method for performing synthesis gas conversion is disclosed which comprises contacting synthesis gas with a hybrid Fischer-Tropsch catalyst formed by impregnating a ZSM-12 zeolite extrudate using a solution, for example, a substantially non-aqueous solution, comprising a cobalt salt and activating the impregnated zeolite extrudate by a reduction-oxidation-reduction cycle. The method results in reduced methane yield and increased yield of liquid hydrocarbons substantially free of solid wax.
摘要翻译： 公开了一种用于进行合成气转化的方法，其包括使合成气与通过使用包含钴盐和活化的溶液例如基本上非水溶液浸渍ZSM-12沸石挤出物而形成的混合费 - 托催化剂接触 浸渍的沸石通过还原 - 氧化 - 还原循环挤出物。 该方法导致甲烷产率降低并且基本上不含固体蜡的液体烃的产率提高。
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38.发明授权Process for conversion of synthesis gas to hydrocarbons using a zeolite-methanol catalyst system 有权使用沸石 - 甲醇催化剂体系将合成气转化为烃的方法公开(公告)号：US07943673B2
公开(公告)日：2011-05-17
申请号：US12316209
申请日：2008-12-10
IPC分类号： C07C27/00
CPC分类号： B01J35/0006 , B01J23/26 , B01J29/87 , B01J35/1019 , B01J37/031 , B01J37/18 , C01B39/082 , C10G2/33 , C10G2/334 , C10L1/06
摘要： A process is described for converting synthesis gas containing carbon monoxide and hydrogen to hydrocarbons via methanol as an intermediate, by contacting the synthesis gas with a catalyst system containing a mixture of gallium silicate zeolite catalyst and a methanol catalyst. The process results in reduced amounts of undesirable low carbon number hydrocarbons, e.g., C4 and lower, undesirable high carbon number hydrocarbons, e.g., C10 and higher, and aromatic hydrocarbons. The process provides higher yields of useful, high octane hydrocarbons boiling in the gasoline range.
摘要翻译： 描述了通过使合成气与含有硅酸镓沸石催化剂和甲醇催化剂的混合物的催化剂体系接触来将含有一氧化碳和氢的合成气转化为甲醇作为中间体的方法。 该方法导致不期望的低碳数烃的量减少，例如C4和更低的不期望的高碳数烃，例如C10和更高级的芳族烃。 该方法提供了在汽油范围内沸腾的有用的高辛烷值的较高产率。
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公开(公告)号：US06676923B1
公开(公告)日：2004-01-13
申请号：US10186905
申请日：2002-06-28
申请人： Stacey Zones , Allen W. Burton, Jr.
发明人： Stacey Zones , Allen W. Burton, Jr.
IPC分类号： C01B3948
CPC分类号： C01B37/02 , C01B39/12 , C01B39/48 , Y10S423/35 , Y10S423/36
摘要： The present invention relates to new crystalline zeolite SSZ-54 prepared using a templating agent comprising N-isopropyl ethylenediamine, or a mixture of 1-N-isopropyl diethylenetriamine and isobutylamine, and processes employing SSZ-54 in a catalyst.
摘要翻译： 本发明涉及使用包含N-异丙基乙二胺或1-N-异丙基二亚乙基三胺和异丁胺的混合物的模板剂制备的新的结晶沸石SSZ-54以及在催化剂中使用SSZ-54的方法。
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40.发明授权Process of synthesis gas conversion to liquid fuels using mixture of synthesis gas conversion catalyst and dual functionality catalyst 有权使用合成气转化催化剂和双官能催化剂的混合物将合成气转化为液体燃料的方法公开(公告)号：US07973087B2
公开(公告)日：2011-07-05
申请号：US12902915
申请日：2010-10-12
申请人： Charles L. Kibby , Kandaswamy Jothimurugesan , Tapan K. Das , Robert J. Saxton , Allen W. Burton, Jr.
发明人： Charles L. Kibby , Kandaswamy Jothimurugesan , Tapan K. Das , Robert J. Saxton , Allen W. Burton, Jr.
IPC分类号： C07C27/00
CPC分类号： C10G2/333 , B01J23/75 , B01J23/894 , B01J29/068 , B01J29/44 , B01J29/74 , B01J35/0006
摘要： A process is disclosed for converting a feed comprising synthesis gas to liquid hydrocarbons within a single reactor at essentially common reaction conditions. The synthesis gas contacts a catalyst bed comprising a mixture of a synthesis gas conversion catalyst on a support containing an acidic component and a dual functionality catalyst including a hydrogenation component and a solid acid component. The hydrocarbons produced are liquid at about 0° C., contain at least 25% by volume C10+ and are substantially free of solid wax.
摘要翻译： 公开了用于在基本上常见的反应条件下将包含合成气的进料转化为单个反应器内的液体烃的方法。 合成气在包含酸性组分的载体和包含氢化组分和固体酸组分的双官能催化剂的催化剂床上接触合成气转化催化剂的混合物。 生产的烃在约0℃是液体的，含有至少25体积％的C 10+，并且基本上不含固体蜡。
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